Atmospheric Chemistry and Physics
Atmospheric Chemistry and Physics
ACP
Articles | Volume 26, issue 10
Articles | Volume 26, issue 10
https://doi.org/10.5194/acp-26-6973-2026
© Author(s) 2026. This work is distributed under
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-26-6973-2026
© Author(s) 2026. This work is distributed under
the Creative Commons Attribution 4.0 License.
Articles | Volume 26, issue 10
Research article
 | 
22 May 2026
Research article |  | 22 May 2026

Reactions of carbonyl oxide with aldehydes: accurate electronic structure methods, kinetic insights, and atmospheric implications

Chaolu Xie and Bo Long

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Short summary
Chemical transformations are fundamental drivers of atmospheric composition. While elucidating these processes is critical, existing quantitative kinetic data remain significantly limited. We develop a computational framework that delivers quantitative kinetics for CH₂OO reactions with aldehydes from small to large systems, revealing fluorination-driven near–collision-limit reactivity and previously unrecognized impacts on nighttime Criegee chemistry and sulfate formation in the atmosphere.
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