Articles | Volume 26, issue 8
https://doi.org/10.5194/acp-26-5713-2026
© Author(s) 2026. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-26-5713-2026
© Author(s) 2026. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
27 Apr 2026
Research article |
| 27 Apr 2026
| 27 Apr 2026
Rapid secondary organic aerosol formation at the air–water interface from methoxyphenols in wildfire emissions: UVA-driven S(IV) photooxidation to organosulfates
Baohua Cai
Shenzhen Key Laboratory of Precision Measurement and Early Warning Technology for Urban Environmental Health Risks, School of Environmental Science and Engineering, Southern University of Science and Technology, Shenzhen 518055, China
Yuanlong Huang
Ningbo Institute of Digital Twin, Eastern Institute of Technology, Ningbo 315201, China
Wenqing Jiang
Department of Environmental Toxicology, University of California, Davis, California 95616, United States
Yanchen Li
Shenzhen Key Laboratory of Precision Measurement and Early Warning Technology for Urban Environmental Health Risks, School of Environmental Science and Engineering, Southern University of Science and Technology, Shenzhen 518055, China
Yali Li
Shenzhen Key Laboratory of Precision Measurement and Early Warning Technology for Urban Environmental Health Risks, School of Environmental Science and Engineering, Southern University of Science and Technology, Shenzhen 518055, China
Jinghao Zhai
Shenzhen Key Laboratory of Precision Measurement and Early Warning Technology for Urban Environmental Health Risks, School of Environmental Science and Engineering, Southern University of Science and Technology, Shenzhen 518055, China
Guangdong Provincial Field Observation and Research Station for Coastal Atmosphere and Climate of the Greater Bay Area, Southern University of Science and Technology, Shenzhen, Guangdong 518055, China
Yaling Zeng
Shenzhen Key Laboratory of Precision Measurement and Early Warning Technology for Urban Environmental Health Risks, School of Environmental Science and Engineering, Southern University of Science and Technology, Shenzhen 518055, China
Guangdong Provincial Field Observation and Research Station for Coastal Atmosphere and Climate of the Greater Bay Area, Southern University of Science and Technology, Shenzhen, Guangdong 518055, China
Jianhuai Ye
Shenzhen Key Laboratory of Precision Measurement and Early Warning Technology for Urban Environmental Health Risks, School of Environmental Science and Engineering, Southern University of Science and Technology, Shenzhen 518055, China
Guangdong Provincial Field Observation and Research Station for Coastal Atmosphere and Climate of the Greater Bay Area, Southern University of Science and Technology, Shenzhen, Guangdong 518055, China
Huizhong Shen
Shenzhen Key Laboratory of Precision Measurement and Early Warning Technology for Urban Environmental Health Risks, School of Environmental Science and Engineering, Southern University of Science and Technology, Shenzhen 518055, China
Guangdong Provincial Field Observation and Research Station for Coastal Atmosphere and Climate of the Greater Bay Area, Southern University of Science and Technology, Shenzhen, Guangdong 518055, China
Chen Wang
Shenzhen Key Laboratory of Precision Measurement and Early Warning Technology for Urban Environmental Health Risks, School of Environmental Science and Engineering, Southern University of Science and Technology, Shenzhen 518055, China
Guangdong Provincial Field Observation and Research Station for Coastal Atmosphere and Climate of the Greater Bay Area, Southern University of Science and Technology, Shenzhen, Guangdong 518055, China
Shenzhen Key Laboratory of Precision Measurement and Early Warning Technology for Urban Environmental Health Risks, School of Environmental Science and Engineering, Southern University of Science and Technology, Shenzhen 518055, China
Guangdong Provincial Field Observation and Research Station for Coastal Atmosphere and Climate of the Greater Bay Area, Southern University of Science and Technology, Shenzhen, Guangdong 518055, China
Tzung-May Fu
Shenzhen Key Laboratory of Precision Measurement and Early Warning Technology for Urban Environmental Health Risks, School of Environmental Science and Engineering, Southern University of Science and Technology, Shenzhen 518055, China
Guangdong Provincial Field Observation and Research Station for Coastal Atmosphere and Climate of the Greater Bay Area, Southern University of Science and Technology, Shenzhen, Guangdong 518055, China
Department of Environmental Toxicology, University of California, Davis, California 95616, United States
Shenzhen Key Laboratory of Precision Measurement and Early Warning Technology for Urban Environmental Health Risks, School of Environmental Science and Engineering, Southern University of Science and Technology, Shenzhen 518055, China
Guangdong Provincial Field Observation and Research Station for Coastal Atmosphere and Climate of the Greater Bay Area, Southern University of Science and Technology, Shenzhen, Guangdong 518055, China
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Saved (final revised paper)
Latest update: 17 Sep 2026
Short summary
This study reveals a novel Ultraviolet A-driven, metal-free mechanism for aqueous-phase tetravalent sulfur (S(IV)) oxidation that leads to organosulfates formation, addressing a critical knowledge gap in atmospheric sulfur and organic aerosol chemistry and highlighting a previously overlooked photochemical pathway with broad environmental implications.
This study reveals a novel Ultraviolet A-driven, metal-free mechanism for aqueous-phase...
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