Articles | Volume 14, issue 22
https://doi.org/10.5194/acp-14-12513-2014
© Author(s) 2014. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-14-12513-2014
© Author(s) 2014. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Competition between water uptake and ice nucleation by glassy organic aerosol particles
Faculty of Chemistry, Bielefeld University, Bielefeld, Germany
Multiphase Chemistry Department, Max Planck Institute for Chemistry, Mainz, Germany
M. Shiraiwa
Multiphase Chemistry Department, Max Planck Institute for Chemistry, Mainz, Germany
U. Pöschl
Multiphase Chemistry Department, Max Planck Institute for Chemistry, Mainz, Germany
Faculty of Chemistry, Bielefeld University, Bielefeld, Germany
Viewed
Total article views: 7,969 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 20 Jun 2014)
HTML | XML | Total | BibTeX | EndNote | |
---|---|---|---|---|---|
3,202 | 4,594 | 173 | 7,969 | 99 | 132 |
- HTML: 3,202
- PDF: 4,594
- XML: 173
- Total: 7,969
- BibTeX: 99
- EndNote: 132
Total article views: 4,235 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 27 Nov 2014)
HTML | XML | Total | BibTeX | EndNote | |
---|---|---|---|---|---|
2,475 | 1,652 | 108 | 4,235 | 88 | 128 |
- HTML: 2,475
- PDF: 1,652
- XML: 108
- Total: 4,235
- BibTeX: 88
- EndNote: 128
Total article views: 3,734 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 20 Jun 2014)
HTML | XML | Total | BibTeX | EndNote | |
---|---|---|---|---|---|
727 | 2,942 | 65 | 3,734 | 11 | 4 |
- HTML: 727
- PDF: 2,942
- XML: 65
- Total: 3,734
- BibTeX: 11
- EndNote: 4
Cited
130 citations as recorded by crossref.
- Ice nucleation ability of ammonium sulfate aerosol particles internally mixed with secondary organics B. Bertozzi et al. 10.5194/acp-21-10779-2021
- Heterogeneous ice nucleation of viscous secondary organic aerosol produced from ozonolysis of <i>α</i>-pinene K. Ignatius et al. 10.5194/acp-16-6495-2016
- Viscous organic aerosol particles in the upper troposphere: diffusivity-controlled water uptake and ice nucleation? D. Lienhard et al. 10.5194/acp-15-13599-2015
- Is Ice Formation by Sea Spray Particles at Cirrus Temperatures Controlled by Crystalline Salts? R. Patnaude et al. 10.1021/acsearthspacechem.1c00228
- Ozonolysis Chemistry and Phase Behavior of 1-Octen-3-ol-Derived Secondary Organic Aerosol K. Fischer et al. 10.1021/acsearthspacechem.0c00092
- Direct observation and assessment of phase states of ambient and lab-generated sub-micron particles upon humidification Z. Cheng et al. 10.1039/D1RA02530A
- Predicting Atmospheric Particle Phase State Using an Explainable Machine Learning Approach Based on Particle Rebound Measurements Y. Qiu et al. 10.1021/acs.est.3c05284
- Water diffusion in atmospherically relevant α-pinene secondary organic material H. Price et al. 10.1039/C5SC00685F
- Progress in the Analysis of Complex Atmospheric Particles A. Laskin et al. 10.1146/annurev-anchem-071015-041521
- Reactive Uptake of Isoprene Epoxydiols Increases the Viscosity of the Core of Phase-Separated Aerosol Particles N. Olson et al. 10.1021/acsearthspacechem.9b00138
- Vapor Condensed and Supercooled Glassy Nanoclusters W. Qi & R. Bowles 10.1021/acsnano.5b07391
- Solid organic-coated ammonium sulfate particles at high relative humidity in the summertime Arctic atmosphere R. Kirpes et al. 10.1073/pnas.2104496119
- Multiphase Chemistry at the Atmosphere–Biosphere Interface Influencing Climate and Public Health in the Anthropocene U. Pöschl & M. Shiraiwa 10.1021/cr500487s
- Amorphous phase state diagrams and viscosity of ternary aqueous organic/organic and inorganic/organic mixtures A. Marsh et al. 10.1039/C8CP00760H
- The Significant Role of New Particle Composition and Morphology on the HNO3-Driven Growth of Particles down to Sub-10 nm Y. Li et al. 10.1021/acs.est.3c09454
- Liquid–Liquid Phase Separation Can Drive Aerosol Droplet Growth in Supersaturated Regimes K. Malek et al. 10.1021/acsenvironau.3c00015
- Heterogeneous ice nucleation ability of aerosol particles generated from Arctic sea surface microlayer and surface seawater samples at cirrus temperatures R. Wagner et al. 10.5194/acp-21-13903-2021
- Coalescence-based assessment of aerosol phase state using dimers prepared through a dual-differential mobility analyzer technique N. Rothfuss & M. Petters 10.1080/02786826.2016.1221050
- Particle Size Distribution Dynamics Can Help Constrain the Phase State of Secondary Organic Aerosol Y. He et al. 10.1021/acs.est.0c05796
- Modelling the effect of condensed-phase diffusion on the homogeneous nucleation of ice in ultra-viscous particles K. Fowler et al. 10.5194/acp-20-683-2020
- Effect of varying experimental conditions on the viscosity of <i>α</i>-pinene derived secondary organic material J. Grayson et al. 10.5194/acp-16-6027-2016
- Role of Organic Hydrocarbons in Atmospheric Ice Formation via Contact Freezing K. Collier & S. Brooks 10.1021/acs.jpca.6b11890
- Heterogeneous ice nucleation of α‐pinene SOA particles before and after ice cloud processing R. Wagner et al. 10.1002/2016JD026401
- Relative humidity-dependent viscosities of isoprene-derived secondary organic material and atmospheric implications for isoprene-dominant forests M. Song et al. 10.5194/acp-15-5145-2015
- Multicomponent diffusion in atmospheric aerosol particles B. Wallace et al. 10.1039/D0EA00008F
