Articles | Volume 17, issue 3
https://doi.org/10.5194/acp-17-1805-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-17-1805-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Differences in BVOC oxidation and SOA formation above and below the forest canopy
Benjamin C. Schulze
Department of Civil and Environmental Engineering, Rice University,
Houston, TX 77005, USA
Henry W. Wallace
Department of Civil and Environmental Engineering, Rice University,
Houston, TX 77005, USA
James H. Flynn
Department of Earth and Atmospheric
Sciences, University of Houston, Houston, TX 77204, USA
Barry L. Lefer
Airborne
Sciences Program, NASA, Washington, DC 20546, USA
Matt H. Erickson
Department of Earth and Atmospheric
Sciences, University of Houston, Houston, TX 77204, USA
B. Tom Jobson
Department of
Civil and Environmental Engineering, Laboratory for Atmospheric Research,
Washington State University, Pullman, WA 99164, USA
Sebastien Dusanter
Mines Douai, SAGE, 59508 Douai, France
Université de
Lille, 59655 Villeneuve d'Ascq, France
School of Public and Environmental Affairs, Indiana
University, Bloomington, IN 47405, USA
Stephen M. Griffith
School of Public and Environmental Affairs, Indiana
University, Bloomington, IN 47405, USA
now at: Department
of Chemistry, The Hong Kong University of Science and
Technology, Kowloon, Hong Kong
Robert F. Hansen
Department of Chemistry,
Indiana University, Bloomington, IN 47405, USA
now at: School of
Chemistry, University of Leeds, Leeds, LS2 9JT, UK
Philip S. Stevens
Department of Chemistry,
Indiana University, Bloomington, IN 47405, USA
Timothy VanReken
Department of
Civil and Environmental Engineering, Laboratory for Atmospheric Research,
Washington State University, Pullman, WA 99164, USA
now at:
National Science Foundation, Washington, DC 22230, USA
Robert J. Griffin
CORRESPONDING AUTHOR
Department of Civil and Environmental Engineering, Rice University,
Houston, TX 77005, USA
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Short summary
The atmospheric chemistry associated with mixing of anthropogenic and natural species was simulated to understand how shade provided by a forest canopy impacts reactions, product distribution, and subsequent phase distribution of the products. This is important to understand, as forested areas downwind of urban areas will be impacted by this phenomenon. It was found that fast transport from below the canopy led to increases in secondary organic aerosol from nitrate radicals above the canopy.
The atmospheric chemistry associated with mixing of anthropogenic and natural species was...
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