Articles | Volume 23, issue 3
https://doi.org/10.5194/acp-23-2089-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-23-2089-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
10 Feb 2023
Research article |
| 10 Feb 2023
| 10 Feb 2023
Biomass burning CO, PM and fuel consumption per unit burned area estimates derived across Africa using geostationary SEVIRI fire radiative power and Sentinel-5P CO data
Department of Geography, King's College London, London, WC2R 2ND, UK
Leverhulme Centre for Wildfires, Environment and Society, London, UK
Jiangping He
Department of Geography, King's College London, London, WC2R 2ND, UK
National Centre for Earth Observation (NCEO), London, UK
Martin J. Wooster
Department of Geography, King's College London, London, WC2R 2ND, UK
Leverhulme Centre for Wildfires, Environment and Society, London, UK
National Centre for Earth Observation (NCEO), London, UK
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This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
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We examine the impact of diurnally varying African biomass burning (BB) emissions on tropospheric ozone using GEOS-Chem simulations with a high-resolution satellite-derived emission inventory. Compared to coarser temporal resolutions, incorporating diurnal variations leads to significant changes in surface ozone and atmospheric oxidation capacity. Our findings highlight the importance of accurately representing BB emission timing in chemical transport models to improve ozone predictions.
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Roland Vernooij, Tom Eames, Jeremy Russell-Smith, Cameron Yates, Robin Beatty, Jay Evans, Andrew Edwards, Natasha Ribeiro, Martin Wooster, Tercia Strydom, Marcos Vinicius Giongo, Marco Assis Borges, Máximo Menezes Costa, Ana Carolina Sena Barradas, Dave van Wees, and Guido R. Van der Werf
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Frederik Kurzrock, Hannah Nguyen, Jerome Sauer, Fabrice Chane Ming, Sylvain Cros, William L. Smith Jr., Patrick Minnis, Rabindra Palikonda, Thomas A. Jones, Caroline Lallemand, Laurent Linguet, and Gilles Lajoie
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The current El Niño event has had a dramatic impact on the amount of Indonesian biomass burning and subsequent greenhouse gas emission. We have used satellite observations of CH4 and CO2 of these fires to probe aspects of their chemical composition. We show large enhancements in the amount of these species, due to the fire emissions. The ability to determine large-scale emission ratios from space allows the combustion behaviour of very large regions of burning to be characterised and understood.
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Fires associated with land use and land cover changes release large amounts of aerosols and trace gases into the atmosphere. Although several inventories of biomass burning emissions cover Brazil, there are still considerable uncertainties and differences among them. However, results indicate that emission derived via similar methods tend to agree with one other, but aerosol emissions from fires with particularly high biomass consumption still lead to an underestimation.
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Landscape fire plume height controls fire emissions release in the atmosphere, in particular their transport that may also affect the longevity, chemical conversion, and fate of the plumes chemical constituents. Here, we review how such landscape-scale fire smoke plume injection heights are represented in large-scale atmospheric transport models aiming to represent the impacts of wildfire emissions on component of the Earth system.
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Landscape fires strongly influence atmospheric chemistry, composition, and climate. Characterizing such fires at very high temporal resolution is best achieved using thermal observations of actively burning fires made from geostationary Earth Observation satellites. Here we detail the Fire Radiative Power (FRP) products generated by the Land Surface Analysis Satellite Applications Facility (LSA SAF) from data collected by the Meteosat geostationary satellites.
G. Roberts, M. J. Wooster, W. Xu, P. H. Freeborn, J.-J. Morcrette, L. Jones, A. Benedetti, H. Jiangping, D. Fisher, and J. W. Kaiser
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Characterising the dynamics of wildfires at high temporal resolution is best achieved using observations from geostationary satellite sensors. The SEVIRI Fire Radiative Power (FRP) products have been developed using such imagery at up to 15-minute temporal frequency. These data are used to estimate wildfire fuel consumption and to the characterise smoke emissions from the 2007 Peloponnese "mega fires" within an atmospheric transport model.
N. Andela, J. W. Kaiser, G. R. van der Werf, and M. J. Wooster
Atmos. Chem. Phys., 15, 8831–8846, https://doi.org/10.5194/acp-15-8831-2015, https://doi.org/10.5194/acp-15-8831-2015, 2015
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The polar orbiting MODIS instruments provide four daily observations of the fire diurnal cycle, resulting in erroneous fire radiative energy (FRE) estimates. Using geostationary SEVIRI data, we explore the fire diurnal cycle and its drivers for Africa to develop a new method to estimate global FRE in near real-time using MODIS. The fire diurnal cycle varied with climate and vegetation type, and including information on the fire diurnal cycle in the model significantly improved the FRE estimates.
S. Gonzi, P. I. Palmer, R. Paugam, M. Wooster, and M. N. Deeter
Atmos. Chem. Phys., 15, 4339–4355, https://doi.org/10.5194/acp-15-4339-2015, https://doi.org/10.5194/acp-15-4339-2015, 2015
R. Paugam, M. Wooster, J. Atherton, S. R. Freitas, M. G. Schultz, and J. W. Kaiser
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acpd-15-9815-2015, https://doi.org/10.5194/acpd-15-9815-2015, 2015
Revised manuscript not accepted
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The transport of Biomass Burning emissions in Chemical Transport Model rely on parametrization of plumes injection height. Using fire observation selected to ensure match-up of fire-atmosphere-plume dynamics; a popular plume rise model was improved and optimized. The resulting model shows response to the effect of atmospheric stability consistent with previous findings and is able to predict higher injection height than any other tested parametrizations, giving a closer match with observation.
T. E. L. Smith, C. Paton-Walsh, C. P. Meyer, G. D. Cook, S. W. Maier, J. Russell-Smith, M. J. Wooster, and C. P. Yates
Atmos. Chem. Phys., 14, 11335–11352, https://doi.org/10.5194/acp-14-11335-2014, https://doi.org/10.5194/acp-14-11335-2014, 2014
S. Turquety, L. Menut, B. Bessagnet, A. Anav, N. Viovy, F. Maignan, and M. Wooster
Geosci. Model Dev., 7, 587–612, https://doi.org/10.5194/gmd-7-587-2014, https://doi.org/10.5194/gmd-7-587-2014, 2014
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Subject: Gases | Research Activity: Remote Sensing | Altitude Range: Troposphere | Science Focus: Chemistry (chemical composition and reactions)
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The Ozone Monitoring Instrument (OMI) was used to understand the evolution of NOx emissions from the Canadian oil sands. OMI NO2 combined with winds and reported stack emissions found emissions from the heavy-hauler mine fleet have remained flat since 2005, whereas the total oil sands mined have more than doubled. This difference is a result of emissions standards that limit NOx emissions becoming more stringent over this period, confirming the efficacy of the policy enacting these standards.
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Atmos. Chem. Phys., 25, 4391–4401, https://doi.org/10.5194/acp-25-4391-2025, https://doi.org/10.5194/acp-25-4391-2025, 2025
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Globally, lockdowns were implemented to limit the spread of COVID-19, leading to a decrease in emissions of key air pollutants. Here, we use novel satellite data and a chemistry model to investigate the impact of the pandemic on tropospheric ozone (O3), a key pollutant, in 2020. Overall, we found substantial decreases of up to 20 %, two-thirds of which came from emission reductions, while one-third was due to a decrease in the stratospheric O3 flux into the troposphere.
Anne Boynard, Catherine Wespes, Juliette Hadji-Lazaro, Selviga Sinnathamby, Daniel Hurtmans, Pierre-François Coheur, Marie Doutriaux-Boucher, Jacobus Onderwaater, Wolfgang Steinbrecht, Elyse A. Pennington, Kevin Bowman, and Cathy Clerbaux
EGUsphere, https://doi.org/10.5194/egusphere-2025-1054, https://doi.org/10.5194/egusphere-2025-1054, 2025
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This study analyzes 16 years of global ozone data to assess its impact on air quality and climate. Using satellite measurements, we observed a global decrease in tropospheric ozone, particularly in tropical and European regions. The study highlights the importance of long-term data for tracking trends, especially during events like the pandemic. We emphasize the need for improved data processing and integrating multiple datasets to better understand ozone trends.
