Articles | Volume 16, issue 8
https://doi.org/10.5194/acp-16-5357-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-16-5357-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
29 Apr 2016
Research article |
| 29 Apr 2016
Seasonal variability of PM2.5 composition and sources in the Klang Valley urban-industrial environment
Norhaniza Amil
School of Environmental and Natural Resource Sciences,
Faculty of Science and Technology, Universiti Kebangsaan Malaysia, 43600
Bangi, Selangor, Malaysia
School of Industrial Technology (Environmental Division),
Universiti Sains Malaysia, 11800 Penang, Malaysia
School of Environmental and Natural Resource Sciences,
Faculty of Science and Technology, Universiti Kebangsaan Malaysia, 43600
Bangi, Selangor, Malaysia
Institute for Environmental and Development (LESTARI),
Universiti Kebangsaan Malaysia, 43600 Bangi, Selangor,
Malaysia
Md Firoz Khan
Centre for Tropical Climate Change System (IKLIM),
Institute of Climate Change, Universiti Kebangsaan Malaysia, 43600 Bangi,
Selangor, Malaysia
Maznorizan Mohamad
Malaysian Meteorological Department, Jalan Sultan, 46667 Petaling Jaya,
Selangor, Malaysia
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Daan Hubert, Klaus-Peter Heue, Jean-Christopher Lambert, Tijl Verhoelst, Marc Allaart, Steven Compernolle, Patrick D. Cullis, Angelika Dehn, Christian Félix, Bryan J. Johnson, Arno Keppens, Debra E. Kollonige, Christophe Lerot, Diego Loyola, Matakite Maata, Sukarni Mitro, Maznorizan Mohamad, Ankie Piters, Fabian Romahn, Henry B. Selkirk, Francisco R. da Silva, Ryan M. Stauffer, Anne M. Thompson, J. Pepijn Veefkind, Holger Vömel, Jacquelyn C. Witte, and Claus Zehner
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M. F. Khan, M. T. Latif, W. H. Saw, N. Amil, M. S. M. Nadzir, M. Sahani, N. M. Tahir, and J. X. Chung
Atmos. Chem. Phys., 16, 597–617, https://doi.org/10.5194/acp-16-597-2016, https://doi.org/10.5194/acp-16-597-2016, 2016
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Trans-boundary haze pollution is a major health and environmental concern during south-west and north-east monsoon in the South East Asian regions. The concentration of PM2.5 exceeds the tolerable limits (WHO; USA EPA) during the summer monsoon. The novelty of this study is the source characterization of PM2.5 and source-specific risk assessment during intense haze pollution, which are yet to be addressed in this region. The outcomes of this study will give an insight about future implications.
Y. Fujii, S. Tohno, N. Amil, M. T. Latif, M. Oda, J. Matsumoto, and A. Mizohata
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Related subject area
Subject: Aerosols | Research Activity: Field Measurements | Altitude Range: Troposphere | Science Focus: Chemistry (chemical composition and reactions)
Marine organic aerosol at Mace Head: effects from phytoplankton and source region variability
Measurement report: Sources and meteorology influencing highly time-resolved PM2.5 trace elements at three urban sites in the extremely polluted Indo-Gangetic Plain in India
Formation of highly absorptive secondary brown carbon through nighttime multiphase chemistry of biomass burning emissions
Measurement report: Vertically resolved atmospheric properties observed over the Southern Great Plains with the ArcticShark uncrewed aerial system
Non-biogenic sources are an important but overlooked contributor to aerosol isoprene-derived organosulfates during winter in northern China
The critical role of aqueous-phase processes in aromatic-derived nitrogen-containing organic aerosol formation in cities with different energy consumption patterns
Characterization of atmospheric water-soluble brown carbon in the Athabasca oil sands region, Canada
Sensitivity of aerosol and cloud properties to coupling strength of marine boundary layer clouds over the northwest Atlantic
Burning conditions and transportation pathways determine biomass-burning aerosol properties in the Ascension Island marine boundary layer
Observations of high-time-resolution and size-resolved aerosol chemical composition and microphysics in the central Arctic: implications for climate-relevant particle properties
Measurement report: Brown carbon aerosol in rural Germany – sources, chemistry, and diurnal variations
Multiple eco-regions contribute to the seasonal cycle of Antarctic aerosol size distributions
Seasonal investigation of ultrafine-particle organic composition in an eastern Amazonian rainforest
High-resolution analyses of concentrations and sizes of refractory black carbon particles deposited in northwestern Greenland over the past 350 years – Part 2: Seasonal and temporal trends in refractory black carbon originated from fossil fuel combustion and biomass burning
Direct measurement of N2O5 heterogeneous uptake coefficients on atmospheric aerosols in southwestern China and evaluation of current parameterizations
Measurement report: Per- and polyfluoroalkyl substances (PFAS) in particulate matter (PM10) from activated sludge aeration
Significant role of biomass burning in heavy haze formation in Nanjing, a megacity in China: molecular-level insights from intensive PM2.5 sampling on winter hazy days
Widespread trace bromine and iodine in remote tropospheric non-sea-salt aerosols
Significant contributions of biomass burning to PM2.5-bound aromatic compounds: insights from field observations and quantum chemical calculations
A 60-year atmospheric nitrate isotope record from a Southeast Greenland ice core with minimal post-depositional alteration
Iron isotopes reveal significant aerosol dissolution over the Pacific Ocean
Formation and chemical evolution of secondary organic aerosol in two different environments: a dual-chamber study
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Measurement report: Oxidation potential of water-soluble aerosol components in the south and north of Beijing
Enhanced daytime secondary aerosol formation driven by gas–particle partitioning in downwind urban plumes
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Understanding the mechanism and importance of brown carbon bleaching across the visible spectrum in biomass burning plumes from the WE-CAN campaign
Influence of terrestrial and marine air mass on the constituents and intermixing of bioaerosols over a coastal atmosphere
A multi-site passive approach to studying the emissions and evolution of smoke from prescribed fires
The annual cycle and sources of relevant aerosol precursor vapors in the central Arctic during the MOSAiC expedition
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African dust transported to Barbados in the Wintertime Lacks Indicators of Chemical Aging
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Machine Learning Assisted Chemical Characterization and Optical Properties of Atmospheric Brown Carbon in Nanjing, China
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Long-range transport of air pollutants increases the concentration of hazardous components of PM2.5 in northern South America
Molecular characterization of organic aerosols in urban and forested areas of Paris using high resolution mass spectrometry
Dominant influence of biomass combustion and cross-border transport on nitrogen-containing organic compound levels in the southeastern Tibetan Plateau
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Impacts of elevated anthropogenic emissions on physicochemical characteristics of black-carbon-containing particles over the Tibetan Plateau
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Atmospheric evolution of environmentally persistent free radicals in the rural North China Plain: effects on water solubility and PM2.5 oxidative potential
Measurement report: Characterization of Aerosol Hygroscopicity over Southeast Asia during the NASA CAMP2Ex Campaign
Two distinct ship emission profiles for organic-sulfate source apportionment of PM in sulfur emission control areas
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Automated compound speciation, cluster analysis, and quantification of organic vapors and aerosols using comprehensive two-dimensional gas chromatography and mass spectrometry
Measurement report: Occurrence of aminiums in PM2.5 during winter in China – aminium outbreak during polluted episodes and potential constraints
Bridging gas and aerosol properties between the northeastern US and Bermuda: analysis of eight transit flights
The behaviour of charged particles (ions) during new particle formation events in urban Leipzig, Germany
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This study presents the first source apportionment of organic aerosol at Mace Head via high-resolution mass spectrometry. Introducing transfer entropy as a novel method reveals that aged organic aerosol originates from both open-ocean ozonolysis and local peat-burning oxidation. Methanesulfonic acid and organic sea spray both mirror phytoplankton activity, with the former closely tied to coccolithophore blooms and the latter linked to diatoms, chlorophytes, and cyanobacteria.
Ashutosh K. Shukla, Sachchida N. Tripathi, Shamitaksha Talukdar, Vishnu Murari, Sreenivas Gaddamidi, Manousos-Ioannis Manousakas, Vipul Lalchandani, Kuldeep Dixit, Vinayak M. Ruge, Peeyush Khare, Mayank Kumar, Vikram Singh, Neeraj Rastogi, Suresh Tiwari, Atul K. Srivastava, Dilip Ganguly, Kaspar Rudolf Daellenbach, and André S. H. Prévôt
Atmos. Chem. Phys., 25, 3765–3784, https://doi.org/10.5194/acp-25-3765-2025, https://doi.org/10.5194/acp-25-3765-2025, 2025
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Our study delves into the elemental composition of aerosols at three sites across the Indo-Gangetic Plain (IGP), revealing distinct patterns during pollution episodes. We found significant increases in chlorine (Cl)-rich and solid fuel combustion (SFC) sources, indicating dynamic emission sources, agricultural burning impacts, and meteorological influences. Surges in Cl-rich particles during cold periods highlight their role in particle growth under high-relative-humidity conditions.
Ye Kuang, Biao Luo, Shan Huang, Junwen Liu, Weiwei Hu, Yuwen Peng, Duohong Chen, Dingli Yue, Wanyun Xu, Bin Yuan, and Min Shao
Atmos. Chem. Phys., 25, 3737–3752, https://doi.org/10.5194/acp-25-3737-2025, https://doi.org/10.5194/acp-25-3737-2025, 2025
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This research reveals the potential importance of nighttime NO3 radical chemistry and aerosol water in the rapid formation of secondary brown carbon from diluted biomass burning emissions. The findings enhance our understanding of nighttime biomass burning evolution and its implications for climate and regional air quality, especially regarding interactions with background aerosol water and water-rich fogs and clouds.
Fan Mei, Qi Zhang, Damao Zhang, Jerome D. Fast, Gourihar Kulkarni, Mikhail S. Pekour, Christopher R. Niedek, Susanne Glienke, Israel Silber, Beat Schmid, Jason M. Tomlinson, Hardeep S. Mehta, Xena Mansoura, Zezhen Cheng, Gregory W. Vandergrift, Nurun Nahar Lata, Swarup China, and Zihua Zhu
Atmos. Chem. Phys., 25, 3425–3444, https://doi.org/10.5194/acp-25-3425-2025, https://doi.org/10.5194/acp-25-3425-2025, 2025
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This study highlights the unique capability of the ArcticShark, an uncrewed aerial system, in measuring vertically resolved atmospheric properties. Data from 32 research flights in 2023 reveal seasonal patterns and correlations with conventional measurements. The consistency and complementarity of in situ and remote sensing methods are highlighted. The study demonstrates the ArcticShark’s versatility in bridging data gaps and improving the understanding of vertical atmospheric structures.
Ting Yang, Yu Xu, Yu-Chen Wang, Yi-Jia Ma, Hong-Wei Xiao, Hao Xiao, and Hua-Yun Xiao
Atmos. Chem. Phys., 25, 2967–2978, https://doi.org/10.5194/acp-25-2967-2025, https://doi.org/10.5194/acp-25-2967-2025, 2025
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Previous measurement–model comparisons of atmospheric isoprene levels showed a significant unidentified source of isoprene in some northern Chinese cities during winter. Here, the first combination of large-scale observations and field combustion experiments provides novel insights into biomass burning emissions as a significant source of isoprene-derived organosulfates during winter in northern cities of China.
Yi-Jia Ma, Yu Xu, Ting Yang, Lin Gui, Hong-Wei Xiao, Hao Xiao, and Hua-Yun Xiao
Atmos. Chem. Phys., 25, 2763–2780, https://doi.org/10.5194/acp-25-2763-2025, https://doi.org/10.5194/acp-25-2763-2025, 2025
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The abundance, potential precursors, and main formation mechanisms of nitrogen-containing organic compounds (NOCs) in PM2.5 during winter were compared among cities with different energy consumption patterns. The aerosol NOC pollution during winter in China is closely associated with the intensity of precursor emissions and the aqueous-phase processes. Our results highlight the importance of emission reduction strategies in controlling aerosol NOCs pollution during winter in China.
Dane Blanchard, Mark Gordon, Duc Huy Dang, Paul Andrew Makar, and Julian Aherne
Atmos. Chem. Phys., 25, 2423–2442, https://doi.org/10.5194/acp-25-2423-2025, https://doi.org/10.5194/acp-25-2423-2025, 2025
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This study offers the first known evaluation of water-soluble brown carbon aerosols in the Athabasca oil sands region (AOSR), Canada. Fluorescence spectroscopy analysis of aerosol samples from five regional sites (collected during the summer of 2021) identified oil sands operations as a measurable brown carbon source. Industrial aerosol emissions were unlikely to impact regional radiative forcing. These findings show that fluorescence spectroscopy can be used to monitor brown carbon in the AOSR.
