Articles | Volume 22, issue 13
https://doi.org/10.5194/acp-22-8805-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-22-8805-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
08 Jul 2022
Research article |
| 08 Jul 2022
| 08 Jul 2022
Viscosity and physical state of sucrose mixed with ammonium sulfate droplets
Rani Jeong
Department of Environment and Energy, Jeonbuk National University, Jeonju, Republic of Korea
Joseph Lilek
Department of Atmospheric and Oceanic Sciences, McGill University, Montréal, Quebec, Canada
Andreas Zuend
Department of Atmospheric and Oceanic Sciences, McGill University, Montréal, Quebec, Canada
Rongshuang Xu
Earth System Science Programme, Faculty of Science, The Chinese University of Hong Kong, Hong Kong, Hong Kong SAR, China
Man Nin Chan
Earth System Science Programme, Faculty of Science, The Chinese University of Hong Kong, Hong Kong, Hong Kong SAR, China
The Institute of Environment, Energy and Sustainability, The Chinese University of Hong Kong, Hong Kong, Hong Kong SAR, China
Dohyun Kim
Department of Environment and Energy, Jeonbuk National University, Jeonju, Republic of Korea
Hi Gyu Moon
Center for Ecological Risk Assessment, Korea Institute of Toxicology (KIT), Jinju 52834, Republic of Korea
Mijung Song
CORRESPONDING AUTHOR
Department of Environment and Energy, Jeonbuk National University, Jeonju, Republic of Korea
Department of Earth and Environmental Sciences, Jeonbuk National University, Jeonju, Republic of Korea
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Cited
18 citations as recorded by crossref.
- Influence of Relative Humidity and Composition on PM2.5 Phases in Northeast Asia C. Seong et al.
- Low-temperature dual balance electrodynamic trap (LT-DBET) for single microparticle aerosol studies V. Ojo et al.
- Morphology and phase state of PM2.5 in urban and coastal-rural areas during summer S. Gaikwad et al.
- Humidity-dependent viscosity and hygroscopicity after aging with SO2 of biomass burning single nanoparticle B. Yang et al.
- Hydrogel network formation triggers atypical hygroscopic behavior in atmospheric aerosols F. Dong et al.
- Comparison of Phase States of PM2.5 over Megacities, Seoul and Beijing, and Their Implications on Particle Size Distribution M. Song et al.
- Direct measurement of the viscosity of ternary aerosol mixtures S. Mahant et al.
- Correlating the Viscosity and Rate of Water Diffusion in Semisolid Gel-Forming Aerosol Particles C. Sheldon et al.
- Temperature–RH dependent viscosity of organic aerosols from 273 to 303 K: implications for global N2O5 uptake A. Ullah et al.
- Exploring the hygroscopicity, water diffusivity, and viscosity of organic–inorganic aerosols – a case study on internally-mixed citric acid and ammonium sulfate particles C. Sheldon et al.
- Equilibration times in viscous and viscoelastic aerosol particles T. Preston & A. Zuend
- Phase Behavior of Polluted and Clean Urban Winter PM2.5 from Optical Observations and Thermodynamic Equilibrium Modeling T. Do et al.
- Viscosity, Glass Formation, and Mixing Times within Secondary Organic Aerosol from Biomass Burning Phenolics K. Kiland et al.
- Viscosity of aqueous ammonium nitrate–organic particles: equilibrium partitioning may be a reasonable assumption for most tropospheric conditions L. Klein et al.
- Hygroscopicity of isoprene-derived secondary organic aerosol mixture proxies: importance of diffusion and salting-in effects N. Ferdousi-Rokib et al.
- Effects of volatility, viscosity, and non-ideality on particle–particle mixing timescales of secondary organic aerosols M. Schervish et al.
- Role of WSOCs and pH on Ammonium Nitrate Aerosol Efflorescence: Insights into Secondary Aerosol Formation J. Sun et al.
- Direct Observation of Liquid–Liquid Phase Separation and Core–Shell Morphology of PM2.5 Collected from Three Northeast Asian Cities and Implications for N2O5 Hydrolysis M. Song et al.
18 citations as recorded by crossref.
- Influence of Relative Humidity and Composition on PM2.5 Phases in Northeast Asia C. Seong et al.
- Low-temperature dual balance electrodynamic trap (LT-DBET) for single microparticle aerosol studies V. Ojo et al.
- Morphology and phase state of PM2.5 in urban and coastal-rural areas during summer S. Gaikwad et al.
- Humidity-dependent viscosity and hygroscopicity after aging with SO2 of biomass burning single nanoparticle B. Yang et al.
- Hydrogel network formation triggers atypical hygroscopic behavior in atmospheric aerosols F. Dong et al.
- Comparison of Phase States of PM2.5 over Megacities, Seoul and Beijing, and Their Implications on Particle Size Distribution M. Song et al.
- Direct measurement of the viscosity of ternary aerosol mixtures S. Mahant et al.
- Correlating the Viscosity and Rate of Water Diffusion in Semisolid Gel-Forming Aerosol Particles C. Sheldon et al.
- Temperature–RH dependent viscosity of organic aerosols from 273 to 303 K: implications for global N2O5 uptake A. Ullah et al.
- Exploring the hygroscopicity, water diffusivity, and viscosity of organic–inorganic aerosols – a case study on internally-mixed citric acid and ammonium sulfate particles C. Sheldon et al.
- Equilibration times in viscous and viscoelastic aerosol particles T. Preston & A. Zuend
- Phase Behavior of Polluted and Clean Urban Winter PM2.5 from Optical Observations and Thermodynamic Equilibrium Modeling T. Do et al.
- Viscosity, Glass Formation, and Mixing Times within Secondary Organic Aerosol from Biomass Burning Phenolics K. Kiland et al.
- Viscosity of aqueous ammonium nitrate–organic particles: equilibrium partitioning may be a reasonable assumption for most tropospheric conditions L. Klein et al.
- Hygroscopicity of isoprene-derived secondary organic aerosol mixture proxies: importance of diffusion and salting-in effects N. Ferdousi-Rokib et al.
- Effects of volatility, viscosity, and non-ideality on particle–particle mixing timescales of secondary organic aerosols M. Schervish et al.
- Role of WSOCs and pH on Ammonium Nitrate Aerosol Efflorescence: Insights into Secondary Aerosol Formation J. Sun et al.
- Direct Observation of Liquid–Liquid Phase Separation and Core–Shell Morphology of PM2.5 Collected from Three Northeast Asian Cities and Implications for N2O5 Hydrolysis M. Song et al.
Saved (final revised paper)
Latest update: 28 Apr 2026
Short summary
In this study, the viscosities of particles of sucrose–H2O, AS–H2O, and sucrose–AS–H2O for OIRs of 4:1, 1:1, and 1:4 for decreasing RH, were quantified by poke-and-flow and bead-mobility techniques at 293 ± 1 K. Based on the viscosity results, the particles of binary and ternary systems ranged from liquid to semisolid, and even the solid state depending on the RH. Moreover, we compared the measured viscosities of ternary systems to the predicted viscosities with excellent agreement.
In this study, the viscosities of particles of sucrose–H2O, AS–H2O, and sucrose–AS–H2O for OIRs...
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