- Isomeric Identification of the Nitroindole Chromophore in Indole + NO3 Organic Aerosol A. Dalton et al. 10.1021/acsphyschemau.4c00044
- Equilibration times in viscous and viscoelastic aerosol particles T. Preston & A. Zuend 10.1039/D2EA00065B
- Observation of viscosity transition in <i>α</i>-pinene secondary organic aerosol E. Järvinen et al. 10.5194/acp-16-4423-2016
- Quantifying the Viscosity of Individual Submicrometer Semisolid Particles Using Atomic Force Microscopy C. Madawala et al. 10.1021/acs.analchem.3c01835
- The dependence of soot particle ice nucleation ability on its volatile content K. Gao et al. 10.1039/D2EM00158F
- The efficiency of secondary organic aerosol particles acting as ice-nucleating particles under mixed-phase cloud conditions W. Frey et al. 10.5194/acp-18-9393-2018
- Temperature‐ and Humidity‐Dependent Phase States of Secondary Organic Aerosols S. Petters et al. 10.1029/2018GL080563
- MIMiX: a Multipurpose In situ Microreactor system for X-ray microspectroscopy to mimic atmospheric aerosol processing J. Förster et al. 10.5194/amt-13-3717-2020
- The Influence of Absolute Mass Loading of Secondary Organic Aerosols on Their Phase State S. Jain et al. 10.3390/atmos9040131
- Models of Isotopic Water Diffusion in Spherical Aerosol Particles A. Moridnejad & T. Preston 10.1021/acs.jpca.6b11241
- Wildfire smoke, Arctic haze, and aerosol effects on mixed-phase and cirrus clouds over the North Pole region during MOSAiC: an introduction R. Engelmann et al. 10.5194/acp-21-13397-2021
- Atmospheric Humic‐Like Substances (HULIS) Act as Ice Active Entities J. Chen et al. 10.1029/2021GL092443
- Kinetically controlled glass transition measurement of organic aerosol thin films using broadband dielectric spectroscopy Y. Zhang et al. 10.5194/amt-11-3479-2018
- Glass Formation Processes in Mixed Inorganic/Organic Aerosol Particles H. Dette & T. Koop 10.1021/jp5106967
- Physicochemical Mixing State of Sea Spray Aerosols: Morphologies Exhibit Size Dependence H. Lee et al. 10.1021/acsearthspacechem.0c00153
- Molecular and physical characteristics of aerosol at a remote free troposphere site: implications for atmospheric aging S. Schum et al. 10.5194/acp-18-14017-2018
- Dynamics and Sorption Kinetics of Methanol Monomers and Clusters on Nopinone Surfaces X. Kong et al. 10.1021/acs.jpca.1c02309
- Ice nucleation by water-soluble macromolecules B. Pummer et al. 10.5194/acp-15-4077-2015
- Hydration of Atmospheric Molecular Clusters II: Organic Acid–Water Clusters J. Kildgaard et al. 10.1021/acs.jpca.8b07713
- Characterization of the temperature and humidity-dependent phase diagram of amorphous nanoscale organic aerosols N. Rothfuss & M. Petters 10.1039/C6CP08593H
- New investigations on homogeneous ice nucleation: the effects of water activity and water saturation formulations M. Baumgartner et al. 10.5194/acp-22-65-2022
- Particle phase-state variability in the North Atlantic free troposphere during summertime is determined by atmospheric transport patterns and sources Z. Cheng et al. 10.5194/acp-22-9033-2022
- Enhanced Ice Nucleation of Simulated Sea Salt Particles with the Addition of Anthropogenic Per- and Polyfluoroalkyl Substances M. Wolf et al. 10.1021/acsearthspacechem.1c00138
- Discontinuities in hygroscopic growth below and above water saturation for laboratory surrogates of oligomers in organic atmospheric aerosols N. Hodas et al. 10.5194/acp-16-12767-2016
- A continuous flow diffusion chamber study of sea salt particles acting as cloud nuclei: deliquescence and ice nucleation X. Kong et al. 10.1080/16000889.2018.1463806
- Toward closure between predicted and observed particle viscosity over a wide range of temperatures and relative humidity S. Kasparoglu et al. 10.5194/acp-21-1127-2021
- Effect of Acidity on Ice Nucleation by Inorganic–Organic Mixed Droplets Z. Lei et al. 10.1021/acsearthspacechem.3c00242
- The viscosity of atmospherically relevant organic particles J. Reid et al. 10.1038/s41467-018-03027-z
- Cloud Activation via Formation of Water and Ice on Various Types of Porous Aerosol Particles E. Jantsch & T. Koop 10.1021/acsearthspacechem.0c00330
- Nanomechanics and Morphology of Simulated Respiratory Particles R. Groth et al. 10.1021/acs.est.2c01829
- Glass Transition Temperatures of Organic Mixtures from Isoprene Epoxydiol-Derived Secondary Organic Aerosol B. Chen et al. 10.1021/acs.jpca.2c08936
- Hygroscopic behavior of aerosols generated from solutions of 3-methyl-1,2,3-butanetricarboxylic acid, its sodium salts, and its mixtures with NaCl L. Wu et al. 10.5194/acp-20-14103-2020
- Diffusion coefficients of organic molecules in sucrose–water solutions and comparison with Stokes–Einstein predictions Y. Chenyakin et al. 10.5194/acp-17-2423-2017
- Recent advances in understanding secondary organic aerosol: Implications for global climate forcing M. Shrivastava et al. 10.1002/2016RG000540
- Predicting the refractive index of amorphous materials using the Bruggeman effective medium approximation M. Sela & C. Haspel 10.1364/AO.402103
- Wildfire smoke triggers cirrus formation: lidar observations over the eastern Mediterranean R. Mamouri et al. 10.5194/acp-23-14097-2023
- The Role of Organic Aerosol in Atmospheric Ice Nucleation: A Review D. Knopf et al. 10.1021/acsearthspacechem.7b00120
