Articles | Volume 22, issue 1
https://doi.org/10.5194/acp-22-273-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-22-273-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Aqueous secondary organic aerosol formation from the direct photosensitized oxidation of vanillin in the absence and presence of ammonium nitrate
Brix Raphael Go
School of Energy and Environment, City University of Hong Kong, Kowloon, Hong Kong, China
City University of Hong Kong Shenzhen Research Institute, Shenzhen, China
Yan Lyu
School of Energy and Environment, City University of Hong Kong, Kowloon, Hong Kong, China
City University of Hong Kong Shenzhen Research Institute, Shenzhen, China
Yan Ji
School of Energy and Environment, City University of Hong Kong, Kowloon, Hong Kong, China
City University of Hong Kong Shenzhen Research Institute, Shenzhen, China
Yong Jie Li
Department of Civil and Environmental Engineering, and Centre for Regional Oceans, Faculty of Science and Technology, University of Macau, Taipa, Macau 999078, China
Dan Dan Huang
State Environmental Protection Key Laboratory of Formation and Prevention of the Urban Air Pollution Complex, Shanghai Academy of Environmental Sciences, Shanghai 200233, China
Xue Li
Institute of Mass Spectrometry and Atmospheric Environment, Jinan University, No. 601 Huangpu Avenue West, Guangzhou 510632, China
Theodora Nah
School of Energy and Environment, City University of Hong Kong, Kowloon, Hong Kong, China
Chun Ho Lam
School of Energy and Environment, City University of Hong Kong, Kowloon, Hong Kong, China
School of Energy and Environment, City University of Hong Kong, Kowloon, Hong Kong, China
City University of Hong Kong Shenzhen Research Institute, Shenzhen, China
Guy Carpenter Asia-Pacific Climate Impact Center, City University of Hong Kong, Kowloon, Hong Kong, China
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Cited
48 citations as recorded by crossref.
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- Aqueous-phase chemistry of atmospheric phenolic compounds: A critical review of laboratory studies F. Li et al. 10.1016/j.scitotenv.2022.158895
- Review of the Mechanisms of Liquid-Phase Transformation of Atmospheric Phenolic Compounds: Implications for Air Quality and Environmental Health Y. Yang et al. 10.3390/atmos15091040
- Influence of urban heat islands on seasonal aerosol acidity and aerosol liquid water content in humid subtropical Hong Kong, South China T. Nah & Y. Lam 10.1016/j.atmosenv.2022.119321
- High spatiotemporal resolution ammonia emission inventory from typical industrial and agricultural province of China from 2000 to 2020 C. Zhu et al. 10.1016/j.scitotenv.2024.170732
- Aqueous-Phase Photoreactions of Mixed Aromatic Carbonyl Photosensitizers Yield More Oxygenated, Oxidized, and less Light-Absorbing Secondary Organic Aerosol (SOA) than Single Systems B. Go et al. 10.1021/acs.est.3c10199
- Complexities of Photosensitization in Atmospheric Particles Z. Liang et al. 10.1021/acsestair.4c00112
- Aqueous photochemical aging of water-soluble smoke particles from crop straws burning Z. Ye et al. 10.1016/j.atmosenv.2024.120897
- Single-particle Raman spectroscopy for studying physical and chemical processes of atmospheric particles Z. Liang et al. 10.5194/acp-22-3017-2022
- Comparison of aqueous secondary organic aerosol (aqSOA) product distributions from guaiacol oxidation by non-phenolic and phenolic methoxybenzaldehydes as photosensitizers in the absence and presence of ammonium nitrate B. Go et al. 10.5194/acp-23-2859-2023
- Photoaging of phenolic secondary organic aerosol in the aqueous phase: evolution of chemical and optical properties and effects of oxidants W. Jiang et al. 10.5194/acp-23-7103-2023
- Photochemical Reactions of Glyoxal during Particulate Ammonium Nitrate Photolysis: Brown Carbon Formation, Enhanced Glyoxal Decay, and Organic Phase Formation R. Zhang et al. 10.1021/acs.est.1c07211
- Production of Volatile Organic Compounds by Ozone Oxidation Chemistry at the South China Sea Surface Microlayer Y. Wang et al. 10.1021/acsearthspacechem.3c00102
- The High Pressure Inside Aerosol Particles Enhances Photochemical Reactions of Biomass Burning Compounds C. Dubois et al. 10.1021/acsearthspacechem.4c00011
- Reactivity of aminophenols in forming nitrogen-containing brown carbon from iron-catalyzed reactions H. Al-Abadleh et al. 10.1038/s42004-022-00732-1
- The complexation of atmospheric Brown carbon surrogates on the generation of hydroxyl radical from transition metals in simulated lung fluid Y. Lyu et al. 10.1016/j.envint.2023.108240
- Heterogeneous chemistry of ozone with floor cleaning agent: Implications of secondary VOCs in the indoor environment J. Xu et al. 10.1016/j.scitotenv.2022.160867
- Optical and chemical properties and oxidative potential of aqueous-phase products from OH and <sup>3</sup>C<sup>∗</sup>-initiated photooxidation of eugenol X. Li et al. 10.5194/acp-22-7793-2022
- Enhanced HONO Formation from Aqueous Nitrate Photochemistry in the Presence of Marine Relevant Organics: Impact of Marine-Dissolved Organic Matter (m-DOM) Concentration on HONO Yields and Potential Synergistic Effects of Compounds within m-DOM S. Mora García et al. 10.1021/acsestair.4c00006