Yujin J. Oak, Daniel J. Jacob, Drew C. Pendergrass, Ruijun Dang, Nadia K. Colombi, Heesung Chong, Seoyoung Lee, Su Keun Kuk, and Jhoon Kim
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We analyze 2015–2023 air quality trends in South Korea using surface and satellite observations. Primary pollutants have decreased, consistent with emissions reductions. Surface O3 continues to increase and PM2.5 has decreased overall, but the nitrate component has not. O3 and PM2.5 nitrate depend on nonlinear responses from precursor emissions. Satellite data indicate a recent shift to NOx-sensitive O3 and nitrate formation, where further NOx reductions will benefit both O3 and PM2.5 pollution.
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The hydroxyl radical (OH) destroys many air pollutants, including methane. Global-mean OH cannot be directly measured, and thus it is inferred with the methyl chloroform (MCF) proxy. MCF is decreasing, and a replacement is needed. We use satellite observations of methane in two spectral ranges as a proxy for OH. We find shortwave infrared observations can characterize yearly OH and its seasonality but not the latitudinal distribution. Thermal infrared observations add little information.
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This study applies an approach that assimilates NO2 vertical column densities from TROPOMI in a mass-conserving manner and inverts daily NOx emissions, presented over rapidly changing regions in China. Source attribution is quantified by the local thermodynamics of the combustion temperature (NOx/NO2). Emission results identify sources which do not exist in the a priori datasets, especially medium industrial sources located next to the Yangtze River.
Amir H. Souri, Gonzalo González Abad, Glenn M. Wolfe, Tijl Verhoelst, Corinne Vigouroux, Gaia Pinardi, Steven Compernolle, Bavo Langerock, Bryan N. Duncan, and Matthew S. Johnson
Atmos. Chem. Phys., 25, 2061–2086, https://doi.org/10.5194/acp-25-2061-2025, https://doi.org/10.5194/acp-25-2061-2025, 2025
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We establish a simple yet robust relationship between ozone production rates and geophysical parameters obtained from several intensive atmospheric composition campaigns. We show that satellite remote sensing data can effectively constrain these parameters, enabling us to produce the first global maps of ozone production rates with unprecedented resolution.
Yu Tian, Siyi Wang, and Xiaomeng Jin
EGUsphere, https://doi.org/10.5194/egusphere-2025-368, https://doi.org/10.5194/egusphere-2025-368, 2025
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We leverage over two-decade ground-based ozone observations alongside space-based observations of ozone precursors (NO2 and formaldehyde) to study the long-term evolution in ozone chemical regimes across global source regions. We find a global trend towards NOx-limited regimes, supported by increasing satellite-based HCHO/NO2 and a diminishing ozone weekend effect.
Norbert Glatthor, Gabriele P. Stiller, Thomas von Clarmann, Bernd Funke, Sylvia Kellmann, and Andrea Linden
Atmos. Chem. Phys., 25, 1175–1208, https://doi.org/10.5194/acp-25-1175-2025, https://doi.org/10.5194/acp-25-1175-2025, 2025
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We present global upper-tropospheric distributions of the pollutants HCN, CO, C2H2, C2H6, PAN, and HCOOH, observed between 2002 and 2012 by the Michelson Interferometer for Passive Atmospheric Sounding (MIPAS) on the Environmental Satellite (Envisat). By comparing the spatial distributions of their volume mixing ratios and by global correlation and regression analyses, we draw conclusions on their sources, such as biomass burning, anthropogenic sources, and biogenic release.
Gijs Leguijt, Joannes D. Maasakkers, Hugo A. C. Denier van der Gon, Arjo J. Segers, Tobias Borsdorff, Ivar R. van der Velde, and Ilse Aben
Atmos. Chem. Phys., 25, 555–574, https://doi.org/10.5194/acp-25-555-2025, https://doi.org/10.5194/acp-25-555-2025, 2025
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The production of steel coincides with large emissions of greenhouse gases and air pollutants including carbon monoxide. European facilities are required to report their emissions, which are estimated using a variety of methods. We evaluate these estimates using carbon monoxide concentrations measured via satellite. We find generally good agreement between our values and those reported but also identify some uncertainties, showing that satellites can provide insights into these emissions.
Chengxin Zhang, Xinhan Niu, Hongyu Wu, Zhipeng Ding, Ka Lok Chan, Jhoon Kim, Thomas Wagner, and Cheng Liu
Atmos. Chem. Phys., 25, 759–770, https://doi.org/10.5194/acp-25-759-2025, https://doi.org/10.5194/acp-25-759-2025, 2025
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This research utilizes hourly air pollution observations from the world’s first geostationary satellite to develop a spatiotemporal neural network model for full-coverage surface NO2 pollution prediction over the next 24 hours, achieving outstanding forecasting performance and efficacy. These results highlight the profound impact of geostationary satellite observations in advancing air quality forecasting models, thereby contributing to future models for health exposure to air pollution.
Lucien Froidevaux, Douglas E. Kinnison, Benjamin Gaubert, Michael J. Schwartz, Nathaniel J. Livesey, William G. Read, Charles G. Bardeen, Jerry R. Ziemke, and Ryan A. Fuller
Atmos. Chem. Phys., 25, 597–624, https://doi.org/10.5194/acp-25-597-2025, https://doi.org/10.5194/acp-25-597-2025, 2025
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We compare observed changes in ozone (O3) and carbon monoxide (CO) in the tropical upper troposphere (10–15 km altitude) for 2005–2020 to predictions from model simulations that track the evolution of natural and industrial emissions transported to this region. An increasing trend in measured upper-tropospheric O3 is well matched by model trends. We find that changes in modeled industrial CO surface emissions lead to better model agreement with observed slight decreases in upper-tropospheric CO.
Vitali Fioletov, Chris A. McLinden, Debora Griffin, Xiaoyi Zhao, and Henk Eskes
Atmos. Chem. Phys., 25, 575–596, https://doi.org/10.5194/acp-25-575-2025, https://doi.org/10.5194/acp-25-575-2025, 2025
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Satellite data were used to estimate urban per capita emissions for 261 major cities worldwide. Three components in tropospheric NO2 data (background NO2, NO2 from urban sources, and NO2 from industrial point sources) were isolated, and then each of these components was analyzed separately. The largest per capita emissions were found in the Middle East and the smallest in India and southern Africa. Urban weekend emissions are 20 %–50 % less than workday emissions for all regions except China.
Roeland Van Malderen, Zhou Zang, Kai-Lan Chang, Robin Björklund, Owen R. Cooper, Jane Liu, Eliane Maillard Barras, Corinne Vigouroux, Irina Petropavlovskikh, Thierry Leblanc, Valérie Thouret, Pawel Wolff, Peter Effertz, Audrey Gaudel, David W. Tarasick, Herman G. J. Smit, Anne M. Thompson, Ryan M. Stauffer, Debra E. Kollonige, Deniz Poyraz, Gérard Ancellet, Marie-Renée De Backer, Matthias M. Frey, James W. Hannigan, José L. Hernandez, Bryan J. Johnson, Nicholas Jones, Rigel Kivi, Emmanuel Mahieu, Isamu Morino, Glen McConville, Katrin Müller, Isao Murata, Justus Notholt, Ankie Piters, Maxime Prignon, Richard Querel, Vincenzo Rizi, Dan Smale, Wolfgang Steinbrecht, Kimberly Strong, and Ralf Sussmann
EGUsphere, https://doi.org/10.5194/egusphere-2024-3745, https://doi.org/10.5194/egusphere-2024-3745, 2025
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Tropospheric ozone is an important greenhouse gas and an air pollutant, whose distribution and time variability is mainly governed by anthropogenic emissions and dynamics. In this paper, we assess regional trends of tropospheric ozone column amounts, based on two different approaches of merging or synthesizing ground-based observations and their trends within specific regions. Our findings clearly demonstrate regional trend differences, but also consistently higher pre- than post-COVID trends.
