Articles | Volume 22, issue 8
https://doi.org/10.5194/acp-22-5377-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-22-5377-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
25 Apr 2022
Research article |
| 25 Apr 2022
| 25 Apr 2022
Micro-spectroscopic and freezing characterization of ice-nucleating particles collected in the marine boundary layer in the eastern North Atlantic
Daniel A. Knopf
CORRESPONDING AUTHOR
School of Marine and Atmospheric Sciences, Stony Brook University, Stony Brook, NY 11794, USA
Joseph C. Charnawskas
School of Marine and Atmospheric Sciences, Stony Brook University, Stony Brook, NY 11794, USA
Peiwen Wang
School of Marine and Atmospheric Sciences, Stony Brook University, Stony Brook, NY 11794, USA
Benny Wong
School of Marine and Atmospheric Sciences, Stony Brook University, Stony Brook, NY 11794, USA
Jay M. Tomlin
Department of Chemistry, Purdue University, West Lafayette, IN 47907, USA
Kevin A. Jankowski
Department of Chemistry, Purdue University, West Lafayette, IN 47907, USA
Matthew Fraund
Ultrafast X-Ray Science Laboratory, Lawrence Berkeley National Laboratory, Berkeley, CA 94720, USA
Daniel P. Veghte
Environmental Molecular Sciences Laboratory/Pacific Northwest National Laboratory, Richland, WA 99354, USA
current address: Center for Electron Microscopy and Analysis, Ohio State University, Columbus, OH 43212, USA
Swarup China
Environmental Molecular Sciences Laboratory/Pacific Northwest National Laboratory, Richland, WA 99354, USA
Alexander Laskin
Department of Chemistry, Purdue University, West Lafayette, IN 47907, USA
Ryan C. Moffet
Sonoma Technology, Inc., Petaluma, CA 94954, USA
Mary K. Gilles
Chemical Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, CA 94720, USA
Josephine Y. Aller
School of Marine and Atmospheric Sciences, Stony Brook University, Stony Brook, NY 11794, USA
Matthew A. Marcus
Advanced Light Source, Lawrence Berkeley National Laboratory, Berkeley, CA 94720, USA
Shira Raveh-Rubin
Department of Earth and Planetary Sciences, Weizmann Institute of Science, Rehovot 76100, Israel
Jian Wang
Center for Aerosol Science and Engineering, Department of Energy, Environmental and Chemical Engineering, Washington University in St. Louis, St. Louis, MO 63130, USA
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Cited
18 citations as recorded by crossref.
- A Method for Separating and Quantifying Organic and Inorganic Ice Nucleating Substances Based on Density Gradient Centrifugation S. Worthy et al. 10.1021/acsearthspacechem.4c00128
- Data analysis in spectroscopic STXM M. Marcus 10.1016/j.elspec.2023.147310
- Physicochemical characterization of free troposphere and marine boundary layer ice-nucleating particles collected by aircraft in the eastern North Atlantic D. Knopf et al. 10.5194/acp-23-8659-2023
- Wildfire smoke triggers cirrus formation: lidar observations over the eastern Mediterranean R. Mamouri et al. 10.5194/acp-23-14097-2023
- Atmospheric ice nucleation D. Knopf & P. Alpert 10.1038/s42254-023-00570-7
- Ice nucleating abilities of deep waters from the Mexican Pacific ocean M. Fernanda Córdoba et al. 10.1016/j.atmosenv.2023.119887
- An automated size and time-resolved aerosol collector platform integrated with environmental sensors to study the vertical profile of aerosols Z. Cheng et al. 10.1039/D2EA00097K
- Influence of open ocean biogeochemistry on aerosol and clouds: Recent findings and perspectives K. Sellegri et al. 10.1525/elementa.2023.00058
- A 1D Model for Nucleation of Ice From Aerosol Particles: An Application to a Mixed‐Phase Arctic Stratus Cloud Layer D. Knopf et al. 10.1029/2023MS003663
- Single particle characteristics and ice nucleation potential of particles collected during Asian dust storms in 2021 L. Zhao et al. 10.1016/j.scitotenv.2024.174829
- Diverse sources and aging change the mixing state and ice nucleation properties of aerosol particles over the western Pacific and Southern Ocean J. Xue et al. 10.5194/acp-24-7731-2024
- Ice-nucleating agents in sea spray aerosol identified and quantified with a holistic multimodal freezing model P. Alpert et al. 10.1126/sciadv.abq6842
- Quantifying and Modeling the Impact of Phase State on the Ice Nucleation Abilities of 2-Methyltetrols as a Key Component of Secondary Organic Aerosol Derived from Isoprene Epoxydiols X. Li et al. 10.1021/acs.est.4c06285
- Measurement report: A comparison of ground-level ice-nucleating-particle abundance and aerosol properties during autumn at contrasting marine and terrestrial locations E. Wilbourn et al. 10.5194/acp-24-5433-2024
- Contact Freezing of Water Droplets by Crystalline Organic Acids Z. Schiffman et al. 10.1021/acs.jpca.5c03258
- Iron (Fe) speciation in size-fractionated aerosol particles in the Pacific Ocean: The role of organic complexation of Fe with humic-like substances in controlling Fe solubility K. Sakata et al. 10.5194/acp-22-9461-2022
- Cloud condensation nuclei activity of internally mixed particle populations at a remote marine free troposphere site in the North Atlantic Ocean Z. Cheng et al. 10.1016/j.scitotenv.2023.166865
- Vertical profiling of residential wood combustion aerosols over Tirana, Albania: First lidar-based observations G. Malollari et al. 10.1016/j.atmosenv.2025.121358
18 citations as recorded by crossref.
