Articles | Volume 22, issue 2
https://doi.org/10.5194/acp-22-805-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-22-805-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
18 Jan 2022
Research article |
| 18 Jan 2022
| 18 Jan 2022
Field observational constraints on the controllers in glyoxal (CHOCHO) reactive uptake to aerosol
Dongwook Kim
Department of Physics and Photon Science, Gwangju Institute of Science
and Technology, Gwangju, South Korea
School of Environmental Sciences and Environmental Engineering,
Gwangju Institute of Science and Technology, Gwangju, South Korea
Department of Chemistry and CIRES, University of Colorado, Boulder, CO,
USA
Changmin Cho
School of Environmental Sciences and Environmental Engineering,
Gwangju Institute of Science and Technology, Gwangju, South Korea
now at: Troposphere (IEK-8), Institute of Energy and Climate Research,
Forschungszentrum Jülich, Jülich, Germany
Seokhan Jeong
School of Environmental Sciences and Environmental Engineering,
Gwangju Institute of Science and Technology, Gwangju, South Korea
now at: Environmental Assessment group, Korea Environment Institute,
Sejong, Korea
Soojin Lee
School of Environmental Sciences and Environmental Engineering,
Gwangju Institute of Science and Technology, Gwangju, South Korea
Benjamin A. Nault
Department of Chemistry and CIRES, University of Colorado, Boulder, CO,
USA
now at: Center for Aerosol and Cloud Chemistry, Aerodyne Research
Inc., Billerica, MA, USA
Pedro Campuzano-Jost
Department of Chemistry and CIRES, University of Colorado, Boulder, CO,
USA
Douglas A. Day
Department of Chemistry and CIRES, University of Colorado, Boulder, CO,
USA
Jason C. Schroder
Department of Chemistry and CIRES, University of Colorado, Boulder, CO,
USA
now at: Colorado Department of Public Health and Environment, Denver,
CO, USA
Jose L. Jimenez
Department of Chemistry and CIRES, University of Colorado, Boulder, CO,
USA
Rainer Volkamer
Department of Chemistry and CIRES, University of Colorado, Boulder, CO,
USA
Donald R. Blake
Department of Chemistry, University of California, Irvine, CA, USA
Armin Wisthaler
Institute for Ion Physics and Applied Physics, University of
Innsbruck, Innsbruck, Austria
Department of Chemistry, University of Oslo, Oslo, Norway
Alan Fried
Institute of Arctic and Alpine Research, University of Colorado,
Boulder, CO, USA
Joshua P. DiGangi
NASA Langley Research Center, Hampton, VA, USA
Glenn S. Diskin
NASA Langley Research Center, Hampton, VA, USA
Sally E. Pusede
Department of Environmental Sciences, University of Virginia,
Charlottesville, VA, USA
Samuel R. Hall
Atmospheric Chemistry Observations and Modeling, National Center for
Atmospheric Research, Boulder, CO, USA
Kirk Ullmann
Atmospheric Chemistry Observations and Modeling, National Center for
Atmospheric Research, Boulder, CO, USA
L. Gregory Huey
School of Earth and Atmospheric Sciences, Georgia Institute of
Technology, Atlanta, GA, USA
David J. Tanner
School of Earth and Atmospheric Sciences, Georgia Institute of
Technology, Atlanta, GA, USA
Jack Dibb
Earth Systems Research Center, Institute for the Study of Earth,
Oceans, and Space, University of New Hampshire, Durham, NH, USA
Christoph J. Knote
Model-Based Environmental Exposure Science, Faculty of Medicine,
University of Augsburg, Augsburg, Germany
Kyung-Eun Min
CORRESPONDING AUTHOR
School of Environmental Sciences and Environmental Engineering,
Gwangju Institute of Science and Technology, Gwangju, South Korea
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Cited
10 citations as recorded by crossref.
