Cluster-dynamics-based parameterization for sulfuric acid–dimethylamine nucleation: comparison and selection through box and three-dimensional modeling
Jiewen Shen,Bin Zhao,Shuxiao Wang,An Ning,Yuyang Li,Runlong Cai,Da Gao,Biwu Chu,Yang Gao,Manish Shrivastava,Jingkun Jiang,Xiuhui Zhang,and Hong He
Jiewen Shen
State Key Joint Laboratory of Environment Simulation and Pollution Control, School of Environment, Tsinghua University, Beijing, 100084, China
State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex, Beijing, 100084, China
Key Laboratory of Cluster Science, Ministry of Education of China, School of Chemistry and Chemical Engineering, Beijing Institute of Technology, Beijing, 100081, China
Yuyang Li
State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex, Beijing, 100084, China
Runlong Cai
Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention (LAP), Department of Environmental Science and Engineering, Fudan University, Shanghai, 200438, China
Da Gao
State Key Joint Laboratory of Environment Simulation and Pollution Control, School of Environment, Tsinghua University, Beijing, 100084, China
State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex, Beijing, 100084, China
State Key Joint Laboratory of Environment Simulation and Pollution Control, Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing, 100085, China
College of Resources and Environment, University of Chinese Academy of Sciences, Beijing, 100049, China
Key Laboratory of Cluster Science, Ministry of Education of China, School of Chemistry and Chemical Engineering, Beijing Institute of Technology, Beijing, 100081, China
State Key Joint Laboratory of Environment Simulation and Pollution Control, Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing, 100085, China
College of Resources and Environment, University of Chinese Academy of Sciences, Beijing, 100049, China
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We extensively compare various cluster-dynamics-based parameterizations for sulfuric acid–dimethylamine nucleation and identify a newly developed parameterization derived from Atmospheric Cluster Dynamic Code (ACDC) simulations as being the most reliable one. This study offers a valuable reference for developing parameterizations of other nucleation systems and is meaningful for the accurate quantification of the environmental and climate impacts of new particle formation.
We extensively compare various cluster-dynamics-based parameterizations for sulfuric...
