Articles | Volume 22, issue 11
https://doi.org/10.5194/acp-22-7489-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-22-7489-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
10 Jun 2022
Research article |
| 10 Jun 2022
| 10 Jun 2022
Distribution and stable carbon isotopic composition of dicarboxylic acids, ketocarboxylic acids and α-dicarbonyls in fresh and aged biomass burning aerosols
Minxia Shen
State Key Laboratory of Loess and Quaternary Geology, Key Laboratory of
Aerosol Chemistry and Physics, Institute of Earth Environment, Chinese
Academy of Sciences, Xi'an 710061, China
University of Chinese Academy of Sciences, Beijing, China
Kin Fai Ho
The Jockey Club School of Public Health and Primary Care, The Chinese
University of Hong Kong, Hong Kong, China
Shenzhen Municipal Key Laboratory for Health Risk Analysis, Shenzhen
Research Institute, The Chinese University of Hong Kong, Shenzhen, China
Wenting Dai
State Key Laboratory of Loess and Quaternary Geology, Key Laboratory of
Aerosol Chemistry and Physics, Institute of Earth Environment, Chinese
Academy of Sciences, Xi'an 710061, China
Suixin Liu
State Key Laboratory of Loess and Quaternary Geology, Key Laboratory of
Aerosol Chemistry and Physics, Institute of Earth Environment, Chinese
Academy of Sciences, Xi'an 710061, China
Ting Zhang
State Key Laboratory of Loess and Quaternary Geology, Key Laboratory of
Aerosol Chemistry and Physics, Institute of Earth Environment, Chinese
Academy of Sciences, Xi'an 710061, China
Qiyuan Wang
State Key Laboratory of Loess and Quaternary Geology, Key Laboratory of
Aerosol Chemistry and Physics, Institute of Earth Environment, Chinese
Academy of Sciences, Xi'an 710061, China
Jingjing Meng
School of Geography and the Environment, Liaocheng University,
Liaocheng 252000, China
Judith C. Chow
State Key Laboratory of Loess and Quaternary Geology, Key Laboratory of
Aerosol Chemistry and Physics, Institute of Earth Environment, Chinese
Academy of Sciences, Xi'an 710061, China
Division of Atmospheric Sciences, Desert of Research Institute, Reno, Nevada, USA
John G. Watson
State Key Laboratory of Loess and Quaternary Geology, Key Laboratory of
Aerosol Chemistry and Physics, Institute of Earth Environment, Chinese
Academy of Sciences, Xi'an 710061, China
Division of Atmospheric Sciences, Desert of Research Institute, Reno, Nevada, USA
Junji Cao
CORRESPONDING AUTHOR
State Key Laboratory of Loess and Quaternary Geology, Key Laboratory of
Aerosol Chemistry and Physics, Institute of Earth Environment, Chinese
Academy of Sciences, Xi'an 710061, China
State Key Laboratory of Loess and Quaternary Geology, Key Laboratory of
Aerosol Chemistry and Physics, Institute of Earth Environment, Chinese
Academy of Sciences, Xi'an 710061, China
CAS Center for Excellence in Quaternary Science and Global Change,
Xi'an 710061, China
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Cited
13 citations as recorded by crossref.