- Ice nucleation on surrogates of boreal forest SOA particles: effect of water content and oxidative age A. Piedehierro et al. 10.5194/acp-21-11069-2021
- The effect of viscosity and diffusion on the HO<sub>2</sub> uptake by sucrose and secondary organic aerosol particles P. Lakey et al. 10.5194/acp-16-13035-2016
- Viscosity controls humidity dependence of N<sub>2</sub>O<sub>5</sub> uptake to citric acid aerosol G. Gržinić et al. 10.5194/acp-15-13615-2015
- Volatility and Viscosity Are Correlated in Terpene Secondary Organic Aerosol Formed in a Flow Reactor W. Champion et al. 10.1021/acs.estlett.9b00412
- Micro-spectroscopic and freezing characterization of ice-nucleating particles collected in the marine boundary layer in the eastern North Atlantic D. Knopf et al. 10.5194/acp-22-5377-2022
- Diurnal and Seasonal Variations in the Phase State of Secondary Organic Aerosol Material over the Contiguous US Simulated in CMAQ Y. Li et al. 10.1021/acsearthspacechem.1c00094
- Low-temperature ice nucleation of sea spray and secondary marine aerosols under cirrus cloud conditions R. Patnaude et al. 10.5194/acp-24-911-2024
- Bouncier Particles at Night: Biogenic Secondary Organic Aerosol Chemistry and Sulfate Drive Diel Variations in the Aerosol Phase in a Mixed Forest J. Slade et al. 10.1021/acs.est.8b07319
- Multiphase Atmospheric Chemistry in Liquid Water: Impacts and Controllability of Organic Aerosol A. Carlton et al. 10.1021/acs.accounts.0c00301
- Emerging investigator series: surfactants, films, and coatings on atmospheric aerosol particles: a review K. Wokosin et al. 10.1039/D2EA00003B
- Heterogeneous Ice Nucleation in the Tropical Tropopause Layer E. Jensen et al. 10.1029/2018JD028949
- A biogenic secondary organic aerosol source of cirrus ice nucleating particles M. Wolf et al. 10.1038/s41467-020-18424-6
- Ice cloud formation potential by free tropospheric particles from long‐range transport over the Northern Atlantic Ocean S. China et al. 10.1002/2016JD025817
- Phase transition observations and discrimination of small cloud particles by light polarization in expansion chamber experiments L. Nichman et al. 10.5194/acp-16-3651-2016
- Diffusion and reactivity in ultraviscous aerosol and the correlation with particle viscosity F. Marshall et al. 10.1039/C5SC03223G
- Heterogeneous oxidation of amorphous organic aerosol surrogates by O<sub>3</sub>, NO<sub>3</sub>, and OH at typical tropospheric temperatures J. Li et al. 10.5194/acp-20-6055-2020
- Condensation Kinetics of Water on Amorphous Aerosol Particles N. Rothfuss et al. 10.1021/acs.jpclett.8b01365
- Physicochemical characterization of free troposphere and marine boundary layer ice-nucleating particles collected by aircraft in the eastern North Atlantic D. Knopf et al. 10.5194/acp-23-8659-2023
- A predictive group-contribution model for the viscosity of aqueous organic aerosol N. Gervasi et al. 10.5194/acp-20-2987-2020
- Unified Description of Diffusion Coefficients from Small to Large Molecules in Organic–Water Mixtures E. Evoy et al. 10.1021/acs.jpca.9b11271
- The characterization of long-range transported North American biomass burning plumes: what can a multi-wavelength Mie–Raman-polarization-fluorescence lidar provide? Q. Hu et al. 10.5194/acp-22-5399-2022
- Anthropogenic influences on the physical state of submicron particulate matter over a tropical forest A. Bateman et al. 10.5194/acp-17-1759-2017
- Phase State and Deliquescence Hysteresis of Ammonium-Sulfate-Seeded Secondary Organic Aerosol E. Saukko et al. 10.1080/02786826.2015.1050085
- Investigating the Heterogeneous Ice Nucleation of Sea Spray Aerosols Using Prochlorococcus as a Model Source of Marine Organic Matter M. Wolf et al. 10.1021/acs.est.8b05150
- Temperature effect on phase state and reactivity controls atmospheric multiphase chemistry and transport of PAHs Q. Mu et al. 10.1126/sciadv.aap7314
- Probing the Water Uptake and Phase State of Individual Sucrose Nanoparticles Using Atomic Force Microscopy C. Madawala et al. 10.1021/acsearthspacechem.1c00101
- Multiphase Chemical Kinetics of OH Radical Uptake by Molecular Organic Markers of Biomass Burning Aerosols: Humidity and Temperature Dependence, Surface Reaction, and Bulk Diffusion A. Arangio et al. 10.1021/jp510489z
- Radiative forcing of anthropogenic aerosols on cirrus clouds using a hybrid ice nucleation scheme J. Zhu & J. Penner 10.5194/acp-20-7801-2020
- Global Distribution of the Phase State and Mixing Times within Secondary Organic Aerosol Particles in the Troposphere Based on Room-Temperature Viscosity Measurements A. Maclean et al. 10.1021/acsearthspacechem.1c00296
- Ozone uptake on glassy, semi-solid and liquid organic matter and the role of reactive oxygen intermediates in atmospheric aerosol chemistry T. Berkemeier et al. 10.1039/C6CP00634E
- Indirect Effects of Secondary Organic Aerosol on Cirrus Clouds J. Zhu & J. Penner 10.1029/2019JD032233
- Atomic Force Microscopy: An Emerging Tool in Measuring the Phase State and Surface Tension of Individual Aerosol Particles H. Lee & A. Tivanski 10.1146/annurev-physchem-090419-110133
- Effects of volatility, viscosity, and non-ideality on particle–particle mixing timescales of secondary organic aerosols M. Schervish et al. 10.1080/02786826.2023.2256827