- A Method for Separating and Quantifying Organic and Inorganic Ice Nucleating Substances Based on Density Gradient Centrifugation S. Worthy et al. 10.1021/acsearthspacechem.4c00128
- Data analysis in spectroscopic STXM M. Marcus 10.1016/j.elspec.2023.147310
- Physicochemical characterization of free troposphere and marine boundary layer ice-nucleating particles collected by aircraft in the eastern North Atlantic D. Knopf et al. 10.5194/acp-23-8659-2023
- Wildfire smoke triggers cirrus formation: lidar observations over the eastern Mediterranean R. Mamouri et al. 10.5194/acp-23-14097-2023
- Atmospheric ice nucleation D. Knopf & P. Alpert 10.1038/s42254-023-00570-7
- Ice nucleating abilities of deep waters from the Mexican Pacific ocean M. Fernanda Córdoba et al. 10.1016/j.atmosenv.2023.119887
- An automated size and time-resolved aerosol collector platform integrated with environmental sensors to study the vertical profile of aerosols Z. Cheng et al. 10.1039/D2EA00097K
- Influence of open ocean biogeochemistry on aerosol and clouds: Recent findings and perspectives K. Sellegri et al. 10.1525/elementa.2023.00058
- A 1D Model for Nucleation of Ice From Aerosol Particles: An Application to a Mixed‐Phase Arctic Stratus Cloud Layer D. Knopf et al. 10.1029/2023MS003663
- Single particle characteristics and ice nucleation potential of particles collected during Asian dust storms in 2021 L. Zhao et al. 10.1016/j.scitotenv.2024.174829
- Diverse sources and aging change the mixing state and ice nucleation properties of aerosol particles over the western Pacific and Southern Ocean J. Xue et al. 10.5194/acp-24-7731-2024
- Ice-nucleating agents in sea spray aerosol identified and quantified with a holistic multimodal freezing model P. Alpert et al. 10.1126/sciadv.abq6842
- Quantifying and Modeling the Impact of Phase State on the Ice Nucleation Abilities of 2-Methyltetrols as a Key Component of Secondary Organic Aerosol Derived from Isoprene Epoxydiols X. Li et al. 10.1021/acs.est.4c06285
- Measurement report: A comparison of ground-level ice-nucleating-particle abundance and aerosol properties during autumn at contrasting marine and terrestrial locations E. Wilbourn et al. 10.5194/acp-24-5433-2024
- Contact Freezing of Water Droplets by Crystalline Organic Acids Z. Schiffman et al. 10.1021/acs.jpca.5c03258
- Iron (Fe) speciation in size-fractionated aerosol particles in the Pacific Ocean: The role of organic complexation of Fe with humic-like substances in controlling Fe solubility K. Sakata et al. 10.5194/acp-22-9461-2022
- Cloud condensation nuclei activity of internally mixed particle populations at a remote marine free troposphere site in the North Atlantic Ocean Z. Cheng et al. 10.1016/j.scitotenv.2023.166865
- Vertical profiling of residential wood combustion aerosols over Tirana, Albania: First lidar-based observations G. Malollari et al. 10.1016/j.atmosenv.2025.121358
Latest update: 30 Oct 2025
Short summary
Marine boundary layer aerosols collected in the remote region of the eastern North Atlantic induce immersion freezing and deposition ice nucleation under typical mixed-phase and cirrus cloud conditions. Corresponding ice nucleation parameterizations for model applications have been derived. Chemical imaging of ambient aerosol and ice-nucleating particles demonstrates that the latter is dominated by sea salt and organics while also representing a major particle type in the particle population.
Marine boundary layer aerosols collected in the remote region of the eastern North Atlantic...
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