Articles | Volume 17, issue 11
https://doi.org/10.5194/acp-17-6925-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Special issue:
https://doi.org/10.5194/acp-17-6925-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
13 Jun 2017
Research article |
| 13 Jun 2017
Multi-model study of mercury dispersion in the atmosphere: vertical and interhemispheric distribution of mercury species
Helmholtz Zentrum Geesthacht, 21052 Geesthacht, Germany
DLR – Deutsches Luft und Raumfahrtzentrum, Münchener Straße 20, 82234 Weßling, Germany
Franz Slemr
Max Planck Institute for Chemistry (MPI), Hahn-Meitner-Weg 1, 55128 Mainz, Germany
Jesse Ambrose
School of Science, Technology, Engineering and Mathematics, University of Washington-Bothell, Bothell, WA, USA
Carl Brenninkmeijer
Max Planck Institute for Chemistry (MPI), Hahn-Meitner-Weg 1, 55128 Mainz, Germany
Steve Brooks
Air Resources Laboratory, National Oceanic and Atmospheric Administration, 5830 University Research Court, College Park, MD 20740, USA
Department of Mechanical, Aerospace and Biomedical Engineering, University of Tennessee Space Institute, 411 BH Goethert Parkway, Tullahoma, TN 37388, USA
Ashu Dastoor
ECCC – Air Quality Research Division, Environment and Climate Change Canada, Dorval, Canada
Francesco DeSimone
CNR Institute of Atmospheric Pollution Research, Division of Rende, Rende, Italy
Ralf Ebinghaus
Helmholtz Zentrum Geesthacht, 21052 Geesthacht, Germany
Christian N. Gencarelli
CNR Institute of Atmospheric Pollution Research, Division of Rende, Rende, Italy
Beate Geyer
Helmholtz Zentrum Geesthacht, 21052 Geesthacht, Germany
Lynne E. Gratz
Environmental Program, Colorado College, Colorado Springs, CO, USA
Ian M. Hedgecock
CNR Institute of Atmospheric Pollution Research, Division of Rende, Rende, Italy
Daniel Jaffe
School of Science, Technology, Engineering and Mathematics, University of Washington-Bothell, Bothell, WA, USA
School of Science, Technology, Engineering and Mathematics, University of Washington-Bothell, Bothell, WA, USA
Paul Kelley
Air Resources Laboratory, National Oceanic and Atmospheric Administration, 5830 University Research Court, College Park, MD 20740, USA
Cooperative Institute for Climate and Satellites, University of Maryland, 5825 University Research Court, College Park, MD 20740, USA
Che-Jen Lin
Center for Advances in Water and Air Quality, Lamar University, Beaumont, Texas, USA
Lyatt Jaegle
University of Washington, Department of Atmospheric Sciences, Seattle, WA 98195, USA
Volker Matthias
Helmholtz Zentrum Geesthacht, 21052 Geesthacht, Germany
Andrei Ryjkov
ECCC – Air Quality Research Division, Environment and Climate Change Canada, Dorval, Canada
Noelle E. Selin
Department of Earth, Atmospheric and Planetary Sciences, Massachusetts Institute of Technology, Cambridge, MA, USA
Institute for Data, Systems, and Society, Massachusetts Institute of Technology, Cambridge, MA, USA
Shaojie Song
Department of Earth, Atmospheric and Planetary Sciences, Massachusetts Institute of Technology, Cambridge, MA, USA
Oleg Travnikov
Meteorological Synthesizing Centre – East of EMEP, Moscow, Russia
Andreas Weigelt
Helmholtz Zentrum Geesthacht, 21052 Geesthacht, Germany
Federal Maritime and Hydrographic Agency (BSH), Hamburg, Germany
Winston Luke
Air Resources Laboratory, National Oceanic and Atmospheric Administration, 5830 University Research Court, College Park, MD 20740, USA
Xinrong Ren
Air Resources Laboratory, National Oceanic and Atmospheric Administration, 5830 University Research Court, College Park, MD 20740, USA
Cooperative Institute for Climate and Satellites, University of Maryland, 5825 University Research Court, College Park, MD 20740, USA
Department of Earth, Ocean, and Atmospheric Science, Florida State University, 117 North Woodward Avenue, Tallahassee, FL 32306, USA
Andreas Zahn
Institut für Meteorologie und Klimaforschung (IMK-ASF), Karlsruhe Institut für Technologie, Hermann-von-Helmholtz-Platz 1, 76344 Leopoldshafen, Germany
Xin Yang
British Antarctic Survey, Cambridge, UK
Yun Zhu
South China University of Technology, School of Environment and Energy, Guangzhou, China
Nicola Pirrone
CNR Institute of Atmospheric Pollution Research, Rome, Italy
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Cited
24 citations as recorded by crossref.