Kira Zeider, Kayla McCauley, Sanja Dmitrovic, Leong Wai Siu, Yonghoon Choi, Ewan C. Crosbie, Joshua P. DiGangi, Glenn S. Diskin, Simon Kirschler, John B. Nowak, Michael A. Shook, Kenneth L. Thornhill, Christiane Voigt, Edward L. Winstead, Luke D. Ziemba, Paquita Zuidema, and Armin Sorooshian
Atmos. Chem. Phys., 25, 2407–2422, https://doi.org/10.5194/acp-25-2407-2025, https://doi.org/10.5194/acp-25-2407-2025, 2025
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In situ aircraft data collected over the northwest Atlantic Ocean are utilized to compare aerosol conditions and turbulence between near-surface and below-cloud-base altitudes for different regimes of coupling strength between those two levels, along with how cloud microphysical properties vary across those regimes. Stronger coupling yields more homogenous aerosol structure vertically along with higher cloud drop concentrations and sea salt influence in clouds.
Amie Dobracki, Ernie R. Lewis, Arthur J. Sedlacek III, Tyler Tatro, Maria A. Zawadowicz, and Paquita Zuidema
Atmos. Chem. Phys., 25, 2333–2363, https://doi.org/10.5194/acp-25-2333-2025, https://doi.org/10.5194/acp-25-2333-2025, 2025
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Biomass-burning aerosol is commonly present in the marine boundary layer over the southeast Atlantic Ocean between June and October. Our research indicates that burning conditions, aerosol transport pathways, and prolonged oxidation processes (heterogeneous and aqueous phases) determine the chemical, microphysical, and optical properties of the boundary layer aerosol. Notably, we find that the aerosol optical properties can be estimated from the chemical properties alone.
Benjamin Heutte, Nora Bergner, Hélène Angot, Jakob B. Pernov, Lubna Dada, Jessica A. Mirrielees, Ivo Beck, Andrea Baccarini, Matthew Boyer, Jessie M. Creamean, Kaspar R. Daellenbach, Imad El Haddad, Markus M. Frey, Silvia Henning, Tiia Laurila, Vaios Moschos, Tuukka Petäjä, Kerri A. Pratt, Lauriane L. J. Quéléver, Matthew D. Shupe, Paul Zieger, Tuija Jokinen, and Julia Schmale
Atmos. Chem. Phys., 25, 2207–2241, https://doi.org/10.5194/acp-25-2207-2025, https://doi.org/10.5194/acp-25-2207-2025, 2025
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Limited aerosol measurements in the central Arctic hinder our understanding of aerosol–climate interactions in the region. Our year-long observations of aerosol physicochemical properties during the MOSAiC expedition reveal strong seasonal variations in aerosol chemical composition, where the short-term variability is heavily affected by storms in the Arctic. Local wind-generated particles are shown to be an important source of cloud seeds, especially in autumn.
Feng Jiang, Harald Saathoff, Uzoamaka Ezenobi, Junwei Song, Hengheng Zhang, Linyu Gao, and Thomas Leisner
Atmos. Chem. Phys., 25, 1917–1930, https://doi.org/10.5194/acp-25-1917-2025, https://doi.org/10.5194/acp-25-1917-2025, 2025
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The chemical composition of brown carbon in the particle and gas phase was determined by mass spectrometry. BrC in the gas phase was mainly controlled by secondary formation and particle-to-gas partitioning. BrC in the particle phase was mainly from secondary formation. This work helps to get a better understanding of diurnal variations and the sources of brown carbon aerosol at a rural location in central Europe.
James Brean, David C. S. Beddows, Eija Asmi, Aki Virkkula, Lauriane L. J. Quéléver, Mikko Sipilä, Floortje Van Den Heuvel, Thomas Lachlan-Cope, Anna Jones, Markus Frey, Angelo Lupi, Jiyeon Park, Young Jun Yoon, Rolf Weller, Giselle L. Marincovich, Gabriela C. Mulena, Roy M. Harrison, and Manuel Dall'Osto
Atmos. Chem. Phys., 25, 1145–1162, https://doi.org/10.5194/acp-25-1145-2025, https://doi.org/10.5194/acp-25-1145-2025, 2025
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Our results emphasise how understanding the geographical variation in surface types across the Antarctic is key to understanding secondary aerosol sources.
Adam E. Thomas, Hayley S. Glicker, Alex B. Guenther, Roger Seco, Oscar Vega Bustillos, Julio Tota, Rodrigo A. F. Souza, and James N. Smith
Atmos. Chem. Phys., 25, 959–977, https://doi.org/10.5194/acp-25-959-2025, https://doi.org/10.5194/acp-25-959-2025, 2025
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We present measurements of the organic composition of ultrafine particles collected from the eastern Amazon, an understudied region that is subjected to increasing human influence. We find that while isoprene chemistry is likely significant for ultrafine-particle growth throughout the year, compounds related to other sources, such as biological-spore emissions and biomass burning, exhibit striking seasonal differences, implying extensive variation in regional ultrafine-particle sources.
Kumiko Goto-Azuma, Yoshimi Ogawa-Tsukagawa, Kaori Fukuda, Koji Fujita, Motohiro Hirabayashi, Remi Dallmayr, Jun Ogata, Nobuhiro Moteki, Tatsuhiro Mori, Sho Ohata, Yutaka Kondo, Makoto Koike, Sumito Matoba, Moe Kadota, Akane Tsushima, Naoko Nagatsuka, and Teruo Aoki
Atmos. Chem. Phys., 25, 657–683, https://doi.org/10.5194/acp-25-657-2025, https://doi.org/10.5194/acp-25-657-2025, 2025
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Monthly ice core records spanning 350 years from Greenland show trends in refractory black carbon (rBC) concentrations and sizes. rBC levels have increased since the 1870s due to the inflow of anthropogenic rBC, with larger diameters than those from biomass burning (BB) rBC. High summer BB rBC peaks may reduce the ice sheet albedo, but BB rBC showed no increase until the early 2000s. These results are vital for validating aerosol and climate models.
Jiayin Li, Tianyu Zhai, Xiaorui Chen, Haichao Wang, Shuyang Xie, Shiyi Chen, Chunmeng Li, Huabin Dong, and Keding Lu
EGUsphere, https://doi.org/10.5194/egusphere-2024-3804, https://doi.org/10.5194/egusphere-2024-3804, 2025
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We directly measured the dinitrogen pentoxide (N2O5) uptake coefficient which critical impact the NOx fate and particulate nitrate formation in a typical highland city, Kunming, in China. We found the performance of current γ(N2O5) parameterizations showed deviations with the varying aerosol liquid water content (ALWC). Such differences would lead to biased estimation on particulate nitrate production potential. Our findings suggest the directions for future studies.
Jishnu Pandamkulangara Kizhakkethil, Zongbo Shi, Anna Bogush, and Ivan Kourtchev
EGUsphere, https://doi.org/10.5194/egusphere-2024-3952, https://doi.org/10.5194/egusphere-2024-3952, 2025
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Pollution with per- and polyfluoroalkyl substances (PFAS) received attention due to their environmental persistence and bioaccumulation. PM10 collected above a scaled-down activated sludge tank treating domestic sewage for a population >10,000 people in the UK were analysed for a range of short-, medium- and long-chain PFAS. Eight PFAS were detected in the PM10. Our results suggest that wastewater treatment processes i.e. activated sludge aeration could aerosolise PFAS into airborne PM.
Mingjie Kang, Mengying Bao, Wenhuai Song, Aduburexiati Abulimiti, Changliu Wu, Fang Cao, Sönke Szidat, and Yanlin Zhang
Atmos. Chem. Phys., 25, 73–91, https://doi.org/10.5194/acp-25-73-2025, https://doi.org/10.5194/acp-25-73-2025, 2025
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Reports on molecular-level knowledge of high-temporal-resolution particulate matter ≤2.5 µm in diameter (PM2.5) on hazy days are limited. We investigated various PM2.5 species and their sources. The results show biomass burning (BB) was the main source of organic carbon. Moreover, BB enhanced fungal spore emissions and secondary aerosol formation. The contribution of non-fossil sources increased with increasing haze pollution, suggesting BB may be an important driver of haze events in winter.
Gregory P. Schill, Karl D. Froyd, Daniel M. Murphy, Christina J. Williamson, Charles A. Brock, Tomás Sherwen, Mat J. Evans, Eric A. Ray, Eric C. Apel, Rebecca S. Hornbrook, Alan J. Hills, Jeff Peischl, Thomas B. Ryerson, Chelsea R. Thompson, Ilann Bourgeois, Donald R. Blake, Joshua P. DiGangi, and Glenn S. Diskin
Atmos. Chem. Phys., 25, 45–71, https://doi.org/10.5194/acp-25-45-2025, https://doi.org/10.5194/acp-25-45-2025, 2025
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Using single-particle mass spectrometry, we show that trace concentrations of bromine and iodine are ubiquitous in remote tropospheric aerosol and suggest that aerosols are an important part of the global reactive iodine budget. Comparisons to a global climate model with detailed iodine chemistry are favorable in the background atmosphere; however, the model cannot replicate our measurements near the ocean surface, in biomass burning plumes, and in the stratosphere.
Yanqin Ren, Zhenhai Wu, Fang Bi, Hong Li, Haijie Zhang, Junling Li, Rui Gao, Fangyun Long, Zhengyang Liu, Yuanyuan Ji, and Gehui Wang
EGUsphere, https://doi.org/10.5194/egusphere-2024-3678, https://doi.org/10.5194/egusphere-2024-3678, 2025
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The daily concentrations of Polycyclic aromatic hydrocarbons (PAHs), oxygenated PAHs (OPAHs), and nitrated phenols (NPs) in PM2.5 were all increased during the heating season. Biomass burning was identified to be the primary source of these aromatic compounds, particularly for PAHs. Phenol and nitrobenzene are two main primary precursors for 4NP, with phenol showing lower reaction barriers. P-Cresol was identified as the primary precursor for the formation of 4-methyl-5-nitrocatechol.
Zhao Wei, Shohei Hattori, Asuka Tsuruta, Zhuang Jiang, Sakiko Ishino, Koji Fujita, Sumito Matoba, Lei Geng, Alexis Lamothe, Ryu Uemura, Naohiro Yoshida, Joel Savarino, and Yoshinori Iizuka
EGUsphere, https://doi.org/10.5194/egusphere-2024-3937, https://doi.org/10.5194/egusphere-2024-3937, 2024
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Nitrate isotope records in ice cores reveal changes in NOₓ emissions, atmospheric acidity, and oxidation chemistry driven by human activity. However, nitrate in snow can be altered by UV-driven post-depositional processes, making snow accumulation rates critical for preserving these records. This study examines nitrate isotopes in an SE-Dome ice core, where high snow accumulation minimizes these effects, providing a reliable archive of atmospheric nitrogen cycling.
Capucine Camin, François Lacan, Catherine Pradoux, Marie Labatut, Anne Johansen, and James W. Murray
EGUsphere, https://doi.org/10.5194/egusphere-2024-3777, https://doi.org/10.5194/egusphere-2024-3777, 2024
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This manuscript presents the chemical composition of aerosols (> 1µm) over the Equatorial and Tropical Pacific Ocean, presenting the first measurements of iron isotopes in aerosols from this region. Iron concentrations and isotopes were determined using a Neptune MC-ICPMS. Our data analysis reveals that a significant portion of the aerosols undergo dissolution and removal during atmospheric transport. These findings contribute to original conclusions about the chemistry and physics of aerosols.
Andreas Aktypis, Dontavious J. Sippial, Christina N. Vasilakopoulou, Angeliki Matrali, Christos Kaltsonoudis, Andrea Simonati, Marco Paglione, Matteo Rinaldi, Stefano Decesari, and Spyros N. Pandis
Atmos. Chem. Phys., 24, 13769–13791, https://doi.org/10.5194/acp-24-13769-2024, https://doi.org/10.5194/acp-24-13769-2024, 2024
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A dual-chamber system was deployed in two different environments (Po Valley, Italy, and Pertouli forest, Greece) to study the potential of ambient air directly injected into the chambers, to form secondary organic aerosol (SOA). In the Po Valley, the system reacts rapidly, forming large amounts of SOA, while in Pertouli the SOA formation chemistry appears to have been practically terminated before the beginning of most experiments, so there is little additional SOA formation potential left.
