Articles | Volume 17, issue 12
https://doi.org/10.5194/acp-17-7807-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-17-7807-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Estimating the atmospheric concentration of Criegee intermediates and their possible interference in a FAGE-LIF instrument
Anna Novelli
Atmospheric Chemistry Department, Max Planck Institute
for Chemistry, 55128 Mainz, Germany
now at: Institute of Energy and Climate Research, IEK-8:
Troposphere, Forschungszentrum Jülich GmbH, 52428 Jülich,
Germany
Korbinian Hens
Atmospheric Chemistry Department, Max Planck Institute
for Chemistry, 55128 Mainz, Germany
Cheryl Tatum Ernest
Atmospheric Chemistry Department, Max Planck Institute
for Chemistry, 55128 Mainz, Germany
now at: Department of Neurology University Medical Center
of the Johannes Gutenberg University Mainz, 55131 Mainz, Germany
Monica Martinez
Atmospheric Chemistry Department, Max Planck Institute
for Chemistry, 55128 Mainz, Germany
Anke C. Nölscher
Atmospheric Chemistry Department, Max Planck Institute
for Chemistry, 55128 Mainz, Germany
now at: Division of Geological and Planetary Sciences,
California Institute of Technology, Pasadena, USA
Vinayak Sinha
Department of Earth and Environmental Sciences, Indian
Institute of Science Education and Research Mohali, Sector 81 S.A.S. Nagar,
Manauli PO, Mohali 140 306, Punjab, India
Pauli Paasonen
Department of Physics., P.O. Box 64. 00014 University of
Helsinki, Helsinki, Finland
Tuukka Petäjä
Department of Physics., P.O. Box 64. 00014 University of
Helsinki, Helsinki, Finland
Mikko Sipilä
Department of Physics., P.O. Box 64. 00014 University of
Helsinki, Helsinki, Finland
Thomas Elste
German Meteorological Service, Meteorological Observatory
Hohenpeissenberg (MOHp), 83282 Hohenpeissenberg, Germany
Christian Plass-Dülmer
German Meteorological Service, Meteorological Observatory
Hohenpeissenberg (MOHp), 83282 Hohenpeissenberg, Germany
Gavin J. Phillips
Atmospheric Chemistry Department, Max Planck Institute
for Chemistry, 55128 Mainz, Germany
Department of Natural Sciences, University of Chester,
Thornton Science Park, Chester, CH2 4NU, UK
Dagmar Kubistin
Atmospheric Chemistry Department, Max Planck Institute
for Chemistry, 55128 Mainz, Germany
German Meteorological Service, Meteorological Observatory
Hohenpeissenberg (MOHp), 83282 Hohenpeissenberg, Germany
University of Wollongong, School of Chemistry,
Wollongong, Australia
Jonathan Williams
Atmospheric Chemistry Department, Max Planck Institute
for Chemistry, 55128 Mainz, Germany
Luc Vereecken
Atmospheric Chemistry Department, Max Planck Institute
for Chemistry, 55128 Mainz, Germany
now at: Institute of Energy and Climate Research, IEK-8:
Troposphere, Forschungszentrum Jülich GmbH, 52428 Jülich,
Germany
Jos Lelieveld
Atmospheric Chemistry Department, Max Planck Institute
for Chemistry, 55128 Mainz, Germany
Atmospheric Chemistry Department, Max Planck Institute
for Chemistry, 55128 Mainz, Germany
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66 citations as recorded by crossref.
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- Study on ozonolysis of asymmetric alkenes with matrix isolation and FT-IR spectroscopy Z. Wang et al. 10.1016/j.chemosphere.2020.126413
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- Implementation of a chemical background method for atmospheric OH measurements by laser-induced fluorescence: characterisation and observations from the UK and China R. Woodward-Massey et al. 10.5194/amt-13-3119-2020
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- Kinetics of CH2OO and syn-CH3CHOO reaction with acrolein X. Zhou et al. 10.1039/D1CP00492A
- Sources, sinks, and chemistry of Stabilized Criegee Intermediates in the Indo-Gangetic Plain M. Shabin et al. 10.1016/j.scitotenv.2023.165281
- Re-examining ammonia addition to the Criegee intermediate: converging to chemical accuracy J. Misiewicz et al. 10.1039/C7CP08582F
- Kinetics of the reaction of the simplest Criegee intermediate with ammonia: a combination of experiment and theory Y. Liu et al. 10.1039/C8CP05920A
- The reaction of peroxy radicals with OH radicals C. Fittschen 10.1016/j.cplett.2019.04.002
- Unimolecular and water reactions of oxygenated and unsaturated Criegee intermediates under atmospheric conditions L. Vereecken et al. 10.1039/D1CP05877K
- Role of Criegee intermediates in the formation of sulfuric acid at a Mediterranean (Cape Corsica) site under influence of biogenic emissions A. Kukui et al. 10.5194/acp-21-13333-2021
- Detection and identification of Criegee intermediates from the ozonolysis of biogenic and anthropogenic VOCs: comparison between experimental measurements and theoretical calculations C. Giorio et al. 10.1039/C7FD00025A
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- OH production from the photolysis of isoprene-derived peroxy radicals: cross-sections, quantum yields and atmospheric implications R. Hansen et al. 10.1039/C6CP06718B
62 citations as recorded by crossref.