Zhuang Wang, Chune Shi, Hao Zhang, Xianguang Ji, Yizhi Zhu, Congzi Xia, Xiaoyun Sun, Xinfeng Lin, Shaowei Yan, Suyao Wang, Yuan Zhou, Chengzhi Xing, Yujia Chen, and Cheng Liu
Atmos. Chem. Phys., 25, 347–366, https://doi.org/10.5194/acp-25-347-2025, https://doi.org/10.5194/acp-25-347-2025, 2025
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This study attempts to explain the surface ozone background and typical and peak trends in eastern China by combining a large number of ground-based and satellite observations. We found diametrically opposed trends in peak (decreasing) and low (increasing) ozone concentrations. Anthropogenic emissions primarily drive trends in low and peak ozone concentrations in eastern China, though meteorological effects also play a role.
Rebekah P. Horner, Eloise A. Marais, Nana Wei, Robert G. Ryan, and Viral Shah
Atmos. Chem. Phys., 24, 13047–13064, https://doi.org/10.5194/acp-24-13047-2024, https://doi.org/10.5194/acp-24-13047-2024, 2024
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Nitrogen oxides (NOx ≡ NO + NO2) affect tropospheric ozone and the hydroxyl radical, influencing climate and atmospheric oxidation. To address the lack of routine observations of NOx, we cloud slice satellite observations of NO2 to derive a new dataset of global vertical profiles of NO2. We evaluate our data against in situ aircraft observations and use these data to critique the contemporary understanding of tropospheric NOx, as simulated by the GEOS-Chem model.
Bryan N. Duncan, Daniel C. Anderson, Arlene M. Fiore, Joanna Joiner, Nickolay A. Krotkov, Can Li, Dylan B. Millet, Julie M. Nicely, Luke D. Oman, Jason M. St. Clair, Joshua D. Shutter, Amir H. Souri, Sarah A. Strode, Brad Weir, Glenn M. Wolfe, Helen M. Worden, and Qindan Zhu
Atmos. Chem. Phys., 24, 13001–13023, https://doi.org/10.5194/acp-24-13001-2024, https://doi.org/10.5194/acp-24-13001-2024, 2024
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Trace gases emitted to or formed within the atmosphere may be chemically or physically removed from the atmosphere. One trace gas, the hydroxyl radical (OH), is responsible for initiating the chemical removal of many trace gases, including some greenhouse gases. Despite its importance, scientists have not been able to adequately measure OH. In this opinion piece, we discuss promising new methods to indirectly constrain OH using satellite data of trace gases that control the abundance of OH.
Emma Sands, Richard J. Pope, Ruth M. Doherty, Fiona M. O'Connor, Chris Wilson, and Hugh Pumphrey
Atmos. Chem. Phys., 24, 11081–11102, https://doi.org/10.5194/acp-24-11081-2024, https://doi.org/10.5194/acp-24-11081-2024, 2024
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Changes in vegetation alongside biomass burning impact regional atmospheric composition and air quality. Using satellite remote sensing, we find a clear linear relationship between forest cover and isoprene and a pronounced non-linear relationship between burned area and nitrogen dioxide in the southern Amazon, a region of substantial deforestation. These quantified relationships can be used for model evaluation and further exploration of biosphere-atmosphere interactions in Earth System Models.
Jieying Ding, Ronald van der A, Henk Eskes, Enrico Dammers, Mark Shephard, Roy Wichink Kruit, Marc Guevara, and Leonor Tarrason
Atmos. Chem. Phys., 24, 10583–10599, https://doi.org/10.5194/acp-24-10583-2024, https://doi.org/10.5194/acp-24-10583-2024, 2024
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Here we applied the existing Daily Emissions Constrained by Satellite Observations (DECSO) inversion algorithm to NH3 observations from the CrIS satellite instrument to estimate NH3 emissions. As NH3 in the atmosphere is influenced by NOx, we implemented DECSO to estimate NOx and NH3 emissions simultaneously. The emissions are derived over Europe for 2020 at a spatial resolution of 0.2° using daily observations from CrIS and TROPOMI. Results are compared to bottom-up emission inventories.
Matthew S. Johnson, Sajeev Philip, Scott Meech, Rajesh Kumar, Meytar Sorek-Hamer, Yoichi P. Shiga, and Jia Jung
Atmos. Chem. Phys., 24, 10363–10384, https://doi.org/10.5194/acp-24-10363-2024, https://doi.org/10.5194/acp-24-10363-2024, 2024
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Satellites, like the Ozone Monitoring Instrument (OMI), retrieve proxy species of ozone (O3) formation (formaldehyde and nitrogen dioxide) and the ratios (FNRs) which can define O3 production sensitivity regimes. Here we investigate trends of OMI FNRs from 2005 to 2021, and they have increased in major cities, suggesting a transition from radical- to NOx-limited regimes. OMI also observed the impact of reduced emissions during the 2020 COVID-19 lockdown that resulted in increased FNRs.
Audrey Gaudel, Ilann Bourgeois, Meng Li, Kai-Lan Chang, Jerald Ziemke, Bastien Sauvage, Ryan M. Stauffer, Anne M. Thompson, Debra E. Kollonige, Nadia Smith, Daan Hubert, Arno Keppens, Juan Cuesta, Klaus-Peter Heue, Pepijn Veefkind, Kenneth Aikin, Jeff Peischl, Chelsea R. Thompson, Thomas B. Ryerson, Gregory J. Frost, Brian C. McDonald, and Owen R. Cooper
Atmos. Chem. Phys., 24, 9975–10000, https://doi.org/10.5194/acp-24-9975-2024, https://doi.org/10.5194/acp-24-9975-2024, 2024
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The study examines tropical tropospheric ozone changes. In situ data from 1994–2019 display increased ozone, notably over India, Southeast Asia, and Malaysia and Indonesia. Sparse in situ data limit trend detection for the 15-year period. In situ and satellite data, with limited sampling, struggle to consistently detect trends. Continuous observations are vital over the tropical Pacific Ocean, Indian Ocean, western Africa, and South Asia for accurate ozone trend estimation in these regions.
Naveed Ahmad, Changqing Lin, Alexis K. H. Lau, Jhoon Kim, Tianshu Zhang, Fangqun Yu, Chengcai Li, Ying Li, Jimmy C. H. Fung, and Xiang Qian Lao
Atmos. Chem. Phys., 24, 9645–9665, https://doi.org/10.5194/acp-24-9645-2024, https://doi.org/10.5194/acp-24-9645-2024, 2024
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This study developed a nested machine learning model to convert the GEMS NO2 column measurements into ground-level concentrations across China. The model directly incorporates the NO2 mixing height (NMH) into the methodological framework. The study underscores the importance of considering NMH when estimating ground-level NO2 from satellite column measurements and highlights the significant advantages of new-generation geostationary satellites in air quality monitoring.
Richard J. Pope, Fiona M. O'Connor, Mohit Dalvi, Brian J. Kerridge, Richard Siddans, Barry G. Latter, Brice Barret, Eric Le Flochmoen, Anne Boynard, Martyn P. Chipperfield, Wuhu Feng, Matilda A. Pimlott, Sandip S. Dhomse, Christian Retscher, Catherine Wespes, and Richard Rigby
Atmos. Chem. Phys., 24, 9177–9195, https://doi.org/10.5194/acp-24-9177-2024, https://doi.org/10.5194/acp-24-9177-2024, 2024
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Ozone is a potent air pollutant in the lower troposphere, with adverse impacts on human health. Satellite records of tropospheric ozone currently show large-scale inconsistencies in long-term trends. Our detailed study of the potential factors (e.g. satellite errors, where the satellite can observe ozone) potentially driving these inconsistencies found that, in North America, Europe, and East Asia, the underlying trends are typically small with large uncertainties.
David P. Edwards, Sara Martínez-Alonso, Duseong S. Jo, Ivan Ortega, Louisa K. Emmons, John J. Orlando, Helen M. Worden, Jhoon Kim, Hanlim Lee, Junsung Park, and Hyunkee Hong
Atmos. Chem. Phys., 24, 8943–8961, https://doi.org/10.5194/acp-24-8943-2024, https://doi.org/10.5194/acp-24-8943-2024, 2024
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Until recently, satellite observations of atmospheric pollutants at any location could only be obtained once a day. New geostationary satellites stare at a region of the Earth to make hourly measurements, and the Geostationary Environment Monitoring Spectrometer is the first looking at Asia. These data and model simulations show how the change seen for one important pollutant that determines air quality depends on a combination of pollution emissions, atmospheric chemistry, and meteorology.
