Articles | Volume 16, issue 5
https://doi.org/10.5194/acp-16-2943-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-16-2943-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
08 Mar 2016
Research article |
| 08 Mar 2016
In situ secondary organic aerosol formation from ambient pine forest air using an oxidation flow reactor
Brett B. Palm
Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, CO, USA
Department of Chemistry and Biochemistry, University of Colorado, Boulder, CO, USA
Pedro Campuzano-Jost
Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, CO, USA
Department of Chemistry and Biochemistry, University of Colorado, Boulder, CO, USA
Amber M. Ortega
Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, CO, USA
Department of Atmospheric and Oceanic Science, University of Colorado, Boulder, CO, USA
Douglas A. Day
Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, CO, USA
Department of Chemistry and Biochemistry, University of Colorado, Boulder, CO, USA
Lisa Kaser
National Center for Atmospheric Research, Boulder, CO, USA
Institute of Ion Physics and Applied Physics, University of Innsbruck, Innsbruck, Austria
Werner Jud
Institute of Ion Physics and Applied Physics, University of Innsbruck, Innsbruck, Austria
Thomas Karl
Institute of Meteorology and Geophysics, University of Innsbruck, Innsbruck, Austria
Armin Hansel
Institute of Ion Physics and Applied Physics, University of Innsbruck, Innsbruck, Austria
James F. Hunter
Department of Civil and Environmental Engineering, Massachusetts Institute of Technology, Cambridge, MA, USA
Eben S. Cross
Department of Civil and Environmental Engineering, Massachusetts Institute of Technology, Cambridge, MA, USA
Jesse H. Kroll
Department of Civil and Environmental Engineering, Massachusetts Institute of Technology, Cambridge, MA, USA
Department of Chemical Engineering, Massachusetts Institute of Technology, Cambridge, MA, USA
Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, CO, USA
Department of Chemistry and Biochemistry, University of Colorado, Boulder, CO, USA
William H. Brune
Department of Meteorology, Pennsylvania State University, State College, PA, USA
Jose L. Jimenez
CORRESPONDING AUTHOR
Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, CO, USA
Department of Chemistry and Biochemistry, University of Colorado, Boulder, CO, USA
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115 citations as recorded by crossref.
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- The Chemical Characteristics and Formation of Potential Secondary Aerosol (PSA) using an Oxidation Flow Reactor (OFR) in the Summer: Focus on the Residential Area, Suwon G. Park et al. 10.5572/KOSAE.2019.35.6.786
- Composition and volatility of secondary organic aerosol (SOA) formed from oxidation of real tree emissions compared to simplified volatile organic compound (VOC) systems A. Ylisirniö et al. 10.5194/acp-20-5629-2020
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- Products and Secondary Organic Aerosol Yields from the OH and NO3 Radical-Initiated Oxidation of Resorcinol Z. Finewax et al. 10.1021/acsearthspacechem.9b00112
- Non-OH chemistry in oxidation flow reactors for the study of atmospheric chemistry systematically examined by modeling Z. Peng et al. 10.5194/acp-16-4283-2016
- Photochemical aging process on PM2.5 bound PAHs emission from solid fuel combustion in traditional and improved stoves Y. Zhang et al. 10.1016/j.atmosres.2021.105807
- Secondary organic aerosol formation from in situ OH, O<sub>3</sub>, and NO<sub>3</sub> oxidation of ambient forest air in an oxidation flow reactor B. Palm et al. 10.5194/acp-17-5331-2017
- Evaluating the impact of new observational constraints on P-S/IVOC emissions, multi-generation oxidation, and chamber wall losses on SOA modeling for Los Angeles, CA P. Ma et al. 10.5194/acp-17-9237-2017
- Comparison of secondary organic aerosol formation from toluene on initially wet and dry ammonium sulfate particles at moderate relative humidity T. Liu et al. 10.5194/acp-18-5677-2018
- Volatile oxidation products and secondary organosiloxane aerosol from D5 + OH at varying OH exposures H. Kang et al. 10.5194/acp-23-14307-2023
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- Oxidation Flow Reactor Results in a Chinese Megacity Emphasize the Important Contribution of S/IVOCs to Ambient SOA Formation W. Hu et al. 10.1021/acs.est.1c03155
- Model Evaluation of New Techniques for Maintaining High-NO Conditions in Oxidation Flow Reactors for the Study of OH-Initiated Atmospheric Chemistry Z. Peng et al. 10.1021/acsearthspacechem.7b00070
- Atmospheric photochemistry and secondary aerosol formation of urban air in Lyon, France S. Sbai et al. 10.1016/j.jes.2020.06.037
- Contrasting impacts of humidity on the ozonolysis of monoterpenes: insights into the multi-generation chemical mechanism S. Zhang et al. 10.5194/acp-23-10809-2023
- Comparison of primary and secondary particle formation from natural gas engine exhaust and of their volatility characteristics J. Alanen et al. 10.5194/acp-17-8739-2017
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Short summary
Ambient pine forest air was oxidized by OH radicals in a PAM oxidation flow reactor during the BEACHON-RoMBAS campaign to study secondary organic aerosol formation. Approximately 4.4 times more secondary organic aerosol was formed in the reactor than could be explained by the volatile organic gases (VOCs) measured in ambient air. The organic aerosol formation can be explained by including an SOA yield from typically unmeasured semivolatile and intermediate-volatility organic gases (S/IVOCs).
Ambient pine forest air was oxidized by OH radicals in a PAM oxidation flow reactor during the...
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