Jie Zhang, Tianyu Zhu, Alexandra Catena, Yaowei Li, Margaret J. Schwab, Pengfei Liu, Akua Asa-Awuku, and James Schwab
Atmos. Chem. Phys., 24, 13445–13456, https://doi.org/10.5194/acp-24-13445-2024, https://doi.org/10.5194/acp-24-13445-2024, 2024
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This study shows the derived organic aerosol hygroscopicity under high-humidity conditions based on a simple optical scatter monitor system, including two nephelometric monitors (pDR-1500), when the aerosol chemical composition is already known.
Wei Yuan, Ru-Jin Huang, Chao Luo, Lu Yang, Wenjuan Cao, Jie Guo, and Huinan Yang
Atmos. Chem. Phys., 24, 13219–13230, https://doi.org/10.5194/acp-24-13219-2024, https://doi.org/10.5194/acp-24-13219-2024, 2024
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We characterized water-soluble oxidative potential (OP) levels in wintertime PM2.5 in the south and north of Beijing. Our results show that the volume-normalized dithiothreitol (DTTv) in the north was comparable to that in the south, while the mass-normalized dithiothreitol (DTTm) in the north was almost twice that in the south. Traffic-related emissions and biomass burning were the main sources of DTTv in the south, and traffic-related emissions contributed the most to DTTv in the north.
Mingfu Cai, Chenshuo Ye, Bin Yuan, Shan Huang, E Zheng, Suxia Yang, Zelong Wang, Yi Lin, Tiange Li, Weiwei Hu, Wei Chen, Qicong Song, Wei Li, Yuwen Peng, Baoling Liang, Qibin Sun, Jun Zhao, Duohong Chen, Jiaren Sun, Zhiyong Yang, and Min Shao
Atmos. Chem. Phys., 24, 13065–13079, https://doi.org/10.5194/acp-24-13065-2024, https://doi.org/10.5194/acp-24-13065-2024, 2024
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This study investigated the daytime secondary organic aerosol (SOA) formation in urban plumes. We observed a significant daytime SOA formation through gas–particle partitioning when the site was affected by urban plumes. A box model simulation indicated that urban pollutants (nitrogen oxide and volatile organic compounds) could enhance the oxidizing capacity, while the elevated volatile organic compounds were mainly responsible for promoting daytime SOA formation.
Qingxiao Meng, Yunjiang Zhang, Sheng Zhong, Jie Fang, Lili Tang, Yongcai Rao, Minfeng Zhou, Jian Qiu, Xiaofeng Xu, Jean-Eudes Petit, Olivier Favez, and Xinlei Ge
EGUsphere, https://doi.org/10.5194/egusphere-2024-2776, https://doi.org/10.5194/egusphere-2024-2776, 2024
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We developed a new method to reconstruct missing elemental carbon (EC) data in four Chinese cities from 2013 to 2023. Using machine learning, we accurately filled data gaps and introduced a new approach to analyze EC trends. Our findings reveal a significant decline in EC due to stricter pollution controls, though this slowed after 2020. This study provides a versatile framework for addressing data gaps and supports strategies to reduce urban air pollution and its climate impacts.
Yingjie Shen, Rudra P. Pokhrel, Amy P. Sullivan, Ezra J. T. Levin, Lauren A. Garofalo, Delphine K. Farmer, Wade Permar, Lu Hu, Darin W. Toohey, Teresa Campos, Emily V. Fischer, and Shane M. Murphy
Atmos. Chem. Phys., 24, 12881–12901, https://doi.org/10.5194/acp-24-12881-2024, https://doi.org/10.5194/acp-24-12881-2024, 2024
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The magnitude and evolution of brown carbon (BrC) absorption remain unclear, with uncertainty in climate models. Data from the WE-CAN airborne experiment show that model parameterizations overestimate the mass absorption cross section (MAC) of BrC. Observed decreases in BrC absorption with chemical markers are due to decreasing organic aerosol (OA) mass rather than a decreasing BrC MAC, which is currently implemented in models. Water-soluble BrC contributes 23 % of total absorption at 660 nm.
Qun He, Zhaowen Wang, Houfeng Liu, Pengju Xu, Rongbao Duan, Caihong Xu, Jianmin Chen, and Min Wei
Atmos. Chem. Phys., 24, 12775–12792, https://doi.org/10.5194/acp-24-12775-2024, https://doi.org/10.5194/acp-24-12775-2024, 2024
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Coastal environments provide an ideal setting for investigating the intermixing of terrestrial and marine aerosols. Terrestrial air mass constituted a larger number of microbes from anthropogenic and soil emissions, whereas saprophytic and gut microbes were predominant in marine samples. Mixed air masses indicated a fusion of marine and terrestrial aerosols, characterized by alterations in the ratio of pathogenic and saprophytic microbes when compared to either terrestrial or marine samples.
Rime El Asmar, Zongrun Li, David J. Tanner, Yongtao Hu, Susan O'Neill, L. Gregory Huey, M. Talat Odman, and Rodney J. Weber
Atmos. Chem. Phys., 24, 12749–12773, https://doi.org/10.5194/acp-24-12749-2024, https://doi.org/10.5194/acp-24-12749-2024, 2024
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Prescribed burning is an important method for managing ecosystems and preventing wildfires. However, smoke from prescribed fires can have a significant impact on air quality. Here, using a network of fixed sites and sampling throughout an extended prescribed burning period in 2 different years, we characterize emissions and evolutions of up to 8 h of PM2.5 mass, black carbon (BC), and brown carbon (BrC) in smoke from burning of forested lands in the southeastern USA.
Matthew Boyer, Diego Aliaga, Lauriane L. J. Quéléver, Silvia Bucci, Hélène Angot, Lubna Dada, Benjamin Heutte, Lisa Beck, Marina Duetsch, Andreas Stohl, Ivo Beck, Tiia Laurila, Nina Sarnela, Roseline C. Thakur, Branka Miljevic, Markku Kulmala, Tuukka Petäjä, Mikko Sipilä, Julia Schmale, and Tuija Jokinen
Atmos. Chem. Phys., 24, 12595–12621, https://doi.org/10.5194/acp-24-12595-2024, https://doi.org/10.5194/acp-24-12595-2024, 2024
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We analyze the seasonal cycle and sources of gases that are relevant for the formation of aerosol particles in the central Arctic. Since theses gases can form new particles, they can influence Arctic climate. We show that the sources of these gases are associated with changes in the Arctic environment during the year, especially with respect to sea ice. Therefore, the concentration of these gases will likely change in the future as the Arctic continues to warm.
Binyu Xiao, Fan Zhang, Zeyu Liu, Yan Zhang, Rui Li, Can Wu, Xinyi Wan, Yi Wang, Yubao Chen, Yong Han, Min Cui, Libo Zhang, Yingjun Chen, and Gehui Wang
EGUsphere, https://doi.org/10.5194/egusphere-2024-3433, https://doi.org/10.5194/egusphere-2024-3433, 2024
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Intermediate/semi-volatile organic compounds in both gas and particle phases from ship exhausts are enhanced due to the switch of fuels from low-sulfur to ultra-low-sulfur. The findings indicate that optimization is necessary for the forthcoming global implementation of an ultra-low-sulfur oil policy. Besides, we find that organic diagnostic markers of hopanes, in conjunction with the ratio of octadecanoic to tetradecanoic could be considered as potential tracers for HFO exhausts.
Hongyu Zhang, Shenbo Wang, Zhangsen Dong, Xiao Li, and Ruiqin Zhang
EGUsphere, https://doi.org/10.5194/egusphere-2024-2869, https://doi.org/10.5194/egusphere-2024-2869, 2024
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To address this, 12-year observational data in Zhengzhou were investigated and revealed that the resuspension of surrounding soil dust determined the rebound of crustal material concentrations after 2019, further elevating the particle pH. Therefore, the future ammonia reduction policies in North China may not lead to a rapid increase in particle acidity buffering by the crustal materials, but it is necessary to consider synergistic control with dust sources.
Haley M. Royer, Michael T. Sheridan, Hope E. Elliott, Nurun Nahar Lata, Zezhen Cheng, Swarup China, Zihua Zhu, Andrew P. Ault, and Cassandra J. Gaston
EGUsphere, https://doi.org/10.5194/egusphere-2024-3288, https://doi.org/10.5194/egusphere-2024-3288, 2024
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Saharan dust transported across the Atlantic to the Caribbean, South America, and North America is hypothesized to undergo chemical processing by inorganic and organic acids that enhances cloud droplet formation, nutrient availability, and reflectivity of. In this study, chemical analysis performed on African dust deposited over Barbados shows that acid tracers are found mostly on sea salt and smoke particles, rather than dust, indicating that dust particles undergo minimal chemical processing.
Imad El Haddad, Danielle Vienneau, Kaspar R. Daellenbach, Robin Modini, Jay G. Slowik, Abhishek Upadhyay, Petros N. Vasilakos, David Bell, Kees de Hoogh, and Andre S. H. Prevot
Atmos. Chem. Phys., 24, 11981–12011, https://doi.org/10.5194/acp-24-11981-2024, https://doi.org/10.5194/acp-24-11981-2024, 2024
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This opinion paper explores how advances in aerosol science inform our understanding of the health impacts of outdoor particulate pollution. We advocate for a shift in the way we target PM pollution, focusing on the most harmful anthropogenic emissions. We highlight key observations, modelling developments, and emission measurements needed to achieve this shift.
Yu Huang, Xingru Li, Dan Dan Huang, Ruoyuan Lei, Binhuang Zhou, Yunjiang Zhang, and Xinlei Ge
EGUsphere, https://doi.org/10.5194/egusphere-2024-2757, https://doi.org/10.5194/egusphere-2024-2757, 2024
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This work performed a comprehensive investigation on the chemical and optical properties of the brown carbon in PM2.5 samples collected in Nanjing, China. In particular, we used the machine learning approach to identify a list of key BrC species, which can be a good reference for future studies. Our findings extend the understanding on BrC properties and are valuable to the assessment of its impact on air quality and radiative forcing.
Pramod Kumar, Khushboo Sharma, Ankita Malu, Rajeev Rajak, Aparna Gupta, Bidyutjyoti Baruah, Shailesh Yadav, Thupstan Angchuk, Jayant Sharma, Rakesh Kumar Ranjan, Anil Kumar Misra, and Nishchal Wanjari
Atmos. Chem. Phys., 24, 11585–11601, https://doi.org/10.5194/acp-24-11585-2024, https://doi.org/10.5194/acp-24-11585-2024, 2024
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This work monitors and assesses air pollution, especially black and brown carbon, its controlling factor, and its effect on the environment of Sikkim Himalayan region. The huge urban sprawl in recent decades has led to regional human-induced air pollution in the region. Black carbon was highest in April 2021 and March 2022, exceeding the WHO limit. The monsoon season causes huge rainfall over the region, which reduces the pollutants by scavenging (rainout and washout).
Maria P. Velásquez-García, K. Santiago Hernández, James A. Vergara-Correa, Richard J. Pope, Miriam Gómez-Marín, and Angela M. Rendón
Atmos. Chem. Phys., 24, 11497–11520, https://doi.org/10.5194/acp-24-11497-2024, https://doi.org/10.5194/acp-24-11497-2024, 2024
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In the Aburrá Valley, northern South America, local emissions determine air quality conditions. However, we found that external sources, such as regional fires, Saharan dust, and volcanic emissions, increase particulate concentrations and worsen chemical composition by introducing elements like heavy metals. Dry winds and source variability contribute to seasonal influences on these events. This study assesses the air quality risks posed by such events, which can affect broad regions worldwide.