- Predicting the glass transition temperature and viscosity of secondary organic material using molecular composition W. DeRieux et al. 10.5194/acp-18-6331-2018
- Particulate matter, air quality and climate: lessons learned and future needs S. Fuzzi et al. 10.5194/acp-15-8217-2015
- The effects of morphology, mobility size, and secondary organic aerosol (SOA) material coating on the ice nucleation activity of black carbon in the cirrus regime C. Zhang et al. 10.5194/acp-20-13957-2020
- Estimation of secondary organic aerosol viscosity from explicit modeling of gas-phase oxidation of isoprene and <i>α</i>-pinene T. Galeazzo et al. 10.5194/acp-21-10199-2021
- Hygroscopic behavior of inorganic–organic aerosol systems including ammonium sulfate, dicarboxylic acids, and oligomer H. Bouzidi et al. 10.1016/j.atmosenv.2020.117481
- Water Uptake and Loss in Viscous Aerosol Particles with Concentration-Dependent Diffusivities B. Wallace & T. Preston 10.1021/acs.jpca.9b00907
- The Role of Cloud Processing for the Ice Nucleating Ability of Organic Aerosol and Coal Fly Ash Particles K. Kilchhofer et al. 10.1029/2020JD033338
- Phase state of ambient aerosol linked with water uptake and chemical aging in the southeastern US A. Pajunoja et al. 10.5194/acp-16-11163-2016
- Atmospheric ice nucleation D. Knopf & P. Alpert 10.1038/s42254-023-00570-7
- Condensed-phase biogenic–anthropogenic interactions with implications for cold cloud formation J. Charnawskas et al. 10.1039/C7FD00010C
- Physical state of 2-methylbutane-1,2,3,4-tetraol in pure and internally mixed aerosols J. Lessmeier et al. 10.5194/acp-18-15841-2018
- Evolution of Sea Spray Aerosol Particle Phase State Across a Phytoplankton Bloom P. Tumminello et al. 10.1021/acsearthspacechem.1c00186
- Evidence for Anthropogenic Organic Aerosols Contributing to Ice Nucleation P. Tian et al. 10.1029/2022GL099990
- Predicting the influence of particle size on the glass transition temperature and viscosity of secondary organic material M. Petters & S. Kasparoglu 10.1038/s41598-020-71490-0
- Optical trapping and light scattering in atmospheric aerosol science A. Rafferty et al. 10.1039/D2CP05301B
- The effect of hydrophobic glassy organic material on the cloud condensation nuclei activity of particles with different morphologies A. Tandon et al. 10.5194/acp-19-3325-2019
- Viscosity, Glass Formation, and Mixing Times within Secondary Organic Aerosol from Biomass Burning Phenolics K. Kiland et al. 10.1021/acsearthspacechem.3c00039
- Experimental Determination of the Relationship Between Organic Aerosol Viscosity and Ice Nucleation at Upper Free Tropospheric Conditions S. Kasparoglu et al. 10.1029/2021JD036296
- Characterising the evaporation kinetics of water and semi-volatile organic compounds from viscous multicomponent organic aerosol particles S. Ingram et al. 10.1039/C7CP05172G
- Predictions of the glass transition temperature and viscosity of organic aerosols from volatility distributions Y. Li et al. 10.5194/acp-20-8103-2020
- Global distribution of particle phase state in atmospheric secondary organic aerosols M. Shiraiwa et al. 10.1038/ncomms15002
- Study on the Mass transfer and hygroscopic behavior of glucose / ammonium sulfate aerosol droplets P. Chang & Z. Chen 10.1016/j.jaerosci.2024.106365
- Influence of Functional Groups on the Viscosity of Organic Aerosol N. Rothfuss & M. Petters 10.1021/acs.est.6b04478
- Utilizing an electrical low-pressure impactor to indirectly probe water uptake via particle bounce measurements K. Fischer & G. Petrucci 10.5194/amt-14-7565-2021
- The Cooling Rate- and Volatility-Dependent Glass-Forming Properties of Organic Aerosols Measured by Broadband Dielectric Spectroscopy Y. Zhang et al. 10.1021/acs.est.9b03317
- Liquid–liquid phase separation and viscosity within secondary organic aerosol generated from diesel fuel vapors M. Song et al. 10.5194/acp-19-12515-2019
- Sunlight can convert atmospheric aerosols into a glassy solid state and modify their environmental impacts V. Baboomian et al. 10.1073/pnas.2208121119
- Aerosol Composition, Mixing State, and Phase State of Free Tropospheric Particles and Their Role in Ice Cloud Formation N. Lata et al. 10.1021/acsearthspacechem.1c00315
- Organic Enrichment, Physical Phase State, and Surface Tension Depression of Nascent Core–Shell Sea Spray Aerosols during Two Phytoplankton Blooms H. Lee et al. 10.1021/acsearthspacechem.0c00032
- Modeling Volatility-Based Aerosol Phase State Predictions in the Amazon Rainforest Q. Rasool et al. 10.1021/acsearthspacechem.1c00255
- Photolytic radical persistence due to anoxia in viscous aerosol particles P. Alpert et al. 10.1038/s41467-021-21913-x
- Tropospheric and stratospheric wildfire smoke profiling with lidar: mass, surface area, CCN, and INP retrieval A. Ansmann et al. 10.5194/acp-21-9779-2021
- Direct imaging of changes in aerosol particle viscosity upon hydration and chemical aging N. Hosny et al. 10.1039/C5SC02959G
- Lifecycle of light-absorbing carbonaceous aerosols in the atmosphere D. Liu et al. 10.1038/s41612-020-00145-8
- Depositional ice nucleation on NX illite and mixtures of NX illite with organic acids K. Primm et al. 10.1007/s10874-016-9340-x
129 citations as recorded by crossref.
