Articles | Volume 25, issue 18
https://doi.org/10.5194/acp-25-11317-2025
https://doi.org/10.5194/acp-25-11317-2025
Research article
 | 
25 Sep 2025
Research article |  | 25 Sep 2025

Homogeneous ice nucleation in adsorbed water films: a theoretical approach

Ari Laaksonen, Golnaz Roudsari, Ana A. Piedehierro, and André Welti

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Interactive discussion

Status: closed

Comment types: AC – author | RC – referee | CC – community | EC – editor | CEC – chief editor | : Report abuse
  • RC1: 'Comment on egusphere-2024-4095', Anonymous Referee #1, 05 Feb 2025
  • RC2: 'Comment on egusphere-2024-4095', Anonymous Referee #2, 19 Jun 2025
  • AC1: 'Response to comments by reviewers 1 and 2', Ari Laaksonen, 03 Jul 2025

Peer review completion

AR: Author's response | RR: Referee report | ED: Editor decision | EF: Editorial file upload
AR by Ari Laaksonen on behalf of the Authors (08 Jul 2025)  Author's response   Author's tracked changes   Manuscript 
ED: Publish as is (09 Jul 2025) by Thomas Berkemeier
AR by Ari Laaksonen on behalf of the Authors (11 Jul 2025)
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Short summary
The mechanisms of ice nucleation at temperatures below 235 K have remained unclear for the past century. We suggest that ice nucleation is caused by the freezing of water adsorbed on aerosol surfaces. To test this hypothesis, we derived theoretical equations to predict the exact atmospheric conditions under which ice nucleation occurs. Our predictions agree well with experiments. The new theory thus provides a basis for an improved description of ice nucleation in the atmosphere.
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