Diana L. Pereira, Chiara Giorio, Aline Gratien, Alexander Zherebker, Gael Noyalet, Servanne Chevaillier, Stéphanie Alage, Elie Almarj, Antonin Bergé, Thomas Bertin, Mathieu Cazaunau, Patrice Coll, Ludovico Di Antonio, Sergio Harb, Johannes Heuser, Cécile Gaimoz, Oscar Guillemant, Brigitte Language, Olivier Lauret, Camilo Macias, Franck Maisonneuve, Bénédicte Picquet-Varrault, Raquel Torres, Sylvain Triquet, Pascal Zapf, Lelia Hawkins, Drew Pronovost, Sydney Riley, Pierre-Marie Flaud, Emilie Perraudin, Pauline Pouyes, Eric Villenave, Alexandre Albinet, Olivier Favez, Robin Aujay-Plouzeau, Vincent Michoud, Christopher Cantrell, Manuela Cirtog, Claudia Di Biagio, Jean-François Doussin, and Paola Formenti
EGUsphere, https://doi.org/10.5194/egusphere-2024-3015, https://doi.org/10.5194/egusphere-2024-3015, 2024
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In order to study aerosols in environments influenced by anthropogenic and biogenic emissions, we performed analysis of samples collected during ACROSS (Atmospheric Chemistry Of the Suburban Forest) campaign in the summer 2022 in the Paris greater area. After analysis of the chemical composition by means of total carbon determination and high resolution mass spectrometry, this work highlights the influence of anthropogenic inputs into the chemical composition of both urban and forested areas.
Meng Wang, Qiyuan Wang, Steven Sai Hang Ho, Jie Tian, Yong Zhang, Shun-cheng Lee, and Junji Cao
Atmos. Chem. Phys., 24, 11175–11189, https://doi.org/10.5194/acp-24-11175-2024, https://doi.org/10.5194/acp-24-11175-2024, 2024
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We studied nitrogen-containing organic compounds (NOCs) in particulate matter <2.5 µm particles on the southeastern Tibetan Plateau. We found that biomass burning and transboundary transport are the main sources of NOCs in the high-altitude area. Understanding these aerosol sources informs how they add to regional and potentially global climate changes. Our findings could help shape effective environmental policies to enhance air quality and address climate impacts in this sensitive region.
Kimmo Teinilä, Sanna Saarikoski, Henna Lintusaari, Teemu Lepistö, Petteri Marjanen, Minna Aurela, Heidi Hellén, Toni Tykkä, Markus Lampimäki, Janne Lampilahti, Luis Barreira, Timo Mäkelä, Leena Kangas, Juha Hatakka, Sami Harni, Joel Kuula, Jarkko V. Niemi, Harri Portin, Jaakko Yli-Ojanperä, Ville Niemelä, Milja Jäppi, Katrianne Lehtipalo, Joonas Vanhanen, Liisa Pirjola, Hanna E. Manninen, Tuukka Petäjä, Topi Rönkkö, and Hilkka Timonen
EGUsphere, https://doi.org/10.5194/egusphere-2024-2235, https://doi.org/10.5194/egusphere-2024-2235, 2024
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Physical and chemical properties of particulate matter and concentrations of trace gases were measured in a street canyon in Helsinki, Finland and an urban background site in January–February 2022 to investigate the effect of wintertime conditions on pollutants. State-of-the-art instruments, a mobile laboratory was used, and the measurement data was further analysed with modelling tools like positive matrix factorization (PMF) and pollution detection algorithm (PDA).
Jinbo Wang, Jiaping Wang, Yuxuan Zhang, Tengyu Liu, Xuguang Chi, Xin Huang, Dafeng Ge, Shiyi Lai, Caijun Zhu, Lei Wang, Qiaozhi Zha, Ximeng Qi, Wei Nie, Congbin Fu, and Aijun Ding
Atmos. Chem. Phys., 24, 11063–11080, https://doi.org/10.5194/acp-24-11063-2024, https://doi.org/10.5194/acp-24-11063-2024, 2024
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In this study, we found large spatial discrepancies in the physical and chemical properties of black carbon over the Tibetan Plateau (TP). Elevated anthropogenic emissions from low-altitude regions can significantly change the mass concentration, mixing state and chemical composition of black-carbon-containing aerosol in the TP region, further altering its light absorption ability. Our study emphasizes the vulnerability of remote plateau regions to intense anthropogenic influences.
Liyuan Zhou, Qianyun Liu, Christian M. Salvador, Michael Le Breton, Mattias Hallquist, Jian Zhen Yu, Chak K. Chan, and Åsa M. Hallquist
Atmos. Chem. Phys., 24, 11045–11061, https://doi.org/10.5194/acp-24-11045-2024, https://doi.org/10.5194/acp-24-11045-2024, 2024
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Our research on city bus emissions reveals that alternative fuels (compressed natural gas and biofuels) reduce fresh particle emissions compared to diesel. However, all fuels lead to secondary air pollution. Aiming at guiding better environmental policies, we studied 76 buses using advanced emission measurement techniques. This work sheds light on the complex effects of bus fuels on urban air quality, emphasizing the need for comprehensive evaluations of future transportation technologies.
Xu Yang, Fobang Liu, Shuqi Yang, Yuling Yang, Yanan Wang, Jingjing Li, Mingyu Zhao, Zhao Wang, Kai Wang, Chi He, and Haijie Tong
Atmos. Chem. Phys., 24, 11029–11043, https://doi.org/10.5194/acp-24-11029-2024, https://doi.org/10.5194/acp-24-11029-2024, 2024
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A study in the rural North China Plain showed environmentally persistent free radicals (EPFRs) in atmospheric particulate matter (PM), with a notable water-soluble fraction likely from atmospheric oxidation during transport. Significant positive correlations between EPFRs and the water-soluble oxidative potential of PM2.5 were found, primarily attributable to the water-soluble fractions of EPFRs. These findings emphasize understanding EPFRs' atmospheric evolution for climate and health impacts.
Genevieve Rose Lorenzo, Luke D. Ziemba, Avelino F. Arellano, Mary C. Barth, Ewan C. Crosbie, Joshua P. DiGangi, Glenn S. Diskin, Richard Ferrare, Miguel Ricardo A. Hilario, Michael A. Shook, Simone Tilmes, Jian Wang, Qian Xiao, Jun Zhang, and Armin Sorooshian
EGUsphere, https://doi.org/10.5194/egusphere-2024-2604, https://doi.org/10.5194/egusphere-2024-2604, 2024
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Novel aerosol hygroscopicity analysis of CAMP2Ex field campaign data show low aerosol hygroscopicity values in Southeast Asia. Organic carbon from smoke decreases hygroscopicity to levels more like those in continental than in polluted marine regions. Hygroscopicity changes at cloud level demonstrate how surface particles impact clouds in the region affecting model representation of aerosol and cloud interactions in similar polluted marine regions with high organic carbon emissions.
Kirsten N. Fossum, Chunshui Lin, Niall O'Sullivan, Lu Lei, Stig Hellebust, Darius Ceburnis, Aqeel Afzal, Anja Tremper, David Green, Srishti Jain, Steigvilė Byčenkienė, Colin O'Dowd, John Wenger, and Jurgita Ovadnevaite
Atmos. Chem. Phys., 24, 10815–10831, https://doi.org/10.5194/acp-24-10815-2024, https://doi.org/10.5194/acp-24-10815-2024, 2024
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The chemical composition and sources of submicron aerosol in the Dublin Port area were investigated over a month-long campaign. Two distinct types of ship emissions were identified and characterised: sulfate-rich plumes from the use of heavy fuel oil with scrubbers and organic-rich plumes from the use of low-sulfur fuels. The latter were more frequent, emitting double the particle number and having a typical V / Ni ratio for ship emission.
Lise Le Berre, Brice Temime-Roussel, Grazia Maria Lanzafame, Barbara D’Anna, Nicolas Marchand, Stéphane Sauvage, Marvin Dufresne, Liselotte Tinel, Thierry Leonardis, Joel Ferreira de Brito, Alexandre Armengaud, Grégory Gille, Ludovic Lanzi, Romain Bourjot, and Henri Wortham
EGUsphere, https://doi.org/10.5194/egusphere-2024-2903, https://doi.org/10.5194/egusphere-2024-2903, 2024
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A summer campaign in a Mediterranean port examined pollution caused by ships. Two stations in the port measured pollution levels and captured over 350 ship plumes to study their chemical composition. Results showed that pollution levels, like ultra-fine particles, were higher in the port than in the city and offer a strong support to improve emission inventories. These findings may also serve as reference for assessing the benefits of a Sulphur Emission Control Area in the Mediterranean in 2025.
Xiao He, Xuan Zheng, Shuwen Guo, Lewei Zeng, Ting Chen, Bohan Yang, Shupei Xiao, Qiongqiong Wang, Zhiyuan Li, Yan You, Shaojun Zhang, and Ye Wu
Atmos. Chem. Phys., 24, 10655–10666, https://doi.org/10.5194/acp-24-10655-2024, https://doi.org/10.5194/acp-24-10655-2024, 2024
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This study introduces an innovative method for identifying and quantifying complex organic vapors and aerosols. By combining advanced analytical techniques and new algorithms, we categorized thousands of compounds from heavy-duty diesel vehicles and ambient air and highlighted specific tracers for emission sources. The innovative approach enhances peak identification, reduces quantification uncertainties, and offers new insights for air quality management and atmospheric chemistry.
Yu Xu, Tang Liu, Yi-Jia Ma, Qi-Bin Sun, Hong-Wei Xiao, Hao Xiao, Hua-Yun Xiao, and Cong-Qiang Liu
Atmos. Chem. Phys., 24, 10531–10542, https://doi.org/10.5194/acp-24-10531-2024, https://doi.org/10.5194/acp-24-10531-2024, 2024
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This study investigates the characteristics of aminiums and ammonium in PM2.5 on clean and polluted winter days in 11 Chinese cities, highlighting the possibility of the competitive uptake of ammonia versus amines on acidic aerosols or the displacement of aminiums by ammonia under high-ammonia conditions. The overall results deepen the understanding of the spatiotemporal differences in aminium characteristics and formation in China.
Cassidy Soloff, Taiwo Ajayi, Yonghoon Choi, Ewan C. Crosbie, Joshua P. DiGangi, Glenn S. Diskin, Marta A. Fenn, Richard A. Ferrare, Francesca Gallo, Johnathan W. Hair, Miguel Ricardo A. Hilario, Simon Kirschler, Richard H. Moore, Taylor J. Shingler, Michael A. Shook, Kenneth L. Thornhill, Christiane Voigt, Edward L. Winstead, Luke D. Ziemba, and Armin Sorooshian
Atmos. Chem. Phys., 24, 10385–10408, https://doi.org/10.5194/acp-24-10385-2024, https://doi.org/10.5194/acp-24-10385-2024, 2024
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Using aircraft measurements over the northwestern Atlantic between the US East Coast and Bermuda and trajectory modeling of continental outflow, we identify trace gas and particle properties that exhibit gradients with offshore distance and quantify these changes with high-resolution measurements of concentrations and particle chemistry, size, and scattering properties. This work furthers our understanding of the complex interactions between continental and marine environments.
Alex Rowell, James Brean, David C. S. Beddows, Zongbo Shi, Avinash Kumar, Matti Rissanen, Miikka Dal Maso, Peter Mettke, Kay Weinhold, Maik Merkel, and Roy M. Harrison
Atmos. Chem. Phys., 24, 10349–10361, https://doi.org/10.5194/acp-24-10349-2024, https://doi.org/10.5194/acp-24-10349-2024, 2024
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Ions enhance the formation and growth rates of new particles, affecting the Earth's radiation budget. Despite these effects, there is little published data exploring the sources of ions in the urban environment and their role in new particle formation (NPF). Here we show that natural ion sources dominate in urban environments, while traffic is a secondary source. Ions contribute up to 12.7 % of the formation rate of particles, indicating that they are important for forming urban PM.
Cited articles
Abas, M. R. B. and Simoneit, B. R. T.: Composition of extractable organic matter of air particles from Malaysia: Initial study, Atmos. Environ., 30, 2779–2793, 1996.
Abdullah, A. M., Abu Samah, M. A., and Jun, T. Y.: An Overview of the Air Pollution Trend in Klang Valley, Malaysia, Open Environ. J., 6, 13–19, https://doi.org/10.2174/1876325101206010013, 2012.
Afroz, R., Hassan, M. N., and Ibrahim, N. A.: Review of air pollution and health impacts in Malaysia, Environ. Res., 92, 71–77, https://doi.org/10.1016/s0013-9351(02)00059-2, 2003.
Aldabe, J., Elustondo, D., Santamaría, C., Lasheras, E., Pandolfi, M., Alastuey, A., Querol, X., and Santamaría, J. M.: Chemical characterisation and source apportionment of PM2.5 and PM10 at rural, urban and traffic sites in Navarra (North of Spain), Atmos. Res., 102, 191–205, https://doi.org/10.1016/j.atmosres.2011.07.003, 2011.