- Seasonal distributions and possible sources of low molecular weight organic acids in PM2.5 from a typical mining city after decade green mining developing in Southeastern Hubei, Central China S. Liu et al. 10.1016/j.atmosenv.2024.120455
- Dual-isotope ratios of carbonaceous aerosols for seasonal observation and their assessment as source indicators A. Mašalaitė et al. 10.1016/j.scitotenv.2024.175094
- Role of aerosol liquid water content on the production of dicarboxylic acids in the dust-laden air masses over the Arabian Sea: Implications for heterogeneous chemistry P. Bikkina et al. 10.1016/j.atmosres.2023.106743
- A year-round observation of δ13C of dicarboxylic acids and related compounds in fine aerosols: Implications from Central European background site P. Vodička et al. 10.1016/j.chemosphere.2023.139393
- Primary and Secondary Emissions of Carboxylic Acids from Solid Fuel Combustion: Insight into the Source Markers and Secondary Formation Mechanism B. Zhang et al. 10.1021/acs.estlett.4c00339
- Comparison of acidity and chemical composition of summertime cloud water and aerosol at an alpine site in Northwest China: Implications for the neutral property of clouds in the free troposphere M. Shen et al. 10.1016/j.scitotenv.2024.171775
- Measurement Report: Investigation on the sources and formation processes of dicarboxylic acids and related species in urban aerosols before and during the COVID-19 lockdown in Jinan, East China J. Meng et al. 10.5194/acp-23-14481-2023
- Influence of vertical transport on chemical evolution of dicarboxylic acids and related secondary organic aerosol from surface emission to the top of Mount Hua, Northwest China M. Shen et al. 10.1016/j.scitotenv.2022.159892
- Effects of photochemical aging on the molecular composition of organic aerosols derived from agricultural biomass burning in whole combustion process L. Li et al. 10.1016/j.scitotenv.2024.174152
- Mixing state and evolutionary mechanism of oxalic acid homologs in Liaocheng, East China: Insights from seasonal and hourly observations J. Ma et al. 10.1016/j.partic.2024.09.011
- Anthropogenic sources and liquid water drive secondary organic aerosol formation over the eastern Himalaya D. Kumar et al. 10.1016/j.scitotenv.2024.175072
- Fates of secondary organic aerosols in the atmosphere identified from compound-specific dual-carbon isotope analysis of oxalic acid B. Xu et al. 10.5194/acp-23-1565-2023
- Effects of atmospheric aging processes on carbonaceous species and water-soluble inorganic ions in biomass burning aerosols X. Guo et al. 10.1016/j.atmosenv.2022.119322
13 citations as recorded by crossref.
- Seasonal distributions and possible sources of low molecular weight organic acids in PM2.5 from a typical mining city after decade green mining developing in Southeastern Hubei, Central China S. Liu et al. 10.1016/j.atmosenv.2024.120455
- Dual-isotope ratios of carbonaceous aerosols for seasonal observation and their assessment as source indicators A. Mašalaitė et al. 10.1016/j.scitotenv.2024.175094
- Role of aerosol liquid water content on the production of dicarboxylic acids in the dust-laden air masses over the Arabian Sea: Implications for heterogeneous chemistry P. Bikkina et al. 10.1016/j.atmosres.2023.106743
- A year-round observation of δ13C of dicarboxylic acids and related compounds in fine aerosols: Implications from Central European background site P. Vodička et al. 10.1016/j.chemosphere.2023.139393
- Primary and Secondary Emissions of Carboxylic Acids from Solid Fuel Combustion: Insight into the Source Markers and Secondary Formation Mechanism B. Zhang et al. 10.1021/acs.estlett.4c00339
- Comparison of acidity and chemical composition of summertime cloud water and aerosol at an alpine site in Northwest China: Implications for the neutral property of clouds in the free troposphere M. Shen et al. 10.1016/j.scitotenv.2024.171775
- Measurement Report: Investigation on the sources and formation processes of dicarboxylic acids and related species in urban aerosols before and during the COVID-19 lockdown in Jinan, East China J. Meng et al. 10.5194/acp-23-14481-2023
- Influence of vertical transport on chemical evolution of dicarboxylic acids and related secondary organic aerosol from surface emission to the top of Mount Hua, Northwest China M. Shen et al. 10.1016/j.scitotenv.2022.159892
- Effects of photochemical aging on the molecular composition of organic aerosols derived from agricultural biomass burning in whole combustion process L. Li et al. 10.1016/j.scitotenv.2024.174152
- Mixing state and evolutionary mechanism of oxalic acid homologs in Liaocheng, East China: Insights from seasonal and hourly observations J. Ma et al. 10.1016/j.partic.2024.09.011
- Anthropogenic sources and liquid water drive secondary organic aerosol formation over the eastern Himalaya D. Kumar et al. 10.1016/j.scitotenv.2024.175072
- Fates of secondary organic aerosols in the atmosphere identified from compound-specific dual-carbon isotope analysis of oxalic acid B. Xu et al. 10.5194/acp-23-1565-2023
- Effects of atmospheric aging processes on carbonaceous species and water-soluble inorganic ions in biomass burning aerosols X. Guo et al. 10.1016/j.atmosenv.2022.119322
Latest update: 23 Nov 2024
Short summary
Looking at characteristics and δ13C compositions of dicarboxylic acids and related compounds in BB aerosols, we used a combined combustion and aging system to generate fresh and aged aerosols from burning straw. The results showed the emission factors (EFaged) of total diacids of aging experiments were around an order of magnitude higher than EFfresh. This meant that dicarboxylic acids are involved with secondary photochemical processes in the atmosphere rather than primary emissions from BB.
Looking at characteristics and δ13C compositions of dicarboxylic acids and related compounds in...
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