Articles | Volume 15, issue 20
https://doi.org/10.5194/acp-15-11835-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-15-11835-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Solar geoengineering using solid aerosol in the stratosphere
D. K. Weisenstein
CORRESPONDING AUTHOR
School of Engineering and Applied Science, Harvard University, Cambridge, MA, USA
D. W. Keith
School of Engineering and Applied Science, Harvard University, Cambridge, MA, USA
Kennedy School of Government, Harvard University, Cambridge, MA, USA
J. A. Dykema
School of Engineering and Applied Science, Harvard University, Cambridge, MA, USA
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69 citations as recorded by crossref.
- Diagnosing the radiative and chemical contributions to future changes in tropical column ozone with the UM-UKCA chemistry–climate model J. Keeble et al. 10.5194/acp-17-13801-2017
- Retrieval of volcanic and man-made stratospheric aerosols from orbital polarimetric measurements M. Mishchenko et al. 10.1364/OE.27.00A158
- Initial velocity and position effect on dynamics of settling particles of variable sizes S. Ghosh et al. 10.1140/epjp/s13360-024-04935-4
- The Climatic Effects of Hygroscopic Growth of Sulfate Aerosols in the Stratosphere K. Krishnamohan et al. 10.1029/2019EF001326
- Solar Geoengineering Modeling and Applications for Mitigating Global Warming: Assessing Key Parameters and the Urban Heat Island Influence A. Feinberg 10.3389/fclim.2022.870071
- Geoengineering with stratospheric aerosols: What do we not know after a decade of research? D. MacMartin et al. 10.1002/2016EF000418
- Removal of non-CO 2 greenhouse gases by large-scale atmospheric solar photocatalysis R. de_Richter et al. 10.1016/j.pecs.2017.01.001
- The Climate and Ozone Impacts of Black Carbon Emissions From Global Rocket Launches C. Maloney et al. 10.1029/2021JD036373
- Relevant climate response tests for stratospheric aerosol injection: A combined ethical and scientific analysis G. Lenferna et al. 10.1002/2016EF000504
- A fully coupled solid-particle microphysics scheme for stratospheric aerosol injections within the aerosol–chemistry–climate model SOCOL-AERv2 S. Vattioni et al. 10.5194/gmd-17-7767-2024
- Diamond-doped silica aerogel for solar geoengineering J. Vukajlovic et al. 10.1016/j.diamond.2021.108474
- Exploring accumulation-mode H<sub>2</sub>SO<sub>4</sub> versus SO<sub>2</sub> stratospheric sulfate geoengineering in a sectional aerosol–chemistry–climate model S. Vattioni et al. 10.5194/acp-19-4877-2019
- Reactivity of the Intramolecular Vicinal Group-13/P- and B/Group-15-Based Frustrate Lewis Pairs with Sulfur Dioxide: Mechanistic Insight from DFT Z. Zhang & M. Su 10.1021/acs.inorgchem.3c01611
- Hydrological Consequences of Solar Geoengineering K. Ricke et al. 10.1146/annurev-earth-031920-083456
- Modulating the Transmission of Light Using Asymmetric Janus Particles P. Sullivan et al. 10.1002/adom.202400419
- The cost of stratospheric climate engineering revisited R. Moriyama et al. 10.1007/s11027-016-9723-y
- Experimental reaction rates constrain estimates of ozone response to calcium carbonate geoengineering Z. Dai et al. 10.1038/s43247-020-00058-7
- An interactive stratospheric aerosol model intercomparison of solar geoengineering by stratospheric injection of SO<sub>2</sub> or accumulation-mode sulfuric acid aerosols D. Weisenstein et al. 10.5194/acp-22-2955-2022
- Heterogeneous reaction of ClONO<sub>2</sub> with TiO<sub>2</sub> and SiO<sub>2</sub> aerosol particles: implications for stratospheric particle injection for climate engineering M. Tang et al. 10.5194/acp-16-15397-2016
- Stratospheric solar geoengineering without ozone loss D. Keith et al. 10.1073/pnas.1615572113
- The Engineering of Climate Engineering D. MacMartin & B. Kravitz 10.1146/annurev-control-053018-023725
- Sensitivity of the radiative forcing by stratospheric sulfur geoengineering to the amount and strategy of the SO<sub>2</sub>injection studied with the LMDZ-S3A model C. Kleinschmitt et al. 10.5194/acp-18-2769-2018
- Models for Simulation of Fractal-like Particle Clusters with Prescribed Fractal Dimension O. Tomchuk 10.3390/fractalfract7120866
- Effects of Aluminum/Carbon and Morphology on Optical Characteristics and Radiative Forcing of Alumina Clusters Emitted by Solid Rockets in the Stratosphere Y. Xu et al. 10.3390/atmos15070812
- The importance of the local structure of fractal aggregates R. Botet et al. 10.1088/1751-8121/ad2c82
- Applying orbital multi-angle photopolarimetric observations to study properties of aerosols in the Earth's atmosphere: Implications of measurements in the 1.378 µm spectral channel to retrieve microphysical characteristics and composition of stratospheric aerosols J. Dlugach et al. 10.1016/j.jqsrt.2020.107483
- Overlooked Long‐Term Atmospheric Chemical Feedbacks Alter the Impact of Solar Geoengineering: Implications for Tropospheric Oxidative Capacity J. Moch et al. 10.1029/2023AV000911
- Governance of Highly Decentralized Nonstate Actors: The Case of Solar Geoengineering J. Reynolds & G. Wagner 10.2139/ssrn.3471699
- Aerosol Dynamics in the Near Field of the SCoPEx Stratospheric Balloon Experiment C. Golja et al. 10.1029/2020JD033438
- A Critical Examination of Geoengineering: Economic and Technological Rationality in Social Context R. Gunderson et al. 10.3390/su10010269