Almeida, S. M., Pio, C. A., Freitas, M. C., Reis, M. A., and Trancoso, M. A.: Source apportionment of fine and coarse particulate matter in a sub-urban area at the Western European Coast, Atmos. Environ., 39, 3127–3138, https://doi.org/10.1016/j.atmosenv.2005.01.048, 2005.
Almeida, S. M., Pio, C. A., Freitas, M. C., Reis, M. A., and Trancoso, M. A.: Approaching PM2.5 and PM2.5 – 10 source apportionment by mass balance analysis, principal component analysis and particle size distribution, Sci. Total Environ., 368, 663–674, 2006.
Amil, N., Latif, M., and Khan, M.: Characterization and Source Apportionment of Fine Particulate Matter during 2011 Haze Episode in UKM Bangi, Malaysia, in: From Sources to Solution, edited by: Aris, A. Z., Tengku Ismail, T. H., Harun, R., Abdullah, A. M., and Ishak, M. Y., Springer Singapore, 363–367, 2014.
Awang, M. B., Jaafar, A. B., Abdullah, A. M., Ismail, M. B., Hassan, M. N., Abdullah, R., Johan, S., and Noor, H.: Air quality in Malaysia: Impacts, management issues and future challenges, Respirology, 5, 183–196, https://doi.org/10.1046/j.1440-1843.2000.00248.x, 2000.
Azmi, S. Z., Latif, M. T., Ismail, A. S., Juneng, L., and Jemain, A. A.: Trend and status of air quality at three different monitoring stations in the Klang Valley, Malaysia, Air Qual. Atmos. Health, 3, 53–64, https://doi.org/10.1007/s11869-009-0051-1, 2010.
Balakrishnaiah, G., Wei, H., Chun-Nan, L., Amit, A., Chuen-Jinn, T., Gwo-Dong, R., Yue-Chuen, W., and Chung-Fang, C.: Source Characterization and Apportionment of PM10, PM2.5 and PM0.1 by Using Positive Matrix Factorization, Aerosol Air Qual. Res., 12, 476–491, https://doi.org/10.4209/aaqr.2012.04.0084, 2012.
Balasubramanian, R., Qian, W. B., Decesari, S., Facchini, M. C., and Fuzzi, S.: Comprehensive characterization of PM2.5 aerosols in Singapore, J. Geophys. Res.-Atmos., 108, 4523, https://doi.org/10.1029/2002JD002517, 2003.
Beckerman, B., Jerrett, M., Brook, J. R., Verma, D. K., Arain, M. A., and Finkelstein, M. M.: Correlation of nitrogen dioxide with other traffic pollutants near a major expressway, Atmos. Environ., 42, 275–290, https://doi.org/10.1016/j.atmosenv.2007.09.042, 2008.
Begum, B. A., Kim, E., Biswas, S. K., and Hopke, P. K.: Investigation of sources of atmospheric aerosol at urban and semi-urban areas in Bangladesh, Atmos. Environ., 38, 3025–3038, https://doi.org/10.1016/j.atmosenv.2004.02.042, 2004.
Bressi, M., Sciare, J., Ghersi, V., Bonnaire, N., Nicolas, J. B., Petit, J.-E., Moukhtar, S., Rosso, A., Mihalopoulos, N., and Féron, A.: A one-year comprehensive chemical characterisation of fine aerosol (PM2.5) at urban, suburban and rural background sites in the region of Paris (France), Atmos. Chem. Phys., 13, 7825–7844, https://doi.org/10.5194/acp-13-7825-2013, 2013.
Cesari, D., Contini, D., Genga, A., Siciliano, M., Elefante, C., Baglivi, F., and Daniele, L.: Analysis of raw soils and their re-suspended PM10 fractions: Characterisation of source profiles and enrichment factors, Appl. Geochem., 27, 1238–1246, https://doi.org/10.1016/j.apgeochem.2012.02.029, 2012.
Chang, D., Song, Y., and Liu, B.: Visibility trends in six megacities in China 1973–2007, Atmos. Res., 94, 161–167, https://doi.org/10.1016/j.atmosres.2009.05.006, 2009.
Cheng, Y., Lee, S. C., Ho, K. F., Chow, J. C., Watson, J. G., Louie, P. K. K., Cao, J. J., and Hai, X.: Chemically-speciated on-road PM2.5 motor vehicle emission factors in Hong Kong, Sci. Total Environ., 408, 1621–1627, https://doi.org/10.1016/j.scitotenv.2009.11.061, 2010.
Cohen, D. D., Garton, D., Stelcer, E., Hawas, O., Wang, T., Poon, S., Kim, J., Choi, B. C., Oh, S. N., Shin, H. J., Ko, M. Y., and Uematsu, M.: Multielemental analysis and characterization of fine aerosols at several key ACE-Asia sites, J. Geophys. Res.-Atmos., 109, 11–18, https://doi.org/10.1029/2003JD003569, 2004.
Contini, D., Cesari, D., Donateo, A., Chirizzi, D., and Belosi, F.: Characterization of PM10 and PM2.5 and Their Metals Content in Different Typologies of Sites in South-Eastern Italy, Atmosphere, 5, 435–453, https://doi.org/10.3390/atmos5020435, 2014.
Diederen, H. S. M. A., Guicherit, R., and HolLonder, J. C. T.: Visibility reduction by air pollution in The Netherlands, Atmos. Environ., 19, 377–383, https://doi.org/10.1016/0004-6981(85)90105-2, 1985.
Dockery, D. W., Pope, C. A., Xu, X., Spengler, J. D., Ware, J. H., Fay, M. E., Ferris, B. G., and Speizer, F. E.: An Association between Air Pollution and Mortality in Six US Cities, New Engl. J. Med., 329, 1753–1759, https://doi.org/10.1056/NEJM199312093292401, 1993.
Dongarrà, G., Manno, E., Varrica, D., Lombardo, M., and Vultaggio, M.: Study on ambient concentrations of PM10, PM10–2.5, PM2.5 and gaseous pollutants. Trace elements and chemical speciation of atmospheric particulates, Atmos. Environ., 44, 5244–5257, https://doi.org/10.1016/j.atmosenv.2010.08.041, 2010.
Doumbia, E. H. T., Liousse, C., Galy-Lacaux, C., Ndiaye, S. A., Diop, B., Ouafo, M., Assamoi, E. M., Gardrat, E., Castera, P., Rosset, R., Akpo, A., and Sigha, L.: Real time black carbon measurements in West and Central Africa urban sites, Atmos. Environ., 54, 529–537, https://doi.org/10.1016/j.atmosenv.2012.02.005, 2012.
Doyle, M. and Dorling, S.: Visibility trends in the UK 1950–1997, Atmos. Environ., 36, 3161–3172 https://doi.org/10.1016/S1352-2310(02)00248-0, 2002.
Eatough, D. J., Long, R. W., Modey, W. K., and Eatough, N. L.: Semi-volatile secondary organic aerosol in urban atmospheres: meeting a measurement challenge, Atmos. Environ., 37, 1277–1292, 2003.
Eatough, D. J., Anderson, R. R., Martello, D. V., Modey, W. K., and Mangelson, N. F.: Apportionment of Ambient Primary and Secondary PM2.5 During a 2001 Summer Intensive Study at the NETL Pittsburgh Site Using PMF2 and EPA UNMIX, Aerosol Sci. Technol., 40, 925–940, https://doi.org/10.1080/02786820600796616, 2006.
Echalar, F., Gaudichet, A., Cachier, H., and Artaxo, P.: Aerosol emissions by tropical forest and savanna biomass burning: Characteristic trace elements and fluxes, Geophy. Res. Lett., 22, 3039–3042, https://doi.org/10.1029/95GL03170, 1995.
Ee-Ling, O., Mustaffa, N. I., Amil, N., Khan, M. F., and Latif, M. T.: Source Contribution of PM2.5 at Different Locations on the Malaysian Peninsula, B. Environ. Contam. Tox., 94, 537–542, https://doi.org/10.1007/s00128-015-1477-9, 2015.
European Commission: Air Quality Standards: http://ec.europa.eu/environment/air/quality/standards.htm, last access: 2 June 2015.
Ewen, C., Anagnostopoulou, M., and Ward, N.: Monitoring of heavy metal levels in roadside dusts of Thessaloniki, Greece in relation to motor vehicle traffic density and flow, Environ. Monit. Assess., 157, 483–498, https://doi.org/10.1007/s10661-008-0550-9, 2009.
Fang, G.-C., Chang, C.-N., Chu, C.-C., Wu, Y.-S., Fu, P. P.-C., Yang, I. L., and Chen, M.-H.: Characterization of particulate, metallic elements of TSP, PM2.5 and PM2.5-10 aerosols at a farm sampling site in Taiwan, Taichung, Sci. Total Environ., 308, 157–166, https://doi.org/10.1016/S0048-9697(02)00648-4, 2003.
Farao, C., Canepari, S., Perrino, C., and Harrison, R. M.: Sources of PM in an Industrial Area: Comparison between Receptor Model Results and Semiempirical Calculations of Source Contributions, Aerosol Air Qual. Res., 14, 1558–1572, https://doi.org/10.4209/aaqr.2013.08.0281, 2014.
Favez, O., El Haddad, I., Piot, C., Boréave, A., Abidi, E., Marchand, N., Jaffrezo, J.-L., Besombes, J.-L., Personnaz, M.-B., Sciare, J., Wortham, H., George, C., and D'Anna, B.: Inter-comparison of source apportionment models for the estimation of wood burning aerosols during wintertime in an Alpine city (Grenoble, France), Atmos. Chem. Phys., 10, 5295–5314, https://doi.org/10.5194/acp-10-5295-2010, 2010.
Fuzzi, S., Baltensperger, U., Carslaw, K., Decesari, S., Denier van der Gon, H., Facchini, M. C., Fowler, D., Koren, I., Langford, B., Lohmann, U., Nemitz, E., Pandis, S., Riipinen, I., Rudich, Y., Schaap, M., Slowik, J. G., Spracklen, D. V., Vignati, E., Wild, M., Williams, M., and Gilardoni, S.: Particulate matter, air quality and climate: lessons learned and future needs, Atmos. Chem. Phys., 15, 8217–8299, https://doi.org/10.5194/acp-15-8217-2015, 2015.
Gehrig, R. and Buchmann, B.: Characterising seasonal variations and spatial distribution of ambient PM10 and PM2.5 concentrations based on long-term Swiss monitoring data, Atmos. Environ., 37, 2571–2580, 2003.
Gibson, M. D., Pierce, J. R., Waugh, D., Kuchta, J. S., Chisholm, L., Duck, T. J., Hopper, J. T., Beauchamp, S., King, G. H., Franklin, J. E., Leaitch, W. R., Wheeler, A. J., Li, Z., Gagnon, G. A., and Palmer, P. I.: Identifying the sources driving observed PM2.5 temporal variability over Halifax, Nova Scotia, during BORTAS-B, Atmos. Chem. Phys., 13, 7199–7213, https://doi.org/10.5194/acp-13-7199-2013, 2013.
Gomišček, B., Hauck, H., Stopper, S., and Preining, O.: Spatial and temporal variations of PM1, PM2.5, PM10 and particle number concentration during the AUPHEP-project, Atmos. Environ., 38, 3917–3934, https://doi.org/10.1016/j.atmosenv.2004.03.056, 2004.
Grossi, C. M. and Brimblecombe, P.: The effect of atmospheric pollution on building materials, J. Phys. IV, 12, 197–210, 2002.
Gugamsetty, B., Wei, H., Liu, C.-N., Awasthi, A., Tsai, C.-J., Roam, G.-D., Wu, Y.-C., and Chen, C.-F.: Source Characterization and Apportionment of PM10, PM2.5 and PM0.1 by Using Positive Matrix Factorization, Aerosol Air Qual. Res., 12, 476–491, https://doi.org/10.4209/aaqr.2012.04.0084, 2012.
Halonen, J.: Acute Cardiorespiratory Health Effects of Size-Segregated Ambient Particulate Air Pollution and Ozone, PhD Faculty of Medicine University of Kuopio, National Institute of Health and Welfare, Kuopio, Finland, 174 pp., 2009.
Han, Y. M., Cao, J. J., Jin, Z. D., and An, Z. S.: Elemental composition of aerosols in Daihai, a rural area in the front boundary of the summer Asian monsoon, Atmos. Res., 92, 229–235, https://doi.org/10.1016/j.atmosres.2008.10.031, 2009.
