Atmospheric Chemistry and Physics
Atmospheric Chemistry and Physics
ACP
Articles | Volume 22, issue 1
Articles | Volume 22, issue 1
https://doi.org/10.5194/acp-22-47-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-22-47-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
Articles | Volume 22, issue 1
Research article
 | 
03 Jan 2022
Research article |  | 03 Jan 2022

Impact of non-ideality on reconstructing spatial and temporal variations in aerosol acidity with multiphase buffer theory

Guangjie Zheng, Hang Su, Siwen Wang, Andrea Pozzer, and Yafang Cheng

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Latest update: 13 Dec 2024
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Short summary
The recently proposed multiphase buffer theory provides a framework to reconstruct long-term trends and spatial variations in aerosol pH, while non-ideality is a major limitation for its broad applications. Here we proposed a parameterization method to estimate the impact of non-ideality and validated it against long-term observations and global simulations. With this method, the multiphase buffer theory can reproduce well aerosol pH variations estimated by comprehensive thermodynamic models.
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