Sören Johansson, Michael Höpfner, Felix Friedl-Vallon, Norbert Glatthor, Thomas Gulde, Vincent Huijnen, Anne Kleinert, Erik Kretschmer, Guido Maucher, Tom Neubert, Hans Nordmeyer, Christof Piesch, Peter Preusse, Martin Riese, Björn-Martin Sinnhuber, Jörn Ungermann, Gerald Wetzel, and Wolfgang Woiwode
Atmos. Chem. Phys., 24, 8125–8138, https://doi.org/10.5194/acp-24-8125-2024, https://doi.org/10.5194/acp-24-8125-2024, 2024
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We present airborne infrared limb sounding GLORIA measurements of ammonia (NH3) in the upper troposphere of air masses within the Asian monsoon and of those connected with biomass burning. Comparing CAMS (Copernicus Atmosphere Monitoring Service) model data, we find that the model reproduces the measured enhanced NH3 within the Asian monsoon well but not that within biomass burning plumes, where no enhanced NH3 is measured in the upper troposphere but considerable amounts are simulated by CAMS.
Sandro Meier, Erik F. M. Koene, Maarten Krol, Dominik Brunner, Alexander Damm, and Gerrit Kuhlmann
Atmos. Chem. Phys., 24, 7667–7686, https://doi.org/10.5194/acp-24-7667-2024, https://doi.org/10.5194/acp-24-7667-2024, 2024
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Nitrogen oxides (NOx = NO + NO2) are important air pollutants. This study addresses the challenge of accurately estimating NOx emissions from NO2 satellite observations. We develop a realistic model to convert NO2 to NOx by using simulated plumes from various power plants. We apply the model to satellite NO2 observations, significantly reducing biases in estimated NOx emissions. The study highlights the potential for a consistent, high-resolution estimation of NOx emissions using satellite data.
Oliver Schneising, Michael Buchwitz, Maximilian Reuter, Michael Weimer, Heinrich Bovensmann, John P. Burrows, and Hartmut Bösch
Atmos. Chem. Phys., 24, 7609–7621, https://doi.org/10.5194/acp-24-7609-2024, https://doi.org/10.5194/acp-24-7609-2024, 2024
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Large quantities of CO and CO2 are emitted during conventional steel production. As satellite-based estimates of CO2 emissions at the facility level are challenging, co-emitted CO can indicate the carbon footprint of steel plants. We estimate CO emissions for German steelworks and use CO2 emissions from emissions trading data to derive a sector-specific CO/CO2 emission ratio for the steel industry; it is a prerequisite to use CO as a proxy for CO2 emissions from similar steel production sites.
Ronald J. van der A, Jieying Ding, and Henk Eskes
Atmos. Chem. Phys., 24, 7523–7534, https://doi.org/10.5194/acp-24-7523-2024, https://doi.org/10.5194/acp-24-7523-2024, 2024
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Using observations of the Sentinel-5P satellite and the latest version of the inversion algorithm DECSO, anthropogenic NOx emissions are derived for Europe for the years 2019–2022 with a spatial resolution of 0.2°. The results are compared with European emissions of the Copernicus Atmosphere Monitoring Service.
Xuehong Gong, Zeyu Liu, Jie Tian, Qiyuan Wang, Guohui Li, Zhisheng An, and Yongming Han
EGUsphere, https://doi.org/10.5194/egusphere-2024-1684, https://doi.org/10.5194/egusphere-2024-1684, 2024
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Our study analyzed CO2 emissions from wildfires in China from 2001 to 2022. Cropland and forest fires contributed the most, while grassland fires were the least. Emissions from forest and shrub fires decreased significantly, while cropland fires increased. The highest emissions were in Heilongjiang and Inner Mongolia. China's effective policy management has reduced wildfire-related CO2 emissions, aiding global climate change efforts.
Bruno Franco, Lieven Clarisse, Nicolas Theys, Juliette Hadji-Lazaro, Cathy Clerbaux, and Pierre Coheur
Atmos. Chem. Phys., 24, 4973–5007, https://doi.org/10.5194/acp-24-4973-2024, https://doi.org/10.5194/acp-24-4973-2024, 2024
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Using IASI global infrared measurements, we retrieve nitrous acid (HONO) in fire plumes from space. We detect large enhancements of pyrogenic HONO worldwide, especially from intense wildfires at Northern Hemisphere mid- and high latitudes. Predominance of IASI nighttime over daytime measurements sheds light on HONO's extended lifetime and secondary formation during long-range transport in smoke plumes. Our findings deepen the understanding of atmospheric HONO, crucial for air quality assessment.
Gitaek T. Lee, Rokjin J. Park, Hyeong-Ahn Kwon, Eunjo S. Ha, Sieun D. Lee, Seunga Shin, Myoung-Hwan Ahn, Mina Kang, Yong-Sang Choi, Gyuyeon Kim, Dong-Won Lee, Deok-Rae Kim, Hyunkee Hong, Bavo Langerock, Corinne Vigouroux, Christophe Lerot, Francois Hendrick, Gaia Pinardi, Isabelle De Smedt, Michel Van Roozendael, Pucai Wang, Heesung Chong, Yeseul Cho, and Jhoon Kim
Atmos. Chem. Phys., 24, 4733–4749, https://doi.org/10.5194/acp-24-4733-2024, https://doi.org/10.5194/acp-24-4733-2024, 2024
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This study evaluates the Geostationary Environment Monitoring Spectrometer (GEMS) HCHO product by comparing its vertical column densities (VCDs) with those of TROPOMI and ground-based observations. Based on some sensitivity tests, obtaining radiance references under clear-sky conditions significantly improves HCHO retrieval quality. GEMS HCHO VCDs captured seasonal and diurnal variations well during the first year of observation, showing consistency with TROPOMI and ground-based observations.
Fei Liu, Steffen Beirle, Joanna Joiner, Sungyeon Choi, Zhining Tao, K. Emma Knowland, Steven J. Smith, Daniel Q. Tong, Siqi Ma, Zachary T. Fasnacht, and Thomas Wagner
Atmos. Chem. Phys., 24, 3717–3728, https://doi.org/10.5194/acp-24-3717-2024, https://doi.org/10.5194/acp-24-3717-2024, 2024
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Using satellite data, we developed a coupled method independent of the chemical transport model to map NOx emissions across US cities. After validating our technique with synthetic data, we charted NOx emissions from 2018–2021 in 39 cities. Our results closely matched EPA estimates but also highlighted some inconsistencies in both magnitude and spatial distribution. This research can help refine strategies for monitoring and managing air quality.
Richard J. Pope, Alexandru Rap, Matilda A. Pimlott, Brice Barret, Eric Le Flochmoen, Brian J. Kerridge, Richard Siddans, Barry G. Latter, Lucy J. Ventress, Anne Boynard, Christian Retscher, Wuhu Feng, Richard Rigby, Sandip S. Dhomse, Catherine Wespes, and Martyn P. Chipperfield
Atmos. Chem. Phys., 24, 3613–3626, https://doi.org/10.5194/acp-24-3613-2024, https://doi.org/10.5194/acp-24-3613-2024, 2024
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Tropospheric ozone is an important short-lived climate forcer which influences the incoming solar short-wave radiation and the outgoing long-wave radiation in the atmosphere (8–15 km) where the balance between the two yields a net positive (i.e. warming) effect at the surface. Overall, we find that the tropospheric ozone radiative effect ranges between 1.21 and 1.26 W m−2 with a negligible trend (2008–2017), suggesting that tropospheric ozone influences on climate have remained stable with time.
Isabelle A. Taylor, Roy G. Grainger, Andrew T. Prata, Simon R. Proud, Tamsin A. Mather, and David M. Pyle
Atmos. Chem. Phys., 23, 15209–15234, https://doi.org/10.5194/acp-23-15209-2023, https://doi.org/10.5194/acp-23-15209-2023, 2023
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This study looks at sulfur dioxide (SO2) and ash emissions from the April 2021 eruption of La Soufrière on St Vincent. Using satellite data, 35 eruptive events were identified. Satellite data were used to track SO2 as it was transported around the globe. The majority of SO2 was emitted into the upper troposphere and lower stratosphere. Similarities with the 1979 eruption of La Soufrière highlight the value of studying these eruptions to be better prepared for future eruptions.