Harrison, R. M., Smith, D. J. T., and Luhana, L.: Source Apportionment of Atmospheric Polycyclic Aromatic Hydrocarbons Collected from an Urban Location in Birmingham, UK, Environ. Sci. Technol., 30, 825–832, https://doi.org/10.1021/es950252d, 1996.
Harrison, R. M., Jones, A. M., and Lawrence, R. G.: A pragmatic mass closure model for airborne particulate matter at urban background and roadside sites, Atmos. Environ., 37, 4927–4933, https://doi.org/10.1016/j.atmosenv.2003.08.025, 2003.
He, K., Zhao, Q., Ma, Y., Duan, F., Yang, F., Shi, Z., and Chen, G.: Spatial and seasonal variability of PM2.5 acidity at two Chinese megacities: insights into the formation of secondary inorganic aerosols, Atmos. Chem. Phys., 12, 1377–1395, https://doi.org/10.5194/acp-12-1377-2012, 2012.
Heal, M. R., Hibbs, L. R., Agius, R. M., and Beverland, I. J.: Interpretation of variations in fine, coarse and black smoke particulate matter concentrations in a northern European city, Atmos. Environ., 39, 3711–3718, 2005.
Hellebust, S., Allanic, A., O'Connor, I. P., Wenger, J. C., and Sodeau, J. R.: The use of real-time monitoring data to evaluate major sources of airborne particulate matter, Atmos. Environ., 44, 1116–1125, 2010.
Hellén, H., Hakola, H., and Laurila, T.: Determination of source contributions of NMHCs in Helsinki (60° N, 25° E) using chemical mass balance and the Unmix multivariate receptor models, Atmos. Environ., 37, 1413–1424, https://doi.org/10.1016/S1352-2310(02)01049-X, 2003.
Heo, J.-B., Hopke, P. K., and Yi, S.-M.: Source apportionment of PM2.5 in Seoul, Korea, Atmos. Chem. Phys., 9, 4957–4971, https://doi.org/10.5194/acp-9-4957-2009, 2009.
Ho, K. F., Cao, J. J., Lee, S. C., and Chan, C. K.: Source apportionment of PM2.5 in urban area of Hong Kong, J. Hazard. Mater., 138, 73–85, https://doi.org/10.1016/j.jhazmat.2006.05.047, 2006.
Hopke, P. K. and Song, X.-H.: The chemical mass balance as a multivariate calibration problem, Chemometrics and Intelligent Laboratory Systems, 37, 5–14, 1997.
Hopke, P. K., Ito, K., Mar, T., Christensen, W. F., Eatough, D. J., Henry, R. C., Kim, E., Laden, F., Lall, R., Larson, T. V., Liu, H., Neas, L., Pinto, J., Stolzel, M., Suh, H., Paatero, P., and Thurston, G. D.: PM source apportionment and health effects: 1. Intercomparison of source apportionment results, J. Expo. Sci. Env. Epid., 16, 275–286, https://doi.org/10.1038/sj.jea.7500458, 2006.
Hopke, P. K., Cohen, D. D., Begum, B. A., Biswas, S. K., Ni, B., Pandit, G. G., Santoso, M., Chung, Y.-S., Davy, P., Markwitz, A., Waheed, S., Siddique, N., Santos, F. L., Pabroa, P. C. B., Seneviratne, M. C. S., Wimolwattanapun, W., Bunprapob, S., Vuong, T. B., Duy Hien, P., and Markowicz, A.: Urban air quality in the Asian region, Sci. Total Environ., 404, 103–112, https://doi.org/10.1016/j.scitotenv.2008.05.039, 2008.
Huang, B., Liu, M., Ren, Z., Bi, X., Zhang, G., Sheng, G., and Fu, J.: Chemical composition, diurnal variation and sources of PM2.5 at two industrial sites of South China, Atmospolres, 4, 298–305, https://doi.org/10.5094/APR.2013.033, 2013.
Hyslop, N. P.: Impaired visibility: the air pollution people see, Atmos. Environ., 43, 182–195, https://doi.org/10.1016/j.atmosenv.2008.09.067, 2009.
Jacobson, M. Z.: Control of fossil-fuel particulate black carbon and organic matter, possibly the most effective method of slowing global warming, J. Geophys. Res.-Atmos., 107, 4410, https://doi.org/10.1029/2001JD001376, 2002.
Jiang, S. Y. N., Yang, F., Chan, K. L., and Ning, Z.: Water solubility of metals in coarse PM and PM2.5 in typical urban environment in Hong Kong, Atmos. Pollut. Res., 5, 236–244, https://doi.org/10.5094/APR.2014.029, 2014.
Juneng, L., Latif, M. T., Tangang, F. T., and Mansor, H.: Spatio-temporal characteristics of PM10 concentration across Malaysia, Atmos. Environ., 43, 4584–4594, https://doi.org/10.1016/j.atmosenv.2009.06.018, 2009.
Juneng, L., Latif, M. T., and Tangang, F.: Factors influencing the variations of PM10 aerosol dust in Klang Valley, Malaysia during the summer, Atmos. Environ., 45, 4370–4378, https://doi.org/10.1016/j.atmosenv.2011.05.045, 2011.
Kalnay, E., Kanamitsu, M., Kistler, R., Collins, W., Deaven, D., Gandin, L., Iredell, M., Saha, S., White, G., Woollen, J., Zhu, Y., Leetmaa, A., Reynolds, R., Chelliah, M., Ebisuzaki, W., Higgins, W., Janowiak, J., Mo, K. C., Ropelewski, C., Wang, J., Jenne, R., and Joseph, D.: The NCEP/NCAR 40-Year Reanalysis Project, Bulletin of the American Meteorological Society, 77, 437–471, 1996.
Karthikeyan, S. and Balasubramanian, R.: Determination of water-soluble inorganic and organic species in atmospheric fine particulate matter, Microchem. J., 82, 49–55, https://doi.org/10.1016/j.microc.2005.07.003, 2006.
Katsouyanni, K., Touloumi, G., Spix, C., Schwartz, J., Balducci, F., Medina, S., Rossi, G., Wojtyniak, B., Sunyer, J., Bacharova, L., Schouten, J. P., Ponka, A., and Anderson, H. R.: Short term effects of ambient sulphur dioxide and particulate matter on mortality in 12 European cities: results from time series data from the APHEA project, BMJ, 314, 1658, 1997.
Keywood, M. D., Ayers, G. P., Gras, J. L., Boers, C. P., and Leong: Haze in the Klang Valley of Malaysia, Atmos. Chem. Phys., 3, 591–605, https://doi.org/10.5194/acp-3-591-2003, 2003.
Khan, M. F., Hirano, K., and Masunaga, S.: Quantifying the sources of hazardous elements of suspended particulate matter aerosol collected in Yokohama, Japan, Atmos. Environ., 44, 2646–2657, https://doi.org/10.1016/j.atmosenv.2010.03.040, 2010a.
Khan, M. F., Shirasuna, Y., Hirano, K., and Masunaga, S.: Characterization of PM2.5, PM2.5–10 and PM10 in ambient air, Yokohama, Japan, Atmos. Res., 96, 159–172, https://doi.org/10.1016/j.atmosres.2009.12.009, 2010b.
Khan, M. F., Latif, M. T., Juneng, L., Amil, N., Nadzir, M. S. M., and Syedul Hoque, H. M.: Physicochemical factors and sources of PM10 at residential-urban environment in Kuala Lumpur, J. Air Waste Manage., 65, 958–969, https://doi.org/10.1080/10962247.2015.1042094, 2015a.
Khan, M. F., Latif, M. T., Lim, C. H., Amil, N., Jaafar, S. A., Dominick, D., Mohd Nadzir, M. S., Sahani, M., and Tahir, N. M.: Seasonal effect and source apportionment of polycyclic aromatic hydrocarbons in PM2.5, Atmos. Environ., 106, 178–190, https://doi.org/10.1016/j.atmosenv.2015.01.077, 2015b.
Khan, M. F., Latif, M. T., Saw, W. H., Amil, N., Nadzir, M. S. M., Sahani, M., Tahir, N. M., and Chung, J. X.: Fine particulate matter in the tropical environment: monsoonal effects, source apportionment, and health risk assessment, Atmos. Chem. Phys., 16, 597–617, https://doi.org/10.5194/acp-16-597-2016, 2016.
Kim, E. and Hopke, P. K.: Source characterization of ambient fine particles at multiple sites in the Seattle area, Atmos. Environ., 42, 6047–6056, https://doi.org/10.1016/j.atmosenv.2008.03.032, 2008.
Kim Oanh, N. T., Upadhyay, N., Zhuang, Y. H., Hao, Z. P., Murthy, D. V. S., Lestari, P., Villarin, J. T., Chengchua, K., Co, H. X., Dung, N. T., and Lindgren, E. S.: Particulate air pollution in six Asian cities: Spatial and temporal distributions, and associated sources, Atmos. Environ., 40, 3367–3380, https://doi.org/10.1016/j.atmosenv.2006.01.050, 2006.
Koçak, M., Theodosi, C., Zarmpas, P., Im, U., Bougiatioti, A., Yenigun, O., and Mihalopoulos, N.: Particulate matter (PM10) in Istanbul: Origin, source areas and potential impact on surrounding regions, Atmos. Environ., 45, 6891–6900, https://doi.org/10.1016/j.atmosenv.2010.10.007, 2011.
Kowalczyk, G. S., Gordon, G. E., and Rheingrover, S. W.: Identification of atmospheric particulate sources in Washington, D.C. using chemical element balances, Environ. Sci. Technol., 16, 79–90, https://doi.org/10.1021/es00096a005, 1982.
Krewski, D., Jerrett, M., Burnett, R. T., Ma, R., Hughes, E., Shi, Y., Turner, M. C., Pope III , C. A., Thurston, G., Calle, E. E., Thun, M. J., Beckerman, B., DeLuca, P., Finkelstein, N., Ito, K., Moore, D. K., Newbold, K. B., Ramsay, T., Ross, Z., Shin, H., and Tempalski, B.: Extended follow-up and spatial analysis of the American Cancer Society study linking particulate air pollution and mortality, HEI Research Report 140, Health Effects Institute, Boston, MA, USA, 5–114, 115–136, 2009.
Kuo, Y.-M., Hung, H.-F., and Yang, T.-T.: Chemical Compositions of PM2.5 in Residential Homes of Southern Taiwan, Aerosol Air Qual. Res., 7, 403–416, https://doi.org/10.4209/aaqr.2007.02.0009, 2007.
Laden, F., Neas, L. M., Dockery, D. W., and Schwartz, J.: Association of fine particulate matter from different sources with daily mortality in six US cities, Environ. Health Persp., 108, 941–947, 2000.
Lanki, T., de Hartog, J. J., Heinrich, J., Hoek, G., Janssen, N. A. H., Peters, A., Stölzel, M., Timonen, K. L., Vallius, M., Vanninen, E., and Pekkanen, J.: Can we identify sources of fine particles respnsible for exercise-induced ischemia on days with elevated air pollution? The ULTRA study, Environ. Health Persp., 114, 655–660, 2006.
Lanz, V. A., Prévôt, A. S. H., Alfarra, M. R., Weimer, S., Mohr, C., DeCarlo, P. F., Gianini, M. F. D., Hueglin, C., Schneider, J., Favez, O., D'Anna, B., George, C., and Baltensperger, U.: Characterization of aerosol chemical composition with aerosol mass spectrometry in Central Europe: an overview, Atmos. Chem. Phys., 10, 10453–10471, https://doi.org/10.5194/acp-10-10453-2010, 2010.
Lawson, D. R. and Winchester, J. W.: A standard crustal aerosol as a reference for elemental enrichment factors, Atmos. Environ., 13, 925–930, https://doi.org/10.1016/0004-6981(79)90003-9, 1979.
Lestari, P. and Mauliadi, Y. D.: Source apportionment of particulate matter at urban mixed site in Indonesia using PMF, Atmos. Environ., 43, 1760–1770, https://doi.org/10.1016/j.atmosenv.2008.12.044, 2009.
Louie, P. K. K., Chow, J. C., Chen, L. W. A., Watson, J. G., Leung, G., and Sin, D. W. M.: PM2.5 chemical composition in Hong Kong: urban and regional variations, Sci. Total Environ., 338, 267–281, https://doi.org/10.1016/j.scitotenv.2004.07.021, 2005.
