Articles | Volume 23, issue 15
https://doi.org/10.5194/acp-23-8789-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-23-8789-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
09 Aug 2023
Research article |
| 09 Aug 2023
| 09 Aug 2023
A dynamic parameterization of sulfuric acid–dimethylamine nucleation and its application in three-dimensional modeling
Yuyang Li
State Key Joint Laboratory of Environment Simulation and Pollution
Control, School of Environment, Tsinghua University, Beijing 100084, China
Jiewen Shen
State Key Joint Laboratory of Environment Simulation and Pollution
Control, School of Environment, Tsinghua University, Beijing 100084, China
State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex, Beijing 100084, China
State Key Joint Laboratory of Environment Simulation and Pollution
Control, School of Environment, Tsinghua University, Beijing 100084, China
State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex, Beijing 100084, China
Runlong Cai
Institute for Atmospheric and Earth System Research/Physics, Faculty of Science, University of Helsinki, 00014 Helsinki, Finland
Shuxiao Wang
State Key Joint Laboratory of Environment Simulation and Pollution
Control, School of Environment, Tsinghua University, Beijing 100084, China
State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex, Beijing 100084, China
Key Laboratory of Marine Environment and Ecology, Ministry of
Education, Ocean University of China, Qingdao 266100, China
Manish Shrivastava
Pacific Northwest National Laboratory, Richland, Washington, USA
Da Gao
State Key Joint Laboratory of Environment Simulation and Pollution
Control, School of Environment, Tsinghua University, Beijing 100084, China
State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex, Beijing 100084, China
Jun Zheng
School of Environmental Science and Engineering, Nanjing University of Information Science & Technology, Nanjing 210044, China
Markku Kulmala
Institute for Atmospheric and Earth System Research/Physics, Faculty of Science, University of Helsinki, 00014 Helsinki, Finland
Aerosol and Haze Laboratory, Beijing Advanced Innovation Center for
Soft Matter Science and Engineering, Beijing University of Chemical
Technology, Beijing 100029, China
Joint International Research Laboratory of Atmospheric and Earth
System Sciences, School of Atmospheric Sciences, Nanjing University, Nanjing, China
Jingkun Jiang
CORRESPONDING AUTHOR
State Key Joint Laboratory of Environment Simulation and Pollution
Control, School of Environment, Tsinghua University, Beijing 100084, China
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Cited
6 citations as recorded by crossref.
- Cluster-dynamics-based parameterization for sulfuric acid–dimethylamine nucleation: comparison and selection through box and three-dimensional modeling J. Shen et al. 10.5194/acp-24-10261-2024
- Overlooked significance of iodic acid in new particle formation in the continental atmosphere A. Ning et al. 10.1073/pnas.2404595121
- A systematic review of reactive nitrogen simulations with chemical transport models in China H. Zhang et al. 10.1016/j.atmosres.2024.107586
- Atmospheric Bases-Enhanced Iodic Acid Nucleation: Altitude-Dependent Characteristics and Molecular Mechanisms J. Li et al. 10.1021/acs.est.4c06053
- Atmospheric amines are a crucial yet missing link in Earth’s climate via airborne aerosol production V. Kanawade & T. Jokinen 10.1038/s43247-025-02063-0
- Intense formation of secondary ultrafine particles from Amazonian vegetation fires and their invigoration of deep clouds and precipitation M. Shrivastava et al. 10.1016/j.oneear.2024.05.015
6 citations as recorded by crossref.
- Cluster-dynamics-based parameterization for sulfuric acid–dimethylamine nucleation: comparison and selection through box and three-dimensional modeling J. Shen et al. 10.5194/acp-24-10261-2024
- Overlooked significance of iodic acid in new particle formation in the continental atmosphere A. Ning et al. 10.1073/pnas.2404595121
- A systematic review of reactive nitrogen simulations with chemical transport models in China H. Zhang et al. 10.1016/j.atmosres.2024.107586
- Atmospheric Bases-Enhanced Iodic Acid Nucleation: Altitude-Dependent Characteristics and Molecular Mechanisms J. Li et al. 10.1021/acs.est.4c06053
- Atmospheric amines are a crucial yet missing link in Earth’s climate via airborne aerosol production V. Kanawade & T. Jokinen 10.1038/s43247-025-02063-0
- Intense formation of secondary ultrafine particles from Amazonian vegetation fires and their invigoration of deep clouds and precipitation M. Shrivastava et al. 10.1016/j.oneear.2024.05.015
Latest update: 21 Feb 2025
Short summary
We set up a new parameterization for 1.4 nm particle formation rates from sulfuric acid–dimethylamine (SA–DMA) nucleation, fully including the effects of coagulation scavenging and cluster stability. Incorporating the new parameterization into 3-D chemical transport models, we achieved better consistencies between simulation results and observation data. This new parameterization provides new insights into atmospheric nucleation simulations and its effects on atmospheric pollution or health.
We set up a new parameterization for 1.4 nm particle formation rates from sulfuric...
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