- Ice nucleation ability of ammonium sulfate aerosol particles internally mixed with secondary organics B. Bertozzi et al. 10.5194/acp-21-10779-2021
- Heterogeneous ice nucleation of viscous secondary organic aerosol produced from ozonolysis of <i>α</i>-pinene K. Ignatius et al. 10.5194/acp-16-6495-2016
- Viscous organic aerosol particles in the upper troposphere: diffusivity-controlled water uptake and ice nucleation? D. Lienhard et al. 10.5194/acp-15-13599-2015
- Is Ice Formation by Sea Spray Particles at Cirrus Temperatures Controlled by Crystalline Salts? R. Patnaude et al. 10.1021/acsearthspacechem.1c00228
- Ozonolysis Chemistry and Phase Behavior of 1-Octen-3-ol-Derived Secondary Organic Aerosol K. Fischer et al. 10.1021/acsearthspacechem.0c00092
- Direct observation and assessment of phase states of ambient and lab-generated sub-micron particles upon humidification Z. Cheng et al. 10.1039/D1RA02530A
- Predicting Atmospheric Particle Phase State Using an Explainable Machine Learning Approach Based on Particle Rebound Measurements Y. Qiu et al. 10.1021/acs.est.3c05284
- Water diffusion in atmospherically relevant α-pinene secondary organic material H. Price et al. 10.1039/C5SC00685F
- Progress in the Analysis of Complex Atmospheric Particles A. Laskin et al. 10.1146/annurev-anchem-071015-041521
- Reactive Uptake of Isoprene Epoxydiols Increases the Viscosity of the Core of Phase-Separated Aerosol Particles N. Olson et al. 10.1021/acsearthspacechem.9b00138
- Vapor Condensed and Supercooled Glassy Nanoclusters W. Qi & R. Bowles 10.1021/acsnano.5b07391
- Solid organic-coated ammonium sulfate particles at high relative humidity in the summertime Arctic atmosphere R. Kirpes et al. 10.1073/pnas.2104496119
- Multiphase Chemistry at the Atmosphere–Biosphere Interface Influencing Climate and Public Health in the Anthropocene U. Pöschl & M. Shiraiwa 10.1021/cr500487s
- Amorphous phase state diagrams and viscosity of ternary aqueous organic/organic and inorganic/organic mixtures A. Marsh et al. 10.1039/C8CP00760H
- The Significant Role of New Particle Composition and Morphology on the HNO3-Driven Growth of Particles down to Sub-10 nm Y. Li et al. 10.1021/acs.est.3c09454
- Liquid–Liquid Phase Separation Can Drive Aerosol Droplet Growth in Supersaturated Regimes K. Malek et al. 10.1021/acsenvironau.3c00015
- Heterogeneous ice nucleation ability of aerosol particles generated from Arctic sea surface microlayer and surface seawater samples at cirrus temperatures R. Wagner et al. 10.5194/acp-21-13903-2021
- Coalescence-based assessment of aerosol phase state using dimers prepared through a dual-differential mobility analyzer technique N. Rothfuss & M. Petters 10.1080/02786826.2016.1221050
- Particle Size Distribution Dynamics Can Help Constrain the Phase State of Secondary Organic Aerosol Y. He et al. 10.1021/acs.est.0c05796
- Modelling the effect of condensed-phase diffusion on the homogeneous nucleation of ice in ultra-viscous particles K. Fowler et al. 10.5194/acp-20-683-2020
- Effect of varying experimental conditions on the viscosity of <i>α</i>-pinene derived secondary organic material J. Grayson et al. 10.5194/acp-16-6027-2016
- Role of Organic Hydrocarbons in Atmospheric Ice Formation via Contact Freezing K. Collier & S. Brooks 10.1021/acs.jpca.6b11890
- Heterogeneous ice nucleation of α‐pinene SOA particles before and after ice cloud processing R. Wagner et al. 10.1002/2016JD026401
- Relative humidity-dependent viscosities of isoprene-derived secondary organic material and atmospheric implications for isoprene-dominant forests M. Song et al. 10.5194/acp-15-5145-2015
- Multicomponent diffusion in atmospheric aerosol particles B. Wallace et al. 10.1039/D0EA00008F
- Isomeric Identification of the Nitroindole Chromophore in Indole + NO3 Organic Aerosol A. Dalton et al. 10.1021/acsphyschemau.4c00044
- Equilibration times in viscous and viscoelastic aerosol particles T. Preston & A. Zuend 10.1039/D2EA00065B
- Observation of viscosity transition in <i>α</i>-pinene secondary organic aerosol E. Järvinen et al. 10.5194/acp-16-4423-2016
- Quantifying the Viscosity of Individual Submicrometer Semisolid Particles Using Atomic Force Microscopy C. Madawala et al. 10.1021/acs.analchem.3c01835
- The dependence of soot particle ice nucleation ability on its volatile content K. Gao et al. 10.1039/D2EM00158F
- The efficiency of secondary organic aerosol particles acting as ice-nucleating particles under mixed-phase cloud conditions W. Frey et al. 10.5194/acp-18-9393-2018
- Temperature‐ and Humidity‐Dependent Phase States of Secondary Organic Aerosols S. Petters et al. 10.1029/2018GL080563
- MIMiX: a Multipurpose In situ Microreactor system for X-ray microspectroscopy to mimic atmospheric aerosol processing J. Förster et al. 10.5194/amt-13-3717-2020
- The Influence of Absolute Mass Loading of Secondary Organic Aerosols on Their Phase State S. Jain et al. 10.3390/atmos9040131
- Models of Isotopic Water Diffusion in Spherical Aerosol Particles A. Moridnejad & T. Preston 10.1021/acs.jpca.6b11241