Richard J. Pope, Brian J. Kerridge, Richard Siddans, Barry G. Latter, Martyn P. Chipperfield, Wuhu Feng, Matilda A. Pimlott, Sandip S. Dhomse, Christian Retscher, and Richard Rigby
Atmos. Chem. Phys., 23, 14933–14947, https://doi.org/10.5194/acp-23-14933-2023, https://doi.org/10.5194/acp-23-14933-2023, 2023
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Ozone is a potent air pollutant, and we present the first study to investigate long-term changes in lower tropospheric column ozone (LTCO3) from space. We have constructed a merged LTCO3 dataset from GOME-1, SCIAMACHY and OMI between 1996 and 2017. Comparing LTCO3 between the 1996–2000 and 2013–2017 5-year averages, we find significant positive increases in the tropics/sub-tropics, while in the northern mid-latitudes, we find small-scale differences.
Daniel H. Cusworth, Andrew K. Thorpe, Charles E. Miller, Alana K. Ayasse, Ralph Jiorle, Riley M. Duren, Ray Nassar, Jon-Paul Mastrogiacomo, and Robert R. Nelson
Atmos. Chem. Phys., 23, 14577–14591, https://doi.org/10.5194/acp-23-14577-2023, https://doi.org/10.5194/acp-23-14577-2023, 2023
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Carbon dioxide (CO2) emissions from combustion sources are uncertain in many places across the globe. Satellites have the ability to detect and quantify emissions from large CO2 point sources, including coal-fired power plants. In this study, we tasked two satellites to routinely observe CO2 emissions at 30 coal-fired power plants between 2021 and 2022. These results present the largest dataset of space-based CO2 emission estimates to date.
Maria Tsivlidou, Bastien Sauvage, Yasmine Bennouna, Romain Blot, Damien Boulanger, Hannah Clark, Eric Le Flochmoën, Philippe Nédélec, Valérie Thouret, Pawel Wolff, and Brice Barret
Atmos. Chem. Phys., 23, 14039–14063, https://doi.org/10.5194/acp-23-14039-2023, https://doi.org/10.5194/acp-23-14039-2023, 2023
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The tropics are a region where the ozone increase has been most apparent since 1980 and where observations are sparse. Using aircraft, satellite, and model data, we document the characteristics of tropospheric ozone and CO over the whole tropics for the last 2 decades. We explore the origin of the observed CO anomalies and investigate transport processes driving the tropical CO and O3 distribution. Our study highlights the importance of anthropogenic emissions, mostly over the northern tropics.
Richard J. Pope, Brian J. Kerridge, Martyn P. Chipperfield, Richard Siddans, Barry G. Latter, Lucy J. Ventress, Matilda A. Pimlott, Wuhu Feng, Edward Comyn-Platt, Garry D. Hayman, Stephen R. Arnold, and Ailish M. Graham
Atmos. Chem. Phys., 23, 13235–13253, https://doi.org/10.5194/acp-23-13235-2023, https://doi.org/10.5194/acp-23-13235-2023, 2023
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In the summer of 2018, Europe experienced several persistent large-scale ozone (O3) pollution episodes. Satellite tropospheric O3 and surface O3 data recorded substantial enhancements in 2018 relative to other years. Targeted model simulations showed that meteorological processes and emissions controlled the elevated surface O3, while mid-tropospheric O3 enhancements were dominated by stratospheric O3 intrusion and advection of North Atlantic O3-rich air masses into Europe.
Rui Wang, Da Pan, Xuehui Guo, Kang Sun, Lieven Clarisse, Martin Van Damme, Pierre-François Coheur, Cathy Clerbaux, Melissa Puchalski, and Mark A. Zondlo
Atmos. Chem. Phys., 23, 13217–13234, https://doi.org/10.5194/acp-23-13217-2023, https://doi.org/10.5194/acp-23-13217-2023, 2023
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Ammonia (NH3) is a key precursor for fine particulate matter (PM2.5) and a primary form of reactive nitrogen, yet it has sparse ground measurements. We perform the first comprehensive comparison between ground observations and satellite retrievals in the US, demonstrating that satellite NH3 data can help fill spatial gaps in the current ground monitoring networks. Trend analyses using both datasets highlight increasing NH3 trends across the US, including the NH3 hotspots and urban areas.
Rimal Abeed, Camille Viatte, William C. Porter, Nikolaos Evangeliou, Cathy Clerbaux, Lieven Clarisse, Martin Van Damme, Pierre-François Coheur, and Sarah Safieddine
Atmos. Chem. Phys., 23, 12505–12523, https://doi.org/10.5194/acp-23-12505-2023, https://doi.org/10.5194/acp-23-12505-2023, 2023
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Ammonia emissions from agricultural activities will inevitably increase with the rise in population. We use a variety of datasets (satellite, reanalysis, and model simulation) to calculate the first regional map of ammonia emission potential during the start of the growing season in Europe. We then apply our developed method using a climate model to show the effect of the temperature increase on future ammonia columns under two possible climate scenarios.
Bianca Zilker, Andreas Richter, Anne-Marlene Blechschmidt, Peter von der Gathen, Ilias Bougoudis, Sora Seo, Tim Bösch, and John Philip Burrows
Atmos. Chem. Phys., 23, 9787–9814, https://doi.org/10.5194/acp-23-9787-2023, https://doi.org/10.5194/acp-23-9787-2023, 2023
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During Arctic spring, near-surface ozone is depleted by bromine released from salty sea ice and/or snow-covered areas under certain meteorological conditions. To study this ozone depletion and the prevailing meteorological conditions, two ozone data sets from Ny-Ålesund, Svalbard, have been evaluated. We found that during ozone depletion events lower pressure over the Barents Sea and higher pressure in the Icelandic Low area led to a transport of cold polar air from the north to Ny-Ålesund.
Gijs Leguijt, Joannes D. Maasakkers, Hugo A. C. Denier van der Gon, Arjo J. Segers, Tobias Borsdorff, and Ilse Aben
Atmos. Chem. Phys., 23, 8899–8919, https://doi.org/10.5194/acp-23-8899-2023, https://doi.org/10.5194/acp-23-8899-2023, 2023
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We present a fast method to evaluate carbon monoxide emissions from cities in Africa. Carbon monoxide is important for climate change in an indirect way, as it is linked to ozone, methane, and carbon dioxide. Our measurements are made with a satellite that sees the entire globe every single day. This means that we can check from space whether the current knowledge of emission rates is up to date. We make the comparison and show that the emission rates in northern Africa are underestimated.
Chantelle R. Lonsdale and Kang Sun
Atmos. Chem. Phys., 23, 8727–8748, https://doi.org/10.5194/acp-23-8727-2023, https://doi.org/10.5194/acp-23-8727-2023, 2023
Short summary
Short summary
The COVID-19 pandemic, which was caused by the SARS-CoV-2 virus, emerged in 2019, and its still evolving variants have resulted in unprecedented shifts in human activities and anthropogenic emissions into the Earth's atmosphere. We present monthly nitrogen oxide emissions over three major continents from May 2018 to January 2023 to capture variations before and after the COVID-19 pandemic. We focus on a diverse collection of 54 cities to quantify the post-COVID-19 perturbations.
Cited articles
Abel, S. J., Haywood, J. M., Highwood, E. J., Li, J., and Buseck, P. R.:
Evolution of biomass burning aerosol properties from an agricultural fire in
southern Africa, Geophys. Res. Lett., 30, 10–13,
https://doi.org/10.1029/2003GL017342, 2003.
Akagi, S. K., Yokelson, R. J., Wiedinmyer, C., Alvarado, M. J., Reid, J. S., Karl, T., Crounse, J. D., and Wennberg, P. O.: Emission factors for open and domestic biomass burning for use in atmospheric models, Atmos. Chem. Phys., 11, 4039–4072, https://doi.org/10.5194/acp-11-4039-2011, 2011.
Andreae, M. O.: Emission of trace gases and aerosols from biomass burning – an updated assessment, Atmos. Chem. Phys., 19, 8523–8546, https://doi.org/10.5194/acp-19-8523-2019, 2019.
