Articles | Volume 16, issue 5
https://doi.org/10.5194/acp-16-2943-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-16-2943-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
In situ secondary organic aerosol formation from ambient pine forest air using an oxidation flow reactor
Brett B. Palm
Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, CO, USA
Department of Chemistry and Biochemistry, University of Colorado, Boulder, CO, USA
Pedro Campuzano-Jost
Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, CO, USA
Department of Chemistry and Biochemistry, University of Colorado, Boulder, CO, USA
Amber M. Ortega
Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, CO, USA
Department of Atmospheric and Oceanic Science, University of Colorado, Boulder, CO, USA
Douglas A. Day
Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, CO, USA
Department of Chemistry and Biochemistry, University of Colorado, Boulder, CO, USA
Lisa Kaser
National Center for Atmospheric Research, Boulder, CO, USA
Institute of Ion Physics and Applied Physics, University of Innsbruck, Innsbruck, Austria
Werner Jud
Institute of Ion Physics and Applied Physics, University of Innsbruck, Innsbruck, Austria
Thomas Karl
Institute of Meteorology and Geophysics, University of Innsbruck, Innsbruck, Austria
Armin Hansel
Institute of Ion Physics and Applied Physics, University of Innsbruck, Innsbruck, Austria
James F. Hunter
Department of Civil and Environmental Engineering, Massachusetts Institute of Technology, Cambridge, MA, USA
Eben S. Cross
Department of Civil and Environmental Engineering, Massachusetts Institute of Technology, Cambridge, MA, USA
Jesse H. Kroll
Department of Civil and Environmental Engineering, Massachusetts Institute of Technology, Cambridge, MA, USA
Department of Chemical Engineering, Massachusetts Institute of Technology, Cambridge, MA, USA
Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, CO, USA
Department of Chemistry and Biochemistry, University of Colorado, Boulder, CO, USA
William H. Brune
Department of Meteorology, Pennsylvania State University, State College, PA, USA
Jose L. Jimenez
CORRESPONDING AUTHOR
Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, CO, USA
Department of Chemistry and Biochemistry, University of Colorado, Boulder, CO, USA
Data sets
Manitou Experimental Forest Observatory Field Campaign UCAR/NCAR - Atmospheric Chemistry Observations and Modeling https://doi.org/10.5065/D61V5CDP
Short summary
Ambient pine forest air was oxidized by OH radicals in a PAM oxidation flow reactor during the BEACHON-RoMBAS campaign to study secondary organic aerosol formation. Approximately 4.4 times more secondary organic aerosol was formed in the reactor than could be explained by the volatile organic gases (VOCs) measured in ambient air. The organic aerosol formation can be explained by including an SOA yield from typically unmeasured semivolatile and intermediate-volatility organic gases (S/IVOCs).
Ambient pine forest air was oxidized by OH radicals in a PAM oxidation flow reactor during the...
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