- Interactions of Water with Mineral Dust Aerosol: Water Adsorption, Hygroscopicity, Cloud Condensation, and Ice Nucleation M. Tang et al. 10.1021/acs.chemrev.5b00529
- First Simulations of Designing Stratospheric Sulfate Aerosol Geoengineering to Meet Multiple Simultaneous Climate Objectives B. Kravitz et al. 10.1002/2017JD026874
- Response of Surface Ultraviolet and Visible Radiation to Stratospheric SO2 Injections S. Madronich et al. 10.3390/atmos9110432
- Spectroscopic Characterization of HSO2• and HOSO• Intermediates Involved in SO2 Geoengineering B. Lu et al. 10.1021/acs.jpca.1c09311
- Sensitivity of tropical monsoon precipitation to the latitude of stratospheric aerosol injections K. Krishnamohan & G. Bala 10.1007/s00382-021-06121-z
- An overview of the Earth system science of solar geoengineering P. Irvine et al. 10.1002/wcc.423
- Coupling free radical catalysis, climate change, and human health J. Anderson & C. Clapp 10.1039/C7CP08331A
- The potential environmental and climate impacts of stratospheric aerosol injection: a review H. Huynh & V. McNeill 10.1039/D3EA00134B
- Sulfur in the Sky with Diamonds: An Inquiry into the Feasibility of Solar Geoengineering M. Grasso 10.1111/1758-5899.12646
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- Climate engineering and the ocean: effects on biogeochemistry and primary production S. Lauvset et al. 10.5194/bg-14-5675-2017
- Mie scattering from optically levitated mixed sulfuric acid–silica core–shell aerosols: observation of core–shell morphology for atmospheric science M. McGrory et al. 10.1039/D1CP04068E
- Quantifying the temperature-independent effect of stratospheric aerosol geoengineering on global-mean precipitation in a multi-model ensemble A. Ferraro & H. Griffiths 10.1088/1748-9326/11/3/034012
- Climate system response to stratospheric sulfate aerosols: sensitivity to altitude of aerosol layer K. Krishnamohan et al. 10.5194/esd-10-885-2019
- Stratospheric ozone changes under solar geoengineering: implications for UV exposure and air quality P. Nowack et al. 10.5194/acp-16-4191-2016
- Stratospheric aerosol injection may impact global systems and human health outcomes S. Tracy et al. 10.1525/elementa.2022.00047
- Towards a comprehensive climate impacts assessment of solar geoengineering P. Irvine et al. 10.1002/2016EF000389
- Climate Response to Aerosol Geoengineering: A Multimethod Comparison H. Muri et al. 10.1175/JCLI-D-17-0620.1
- Highly decentralized solar geoengineering J. Reynolds & G. Wagner 10.1080/09644016.2019.1648169
- Development of geopolitically relevant ranking criteria for geoengineering methods P. Boyd 10.1002/2016EF000447
- The cost of stratospheric aerosol injection through 2100 W. Smith 10.1088/1748-9326/aba7e7
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- Spectroscopy and Photochemistry of Aluminum-Bearing Species in the Universe T. Trabelsi et al. 10.1021/acs.accounts.3c00481
- Chemical Impact of Stratospheric Alumina Particle Injection for Solar Radiation Modification and Related Uncertainties S. Vattioni et al. 10.1029/2023GL105889
- Radiative and chemical implications of the size and composition of aerosol particles in the existing or modified global stratosphere D. Murphy et al. 10.5194/acp-21-8915-2021
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- Climate scientists ponder spraying diamond dust in the sky to cool planet A. Extance 10.1038/nature.2015.18634
- Solar geoengineering reduces atmospheric carbon burden D. Keith et al. 10.1038/nclimate3376
- Heterogeneous Reactivity of HCl on CaCO3 Aerosols at Stratospheric Temperature H. Huynh & V. McNeill 10.1021/acsearthspacechem.1c00151
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- Stratospheric ozone over the United States in summer linked to observations of convection and temperature via chlorine and bromine catalysis J. Anderson et al. 10.1073/pnas.1619318114
- Heterogeneous Chemistry of CaCO3 Aerosols with HNO3 and HCl H. Huynh & V. McNeill 10.1021/acs.jpca.9b11691
- Improved aerosol radiative properties as a foundation for solar geoengineering risk assessment J. Dykema et al. 10.1002/2016GL069258
- Legitimacy and Non-Domination in Solar Radiation Management Research P. Smith 10.1080/21550085.2018.1562528
2 citations as recorded by crossref.
- Fighting global warming by greenhouse gas removal: destroying atmospheric nitrous oxide thanks to synergies between two breakthrough technologies T. Ming et al. 10.1007/s11356-016-6103-9
- What is the limit of climate engineering by stratospheric injection of SO<sub>2</sub>? U. Niemeier & C. Timmreck 10.5194/acp-15-9129-2015
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Short summary
We investigate stratospheric aerosol geoengineering with solid particle injection by modeling the fractal structure of alumina aerosols and their interaction with background sulfate. We analyze the efficacy (W m^-2 of radiative forcing per megaton of injection) and risks (ozone loss, s) for both alumina and diamond particles as a function of injected monomer radius, finding 240nm alumina and 160nm diamond optimal. We discuss the limitations of our 2-D model study and associated uncertainties.
We investigate stratospheric aerosol geoengineering with solid particle injection by modeling...
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