Articles | Volume 22, issue 5
https://doi.org/10.5194/acp-22-3203-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-22-3203-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| Highlight paper
| 
10 Mar 2022
Research article | Highlight paper |
| 10 Mar 2022
| 10 Mar 2022
A predictive viscosity model for aqueous electrolytes and mixed organic–inorganic aerosol phases
Joseph Lilek
Department of Atmospheric and Oceanic Sciences, McGill University, Montréal, Quebec, H3A 0B9, Canada
Department of Atmospheric and Oceanic Sciences, McGill University, Montréal, Quebec, H3A 0B9, Canada
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Cited
18 citations as recorded by crossref.
- Prediction of Dynamic Viscosity and Sensitivity Study of Potassium Amino-Acid Salt Aqueous Solutions by an Artificial Neural Network According to the Structure A. Delanney et al. 10.1021/acs.iecr.3c02083
- Viscosity, Glass Formation, and Mixing Times within Secondary Organic Aerosol from Biomass Burning Phenolics K. Kiland et al. 10.1021/acsearthspacechem.3c00039
- Enhanced Nitrate Fraction: Enabling Urban Aerosol Particles to Remain in a Liquid State at Reduced Relative Humidity Y. Liu et al. 10.1029/2023GL105505
- Influence of Relative Humidity and Composition on PM2.5 Phases in Northeast Asia C. Seong et al. 10.1021/acsearthspacechem.4c00019
- The viscosity of aqueous solutions as analogs to cryovolcanic liquids A. Morrison et al. 10.1016/j.gca.2022.10.019
- Probe molecular diffusivity in single ternary inorganic–organic microdroplets via interfacial ozonolysis of thiosulfate T. Hung et al. 10.1039/D4EA00072B
- OH Radical Oxidation of Organosulfates in the Atmospheric Aqueous Phase D. Gweme & S. Styler 10.1021/acs.jpca.4c02877
- Viscosity and physical state of sucrose mixed with ammonium sulfate droplets R. Jeong et al. 10.5194/acp-22-8805-2022
- Microscopic observation of a liquid-liquid-(semi)solid phase in polluted PM2.5 S. Gaikwad et al. 10.3389/fenvs.2022.947924
- Hydrogel network formation triggers atypical hygroscopic behavior in atmospheric aerosols F. Dong et al. 10.1016/j.scitotenv.2024.177298
- Machine-Learning-Based Prediction of the Glass Transition Temperature of Organic Compounds Using Experimental Data G. Armeli et al. 10.1021/acsomega.2c08146
- Changes in Physicochemical Properties of Organic Aerosol During Photochemical Aging of Cooking and Burning Emissions W. Xu et al. 10.1029/2022JD037911
- Equilibration times in viscous and viscoelastic aerosol particles T. Preston & A. Zuend 10.1039/D2EA00065B
- Comparison of Phase States of PM2.5 over Megacities, Seoul and Beijing, and Their Implications on Particle Size Distribution M. Song et al. 10.1021/acs.est.2c06377
- Direct measurement of the viscosity of ternary aerosol mixtures S. Mahant et al. 10.1039/D2EA00160H
- Simulated phase state and viscosity of secondary organic aerosols over China Z. Zhang et al. 10.5194/acp-24-4809-2024
- Viscosity and phase state of aerosol particles consisting of sucrose mixed with inorganic salts Y. Song et al. 10.5194/acp-21-10215-2021
- Integration of Semi-Empirical and Artificial Neural Network (ANN) for Modeling Lithium-Ion Electrolyte Systems Dynamic Viscosity F. Azeez & A. Refaie 10.1149/1945-7111/ac4840
16 citations as recorded by crossref.
- Prediction of Dynamic Viscosity and Sensitivity Study of Potassium Amino-Acid Salt Aqueous Solutions by an Artificial Neural Network According to the Structure A. Delanney et al. 10.1021/acs.iecr.3c02083
- Viscosity, Glass Formation, and Mixing Times within Secondary Organic Aerosol from Biomass Burning Phenolics K. Kiland et al. 10.1021/acsearthspacechem.3c00039
- Enhanced Nitrate Fraction: Enabling Urban Aerosol Particles to Remain in a Liquid State at Reduced Relative Humidity Y. Liu et al. 10.1029/2023GL105505
- Influence of Relative Humidity and Composition on PM2.5 Phases in Northeast Asia C. Seong et al. 10.1021/acsearthspacechem.4c00019
- The viscosity of aqueous solutions as analogs to cryovolcanic liquids A. Morrison et al. 10.1016/j.gca.2022.10.019
- Probe molecular diffusivity in single ternary inorganic–organic microdroplets via interfacial ozonolysis of thiosulfate T. Hung et al. 10.1039/D4EA00072B
- OH Radical Oxidation of Organosulfates in the Atmospheric Aqueous Phase D. Gweme & S. Styler 10.1021/acs.jpca.4c02877
- Viscosity and physical state of sucrose mixed with ammonium sulfate droplets R. Jeong et al. 10.5194/acp-22-8805-2022
- Microscopic observation of a liquid-liquid-(semi)solid phase in polluted PM2.5 S. Gaikwad et al. 10.3389/fenvs.2022.947924
- Hydrogel network formation triggers atypical hygroscopic behavior in atmospheric aerosols F. Dong et al. 10.1016/j.scitotenv.2024.177298
- Machine-Learning-Based Prediction of the Glass Transition Temperature of Organic Compounds Using Experimental Data G. Armeli et al. 10.1021/acsomega.2c08146
- Changes in Physicochemical Properties of Organic Aerosol During Photochemical Aging of Cooking and Burning Emissions W. Xu et al. 10.1029/2022JD037911
- Equilibration times in viscous and viscoelastic aerosol particles T. Preston & A. Zuend 10.1039/D2EA00065B
- Comparison of Phase States of PM2.5 over Megacities, Seoul and Beijing, and Their Implications on Particle Size Distribution M. Song et al. 10.1021/acs.est.2c06377
- Direct measurement of the viscosity of ternary aerosol mixtures S. Mahant et al. 10.1039/D2EA00160H
- Simulated phase state and viscosity of secondary organic aerosols over China Z. Zhang et al. 10.5194/acp-24-4809-2024
2 citations as recorded by crossref.
- Viscosity and phase state of aerosol particles consisting of sucrose mixed with inorganic salts Y. Song et al. 10.5194/acp-21-10215-2021
- Integration of Semi-Empirical and Artificial Neural Network (ANN) for Modeling Lithium-Ion Electrolyte Systems Dynamic Viscosity F. Azeez & A. Refaie 10.1149/1945-7111/ac4840
Latest update: 23 Nov 2024
Short summary
Depending on temperature and chemical makeup, certain aerosols can be highly viscous or glassy, with atmospheric implications. We have therefore implemented two major upgrades to the predictive viscosity model AIOMFAC-VISC. First, we created a new viscosity model for aqueous electrolyte solutions containing an arbitrary number of ion species. Second, we integrated the electrolyte model within the existing AIOMFAC-VISC framework to enable viscosity predictions for organic–inorganic mixtures.
Depending on temperature and chemical makeup, certain aerosols can be highly viscous or glassy,...
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