Articles | Volume 23, issue 14
https://doi.org/10.5194/acp-23-8383-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-23-8383-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
26 Jul 2023
Research article |
| 26 Jul 2023
| 26 Jul 2023
Large differences of highly oxygenated organic molecules (HOMs) and low-volatile species in secondary organic aerosols (SOAs) formed from ozonolysis of β-pinene and limonene
Dandan Liu
Institute of Surface-Earth System Science, School of Earth System Science, Tianjin University, Tianjin 300072, China
Yun Zhang
Innovation Center of Pesticide Research, Department of Applied Chemistry, College of Science, China Agricultural University, Beijing 100193, China
Institute of Chemistry, Johannes Gutenberg University, Mainz 55128, Germany
Shujun Zhong
Institute of Surface-Earth System Science, School of Earth System Science, Tianjin University, Tianjin 300072, China
Shuang Chen
Institute of Surface-Earth System Science, School of Earth System Science, Tianjin University, Tianjin 300072, China
Qiaorong Xie
Institute of Surface-Earth System Science, School of Earth System Science, Tianjin University, Tianjin 300072, China
Donghuan Zhang
Institute of Surface-Earth System Science, School of Earth System Science, Tianjin University, Tianjin 300072, China
Qiang Zhang
Institute of Surface-Earth System Science, School of Earth System Science, Tianjin University, Tianjin 300072, China
Institute of Surface-Earth System Science, School of Earth System Science, Tianjin University, Tianjin 300072, China
Junjun Deng
Institute of Surface-Earth System Science, School of Earth System Science, Tianjin University, Tianjin 300072, China
Libin Wu
Institute of Surface-Earth System Science, School of Earth System Science, Tianjin University, Tianjin 300072, China
Chao Ma
Institute of Surface-Earth System Science, School of Earth System Science, Tianjin University, Tianjin 300072, China
Multiphase Chemistry Department, Max Planck Institute for Chemistry, Mainz 55128, Germany
Institute of Surface Science, Helmholtz-Zentrum Hereon, Geesthacht 21502, Germany
Institute of Surface-Earth System Science, School of Earth System Science, Tianjin University, Tianjin 300072, China
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Cited
7 citations as recorded by crossref.
- Long-term evolution of carbonaceous aerosols in PM2.5 during over a decade of atmospheric pollution outbreaks and control in polluted central China Z. Dong et al. 10.1016/j.scitotenv.2024.173089
- Regional differences in molecular characteristics of atmospheric water-soluble organic carbon over northern China: Comparison of remote, rural, and urban environments H. Wen et al. 10.1016/j.scitotenv.2024.174170
- Volatility and chemical composition of secondary organic aerosol derived from acenaphthylene and acenaphthene under various oxidant conditions W. Xiang et al. 10.1016/j.atmosenv.2024.120563
- Enhanced sulfate formation in mixed biomass burning and sea-salt interactions mediated by photosensitization: effects of chloride, nitrogen-containing compounds, and atmospheric aging R. Tang et al. 10.5194/acp-25-425-2025
- Unraveling the Autoxidation Mechanisms of Limonene, α-Pinene, and β-Pinene: A Computational Study with Reactivity Prediction Models A. Bhavadharini et al. 10.1021/acs.jpca.4c06819
- Chemical Characterization of Rural Organic Aerosol in the North China Plain Using Ultrahigh-Resolution Mass Spectrometry Y. Zhang et al. 10.3390/atmos14111636
- Efficient Formation of Secondary Organic Aerosols from the Aqueous Oxidation of Terpenoic 1,2-Diols by OH P. Jain et al. 10.1021/acs.est.4c06347
7 citations as recorded by crossref.
- Long-term evolution of carbonaceous aerosols in PM2.5 during over a decade of atmospheric pollution outbreaks and control in polluted central China Z. Dong et al. 10.1016/j.scitotenv.2024.173089
- Regional differences in molecular characteristics of atmospheric water-soluble organic carbon over northern China: Comparison of remote, rural, and urban environments H. Wen et al. 10.1016/j.scitotenv.2024.174170
- Volatility and chemical composition of secondary organic aerosol derived from acenaphthylene and acenaphthene under various oxidant conditions W. Xiang et al. 10.1016/j.atmosenv.2024.120563
- Enhanced sulfate formation in mixed biomass burning and sea-salt interactions mediated by photosensitization: effects of chloride, nitrogen-containing compounds, and atmospheric aging R. Tang et al. 10.5194/acp-25-425-2025
- Unraveling the Autoxidation Mechanisms of Limonene, α-Pinene, and β-Pinene: A Computational Study with Reactivity Prediction Models A. Bhavadharini et al. 10.1021/acs.jpca.4c06819
- Chemical Characterization of Rural Organic Aerosol in the North China Plain Using Ultrahigh-Resolution Mass Spectrometry Y. Zhang et al. 10.3390/atmos14111636
- Efficient Formation of Secondary Organic Aerosols from the Aqueous Oxidation of Terpenoic 1,2-Diols by OH P. Jain et al. 10.1021/acs.est.4c06347
Latest update: 18 Jan 2025
Short summary
Based on ultra-high-resolution mass spectrometry analysis, we found that β-pinene oxidation-derived highly oxygenated organic molecules (HOMs) exhibit higher yield at high ozone concentration, while limonene oxidation-derived HOMs exhibit higher yield at moderate ozone concentration. The distinct molecular response of HOMs and low-volatile species in different biogenic secondary organic aerosols to ozone concentrations provides a new clue for more accurate air quality prediction and management.
Based on ultra-high-resolution mass spectrometry analysis, we found that β-pinene...
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