- Kinetics of the Simplest Criegee Intermediate CH2OO Reaction with tert-Butylamine Y. Chen et al. 10.1021/acs.jpca.2c07854
- Year-round modeling of sulfate aerosol over Asia through updates of aqueous-phase oxidation and gas-phase reactions with stabilized Criegee intermediates S. Itahashi et al. 10.1016/j.aeaoa.2021.100123
- ROOOH: a missing piece of the puzzle for OH measurements in low-NO environments? C. Fittschen et al. 10.5194/acp-19-349-2019
- Criegee Intermediate Reactions with Carboxylic Acids: A Potential Source of Secondary Organic Aerosol in the Atmosphere R. Chhantyal-Pun et al. 10.1021/acsearthspacechem.8b00069
- Oligomer formation from the gas-phase reactions of Criegee intermediates with hydroperoxide esters: mechanism and kinetics L. Chen et al. 10.5194/acp-22-14529-2022
- The simplest Criegee intermediate CH2OO reaction with dimethylamine and trimethylamine: kinetics and atmospheric implications Y. Chen et al. 10.1039/D3CP02948D
- Dynamics Insight into Isomerization and Dissociation of Hot Criegee Intermediate CH3CHOO Z. Wang et al. 10.1021/acs.jpca.8b11908
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- Reactions with criegee intermediates are the dominant gas-phase sink for formyl fluoride in the atmosphere Y. Xia et al. 10.1016/j.fmre.2023.02.012
- Study on ozonolysis of asymmetric alkenes with matrix isolation and FT-IR spectroscopy Z. Wang et al. 10.1016/j.chemosphere.2020.126413
- Effects of stabilized Criegee intermediates (sCIs) on sulfate formation: a sensitivity analysis during summertime in Beijing–Tianjin–Hebei (BTH), China L. Liu et al. 10.5194/acp-19-13341-2019
- Quantitative kinetics for the atmospheric reactions of Criegee intermediates with acetonitrile Y. Zhang et al. 10.1039/D2CP02849B
- An Extended Computational Study of Criegee Intermediate–Alcohol Reactions N. Watson et al. 10.1021/acs.jpca.8b09349
- Application of chemical derivatization techniques combined with chemical ionization mass spectrometry to detect stabilized Criegee intermediates and peroxy radicals in the gas phase A. Zaytsev et al. 10.5194/amt-14-2501-2021
- Unimolecular decay strongly limits the atmospheric impact of Criegee intermediates L. Vereecken et al. 10.1039/C7CP05541B
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- Reconciling Observed and Predicted Tropical Rainforest OH Concentrations D. Jeong et al. 10.1029/2020JD032901
- Criegee intermediates and their impacts on the troposphere M. Khan et al. 10.1039/C7EM00585G
- Nitrous acid (HONO) as a sink of the simplest Criegee intermediate in the atmosphere A. Kumar et al. 10.1039/D1CP03605J
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- Direct measurements of NO<sub>3</sub> reactivity in and above the boundary layer of a mountaintop site: identification of reactive trace gases and comparison with OH reactivity J. Liebmann et al. 10.5194/acp-18-12045-2018
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- Kinetics for the reaction of Criegee intermediate CH2OO with n-butyraldehyde and its atmospheric implications S. Liu et al. 10.1016/j.atmosenv.2023.120012
- Direct kinetic measurements and theoretical predictions of an isoprene-derived Criegee intermediate R. Caravan et al. 10.1073/pnas.1916711117
- Investigation of kinetics and mechanistic insights of the reaction of criegee intermediate (CH2OO) with methyl-ethyl ketone (MEK) under tropospherically relevant conditions A. Debnath & B. Rajakumar 10.1016/j.chemosphere.2022.137217
- Temperature-Dependent Rate Coefficient for the Reaction of CH3SH with the Simplest Criegee Intermediate Y. Li et al. 10.1021/acs.jpca.8b12553
- Measurements of a potential interference with laser-induced fluorescence measurements of ambient OH from the ozonolysis of biogenic alkenes P. Rickly & P. Stevens 10.5194/amt-11-1-2018