Andreae, M. O. and Merlet, P.: Emissions of trace gases and aerosols from
biomass burning, Global Biogeochem. Cy., 15, 955–966,
https://doi.org/10.1029/2000GB001382, 2001.
Baldassarre, G., Pozzoli, L., Schmidt, C. C., Unal, A., Kindap, T., Menzel, W. P., Whitburn, S., Coheur, P.-F., Kavgaci, A., and Kaiser, J. W.: Using SEVIRI fire observations to drive smoke plumes in the CMAQ air quality model: a case study over Antalya in 2008, Atmos. Chem. Phys., 15, 8539–8558, https://doi.org/10.5194/acp-15-8539-2015, 2015.
Borsdorff, T., aan de Brugh, J., Hu, H., Hasekamp, O., Sussmann, R., Rettinger, M., Hase, F., Gross, J., Schneider, M., Garcia, O., Stremme, W., Grutter, M., Feist, D. G., Arnold, S. G., De Mazière, M., Kumar Sha, M., Pollard, D. F., Kiel, M., Roehl, C., Wennberg, P. O., Toon, G. C., and Landgraf, J.: Mapping carbon monoxide pollution from space down to city scales with daily global coverage, Atmos. Meas. Tech., 11, 5507–5518, https://doi.org/10.5194/amt-11-5507-2018, 2018.
Borsdorff, T., aan de Brugh, J., Schneider, A., Lorente, A., Birk, M., Wagner, G., Kivi, R., Hase, F., Feist, D. G., Sussmann, R., Rettinger, M., Wunch, D., Warneke, T., and Landgraf, J.: Improving the TROPOMI CO data product: update of the spectroscopic database and destriping of single orbits, Atmos. Meas. Tech., 12, 5443–5455, https://doi.org/10.5194/amt-12-5443-2019, 2019.
Bowman, D. M. J. S., Balch, J. K., Artaxo, P., Bond, W. J., Carlson, J. M.,
Cochrane, M. A., D'Antonio, C. M., DeFries, R. S., Doyle, J. C., Harrison,
S. P., Johnston, F. H., Keeley, J. E., Krawchuk, M. A., Kull, C. A.,
Marston, J. B., Moritz, M. A., Prentice, I. C., Roos, C. I., Scott, A. C.,
Swetnam, T. W., van der Werf, G. R., and Pyne, S. J.: Fire in the earth
system, Science, 324, 481–484, https://doi.org/10.1126/science.1163886,
2009.
Cheng, Z., Wang, S., Fu, X., Watson, J. G., Jiang, J., Fu, Q., Chen, C., Xu, B., Yu, J., Chow, J. C., and Hao, J.: Impact of biomass burning on haze pollution in the Yangtze River delta, China: a case study in summer 2011, Atmos. Chem. Phys., 14, 4573–4585, https://doi.org/10.5194/acp-14-4573-2014, 2014.
Chevallier, F., Fortems, A., Bousquet, P., Pison, I., Szopa, S., Devaux, M., and Hauglustaine, D. A.: African CO emissions between years 2000 and 2006 as estimated from MOPITT observations, Biogeosciences, 6, 103–111, https://doi.org/10.5194/bg-6-103-2009, 2009.
Chin, M., Ginoux, P., Kinne, S., Torres, O., Holben, B., Duncan, B. N.,
Martin, R. V, Logan, J. A., Higurashi, A., and Nakajima, T.: Tropospheric
Aerosol Optical Thickness from the GOCART Model and Comparisons with
Satellite and Sun Photometer Measurements, J. Atmos. Sci., 59, 461–483,
https://doi.org/10.1175/1520-0469(2002)059<0461:TAOTFT>2.0.CO;2,
2002.
Choi, M. W., Lee, J. H., Woo, J. W., Kim, C. H., and Lee, S. H.: Comparison
of PM2.5 chemical components over East Asia simulated by the WRF-Chem and
WRF/CMAQ models: On the models' prediction inconsistency, Atmosphere, 10, 618, https://doi.org/10.3390/atmos10100618, 2019.
Formenti, P., Elbert, W., Maenhaut, W., Haywood, J., Osborne, S., and Andreae, M. O.: Inorganic and carbonaceous aerosols during the Southern African Regional Science Initiative (SAFARI 2000) experiment: Chemical characteristics, physical properties, and emission data for smoke from African biomass burning, J. Geophys. Res., 108, 8488, https://doi.org/10.1029/2002JD002408, 2003.
Forster, P., Ramaswamy, V., Artaxo, P., Berntsen, T., Betts, R., Fahey, D.
W., Haywood, J. M., Lean, J., Lowe, D. C., Myhre, G., Nganga, J., Prinn, R.,
Raga, G., Schulz, M., and Van Dorland, R.: Changes in Atmospheric
Constituents and in Radiative Forcing (IPCC 2007), Change, 30, 129–234,
https://doi.org/10.1103/PhysRevB.77.220407, 2007.
Freeborn, P. H., Wooster, M. J., Hao, W. M., Ryan, C. A., Nordgren, B. L.,
Baker, S. P., and Ichoku, C.: Relationships between energy release, fuel
mass loss, and trace gas and aerosol emissions during laboratory biomass
fires, J. Geophys. Res., 113, 1–17, https://doi.org/10.1029/2007JD008679, 2008.
Freeborn, P. H., Wooster, M. J., Roberts, G., Malamud, B. D., and Xu, W.:
Development of a virtual active fire product for Africa through a synthesis
of geostationary and polar orbiting satellite data, Remote Sens. Environ.,
113, 1700–1711, https://doi.org/10.1016/j.rse.2009.03.013, 2009.
Garcia-Menendez, F., Hu, Y., and Odman, M. T.: Science of the Total
Environment Simulating smoke transport from wildland fires with a
regional-scale air quality model: Sensitivity to spatiotemporal allocation
of fire emissions, Sci. Total Environ., 493, 544–553,
https://doi.org/10.1016/j.scitotenv.2014.05.108, 2014.
Giglio, L., Schroeder, W., and Justice, C. O.: The collection 6 MODIS active
fire detection algorithm and fire products, Remote Sens. Environ., 178,
31–41, https://doi.org/10.1016/j.rse.2016.02.054, 2016.
Hall, J. V., Zhang, R., Schroeder, W., Huang, C., and Giglio, L.: Validation
of GOES-16 ABI and MSG SEVIRI active fire products, Int. J. Appl. Earth Obs.
Geoinf., 83, 101928, https://doi.org/10.1016/j.jag.2019.101928, 2019.
Hawbaker, T. J., Vanderhoof, M. K., Beal, Y. J., Takacs, J. D., Schmidt, G.
L., Falgout, J. T., Williams, B., Fairaux, N. M., Caldwell, M. K., Picotte,
J. J., Howard, S. M., Stitt, S., and Dwyer, J. L.: Mapping burned areas using
dense time-series of Landsat data, Remote Sens. Environ., 198,
504–522, https://doi.org/10.1016/j.rse.2017.06.027, 2017.
Holben, B., Tanre, D., Smirnov, A., Eck, T. F., Slutsker, I., Abuhassan, N.,
Newcomb, W. W., Schafer, J. S., Chatenet, B., Lavenu, F., Kaufman, Y.,
Castle, J. V., Setzer, A., Markham, B., Clark, D., Frouin, R., Halthore, R.,
Karneli, A., and O'Neill, N. T.: An Emerging Ground- based Aerosol
Climatology: Aerosol Optical Depth from AERONET, J. Geophys. Res., 106,
12067–12097, 2001.
Hu, J., Chen, J., Ying, Q., and Zhang, H.: One-year simulation of ozone and particulate matter in China using WRF/CMAQ modeling system, Atmos. Chem. Phys., 16, 10333–10350, https://doi.org/10.5194/acp-16-10333-2016, 2016.
Ichoku, C. and Ellison, L.: Global top-down smoke-aerosol emissions estimation using satellite fire radiative power measurements, Atmos. Chem. Phys., 14, 6643–6667, https://doi.org/10.5194/acp-14-6643-2014, 2014.
Kaiser, J. W., Heil, A., Andreae, M. O., Benedetti, A., Chubarova, N., Jones, L., Morcrette, J.-J., Razinger, M., Schultz, M. G., Suttie, M., and van der Werf, G. R.: Biomass burning emissions estimated with a global fire assimilation system based on observed fire radiative power, Biogeosciences, 9, 527–554, https://doi.org/10.5194/bg-9-527-2012, 2012.