- Photochemistry of oxidized Hg(I) and Hg(II) species suggests missing mercury oxidation in the troposphere A. Saiz-Lopez et al. 10.1073/pnas.1922486117
- Effects of temperature and relative humidity on the partitioning of atmospheric oxidized mercury at a high-altitude mountain background site in Taiwan L. Nguyen et al. 10.1016/j.atmosenv.2021.118572
- Impact of Athabasca oil sands operations on mercury levels in air and deposition A. Dastoor et al. 10.5194/acp-21-12783-2021
- Global Mercury Assimilation by Vegetation J. Zhou & D. Obrist 10.1021/acs.est.1c03530
- The first simultaneous and continuous underway measurements of atmospheric gaseous elemental mercury, carbon dioxide and methane in the marine boundary layer: Results of cruise study in the Sea of Japan in May 2018 V. Kalinchuk et al. 10.1016/j.apr.2022.101458
- Earth system modeling of mercury using CESM2 – Part 1: Atmospheric model CAM6-Chem/Hg v1.0 P. Zhang & Y. Zhang 10.5194/gmd-15-3587-2022
- The 3D biogeochemical marine mercury cycling model MERCY v2.0 – linking atmospheric Hg to methylmercury in fish J. Bieser et al. 10.5194/gmd-16-2649-2023
- Source contribution analysis of mercury deposition using an enhanced CALPUFF-Hg in the central Pearl River Delta, China H. Xu et al. 10.1016/j.envpol.2019.04.008
- Atmospheric Chemistry of Gaseous Oxidized Mercury at a Coastal Site in Atlantic Canada I. Cheng et al. 10.1175/JAS-D-19-0120.1
- Understanding mercury oxidation and air–snow exchange on the East Antarctic Plateau: a modeling study S. Song et al. 10.5194/acp-18-15825-2018
- Mercury distribution in the upper troposphere and lowermost stratosphere according to measurements by the IAGOS-CARIBIC observatory: 2014–2016 F. Slemr et al. 10.5194/acp-18-12329-2018
- Atmospheric Modelling of Mercury in the Southern Hemisphere and Future Research Needs: A Review J. Leiva González et al. 10.3390/atmos13081226
- Recent Advances in Atmospheric Chemistry of Mercury L. Si & P. Ariya 10.3390/atmos9020076
- Global evaluation and calibration of a passive air sampler for gaseous mercury D. McLagan et al. 10.5194/acp-18-5905-2018
- Toward an Understanding of Fundamentals Governing the Elemental Mercury Sequestration by Metal Chalcogenides Z. Yang et al. 10.1021/acs.est.0c02568
- Identifying and evaluating urban mercury emission sources through passive sampler-based mapping of atmospheric concentrations D. McLagan et al. 10.1088/1748-9326/aac8e6
- Trans-boundary movement of mercury in the Northeast Asian region predicted by CAMQ-Hg from anthropogenic emissions distribution J. Sung et al. 10.1016/j.atmosres.2017.12.015
- Assessment of Regional Mercury Deposition and Emission Outflow in Mainland China X. Wang et al. 10.1029/2018JD028350
- Unequal Anthropogenic Enrichment of Mercury in Earth’s Northern and Southern Hemispheres C. Li et al. 10.1021/acsearthspacechem.0c00220
- A vegetation control on seasonal variations in global atmospheric mercury concentrations M. Jiskra et al. 10.1038/s41561-018-0078-8
- Correction: Recent Advances in Atmospheric Chemistry of Mercury L. Si & P. Ariya 10.3390/atmos9060211
- Previously unaccounted atmospheric mercury deposition in a midlatitude deciduous forest D. Obrist et al. 10.1073/pnas.2105477118
- A new mechanism for atmospheric mercury redox chemistry: implications for the global mercury budget H. Horowitz et al. 10.5194/acp-17-6353-2017
- Sensitivity model study of regional mercury dispersion in the atmosphere C. Gencarelli et al. 10.5194/acp-17-627-2017
22 citations as recorded by crossref.