Mallet, M., Dulac, F., Formenti, P., Nabat, P., Sciare, J., Roberts, G., Pelon, J., Ancellet, G., Tanré, D., Parol, F., Denjean, C., Brogniez, G., di Sarra, A., Alados-Arboledas, L., Arndt, J., Auriol, F., Blarel, L., Bourrianne, T., Chazette, P., Chevaillier, S., Claeys, M., D'Anna, B., Derimian, Y., Desboeufs, K., Di Iorio, T., Doussin, J.-F., Durand, P., Féron, A., Freney, E., Gaimoz, C., Goloub, P., Gómez-Amo, J. L., Granados-Muñoz, M. J., Grand, N., Hamonou, E., Jankowiak, I., Jeannot, M., Léon, J.-F., Maillé, M., Mailler, S., Meloni, D., Menut, L., Momboisse, G., Nicolas, J., Podvin, T., Pont, V., Rea, G., Renard, J.-B., Roblou, L., Schepanski, K., Schwarzenboeck, A., Sellegri, K., Sicard, M., Solmon, F., Somot, S., Torres, B., Totems, J., Triquet, S., Verdier, N., Verwaerde, C., Waquet, F., Wenger, J., and Zapf, P.: Overview of the Chemistry-Aerosol Mediterranean Experiment/Aerosol Direct Radiative Forcing on the Mediterranean Climate (ChArMEx/ADRIMED) summer 2013 campaign, Atmos. Chem. Phys., 16, 455–504, https://doi.org/10.5194/acp-16-455-2016, 2016.
Megaritis, A. G., Fountoukis, C., Charalampidis, P. E., Denier van der Gon, H. A. C., Pilinis, C., and Pandis, S. N.: Linking climate and air quality over Europe: effects of meteorology on PM2.5 concentrations, Atmos. Chem. Phys., 14, 10283–10298, https://doi.org/10.5194/acp-14-10283-2014, 2014.
METMalaysia: General Climate of Malaysia: http://www.met.gov.my/en/web/metmalaysia/education/climate/generalclimateofmalaysia (last access: 1 July 2015), 2013.
Meyer, N. K.: Particulate, black carbon and organic emissions from small-scale residential wood combustion appliances in Switzerland, Biomass. Bioenerg., 36, 31–42, https://doi.org/10.1016/j.biombioe.2011.09.023, 2012.
Ministry of Works: Road Traffic Volume Malaysia Malaysian Institute of Road Safety Research (MIROS), Selangor, Malaysia, 2011.
Moldanová, J., Fridell, E., Winnes, H., Holmin-Fridell, S., Boman, J., Jedynska, A., Tishkova, V., Demirdjian, B., Joulie, S., Bladt, H., Ivleva, N. P., and Niessner, R.: Physical and chemical characterisation of PM emissions from two ships operating in European Emission Control Areas, Atmos. Meas. Tech., 6, 3577–3596, https://doi.org/10.5194/amt-6-3577-2013, 2013.
Mooibroek, D., Schaap, M., Weijers, E. P., and Hoogerbrugge, R.: Source apportionment and spatial variability of PM2.5 using measurements at five sites in the Netherlands, Atmos. Environ., 45, 4180–4191, https://doi.org/10.1016/j.atmosenv.2011.05.017, 2011.
Mueller, D., Uibel, S., Takemura, M., Klingelhoefer, D., and Groneberg, D.: Ships, ports and particulate air pollution – an analysis of recent studies, J. Occup. Med. Toxicol., 6, 1–6, https://doi.org/10.1186/1745-6673-6-31, 2011.
Mustaffa, N. I., Latif, M. T., Ali, M. M., and Khan, M. F.: Source apportionment of surfactants in marine aerosols at different locations along the Malacca Straits, Environ. Sci. Pollut. Res., 21, 6590–6602, https://doi.org/10.1007/s11356-014-2562-z, 2014.
NOAA: NCEP/NCAR Reanalysis 1: Pressure: http://www.esrl.noaa.gov/psd/data/gridded/data.ncep.reanalysis.pressure.html, last access: 3 March 2015.
Norela, S., Saidah, M. S., and Mastura, M.: Chemical composition of the haze in Malaysia 2005, Atmos. Environ., https://doi.org/10.1016/j.atmosenv.2013.05.024, 2013.
Paatero, P. and Tapper, U.: Analysis of different modes of factor analysis as least squares fit problems, Chemometer. Intell. Lab., 18, 183–194, https://doi.org/10.1016/0169-7439(93)80055-M, 1993.
Paatero, P. and Tapper, U.: Positive Matrix Factorization – A Nonnegative Factor Model With Optimal Utilization of Error – Estimates of Data Values, Environmetrics, 5, 111–126, https://doi.org/10.1002/env.3170050203, 1994.
Paatero, P., Eberly, S., Brown, S. G., and Norris, G. A.: Methods for estimating uncertainty in factor analytic solutions, Atmos. Meas. Tech., 7, 781–797, https://doi.org/10.5194/amt-7-781-2014, 2014.
Pachauri, T., Satsangi, A., Singla, V., Lakhani, A., and Kumari, K. M.: Characteristics and Sources of Carbonaceous Aerosols in PM2.5 during Wintertime in Agra, India, Aerosol Air Qual. Res., 13, 977–991, 2013.
Park, S. S., Kim, Y. J., and Fung, K.: PM2.5 carbon measurements in two urban areas: Seoul and Kwangju, Korea, Atmos. Environ., 36, 1287–1297, 2002.
Pastuszka, J., Rogula-Kozlowska, W., and Zajusz-Zubek, E.: Characterization of PM10 and PM2.5 and associated heavy metals at the crossroads and urban background site in Zabrze, Upper Silesia, Poland, during the smog episodes, Environ. Monit. Assess., 168, 613–627, https://doi.org/10.1007/s10661-009-1138-8, 2010.
Pey, J., Querol, X., Alastuey, A., Rodríguez, S., Putaud, J. P., and Van Dingenen, R.: Source apportionment of urban fine and ultra-fine particle number concentration in a Western Mediterranean city, Atmos. Environ., 43, 4407–4415, https://doi.org/10.1016/j.atmosenv.2009.05.024, 2009.
Pope III, C. A.: Epidemiology of fine particulate air pollution and human health: Biologic mechanisms and who's at risk?, Environ. Health Persp., 108, 713–723, 2000.
Pope III, C. A. and Dockery, D. W.: Health effects of fine particulate air pollution: Lines that connect, J. Air Waste Manage., 56, 709–742, 2006.
Querol, X., Viana, M., Alastuey, A., Amato, F., Moreno, T., Castillo, S., Pey, J., de la Rosa, J., Sánchez de la Campa, A., Artíñano, B., Salvador, P., García Dos Santos, S., Fernández-Patier, R., Moreno-Grau, S., Negral, L., Minguillón, M. C., Monfort, E., Gil, J. I., Inza, A., Ortega, L. A., Santamaría, J. M., and Zabalza, J.: Source origin of trace elements in PM from regional background, urban and industrial sites of Spain, Atmos. Environ., 41, 7219–7231, https://doi.org/10.1016/j.atmosenv.2007.05.022, 2007.
Querol, X., Pey, J., Minguillón, M. C., Pérez, N., Alastuey, A., Viana, M., Moreno, T., Bernabé, R. M., Blanco, S., Cárdenas, B., Vega, E., Sosa, G., Escalona, S., Ruiz, H., and Artíñano, B.: PM speciation and sources in Mexico during the MILAGRO-2006 Campaign, Atmos. Chem. Phys., 8, 111–128, https://doi.org/10.5194/acp-8-111-2008, 2008.
Rahman, S. A., Hamzah, M. S., Wood, A. K., Elias, M. S., Adullah Salim, N. A., and Sanuri, E.: Sources apportionment of fine and coarse aerosol in Klang Valley, Kuala Lumpur using positive matrix factorization, Atmos. Pollut. Res., 2, 197–206, https://doi.org/10.5094/APR.2011.025, 2011.
Rashid, M. and Griffiths, R. F.: Trends of atmospheric fine and coarse particulates in Kuala Lumpur, Malaysia (1986–1990), Environ. Technol., 16, 25–34, 1995.
Reche, C., Viana, M., Amato, F., Alastuey, A., Moreno, T., Hillamo, R., Teinilä, K., Saarnio, K., Seco, R., Peñuelas, J., Mohr, C., Prévôt, A. S. H., and Querol, X.: Biomass burning contributions to urban aerosols in a coastal Mediterranean City, Sci. Total Environ., 427, 175–190, https://doi.org/10.1016/j.scitotenv.2012.04.012, 2012.
Reid, J. S., Hyer, E. J., Johnson, R. S., Holben, B. N., Yokelson, R. J., Zhang, J., Campbell, J. R., Christopher, S. A., Di Girolamo, L., Giglio, L., Holz, R. E., Kearney, C., Miettinen, J., Reid, E. A., Turk, F. J., Wang, J., Xian, P., Zhao, G., Balasubramanian, R., Chew, B. N., Janjai, S., Lagrosas, N., Lestari, P., Lin, N.-H., Mahmud, M., Nguyen, A. X., Norris, B., Oanh, N. T. K., Oo, M., Salinas, S. V., Welton, E. J., and Liew, S. C.: Observing and understanding the Southeast Asian aerosol system by remote sensing: An initial review and analysis for the Seven Southeast Asian Studies (7SEAS) program, Atmos. Res., 122, 403–468, https://doi.org/10.1016/j.atmosres.2012.06.005, 2013.
Reisen, F., Meyer, C. P., and Keywood, M. D.: Impact of biomass burning sources on seasonal aerosol air quality, Atmos. Environ., 67, 437–447, https://doi.org/10.1016/j.atmosenv.2012.11.004, 2013.
Remoundaki, E., Kassomenos, P., Mantas, E., Mihalopoulos, N., and Tsezos, M.: Composition and Mass Closure of PM2.5 in Urban Environment (Athens, Greece), Aerosol Air Qual. Res., 13, 72–82, https://doi.org/10.4209/aaqr.2012.03.0054, 2013.
Rengarajan, R., Sudheer, A. K., and Sarin, M. M.: Wintertime PM2.5 and PM10 carbonaceous and inorganic constituents from urban site in western India, Atmos. Res., 102, 420–431, https://doi.org/10.1016/j.atmosres.2011.09.005, 2011.
Richard, A., Gianini, M. F. D., Mohr, C., Furger, M., Bukowiecki, N., Minguillón, M. C., Lienemann, P., Flechsig, U., Appel, K., DeCarlo, P. F., Heringa, M. F., Chirico, R., Baltensperger, U., and Prévôt, A. S. H.: Source apportionment of size and time resolved trace elements and organic aerosols from an urban courtyard site in Switzerland, Atmos. Chem. Phys., 11, 8945–8963, https://doi.org/10.5194/acp-11-8945-2011, 2011.
Richmond-Bryant, J., Saganich, C., Bukiewicz, L., and Kalin, R.: Associations of PM2.5 and black carbon concentrations with traffic, idling, background pollution, and meteorology during school dismissals, Sci. Total Environ., 407, 3357–3364, https://doi.org/10.1016/j.scitotenv.2009.01.046, 2009.
Ross, Z., Ito, K., Johnson, S., Yee, M., Pezeshki, G., Clougherty, J. E., Savitz, D., and Matte, T.: Spatial and temporal estimation of air pollutants in New York City: exposure assignment for use in a birth outcomes study, Environ. Health, 12, 1–13, https://doi.org/10.1186/1476-069x-12-51, 2013.
Ruuskanen, J., Tuch, T., Ten Brink, H., Peters, A., Khlystov, A., Mirme, A., Kos, G. P. A., Brunekreef, B., Wichmann, H. E., Buzorius, G., Vallius, M., Kreyling, W. G., and Pekkanen, J.: Concentrations of ultrafine, fine and PM2.5 particles in three European cities, Atmos. Environ., 35, 3729–3738, 2001.
Sánchez de la Campa, A. M., de la Rosa, J. D., Sánchez-Rodas, D., Oliveira, V., Alastuey, A., Querol, X., and Gómez Ariza, J. L.: Arsenic speciation study of PM2.5 in an urban area near a copper smelter, Atmos. Environ., 42, 6487–6495, https://doi.org/10.1016/j.atmosenv.2008.04.016, 2008.
Santoso, M., Hopke, P. K., Hidayat, A., and Diah Dwiana, L.: Sources identification of the atmospheric aerosol at urban and suburban sites in Indonesia by positive matrix factorization, Sci. Total Environ., 397, 229–237, https://doi.org/10.1016/j.scitotenv.2008.01.057, 2008.