Keywood, M., Kanakidou, M., Stohl, A., Dentener, F., Grassi, G., Meyer, C.
P., Torseth, K., Edwards, D., Thompson, A. M., Lohmann, U., and Burrows, J.:
Fire in the air: Biomass burning impacts in a changing climate, Crit. Rev.
Environ. Sci. Technol., 43, 40–83, https://doi.org/10.1080/10643389.2011.604248,
2013.
Kopacz, M., Jacob, D. J., Fisher, J. A., Logan, J. A., Zhang, L., Megretskaia, I. A., Yantosca, R. M., Singh, K., Henze, D. K., Burrows, J. P., Buchwitz, M., Khlystova, I., McMillan, W. W., Gille, J. C., Edwards, D. P., Eldering, A., Thouret, V., and Nedelec, P.: Global estimates of CO sources with high resolution by adjoint inversion of multiple satellite datasets (MOPITT, AIRS, SCIAMACHY, TES), Atmos. Chem. Phys., 10, 855–876, https://doi.org/10.5194/acp-10-855-2010, 2010.
Koplitz, S. N., Nolte, C. G., Pouliot, G., Vukovich, J. M., and Beidler, J.:
Influence of uncertainties in burned area estimates on modeled wildland fire
PM2.5 and ozone pollution in the contiguous U.S., Atmos. Environ., 191,
328–339, https://doi.org/10.1016/j.atmosenv.2018.08.020, 2018.
Kuik, F., Lauer, A., Beukes, J. P., Van Zyl, P. G., Josipovic, M., Vakkari, V., Laakso, L., and Feig, G. T.: The anthropogenic contribution to atmospheric black carbon concentrations in southern Africa: a WRF-Chem modeling study, Atmos. Chem. Phys., 15, 8809–8830, https://doi.org/10.5194/acp-15-8809-2015, 2015.
Kukkonen, J., Olsson, T., Schultz, D. M., Baklanov, A., Klein, T., Miranda, A. I., Monteiro, A., Hirtl, M., Tarvainen, V., Boy, M., Peuch, V.-H., Poupkou, A., Kioutsioukis, I., Finardi, S., Sofiev, M., Sokhi, R., Lehtinen, K. E. J., Karatzas, K., San José, R., Astitha, M., Kallos, G., Schaap, M., Reimer, E., Jakobs, H., and Eben, K.: A review of operational, regional-scale, chemical weather forecasting models in Europe, Atmos. Chem. Phys., 12, 1–87, https://doi.org/10.5194/acp-12-1-2012, 2012.
Landgraf, J., aan de Brugh, J., Scheepmaker, R., Borsdorff, T., Hu, H., Houweling, S., Butz, A., Aben, I., and Hasekamp, O.: Carbon monoxide total column retrievals from TROPOMI shortwave infrared measurements, Atmos. Meas. Tech., 9, 4955–4975, https://doi.org/10.5194/amt-9-4955-2016, 2016.
Langmann, B., Duncan, B., Textor, C., Trentmann, J., and van der Werf, G. R.:
Vegetation fire emissions and their impact on air pollution and climate,
Atmos. Environ., 43, 107–116, https://doi.org/10.1016/j.atmosenv.2008.09.047, 2009.
Lavorel, S., Flannigan, M. D., Lambin, E. F., and Scholes, M. C.:
Vulnerability of land systems to fire: Interactions among humans, climate,
the atmosphere, and ecosystems, Mitig. Adapt. Strateg. Glob. Chang., 12,
33–53, https://doi.org/10.1007/s11027-006-9046-5, 2007.
van Leeuwen, T. T., van der Werf, G. R., Hoffmann, A. A., Detmers, R. G., Rücker, G., French, N. H. F., Archibald, S., Carvalho Jr., J. A., Cook, G. D., de Groot, W. J., Hély, C., Kasischke, E. S., Kloster, S., McCarty, J. L., Pettinari, M. L., Savadogo, P., Alvarado, E. C., Boschetti, L., Manuri, S., Meyer, C. P., Siegert, F., Trollope, L. A., and Trollope, W. S. W.: Biomass burning fuel consumption rates: a field measurement database, Biogeosciences, 11, 7305–7329, https://doi.org/10.5194/bg-11-7305-2014, 2014.
Lyapustin, A., Wang, Y., Korkin, S., and Huang, D.: MODIS Collection 6 MAIAC algorithm, Atmos. Meas. Tech., 11, 5741–5765, https://doi.org/10.5194/amt-11-5741-2018, 2018.
Marengo, J. A., Tomasella, J., Alves, L. M., Soares, W. R., and Rodriguez, D.
A.: The drought of 2010 in the context of historical droughts in the Amazon
region, Geophys. Res. Lett., 38, 1–5, https://doi.org/10.1029/2011GL047436, 2011.
Mota, B. and Wooster, M. J.: A new top-down approach for directly estimating
biomass burning emissions and fuel consumption rates and totals from
geostationary satellite fire radiative power (FRP), Remote Sens.
Environ., 206, 45–62, https://doi.org/10.1016/j.rse.2017.12.016, 2018.
Nguyen, H. M. and Wooster, M. J.: Advances in the estimation of high
Spatio-temporal resolution pan-African top-down biomass burning emissions
made using geostationary fire radiative power (FRP) and MAIAC aerosol
optical depth (AOD) data, Remote Sens. Environ., 248, 111971,
https://doi.org/10.1016/j.rse.2020.111971, 2020.
Pechony, O., Shindell, D. T., and Faluvegi, G.: Direct top-down estimates of
biomass burning CO emissions using TES and MOPITT versus bottom-up GFED
inventory, J. Geophys. Res.-Atmos., 118, 8054–8066,
https://doi.org/10.1002/jgrd.50624, 2013.
Quennehen, B., Schwarzenboeck, A., Matsuki, A., Burkhart, J. F., Stohl, A., Ancellet, G., and Law, K. S.: Anthropogenic and forest fire pollution aerosol transported to the Arctic: observations from the POLARCAT-France spring campaign, Atmos. Chem. Phys., 12, 6437–6454, https://doi.org/10.5194/acp-12-6437-2012, 2012.
Randerson, J. T., Chen, Y., van der Werf, G. R., Rogers, B. M., and Morton,
D. C.: Global burned area and biomass burning emissions from small fires, J.
Geophys. Res.-Biogeo., 117, https://doi.org/10.1029/2012JG002128, 2012.
Reddington, C. L., Spracklen, D. V., Artaxo, P., Ridley, D. A., Rizzo, L. V., and Arana, A.: Analysis of particulate emissions from tropical biomass burning using a global aerosol model and long-term surface observations, Atmos. Chem. Phys., 16, 11083–11106, https://doi.org/10.5194/acp-16-11083-2016, 2016.
Reid, J. S., Eck, T. F., Christopher, S. A., Koppmann, R., Dubovik, O., Eleuterio, D. P., Holben, B. N., Reid, E. A., and Zhang, J.: A review of biomass burning emissions part III: intensive optical properties of biomass burning particles, Atmos. Chem. Phys., 5, 827–849, https://doi.org/10.5194/acp-5-827-2005, 2005.
Reid, J. S., Hyer, E. J., Prins, E., Westphal, D. L., Zhang, J., Wang, J.,
Christopher, S. A., Curtis, C. A., Schmidt, C. C., Eleuterio, D. P.,
Richardson, K. A., and Hoffman, J.: Global monitoring and forecasting of
biomass-burning smoke: Description of and lessons from the fire Locating and
Modeling of Burning Emissions (FLAMBE) program, IEEE J. Sel. Top. Appl.
Earth Obs. Remote Sens., 2, 144–162, https://doi.org/10.1109/JSTARS.2009.2027443,
2009.
Roberts, G., Wooster, M. J., Perry, G. L. W., Drake, N., Rebelo, L. M., and
Dipotso, F.: Retrieval of biomass combustion rates and totals from fire
radiative power observations: Application to southern Africa using
geostationary SEVIRI imagery, J. Geophys. Res.-Atmos., 110, 1–19,
https://doi.org/10.1029/2005JD006018, 2005.