- Wildfire smoke, Arctic haze, and aerosol effects on mixed-phase and cirrus clouds over the North Pole region during MOSAiC: an introduction R. Engelmann et al. 10.5194/acp-21-13397-2021
- Atmospheric Humic‐Like Substances (HULIS) Act as Ice Active Entities J. Chen et al. 10.1029/2021GL092443
- Kinetically controlled glass transition measurement of organic aerosol thin films using broadband dielectric spectroscopy Y. Zhang et al. 10.5194/amt-11-3479-2018
- Glass Formation Processes in Mixed Inorganic/Organic Aerosol Particles H. Dette & T. Koop 10.1021/jp5106967
- Physicochemical Mixing State of Sea Spray Aerosols: Morphologies Exhibit Size Dependence H. Lee et al. 10.1021/acsearthspacechem.0c00153
- Molecular and physical characteristics of aerosol at a remote free troposphere site: implications for atmospheric aging S. Schum et al. 10.5194/acp-18-14017-2018
- Dynamics and Sorption Kinetics of Methanol Monomers and Clusters on Nopinone Surfaces X. Kong et al. 10.1021/acs.jpca.1c02309
- Ice nucleation by water-soluble macromolecules B. Pummer et al. 10.5194/acp-15-4077-2015
- Hydration of Atmospheric Molecular Clusters II: Organic Acid–Water Clusters J. Kildgaard et al. 10.1021/acs.jpca.8b07713
- Characterization of the temperature and humidity-dependent phase diagram of amorphous nanoscale organic aerosols N. Rothfuss & M. Petters 10.1039/C6CP08593H
- New investigations on homogeneous ice nucleation: the effects of water activity and water saturation formulations M. Baumgartner et al. 10.5194/acp-22-65-2022
- Particle phase-state variability in the North Atlantic free troposphere during summertime is determined by atmospheric transport patterns and sources Z. Cheng et al. 10.5194/acp-22-9033-2022
- Enhanced Ice Nucleation of Simulated Sea Salt Particles with the Addition of Anthropogenic Per- and Polyfluoroalkyl Substances M. Wolf et al. 10.1021/acsearthspacechem.1c00138
- Discontinuities in hygroscopic growth below and above water saturation for laboratory surrogates of oligomers in organic atmospheric aerosols N. Hodas et al. 10.5194/acp-16-12767-2016
- A continuous flow diffusion chamber study of sea salt particles acting as cloud nuclei: deliquescence and ice nucleation X. Kong et al. 10.1080/16000889.2018.1463806
- Toward closure between predicted and observed particle viscosity over a wide range of temperatures and relative humidity S. Kasparoglu et al. 10.5194/acp-21-1127-2021
- Effect of Acidity on Ice Nucleation by Inorganic–Organic Mixed Droplets Z. Lei et al. 10.1021/acsearthspacechem.3c00242
- The viscosity of atmospherically relevant organic particles J. Reid et al. 10.1038/s41467-018-03027-z
- Cloud Activation via Formation of Water and Ice on Various Types of Porous Aerosol Particles E. Jantsch & T. Koop 10.1021/acsearthspacechem.0c00330
- Nanomechanics and Morphology of Simulated Respiratory Particles R. Groth et al. 10.1021/acs.est.2c01829
- Glass Transition Temperatures of Organic Mixtures from Isoprene Epoxydiol-Derived Secondary Organic Aerosol B. Chen et al. 10.1021/acs.jpca.2c08936
- Hygroscopic behavior of aerosols generated from solutions of 3-methyl-1,2,3-butanetricarboxylic acid, its sodium salts, and its mixtures with NaCl L. Wu et al. 10.5194/acp-20-14103-2020
- Diffusion coefficients of organic molecules in sucrose–water solutions and comparison with Stokes–Einstein predictions Y. Chenyakin et al. 10.5194/acp-17-2423-2017
- Recent advances in understanding secondary organic aerosol: Implications for global climate forcing M. Shrivastava et al. 10.1002/2016RG000540
- Predicting the refractive index of amorphous materials using the Bruggeman effective medium approximation M. Sela & C. Haspel 10.1364/AO.402103
- Wildfire smoke triggers cirrus formation: lidar observations over the eastern Mediterranean R. Mamouri et al. 10.5194/acp-23-14097-2023
- The Role of Organic Aerosol in Atmospheric Ice Nucleation: A Review D. Knopf et al. 10.1021/acsearthspacechem.7b00120
- Ice nucleation on surrogates of boreal forest SOA particles: effect of water content and oxidative age A. Piedehierro et al. 10.5194/acp-21-11069-2021
- The effect of viscosity and diffusion on the HO<sub>2</sub> uptake by sucrose and secondary organic aerosol particles P. Lakey et al. 10.5194/acp-16-13035-2016
- Viscosity controls humidity dependence of N<sub>2</sub>O<sub>5</sub> uptake to citric acid aerosol G. Gržinić et al. 10.5194/acp-15-13615-2015
- Volatility and Viscosity Are Correlated in Terpene Secondary Organic Aerosol Formed in a Flow Reactor W. Champion et al. 10.1021/acs.estlett.9b00412
- Micro-spectroscopic and freezing characterization of ice-nucleating particles collected in the marine boundary layer in the eastern North Atlantic D. Knopf et al. 10.5194/acp-22-5377-2022
- Diurnal and Seasonal Variations in the Phase State of Secondary Organic Aerosol Material over the Contiguous US Simulated in CMAQ Y. Li et al. 10.1021/acsearthspacechem.1c00094