- Sources of organic aerosols in eastern China: a modeling study with high-resolution intermediate-volatility and semivolatile organic compound emissions J. An et al. 10.5194/acp-23-323-2023
- Airborne glyoxal measurements in the marine and continental atmosphere: comparison with TROPOMI observations and EMAC simulations F. Kluge et al. 10.5194/acp-23-1369-2023
- Modeling Secondary Organic Aerosols in China: State of the Art and Perspectives J. Li et al. 10.1007/s40726-022-00246-3
- Gas-liquid interfacial reaction mechanisms of typical small α-dicarbonyls in the neutral and acidic droplets: Implications for secondary organic aerosol formation Q. Shi et al. 10.1016/j.atmosenv.2024.120859
- Using observed urban NOx sinks to constrain VOC reactivity and the ozone and radical budget in the Seoul Metropolitan Area B. Nault et al. 10.5194/acp-24-9573-2024
- Modeling the molecular composition of secondary organic aerosol under highly polluted conditions: A case study in the Yangtze River Delta Region in China Q. Huang et al. 10.1016/j.scitotenv.2024.173327
- Reversible and irreversible gas–particle partitioning of dicarbonyl compounds observed in the real atmosphere J. Hu et al. 10.5194/acp-22-6971-2022
- Satellite Evidence for Glyoxal Depletion in Elevated Fire Plumes C. Lerot et al. 10.1029/2022GL102195
- Online headspace monitoring of volatile organic compounds using proton transfer reaction-mass spectrometry: Application to the multiphase atmospheric fate of 2,4-hexadienedial N. Brun et al. 10.1016/j.talanta.2024.126176
- How non-equilibrium aerosol chemistry impacts particle acidity: the GMXe AERosol CHEMistry (GMXe–AERCHEM, v1.0) sub-submodel of MESSy S. Rosanka et al. 10.5194/gmd-17-2597-2024
10 citations as recorded by crossref.
- Sources of organic aerosols in eastern China: a modeling study with high-resolution intermediate-volatility and semivolatile organic compound emissions J. An et al. 10.5194/acp-23-323-2023
- Airborne glyoxal measurements in the marine and continental atmosphere: comparison with TROPOMI observations and EMAC simulations F. Kluge et al. 10.5194/acp-23-1369-2023
- Modeling Secondary Organic Aerosols in China: State of the Art and Perspectives J. Li et al. 10.1007/s40726-022-00246-3
- Gas-liquid interfacial reaction mechanisms of typical small α-dicarbonyls in the neutral and acidic droplets: Implications for secondary organic aerosol formation Q. Shi et al. 10.1016/j.atmosenv.2024.120859
- Using observed urban NOx sinks to constrain VOC reactivity and the ozone and radical budget in the Seoul Metropolitan Area B. Nault et al. 10.5194/acp-24-9573-2024
- Modeling the molecular composition of secondary organic aerosol under highly polluted conditions: A case study in the Yangtze River Delta Region in China Q. Huang et al. 10.1016/j.scitotenv.2024.173327
- Reversible and irreversible gas–particle partitioning of dicarbonyl compounds observed in the real atmosphere J. Hu et al. 10.5194/acp-22-6971-2022
- Satellite Evidence for Glyoxal Depletion in Elevated Fire Plumes C. Lerot et al. 10.1029/2022GL102195
- Online headspace monitoring of volatile organic compounds using proton transfer reaction-mass spectrometry: Application to the multiphase atmospheric fate of 2,4-hexadienedial N. Brun et al. 10.1016/j.talanta.2024.126176
- How non-equilibrium aerosol chemistry impacts particle acidity: the GMXe AERosol CHEMistry (GMXe–AERCHEM, v1.0) sub-submodel of MESSy S. Rosanka et al. 10.5194/gmd-17-2597-2024
Latest update: 13 Dec 2024
Short summary
CHOCHO was simulated using a 0-D box model constrained by measurements during the KORUS-AQ mission. CHOCHO concentration was high in large cities, aromatics being the most important precursors. Loss path to aerosol was the highest sink, contributing to ~ 20 % of secondary organic aerosol formation. Our work highlights that simple CHOCHO surface uptake approach is valid only for low aerosol conditions and more work is required to understand CHOCHO solubility in high-aerosol conditions.
CHOCHO was simulated using a 0-D box model constrained by measurements during the KORUS-AQ...
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