Articles | Volume 22, issue 6
https://doi.org/10.5194/acp-22-4237-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-22-4237-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
01 Apr 2022
Research article |
| 01 Apr 2022
| 01 Apr 2022
Formation of organic sulfur compounds through SO2-initiated photochemistry of PAHs and dimethylsulfoxide at the air-water interface
Haoyu Jiang
State Key Laboratory of Organic Geochemistry and Guangdong Provincial Key Laboratory of Environmental Protection and Resources Utilization, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510 640, China
Guangdong-Hong Kong-Macao Joint Laboratory for Environmental Pollution and Control, Guangzhou Institute of Geochemistry, Chinese Academy of Science, Guangzhou 510640, China
Chinese Academy of Science, Center for Excellence in Deep Earth
Science, Guangzhou, 510640, China
Yingyao He
School of Marine Sciences, Sun Yat-sen University, Guangzhou 510006, China
Yiqun Wang
State Key Laboratory of Organic Geochemistry and Guangdong Provincial Key Laboratory of Environmental Protection and Resources Utilization, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510 640, China
Guangdong-Hong Kong-Macao Joint Laboratory for Environmental Pollution and Control, Guangzhou Institute of Geochemistry, Chinese Academy of Science, Guangzhou 510640, China
Sheng Li
Hunan Research Academy of Environmental sciences, Changsha, 410004,
China
Bin Jiang
State Key Laboratory of Organic Geochemistry and Guangdong Provincial Key Laboratory of Environmental Protection and Resources Utilization, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510 640, China
Guangdong-Hong Kong-Macao Joint Laboratory for Environmental Pollution and Control, Guangzhou Institute of Geochemistry, Chinese Academy of Science, Guangzhou 510640, China
Luca Carena
Dipartimento di Chimica, Università di Torino, Via Pietro Giuria 5, 10125 Torino, Italy
Xue Li
Institute of Mass Spectrometry and Atmospheric Environment, Jinan
University, Guangzhou 510632, China
Lihua Yang
School of Marine Sciences, Sun Yat-sen University, Guangzhou 510006, China
Tiangang Luan
School of Marine Sciences, Sun Yat-sen University, Guangzhou 510006, China
Davide Vione
Dipartimento di Chimica, Università di Torino, Via Pietro Giuria 5, 10125 Torino, Italy
Sasho Gligorovski
CORRESPONDING AUTHOR
State Key Laboratory of Organic Geochemistry and Guangdong Provincial Key Laboratory of Environmental Protection and Resources Utilization, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510 640, China
Guangdong-Hong Kong-Macao Joint Laboratory for Environmental Pollution and Control, Guangzhou Institute of Geochemistry, Chinese Academy of Science, Guangzhou 510640, China
Chinese Academy of Science, Center for Excellence in Deep Earth
Science, Guangzhou, 510640, China
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Cited
13 citations as recorded by crossref.
- Chemical transformation of a long-chain alkyl organosulfate via heterogeneous OH oxidation: a case study of sodium dodecyl sulfate S. Madeleine Ng et al. 10.1039/D2EA00026A
- Heterogeneous chemistry of ozone with floor cleaning agent: Implications of secondary VOCs in the indoor environment J. Xu et al. 10.1016/j.scitotenv.2022.160867
- Beyond the formation: unveiling the atmospheric transformation of organosulfatesviaheterogeneous OH oxidation S. Ng & M. Chan 10.1039/D3CC03700B
- Characteristics, formation, and sources of PM2.5 in 2020 in Suzhou, Yangtze River Delta, China Y. Li et al. 10.1016/j.envres.2022.113545
- Tracking the history of polycyclic aromatic compounds in London through a River Thames sediment core and ultrahigh resolution mass spectrometry R. Downham et al. 10.1016/j.jhazmat.2024.134605
- Daytime SO 2 chemistry on ubiquitous urban surfaces as a source of organic sulfur compounds in ambient air H. Deng et al. 10.1126/sciadv.abq6830
- Polycyclic aromatic hydrocarbons in coarse particles (PM10) over the coastal urban region in Poland: Distribution, source analysis and human health risk implications P. Siudek 10.1016/j.chemosphere.2022.137130
- Measurements of particulate methanesulfonic acid above the remote Arctic Ocean using a high resolution aerosol mass spectrometer Y. Zhang et al. 10.1016/j.atmosenv.2024.120538
- The Effect of Human Occupancy on Indoor Air Quality through Real-Time Measurements of Key Pollutants H. Deng et al. 10.1021/acs.est.2c04609
- Observations of atmospheric new particle formation impacts on cloud condensation nuclei in summer at Mt.Tian Z. Wu et al. 10.1016/j.atmosenv.2023.120002
- Design of a new nanocomposite based on Keggin-type [ZnW12O40]6− anionic cluster anchored on NiZn2O4 ceramics as a promising material towards the electrocatalytic hydrogen storage M. Rezvani et al. 10.1038/s41598-024-61871-0
- Synthesis, characterization, and electrochemical evaluation of SnFe2O4@MWCNTS nanocomposite as a potential hydrogen storage material M. Shaterian et al. 10.1016/j.heliyon.2023.e16648
- Characteristics of dissolved black carbon in riverine surface microlayer V. Vaezzadeh et al. 10.1016/j.marpolbul.2023.115301
13 citations as recorded by crossref.