- Surprisingly long lifetime of methacrolein oxide, an isoprene derived Criegee intermediate, under humid conditions Y. Lin et al. 10.1038/s42004-021-00451-z
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- OH and HO<sub>2</sub> radical chemistry at a suburban site during the EXPLORE-YRD campaign in 2018 X. Ma et al. 10.5194/acp-22-7005-2022
- Criegee Intermediate–Alcohol Reactions, A Potential Source of Functionalized Hydroperoxides in the Atmosphere M. McGillen et al. 10.1021/acsearthspacechem.7b00108
- Atmospheric Kinetics: Bimolecular Reactions of Carbonyl Oxide by a Triple-Level Strategy B. Long et al. 10.1021/jacs.1c02029
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- A theoretical study of the addition of CH2OO to hydroxymethyl hydroperoxide and its implications on SO3 formation in the atmosphere R. Chow & D. Mok 10.1039/D0CP00961J
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- An Experimental and Master Equation Investigation of Kinetics of the CH2OO + RCN Reactions (R = H, CH3, C2H5) and Their Atmospheric Relevance L. Franzon et al. 10.1021/acs.jpca.2c07073
- Perspective on Mechanism Development and Structure‐Activity Relationships for Gas‐Phase Atmospheric Chemistry L. Vereecken et al. 10.1002/kin.21172
- Reactivity of Criegee Intermediates toward Carbon Dioxide Y. Lin et al. 10.1021/acs.jpclett.7b03154
- Kinetics of the simplest criegee intermediate CH2OO reacting with CF3CF=CF2 Y. Chen et al. 10.1063/1674-0068/cjcp2002025
- Kinetics of CH2OO and syn-CH3CHOO reaction with acrolein X. Zhou et al. 10.1039/D1CP00492A
- Sources, sinks, and chemistry of Stabilized Criegee Intermediates in the Indo-Gangetic Plain M. Shabin et al. 10.1016/j.scitotenv.2023.165281
- Re-examining ammonia addition to the Criegee intermediate: converging to chemical accuracy J. Misiewicz et al. 10.1039/C7CP08582F
- Kinetics of the reaction of the simplest Criegee intermediate with ammonia: a combination of experiment and theory Y. Liu et al. 10.1039/C8CP05920A
- The reaction of peroxy radicals with OH radicals C. Fittschen 10.1016/j.cplett.2019.04.002
- Unimolecular and water reactions of oxygenated and unsaturated Criegee intermediates under atmospheric conditions L. Vereecken et al. 10.1039/D1CP05877K
- Role of Criegee intermediates in the formation of sulfuric acid at a Mediterranean (Cape Corsica) site under influence of biogenic emissions A. Kukui et al. 10.5194/acp-21-13333-2021
4 citations as recorded by crossref.
- Detection and identification of Criegee intermediates from the ozonolysis of biogenic and anthropogenic VOCs: comparison between experimental measurements and theoretical calculations C. Giorio et al. 10.1039/C7FD00025A
- Significant OH production under surface cleaning and air cleaning conditions: Impact on indoor air quality N. Carslaw et al. 10.1111/ina.12394
- Reaction of SO2with OH in the atmosphere B. Long et al. 10.1039/C7CP00497D
- OH production from the photolysis of isoprene-derived peroxy radicals: cross-sections, quantum yields and atmospheric implications R. Hansen et al. 10.1039/C6CP06718B
Latest update: 26 Sep 2023
Short summary
The ambient concentration of stabilised Criegee intermediates (SCIs) was estimated for two
environments using field data. The low concentrations predicted indicate that SCIs are
unlikely to have a large impact on atmospheric chemistry. Concurrent measurements of an OH background signal using the Mainz IPI-LIF-FAGE instrument were found to be consistent with the chemistry of SCIs during the measurement campaigns.
The ambient concentration of stabilised Criegee intermediates (SCIs) was estimated for two...
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