Articles | Volume 25, issue 2
https://doi.org/10.5194/acp-25-771-2025
© Author(s) 2025. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-25-771-2025
© Author(s) 2025. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Exploring the processes controlling secondary inorganic aerosol: evaluating the global GEOS-Chem simulation using a suite of aircraft campaigns
Olivia G. Norman
CORRESPONDING AUTHOR
Department of Earth, Atmospheric and Planetary Sciences, Massachusetts Institute of Technology, Cambridge, MA, USA
Colette L. Heald
CORRESPONDING AUTHOR
Department of Earth, Atmospheric and Planetary Sciences, Massachusetts Institute of Technology, Cambridge, MA, USA
Department of Civil and Environmental Engineering, Massachusetts Institute of Technology, Cambridge, MA, USA
now at: Department of Environmental Systems Science, ETH Zurich, Zurich, Switzerland
Solomon Bililign
Department of Physics, North Carolina Agricultural and Technical State University, Greensboro, NC, USA
Pedro Campuzano-Jost
Department of Chemistry and Cooperative Institute for Research in Environmental Science (CIRES), University of Colorado, Boulder, CO, USA
Department of Earth and Environmental Sciences, University of Manchester, Oxford Road, Manchester, M13 1QD, UK
National Centre for Atmospheric Sciences, University of Manchester, Oxford Road, Manchester, M13 1QD, UK
Marc N. Fiddler
Department of Chemistry, North Carolina Agricultural and Technical State University, Greensboro, NC, USA
Jaime R. Green
Department of Environmental Sciences & Engineering, University of North Carolina, Chapel Hill, NC, USA
Jose L. Jimenez
Department of Chemistry and Cooperative Institute for Research in Environmental Science (CIRES), University of Colorado, Boulder, CO, USA
Katharina Kaiser
Particle Chemistry Department, Max Planck Institute for Chemistry, Mainz, Germany
Jin Liao
NASA Goddard Space Flight Center, Greenbelt, MD, USA
Goddard Earth Sciences Technology and Research (GESTAR) II, University of Maryland, College Park, MD, USA
Ann M. Middlebrook
NOAA Chemical Sciences Laboratory, Boulder, CO, USA
Benjamin A. Nault
Department of Chemistry and Cooperative Institute for Research in Environmental Science (CIRES), University of Colorado, Boulder, CO, USA
Department of Environmental Health and Engineering, Johns Hopkins University, Baltimore, MD, USA
Center for Aerosol and Cloud Chemistry, Aerodyne Research, Inc., Billerica, MA, USA
John B. Nowak
NASA Langley Research Center, Hampton, VA, USA
Johannes Schneider
Particle Chemistry Department, Max Planck Institute for Chemistry, Mainz, Germany
André Welti
Finnish Meteorological Institute, Helsinki, Finland
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Short summary
This study finds that one component of secondary inorganic aerosols, nitrate, is greatly overestimated by a global atmospheric chemistry model compared to observations from 11 flight campaigns. None of the loss and production pathways explored can explain the nitrate bias alone. The model’s inability to capture the variability in the observations remains and requires future investigation to avoid biases in policy-related studies (i.e., air quality, health, climate impacts of these aerosols).
This study finds that one component of secondary inorganic aerosols, nitrate, is greatly...
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