Schwartz, J., Dockery, D. W., and Neas, L. M.: Is daily mortality associated specifically with fine particles?, J. Air Waste Manage., 46, 927–939, 1996.
Song, C. H. and Carmichael, G. R.: The aging process of naturally emitted aerosol (sea-salt and mineral aerosol) during long range transport, Atmos. Environ., 33, 2203–2218, https://doi.org/10.1016/S1352-2310(98)00301-X, 1999.
Song, Y., Xie, S., Zhang, Y., Zeng, L., Salmon, L. G., and Zheng, M.: Source apportionment of PM2.5 in Beijing using principal component analysis/absolute principal component scores and UNMIX, Sci. Total Environ., 372, 278–286, https://doi.org/10.1016/j.scitotenv.2006.08.041, 2006.
Speer, R. E., Barnes, H. M., and Brown, R.: An instrument for measuring the liquid water content of aerosols, Aerosol Sci. Technol., 27, 50–61, 1997.
Squizzato, S., Masiol, M., Brunelli, A., Pistollato, S., Tarabotti, E., Rampazzo, G., and Pavoni, B.: Factors determining the formation of secondary inorganic aerosol: a case study in the Po Valley (Italy), Atmos. Chem. Phys., 13, 1927–1939, https://doi.org/10.5194/acp-13-1927-2013, 2013.
Srimuruganandam, B. and Shiva Nagendra, S. M.: Source characterization of PM10 and PM2.5 mass using a chemical mass balance model at urban roadside, Sci. Total Environ., 433, 8–19, https://doi.org/10.1016/j.scitotenv.2012.05.082, 2012a.
Srimuruganandam, B. and Shiva Nagendra, S. M.: Application of positive matrix factorization in characterization of PM10 and PM2.5 emission sources at urban roadside, Chemosphere, 88, 120–130, https://doi.org/10.1016/j.chemosphere.2012.02.083, 2012b.
Stortini, A. M., Freda, A., Cesari, D., Cairns, W. R. L., Contini, D., Barbante, C., Prodi, F., Cescon, P., and Gambaro, A.: An evaluation of the PM2.5 trace elemental composition in the Venice Lagoon area and an analysis of the possible sources, Atmos. Environ., 43, 6296–6304, https://doi.org/10.1016/j.atmosenv.2009.09.033, 2009.
Tagaris, E., Liao, K.-J., DeLucia, A. J., Deck, L., Amar, P., and Russell, A. G.: Potential Impact of Climate Change on Air Pollution-Related Human Health Effects, Environ. Sci. Technol., 43, 4979–4988, https://doi.org/10.1021/es803650w, 2009.
Tahir, N. M., Koh, M., and Suratman, S.: PM2.5 and associated ionic species in a sub-urban coastal area of Kuala Terengganu, Southern South China Sea (Malaysia), Sains Malays., 42, 1065–1072, 2013a.
Tahir, N. M., Suratman, S., Fong, F. T., Hamzah, M. S., and Latif, M. T.: Temporal Distribution and Chemical Characterization of Atmospheric Particulate Matter in the Eastern Coast of Peninsular Malaysia, Aerosol Air Qual. Res., 13, 584–595, https://doi.org/10.4209/aaqr.2012.08.0216, 2013b.
Tai, A. P. K., Mickley, L. J., and Jacob, D. J.: Correlations between fine particulate matter (PM2.5) and meteorological variables in the United States: Implications for the sensitivity of PM2.5 to climate change, Atmos. Environ., 44, 3976–3984, https://doi.org/10.1016/j.atmosenv.2010.06.060, 2010.
Tai, A. P. K., Mickley, L. J., Jacob, D. J., Leibensperger, E. M., Zhang, L., Fisher, J. A., and Pye, H. O. T.: Meteorological modes of variability for fine particulate matter (PM2.5) air quality in the United States: implications for PM2.5 sensitivity to climate change, Atmos. Chem. Phys., 12, 3131–3145, https://doi.org/10.5194/acp-12-3131-2012, 2012.
Thurston, G. D., Ito, K., and Lall, R.: A source apportionment of US fine particulate matter air pollution, Atmos. Environ., 45, 3924–3936, https://doi.org/10.1016/j.atmosenv.2011.04.070, 2011.
USEPA: National Ambient Air Quality Standards (NAAQS): http://www.epa.gov/air/criteria.html, last access: 30 April 2015.
Vallius, M., Ruuskanen, J., and Pekkanen, J.: Comparison of multivariate source apportionment of urban PM2. 5 with chemical mass closure, Boreal Environ. Res., 13, 347–358, 2008.
Vecchi, R., Chiari, M., D'Alessandro, A., Fermo, P., Lucarelli, F., Mazzei, F., Nava, S., Piazzalunga, A., Prati, P., Silvani, F., and Valli, G.: A mass closure and PMF source apportionment study on the sub-micron sized aerosol fraction at urban sites in Italy, Atmos. Environ., 42, 2240–2253, 2008.
Viana, M., Kuhlbusch, T. A. J., Querol, X., Alastuey, A., Harrison, R. M., Hopke, P. K., Winiwarter, W., Vallius, M., Szidat, S., Prévôt, A. S. H., Hueglin, C., Bloemen, H., Wåhlin, P., Vecchi, R., Miranda, A. I., Kasper-Giebl, A., Maenhaut, W., and Hitzenberger, R.: Source apportionment of particulate matter in Europe: A review of methods and results, J. Aerosol Sci., 39, 827–849, https://doi.org/10.1016/j.jaerosci.2008.05.007, 2008.
Vieno, M., Heal, M. R., Hallsworth, S., Famulari, D., Doherty, R. M., Dore, A. J., Tang, Y. S., Braban, C. F., Leaver, D., Sutton, M. A., and Reis, S.: The role of long-range transport and domestic emissions in determining atmospheric secondary inorganic particle concentrations across the UK, Atmos. Chem. Phys., 14, 8435–8447, https://doi.org/10.5194/acp-14-8435-2014, 2014.
Viidanoja, J., Sillanpää, M., Laakia, J., Kerminen, V.-M., Hillamo, R., Aarnio, P., and Koskentalo, T.: Organic and black carbon in PM2.5 and PM10: 1 year of data from an urban site in Helsinki, Finland, Atmos. Environ., 36, 3183–3193, https://doi.org/10.1016/S1352-2310(02)00205-4, 2002.
Wagstrom, K. M. and Pandis, S. N.: Source–receptor relationships for fine particulate matter concentrations in the Eastern United States, Atmos. Environ., 45, 347–356, https://doi.org/10.1016/j.atmosenv.2010.10.019, 2011.
Wahid, N. B. A., Latif, M. T., and Suratman, S.: Composition and source apportionment of surfactants in atmospheric aerosols of urban and semi-urban areas in Malaysia, Chemosphere, 91, 1508–1516, https://doi.org/10.1016/j.chemosphere.2012.12.029, 2013.
Wåhlin, P., Berkowicz, R., and Palmgren, F.: Characterisation of traffic-generated particulate matter in Copenhagen, Atmos. Environ., 40, 2151–2159, https://doi.org/10.1016/j.atmosenv.2005.11.049, 2006.
Wang, Y., Zhuang, G., Sun, Y., and An, Z.: Water-soluble part of the aerosol in the dust storm season-evidence of the mixing between mineral and pollution aerosols, Atmos. Environ., 39, 7020–7029, https://doi.org/10.1016/j.atmosenv.2005.08.005, 2005.
Watson, J. G.: Visibility: Science and Regulation, J. Air Waste Manage., 52, 628–713, 2002.
Watson, J. G. and Chow, J. C.: Source characterization of major emission sources in the Imperial and Mexicali Valleys along the US/Mexico border, Sci. Total Environ., 276, 33–47, 2001.
Watson, J. G., Zhu, T., Chow, J. C., Engelbrecht, J., Fujita, E. M., and Wilson, W. E.: Receptor modeling application framework for particle source apportionment, Chemosphere, 49, 1093–1136, 2002.
WHO: WHO Air Quality Guidelines Global Updates 2005: Particulate matter, ozone, nitrogen dioxide and sulfur dioxide, Copenhagen, Denmark, 2006.
WHO: Health Effects of Particulate Matter, WHO Regional Office for Europe, UN City, Marmorvej 51, 2100 Copenhagen, Denmark, 2013.
Wiwolwattanapun, W., Hopke, P. K., and Pongkiatkul, P.: Source Apportionment and Potential Source Locations of PM2.5 and PM2.5-PM10 at Residential Sites in Metropolitan Bangkok, APR, 2, 172–181, https://doi.org/10.5094/APR.2011.022, 2011.
Ye, B., Ji, X., Yang, H., Yao, X., Chan, C. K., Cadle, S. H., Chan, T., and Mulawa, P. A.: Concentration and chemical composition of PM2.5 in Shanghai for a 1-year period, Atmos. Environ., 37, 499–510, 2003.
Yin, J., Allen, A. G., Harrison, R. M., Jennings, S. G., Wright, E., Fitzpatrick, M., Healy, T., Barry, E., Ceburnis, D., and McCusker, D.: Major component composition of urban PM10 and PM2.5 in Ireland, Atmos. Res., 78, 149–165, https://doi.org/10.1016/j.atmosres.2005.03.006, 2005.
Yin, J., Harrison, R. M., Chen, Q., Rutter, A., and Schauer, J. J.: Source apportionment of fine particles at urban background and rural sites in the UK atmosphere, Atmos. Environ., 44, 841–851, https://doi.org/10.1016/j.atmosenv.2009.11.026, 2010.
Yu, L., Wang, G., Zhang, R., Zhang, L., Song, Y., Wu, B., Li, X., An, K., and Chu, J.: Characterization and source apportionment of PM2.5 in an urban environment in Beijing, Aerosol Air Qual. Res., 13, 574–583, 2013.
Zaki, N. S., Barbooti, M. M., Baha-Uddin, S. S., and Hassan, E. B.: Determination of Trace Metals and Their Distribution in Heavy Crude Oil Distillates (350 °C+) by Atomic Absorption Spectrophotometry, Appl. Spectrosc., 43, 1257–1259, 1989.
Zhang, R., Jing, J., Tao, J., Hsu, S.-C., Wang, G., Cao, J., Lee, C. S. L., Zhu, L., Chen, Z., Zhao, Y., and Shen, Z.: Chemical characterization and source apportionment of PM2.5 in Beijing: seasonal perspective, Atmos. Chem. Phys., 13, 7053–7074, https://doi.org/10.5194/acp-13-7053-2013, 2013.
Zhang, T., Cao, J. J., Tie, X. X., Shen, Z. X., Liu, S. X., Ding, H., Han, Y. M., Wang, G. H., Ho, K. F., Qiang, J., and Li, W. T.: Water-soluble ions in atmospheric aerosols measured in Xi'an, China: Seasonal variations and sources, Atmos. Res., 102, 110–119, https://doi.org/10.1016/j.atmosres.2011.06.014, 2011.
Zhao, M., Zhang, Y., Ma, W., Fu, Q., Yang, X., Li, C., Zhou, B., Yu, Q., and Chen, L.: Characteristics and ship traffic source identification of air pollutants in China's largest port, Atmos. Environ., 64, 277–286, https://doi.org/10.1016/j.atmosenv.2012.10.007, 2013.
Zheng, J., He, M., Shen, X., Yin, S., and Yuan, Z.: High resolution of black carbon and organic carbon emissions in the Pearl River Delta region, China, Sci. Total Environ., 438, 189–200, https://doi.org/10.1016/j.scitotenv.2012.08.068, 2012.
Zheng, M., Salmon, L. G., Schauer, J. J., Zeng, L., Kiang, C. S., Zhang, Y., and Cassa, G. R.: Seasonal trends in PM2.5 source contributions in Beijing, China, Atmos. Environ., 39, 3967–3976, https://doi.org/10.1016/j.atmosenv.2005.03.036, 2005.
Short summary
This study investigates the PM2.5 variability in the Klang Valley urban-industrial environment. Source apportionment analysis reveals two major contributors of PM2.5 in the study area: secondary inorganic aerosols and biomass burning. The chemical constituents and sources of PM2.5 in this study area were greatly influenced and characterised by meteorological and gaseous parameters which largely vary with season.
This study investigates the PM2.5 variability in the Klang Valley urban-industrial environment....
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