- Low-temperature ice nucleation of sea spray and secondary marine aerosols under cirrus cloud conditions R. Patnaude et al. 10.5194/acp-24-911-2024
- Bouncier Particles at Night: Biogenic Secondary Organic Aerosol Chemistry and Sulfate Drive Diel Variations in the Aerosol Phase in a Mixed Forest J. Slade et al. 10.1021/acs.est.8b07319
- Multiphase Atmospheric Chemistry in Liquid Water: Impacts and Controllability of Organic Aerosol A. Carlton et al. 10.1021/acs.accounts.0c00301
- Emerging investigator series: surfactants, films, and coatings on atmospheric aerosol particles: a review K. Wokosin et al. 10.1039/D2EA00003B
- Heterogeneous Ice Nucleation in the Tropical Tropopause Layer E. Jensen et al. 10.1029/2018JD028949
- A biogenic secondary organic aerosol source of cirrus ice nucleating particles M. Wolf et al. 10.1038/s41467-020-18424-6
- Ice cloud formation potential by free tropospheric particles from long‐range transport over the Northern Atlantic Ocean S. China et al. 10.1002/2016JD025817
- Phase transition observations and discrimination of small cloud particles by light polarization in expansion chamber experiments L. Nichman et al. 10.5194/acp-16-3651-2016
- Diffusion and reactivity in ultraviscous aerosol and the correlation with particle viscosity F. Marshall et al. 10.1039/C5SC03223G
- Heterogeneous oxidation of amorphous organic aerosol surrogates by O<sub>3</sub>, NO<sub>3</sub>, and OH at typical tropospheric temperatures J. Li et al. 10.5194/acp-20-6055-2020
- Condensation Kinetics of Water on Amorphous Aerosol Particles N. Rothfuss et al. 10.1021/acs.jpclett.8b01365
- Physicochemical characterization of free troposphere and marine boundary layer ice-nucleating particles collected by aircraft in the eastern North Atlantic D. Knopf et al. 10.5194/acp-23-8659-2023
- A predictive group-contribution model for the viscosity of aqueous organic aerosol N. Gervasi et al. 10.5194/acp-20-2987-2020
- Unified Description of Diffusion Coefficients from Small to Large Molecules in Organic–Water Mixtures E. Evoy et al. 10.1021/acs.jpca.9b11271
- The characterization of long-range transported North American biomass burning plumes: what can a multi-wavelength Mie–Raman-polarization-fluorescence lidar provide? Q. Hu et al. 10.5194/acp-22-5399-2022
- Anthropogenic influences on the physical state of submicron particulate matter over a tropical forest A. Bateman et al. 10.5194/acp-17-1759-2017
- Phase State and Deliquescence Hysteresis of Ammonium-Sulfate-Seeded Secondary Organic Aerosol E. Saukko et al. 10.1080/02786826.2015.1050085
- Investigating the Heterogeneous Ice Nucleation of Sea Spray Aerosols Using Prochlorococcus as a Model Source of Marine Organic Matter M. Wolf et al. 10.1021/acs.est.8b05150
- Temperature effect on phase state and reactivity controls atmospheric multiphase chemistry and transport of PAHs Q. Mu et al. 10.1126/sciadv.aap7314
- Probing the Water Uptake and Phase State of Individual Sucrose Nanoparticles Using Atomic Force Microscopy C. Madawala et al. 10.1021/acsearthspacechem.1c00101
- Multiphase Chemical Kinetics of OH Radical Uptake by Molecular Organic Markers of Biomass Burning Aerosols: Humidity and Temperature Dependence, Surface Reaction, and Bulk Diffusion A. Arangio et al. 10.1021/jp510489z
- Radiative forcing of anthropogenic aerosols on cirrus clouds using a hybrid ice nucleation scheme J. Zhu & J. Penner 10.5194/acp-20-7801-2020
- Global Distribution of the Phase State and Mixing Times within Secondary Organic Aerosol Particles in the Troposphere Based on Room-Temperature Viscosity Measurements A. Maclean et al. 10.1021/acsearthspacechem.1c00296
- Ozone uptake on glassy, semi-solid and liquid organic matter and the role of reactive oxygen intermediates in atmospheric aerosol chemistry T. Berkemeier et al. 10.1039/C6CP00634E
- Indirect Effects of Secondary Organic Aerosol on Cirrus Clouds J. Zhu & J. Penner 10.1029/2019JD032233
- Atomic Force Microscopy: An Emerging Tool in Measuring the Phase State and Surface Tension of Individual Aerosol Particles H. Lee & A. Tivanski 10.1146/annurev-physchem-090419-110133
- Effects of volatility, viscosity, and non-ideality on particle–particle mixing timescales of secondary organic aerosols M. Schervish et al. 10.1080/02786826.2023.2256827
- Predicting the glass transition temperature and viscosity of secondary organic material using molecular composition W. DeRieux et al. 10.5194/acp-18-6331-2018
- Particulate matter, air quality and climate: lessons learned and future needs S. Fuzzi et al. 10.5194/acp-15-8217-2015
- The effects of morphology, mobility size, and secondary organic aerosol (SOA) material coating on the ice nucleation activity of black carbon in the cirrus regime C. Zhang et al. 10.5194/acp-20-13957-2020
- Estimation of secondary organic aerosol viscosity from explicit modeling of gas-phase oxidation of isoprene and <i>α</i>-pinene T. Galeazzo et al. 10.5194/acp-21-10199-2021
- Hygroscopic behavior of inorganic–organic aerosol systems including ammonium sulfate, dicarboxylic acids, and oligomer H. Bouzidi et al. 10.1016/j.atmosenv.2020.117481