Roberts, G., Wooster, M. J., Xu, W., Freeborn, P. H., Morcrette, J.-J., Jones, L., Benedetti, A., Jiangping, H., Fisher, D., and Kaiser, J. W.: LSA SAF Meteosat FRP products – Part 2: Evaluation and demonstration for use in the Copernicus Atmosphere Monitoring Service (CAMS), Atmos. Chem. Phys., 15, 13241–13267, https://doi.org/10.5194/acp-15-13241-2015, 2015.
Roberts, G., Wooster, M. J., Lauret, N., Gastellu-Etchegorry, J. P., Lynham,
T., and McRae, D.: Investigating the impact of overlying vegetation canopy
structures on fire radiative power (FRP) retrieval through simulation and
measurement, Remote Sens. Environ., 217, 158–171,
https://doi.org/10.1016/j.rse.2018.08.015, 2018.
Roteta, E., Bastarrika, A., Padilla, M., Storm, T., and Chuvieco, E.:
Development of a Sentinel-2 burned area algorithm: Generation of a small
fire database for sub-Saharan Africa, Remote Sens. Environ., 222,
1–17, https://doi.org/10.1016/j.rse.2018.12.011, 2019.
Seiler, W. and Crutzen, P. J.: Estimates of gross and net fluxes of carbon
between the biosphere and the atmosphere from biomass burning, Clim. Change,
2, 207–247, https://doi.org/10.1007/BF00137988, 1980.
Tomasella, J., Pinho, P. F., Borma, L. S., Marengo, J. A., Nobre, C. A.,
Bittencourt, O. R. F. O., Prado, M. C. R., Rodriguez, D. A., and Cuartas, L.
A.: The droughts of 1997 and 2005 in Amazonia: Floodplain hydrology and its
potential ecological and human impacts, Clim. Change, 116, 723–746,
https://doi.org/10.1007/s10584-012-0508-3, 2013.
Tsela, P. L., Van Helden, P., Frost, P., Wessels, K., and Archibald, S.:
Validation of the modis burned-area products across different biomes in
South Africa, Int. Geosci. Remote Sens. Symp., Honolulu, HI, USA, 3652–3655,
https://doi.org/10.1109/IGARSS.2010.5650253, 2010.
Vermote, E., Ellicott, E., Dubovik, O., Lapyonok, T., Chin, M., Giglio, L., and Roberts, G.: An approach to estimate global biomass burning emissions of
organic and black carbon from MODIS fire radiative power, J. Geophys. Res.-Atmos., 114, 1–22, https://doi.org/10.1029/2008JD011188, 2009.
Vongruang, P., Wongwises, P., and Pimonsree, S.: Assessment of fire emission
inventories for simulating particulate matter in Upper Southeast Asia using
WRF-CMAQ, Atmos. Pollut. Res., 8, 921–929,
https://doi.org/10.1016/j.apr.2017.03.004, 2017.
van der Werf, G. R., Randerson, J. T., Giglio, L., Collatz, G. J., Kasibhatla, P. S., and Arellano Jr., A. F.: Interannual variability in global biomass burning emissions from 1997 to 2004, Atmos. Chem. Phys., 6, 3423–3441, https://doi.org/10.5194/acp-6-3423-2006, 2006.
van der Werf, G. R., Randerson, J. T., Giglio, L., Collatz, G. J., Mu, M., Kasibhatla, P. S., Morton, D. C., DeFries, R. S., Jin, Y., and van Leeuwen, T. T.: Global fire emissions and the contribution of deforestation, savanna, forest, agricultural, and peat fires (1997–2009), Atmos. Chem. Phys., 10, 11707–11735, https://doi.org/10.5194/acp-10-11707-2010, 2010.
van der Werf, G. R., Randerson, J. T., Giglio, L., van Leeuwen, T. T., Chen, Y., Rogers, B. M., Mu, M., van Marle, M. J. E., Morton, D. C., Collatz, G. J., Yokelson, R. J., and Kasibhatla, P. S.: Global fire emissions estimates during 1997–2016, Earth Syst. Sci. Data, 9, 697–720, https://doi.org/10.5194/essd-9-697-2017, 2017.
Wiedinmyer, C., Akagi, S. K., Yokelson, R. J., Emmons, L. K., Al-Saadi, J. A., Orlando, J. J., and Soja, A. J.: The Fire INventory from NCAR (FINN): a high resolution global model to estimate the emissions from open burning, Geosci. Model Dev., 4, 625–641, https://doi.org/10.5194/gmd-4-625-2011, 2011.
Wooster, M. J., Freeborn, P. H., Archibald, S., Oppenheimer, C., Roberts, G. J., Smith, T. E. L., Govender, N., Burton, M., and Palumbo, I.: Field determination of biomass burning emission ratios and factors via open-path FTIR spectroscopy and fire radiative power assessment: headfire, backfire and residual smouldering combustion in African savannahs, Atmos. Chem. Phys., 11, 11591–11615, https://doi.org/10.5194/acp-11-11591-2011, 2011.
Wooster, M. J., Roberts, G., Freeborn, P. H., Xu, W., Govaerts, Y., Beeby, R., He, J., Lattanzio, A., Fisher, D., and Mullen, R.: LSA SAF Meteosat FRP products – Part 1: Algorithms, product contents, and analysis, Atmos. Chem. Phys., 15, 13217–13239, https://doi.org/10.5194/acp-15-13217-2015, 2015.
Xu, W., Wooster, M. J., Roberts, G., and Freeborn, P. H.: New GOES imager
algorithms for cloud and active fire detection and fire radiative power
assessment across North, South and Central America, Remote Sens. Environ.,
114, 1876–1895, https://doi.org/10.1016/j.rse.2010.03.012, 2010.
Xu, W., Wooster, M. J., Kaneko, T., He, J., Zhang, T., and Fisher, D.: Major
advances in geostationary fire radiative power (FRP) retrieval over Asia and
Australia stemming from use of Himarawi-8 AHI, Remote Sens. Environ., 193,
138–149, https://doi.org/10.1016/j.rse.2017.02.024, 2017.
Yang, Z., Wang, J., Ichoku, C., Hyer, E. J., and Zeng, J.: Mesoscale modeling
and satellite observation of transport and mixing of smoke and dust
particles over northern sub-Saharan African region, J. Geophys. Res.-Atmos.,
118, 12139–12157, https://doi.org/10.1002/2013JD020644, 2013.
Yu, S., Eder, B., Dennis, R., Chu, S.-H., and Schwartz, S. E.: New unbiased
symmetric metrics for evaluation of air quality models, Atmos. Sci. Lett.,
7, 26–34, https://doi.org/10.1002/asl.125, 2006.
Zhang, F., Wang, J., Ichoku, C., Hyer, E. J., Yang, Z., Ge, C., Su, S.,
Zhang, X., Kondragunta, S., Kaiser, J. W., Wiedinmyer, C., and Da Silva, A.:
Sensitivity of mesoscale modeling of smoke direct radiative effect to the
emission inventory: A case study in northern sub-Saharan African region,
Environ. Res. Lett., 9, 7, https://doi.org/10.1088/1748-9326/9/7/075002, 2014.
Zhang, X., Kondragunta, S., Schmidt, C., and Kogan, F.: Near real time
monitoring of biomass burning particulate emissions (PM2.5) across
contiguous United States using multiple satellite instruments, Atmos.
Environ., 42, 6959–6972, https://doi.org/10.1016/j.atmosenv.2008.04.060, 2008.
Zheng, B., Chevallier, F., Ciais, P., Yin, Y., and Wang, Y.: On the Role of
the Flaming to Smoldering Transition in the Seasonal Cycle of African Fire
Emissions, Geophys. Res. Lett., 45, 11998–12007,
https://doi.org/10.1029/2018GL079092, 2018.
Short summary
This work presents novel advances in the estimation of open biomass burning emissions via the first fully "top-down" approach to exploit satellite-derived observations of fire radiative power and carbon monoxide over Africa. We produce a 16-year record of fire-generated CO emissions and dry matter consumed per unit area for Africa and evaluate these emissions estimates through their use in an atmospheric model, whose simulation output is then compared to independent satellite observations of CO.
This work presents novel advances in the estimation of open biomass burning emissions via the...
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