- Photochemistry of oxidized Hg(I) and Hg(II) species suggests missing mercury oxidation in the troposphere A. Saiz-Lopez et al. 10.1073/pnas.1922486117
- Effects of temperature and relative humidity on the partitioning of atmospheric oxidized mercury at a high-altitude mountain background site in Taiwan L. Nguyen et al. 10.1016/j.atmosenv.2021.118572
- Impact of Athabasca oil sands operations on mercury levels in air and deposition A. Dastoor et al. 10.5194/acp-21-12783-2021
- Global Mercury Assimilation by Vegetation J. Zhou & D. Obrist 10.1021/acs.est.1c03530
- The first simultaneous and continuous underway measurements of atmospheric gaseous elemental mercury, carbon dioxide and methane in the marine boundary layer: Results of cruise study in the Sea of Japan in May 2018 V. Kalinchuk et al. 10.1016/j.apr.2022.101458
- Earth system modeling of mercury using CESM2 – Part 1: Atmospheric model CAM6-Chem/Hg v1.0 P. Zhang & Y. Zhang 10.5194/gmd-15-3587-2022
- The 3D biogeochemical marine mercury cycling model MERCY v2.0 – linking atmospheric Hg to methylmercury in fish J. Bieser et al. 10.5194/gmd-16-2649-2023
- Source contribution analysis of mercury deposition using an enhanced CALPUFF-Hg in the central Pearl River Delta, China H. Xu et al. 10.1016/j.envpol.2019.04.008
- Atmospheric Chemistry of Gaseous Oxidized Mercury at a Coastal Site in Atlantic Canada I. Cheng et al. 10.1175/JAS-D-19-0120.1
- Understanding mercury oxidation and air–snow exchange on the East Antarctic Plateau: a modeling study S. Song et al. 10.5194/acp-18-15825-2018
- Mercury distribution in the upper troposphere and lowermost stratosphere according to measurements by the IAGOS-CARIBIC observatory: 2014–2016 F. Slemr et al. 10.5194/acp-18-12329-2018
- Atmospheric Modelling of Mercury in the Southern Hemisphere and Future Research Needs: A Review J. Leiva González et al. 10.3390/atmos13081226
- Recent Advances in Atmospheric Chemistry of Mercury L. Si & P. Ariya 10.3390/atmos9020076
- Global evaluation and calibration of a passive air sampler for gaseous mercury D. McLagan et al. 10.5194/acp-18-5905-2018
- Toward an Understanding of Fundamentals Governing the Elemental Mercury Sequestration by Metal Chalcogenides Z. Yang et al. 10.1021/acs.est.0c02568
- Identifying and evaluating urban mercury emission sources through passive sampler-based mapping of atmospheric concentrations D. McLagan et al. 10.1088/1748-9326/aac8e6
- Trans-boundary movement of mercury in the Northeast Asian region predicted by CAMQ-Hg from anthropogenic emissions distribution J. Sung et al. 10.1016/j.atmosres.2017.12.015
- Assessment of Regional Mercury Deposition and Emission Outflow in Mainland China X. Wang et al. 10.1029/2018JD028350
- Unequal Anthropogenic Enrichment of Mercury in Earth’s Northern and Southern Hemispheres C. Li et al. 10.1021/acsearthspacechem.0c00220
- A vegetation control on seasonal variations in global atmospheric mercury concentrations M. Jiskra et al. 10.1038/s41561-018-0078-8
- Correction: Recent Advances in Atmospheric Chemistry of Mercury L. Si & P. Ariya 10.3390/atmos9060211
- Previously unaccounted atmospheric mercury deposition in a midlatitude deciduous forest D. Obrist et al. 10.1073/pnas.2105477118
Latest update: 18 Apr 2024
Short summary
We conducted a multi model study to investigate our ability to reproduce the vertical distribution of mercury in the atmosphere. For this, we used observational data from over 40 aircraft flights in EU and US. We compared observations to the results of seven chemistry transport models and found that the models are able to reproduce vertical gradients of total and elemental Hg. Finally, we found that different chemical reactions seem responsible for the oxidation of Hg depending on altitude.
We conducted a multi model study to investigate our ability to reproduce the vertical...
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