- Chemical transformation of a long-chain alkyl organosulfate via heterogeneous OH oxidation: a case study of sodium dodecyl sulfate S. Madeleine Ng et al. 10.1039/D2EA00026A
- Heterogeneous chemistry of ozone with floor cleaning agent: Implications of secondary VOCs in the indoor environment J. Xu et al. 10.1016/j.scitotenv.2022.160867
- Beyond the formation: unveiling the atmospheric transformation of organosulfatesviaheterogeneous OH oxidation S. Ng & M. Chan 10.1039/D3CC03700B
- Characteristics, formation, and sources of PM2.5 in 2020 in Suzhou, Yangtze River Delta, China Y. Li et al. 10.1016/j.envres.2022.113545
- Tracking the history of polycyclic aromatic compounds in London through a River Thames sediment core and ultrahigh resolution mass spectrometry R. Downham et al. 10.1016/j.jhazmat.2024.134605
- Daytime SO 2 chemistry on ubiquitous urban surfaces as a source of organic sulfur compounds in ambient air H. Deng et al. 10.1126/sciadv.abq6830
- Polycyclic aromatic hydrocarbons in coarse particles (PM10) over the coastal urban region in Poland: Distribution, source analysis and human health risk implications P. Siudek 10.1016/j.chemosphere.2022.137130
- Measurements of particulate methanesulfonic acid above the remote Arctic Ocean using a high resolution aerosol mass spectrometer Y. Zhang et al. 10.1016/j.atmosenv.2024.120538
- The Effect of Human Occupancy on Indoor Air Quality through Real-Time Measurements of Key Pollutants H. Deng et al. 10.1021/acs.est.2c04609
- Observations of atmospheric new particle formation impacts on cloud condensation nuclei in summer at Mt.Tian Z. Wu et al. 10.1016/j.atmosenv.2023.120002
- Design of a new nanocomposite based on Keggin-type [ZnW12O40]6− anionic cluster anchored on NiZn2O4 ceramics as a promising material towards the electrocatalytic hydrogen storage M. Rezvani et al. 10.1038/s41598-024-61871-0
- Synthesis, characterization, and electrochemical evaluation of SnFe2O4@MWCNTS nanocomposite as a potential hydrogen storage material M. Shaterian et al. 10.1016/j.heliyon.2023.e16648
- Characteristics of dissolved black carbon in riverine surface microlayer V. Vaezzadeh et al. 10.1016/j.marpolbul.2023.115301
Latest update: 29 Jun 2024
Short summary
Heterogeneous oxidation of SO2 is suggested to be one of the most important pathways for sulfate formation during extreme haze events in China, yet the exact mechanism remains highly uncertain. Our study reveals that ubiquitous compounds at the sea surface PAHS and DMSO, when exposed to SO2 under simulated sunlight irradiation, generate abundant organic sulfur compounds, providing implications for air-sea interaction and secondary organic aerosols formation processes.
Heterogeneous oxidation of SO2 is suggested to be one of the most important pathways for sulfate...
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