Articles | Volume 24, issue 13
https://doi.org/10.5194/acp-24-7499-2024
© Author(s) 2024. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-24-7499-2024
© Author(s) 2024. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
The influence of extratropical cross-tropopause mixing on the correlation between ozone and sulfate aerosol in the lowermost stratosphere
Institute for Atmospheric Physics, Johannes Gutenberg University Mainz, Mainz, Germany
Particle Chemistry Department, Max Planck Institute for Chemistry, Mainz, Germany
Johannes Schneider
Particle Chemistry Department, Max Planck Institute for Chemistry, Mainz, Germany
Katharina Kaiser
Institute for Atmospheric Physics, Johannes Gutenberg University Mainz, Mainz, Germany
Particle Chemistry Department, Max Planck Institute for Chemistry, Mainz, Germany
Horst Fischer
Atmospheric Chemistry Department, Max Planck Institute for Chemistry, Mainz, Germany
Peter Hoor
Institute for Atmospheric Physics, Johannes Gutenberg University Mainz, Mainz, Germany
Daniel Kunkel
Institute for Atmospheric Physics, Johannes Gutenberg University Mainz, Mainz, Germany
Hans-Christoph Lachnitt
Institute for Atmospheric Physics, Johannes Gutenberg University Mainz, Mainz, Germany
Andreas Marsing
Institute of Atmospheric Physics, Deutsches Zentrum für Luft- und Raumfahrt (DLR), Oberpfaffenhofen, Germany
Lenard Röder
Atmospheric Chemistry Department, Max Planck Institute for Chemistry, Mainz, Germany
Hans Schlager
Institute of Atmospheric Physics, Deutsches Zentrum für Luft- und Raumfahrt (DLR), Oberpfaffenhofen, Germany
Laura Tomsche
Institute for Atmospheric Physics, Johannes Gutenberg University Mainz, Mainz, Germany
Institute of Atmospheric Physics, Deutsches Zentrum für Luft- und Raumfahrt (DLR), Oberpfaffenhofen, Germany
Christiane Voigt
Institute for Atmospheric Physics, Johannes Gutenberg University Mainz, Mainz, Germany
Institute of Atmospheric Physics, Deutsches Zentrum für Luft- und Raumfahrt (DLR), Oberpfaffenhofen, Germany
Andreas Zahn
Karlsruhe Institute of Technology, Institute of Meteorology and Climate Research, Karlsruhe, Germany
Stephan Borrmann
Institute for Atmospheric Physics, Johannes Gutenberg University Mainz, Mainz, Germany
Particle Chemistry Department, Max Planck Institute for Chemistry, Mainz, Germany
Data sets
HALO: Mission: CAFE-EU HALO https://halo-db.pa.op.dlr.de/mission/120
Mission: BLUESKY HALO https://halo-db.pa.op.dlr.de/mission/119
Sulfate anomaly during CAFE-EU/BLUESKY 10 days LAGRANTO back trajectories Daniel Kunkel and Philipp Joppe https://doi.org/10.5281/zenodo.11092106
Short summary
From aircraft measurements in the upper troposphere/lower stratosphere, we find a correlation between the ozone and particulate sulfate in the lower stratosphere. The correlation exhibits some variability over the measurement period exceeding the background sulfate-to-ozone correlation. From our analysis, we conclude that gas-to-particle conversion of volcanic sulfur dioxide leads to observed enhanced sulfate aerosol mixing ratios.
From aircraft measurements in the upper troposphere/lower stratosphere, we find a correlation...
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