- Water Uptake and Loss in Viscous Aerosol Particles with Concentration-Dependent Diffusivities B. Wallace & T. Preston 10.1021/acs.jpca.9b00907
- The Role of Cloud Processing for the Ice Nucleating Ability of Organic Aerosol and Coal Fly Ash Particles K. Kilchhofer et al. 10.1029/2020JD033338
- Phase state of ambient aerosol linked with water uptake and chemical aging in the southeastern US A. Pajunoja et al. 10.5194/acp-16-11163-2016
- Atmospheric ice nucleation D. Knopf & P. Alpert 10.1038/s42254-023-00570-7
- Condensed-phase biogenic–anthropogenic interactions with implications for cold cloud formation J. Charnawskas et al. 10.1039/C7FD00010C
- Physical state of 2-methylbutane-1,2,3,4-tetraol in pure and internally mixed aerosols J. Lessmeier et al. 10.5194/acp-18-15841-2018
- Evolution of Sea Spray Aerosol Particle Phase State Across a Phytoplankton Bloom P. Tumminello et al. 10.1021/acsearthspacechem.1c00186
- Evidence for Anthropogenic Organic Aerosols Contributing to Ice Nucleation P. Tian et al. 10.1029/2022GL099990
- Predicting the influence of particle size on the glass transition temperature and viscosity of secondary organic material M. Petters & S. Kasparoglu 10.1038/s41598-020-71490-0
- Optical trapping and light scattering in atmospheric aerosol science A. Rafferty et al. 10.1039/D2CP05301B
- The effect of hydrophobic glassy organic material on the cloud condensation nuclei activity of particles with different morphologies A. Tandon et al. 10.5194/acp-19-3325-2019
- Viscosity, Glass Formation, and Mixing Times within Secondary Organic Aerosol from Biomass Burning Phenolics K. Kiland et al. 10.1021/acsearthspacechem.3c00039
- Experimental Determination of the Relationship Between Organic Aerosol Viscosity and Ice Nucleation at Upper Free Tropospheric Conditions S. Kasparoglu et al. 10.1029/2021JD036296
- Characterising the evaporation kinetics of water and semi-volatile organic compounds from viscous multicomponent organic aerosol particles S. Ingram et al. 10.1039/C7CP05172G
- Predictions of the glass transition temperature and viscosity of organic aerosols from volatility distributions Y. Li et al. 10.5194/acp-20-8103-2020
- Global distribution of particle phase state in atmospheric secondary organic aerosols M. Shiraiwa et al. 10.1038/ncomms15002
- Study on the Mass transfer and hygroscopic behavior of glucose / ammonium sulfate aerosol droplets P. Chang & Z. Chen 10.1016/j.jaerosci.2024.106365
- Influence of Functional Groups on the Viscosity of Organic Aerosol N. Rothfuss & M. Petters 10.1021/acs.est.6b04478
- Utilizing an electrical low-pressure impactor to indirectly probe water uptake via particle bounce measurements K. Fischer & G. Petrucci 10.5194/amt-14-7565-2021
- The Cooling Rate- and Volatility-Dependent Glass-Forming Properties of Organic Aerosols Measured by Broadband Dielectric Spectroscopy Y. Zhang et al. 10.1021/acs.est.9b03317
- Liquid–liquid phase separation and viscosity within secondary organic aerosol generated from diesel fuel vapors M. Song et al. 10.5194/acp-19-12515-2019
- Sunlight can convert atmospheric aerosols into a glassy solid state and modify their environmental impacts V. Baboomian et al. 10.1073/pnas.2208121119
- Aerosol Composition, Mixing State, and Phase State of Free Tropospheric Particles and Their Role in Ice Cloud Formation N. Lata et al. 10.1021/acsearthspacechem.1c00315
- Organic Enrichment, Physical Phase State, and Surface Tension Depression of Nascent Core–Shell Sea Spray Aerosols during Two Phytoplankton Blooms H. Lee et al. 10.1021/acsearthspacechem.0c00032
- Modeling Volatility-Based Aerosol Phase State Predictions in the Amazon Rainforest Q. Rasool et al. 10.1021/acsearthspacechem.1c00255
- Photolytic radical persistence due to anoxia in viscous aerosol particles P. Alpert et al. 10.1038/s41467-021-21913-x
- Tropospheric and stratospheric wildfire smoke profiling with lidar: mass, surface area, CCN, and INP retrieval A. Ansmann et al. 10.5194/acp-21-9779-2021
- Direct imaging of changes in aerosol particle viscosity upon hydration and chemical aging N. Hosny et al. 10.1039/C5SC02959G
- Lifecycle of light-absorbing carbonaceous aerosols in the atmosphere D. Liu et al. 10.1038/s41612-020-00145-8
1 citations as recorded by crossref.
Saved (final revised paper)
Saved (final revised paper)
Saved (preprint)
Latest update: 06 Oct 2024
Short summary
Glassy organic particles can serve as ice nuclei at low temperatures. We provide a rationale for these findings using a numerical aerosol diffusion model that describes particle phase state and its kinetics during simulated atmospheric updrafts dependent upon composition, size, updraft velocity, temperature and humidity. Our simulations suggest that aerosols from anthropogenic aromatic organics can be particularly relevant for ice cloud formation.
Glassy organic particles can serve as ice nuclei at low temperatures. We provide a rationale for...
Altmetrics
Final-revised paper
Preprint