Articles | Volume 17, issue 20
https://doi.org/10.5194/acp-17-12361-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Special issue:
https://doi.org/10.5194/acp-17-12361-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
17 Oct 2017
Research article |
| 17 Oct 2017
Fast heterogeneous N2O5 uptake and ClNO2 production in power plant and industrial plumes observed in the nocturnal residual layer over the North China Plain
Department of Civil and Environmental Engineering, The Hong Kong Polytechnic University, Hong Kong, China
Weihao Wang
Department of Civil and Environmental Engineering, The Hong Kong Polytechnic University, Hong Kong, China
Yee Jun Tham
Department of Civil and Environmental Engineering, The Hong Kong Polytechnic University, Hong Kong, China
now at: Department of Physics, University of Helsinki, Helsinki, Finland
Department of Civil and Environmental Engineering, The Hong Kong Polytechnic University, Hong Kong, China
Hao Wang
Environment Research Institute, Shandong University, Jinan, China
Liang Wen
Environment Research Institute, Shandong University, Jinan, China
Xinfeng Wang
Environment Research Institute, Shandong University, Jinan, China
Department of Civil and Environmental Engineering, The Hong Kong Polytechnic University, Hong Kong, China
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Latest update: 14 Dec 2024
Short summary
This work addresses unclear roles of heterogeneous N2O5 reactions and chlorine activation processes in the polluted residual layer from a mountaintop measurement in northern China. The results revealed efficient ClNO2 production in the coal-fired plumes in this region, having large impacts on next-morning photochemistry. Fast heterogeneous N2O5 reactions dominate the nocturnal NOx loss and contribute to substantial nitrate formation, which may boost the haze pollution in northern China.
This work addresses unclear roles of heterogeneous N2O5 reactions and chlorine activation...
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