- Aqueous Photosensitization of Syringaldehyde: Reactivity, Effects of Environmental Factors, and Formation of Brown Carbon Products F. Li et al. 10.1021/acsearthspacechem.4c00004
- Sulfate Formation in Incense Burning Particles: A Single-Particle Mass Spectrometric Study Z. Liang et al. 10.1021/acs.estlett.2c00492
- Wavelength-resolved quantum yields for vanillin photochemistry: self-reaction and ionic-strength implications for wildfire brown carbon lifetime G. Drozd et al. 10.1039/D4EA00002A
- Chemical evolution of primary and secondary biomass burning aerosols during daytime and nighttime A. Yazdani et al. 10.5194/acp-23-7461-2023
- Photoinduced Reactions of Nitrate in Aqueous Microdroplets by Triplet Energy Transfer P. Kim et al. 10.1021/acs.jpclett.3c02178
- Sulfate formation via aerosol-phase SO2 oxidation by model biomass burning photosensitizers: 3,4-dimethoxybenzaldehyde, vanillin and syringaldehyde using single-particle mixing-state analysis L. Zhou et al. 10.5194/acp-23-5251-2023
- Co-photolysis of mixed chromophores affects atmospheric lifetimes of brown carbon Y. Wang et al. 10.1039/D3EA00073G
- The Effect of Human Occupancy on Indoor Air Quality through Real-Time Measurements of Key Pollutants H. Deng et al. 10.1021/acs.est.2c04609
- Surface Oxidation of Phenolic Aldehydes: Fragmentation, Functionalization, and Coupling Reactions M. Rana & M. Guzman 10.1021/acs.jpca.2c04963
- Role of Direct and Sensitized Photolysis in the Photomineralization of Dissolved Organic Matter and Model Chromophores to Carbon Dioxide S. Buckley et al. 10.1021/acs.est.4c01530
- Photoinduced production of substances with humic-like fluorescence, upon irradiation of water samples from alpine lakes L. Carena et al. 10.1016/j.chemosphere.2023.137972
- Simultaneous Measurement of Gaseous HONO and NO2− in Solutions from Aqueous Nitrate Photolysis Mediated by Organics Y. Zhao et al. 10.3390/atmos15111279
- Role of WSOCs and pH on Ammonium Nitrate Aerosol Efflorescence: Insights into Secondary Aerosol Formation J. Sun et al. 10.1021/acs.est.3c07603
- Contribution of Carbonyl Chromophores in Secondary Brown Carbon from Nighttime Oxidation of Unsaturated Heterocyclic Volatile Organic Compounds K. Chen et al. 10.1021/acs.est.3c08872
- Aqueous-Phase Photooxidation of Vanillin in the Presence of Nitrite: Characteristics, Products, and Mechanism M. Cai et al. 10.1021/acsestair.4c00013
- Daytime SO 2 chemistry on ubiquitous urban surfaces as a source of organic sulfur compounds in ambient air H. Deng et al. 10.1126/sciadv.abq6830
- Metal–organic framework-reduced graphene oxide (Zn-BDC@rGO) composite for selective discrimination among ammonia, carbon monoxide, and sulfur dioxide M. More et al. 10.1007/s00339-023-07103-0
- Enhanced Sulfate Formation through Synergistic Effects of Chlorine Chemistry and Photosensitization in Atmospheric Particles R. Zhang & C. Chan 10.1021/acsestair.3c00030
- Evaluating the potential secondary contribution of photosensitized chemistry to OH production in aqueous aerosols E. Petersen-Sonn et al. 10.1039/D4EA00103F
- pH affects the aqueous-phase nitrate-mediated photooxidation of phenolic compounds: implications for brown carbon formation and evolution J. Yang et al. 10.1039/D2EM00004K
- The interplay of Brown carbon (BrC) surrogates and copper: Implications for the oxidative potential of ambient particles D. Wu et al. 10.1016/j.jhazmat.2024.136276
- Phototransformation of Vanillin in Artificial Snow by Direct Photolysis and Mediated by Nitrite L. Carena et al. 10.1021/acs.est.3c01931
- Effects of copper on chemical kinetics and brown carbon formation in the aqueous ˙OH oxidation of phenolic compounds J. Yang et al. 10.1039/D4EM00191E
- Rapid aqueous-phase dark reaction of phenols with nitrosonium ions: Novel mechanism for atmospheric nitrosation and nitration at low pH B. Cai et al. 10.1093/pnasnexus/pgae385
- Deciphering the key drivers of oxidative potential during ammonium nitrate-mediated aqueous-phase photoreaction of methoxyphenols R. Lai et al. 10.1016/j.atmosenv.2024.120895
- Unsaturated Fatty Acids Enhance Aqueous Atmospheric Oxidation Ability by Producing Oxygen‐Containing Radicals in Fog Droplets N. Yang et al. 10.1029/2022JD038069
- Seasonal variations in the production of singlet oxygen and organic triplet excited states in aqueous PM2.5 in Hong Kong SAR, South China Y. Lyu et al. 10.5194/acp-23-9245-2023
- Significantly alleviated PM2.5 pollution in cold seasons in the Beijing-Tianjin-Hebei and surrounding area: Insights from regional observation Y. Chu et al. 10.1016/j.atmosres.2023.107136
- Decay Kinetics and Absorption Changes of Methoxyphenols and Nitrophenols during Nitrate-Mediated Aqueous Photochemical Oxidation at 254 and 313 nm Y. Wang et al. 10.1021/acsearthspacechem.2c00021
48 citations as recorded by crossref.
- Particulate nitrate photolysis in the atmosphere M. Gen et al. 10.1039/D1EA00087J
- Aqueous-phase chemistry of atmospheric phenolic compounds: A critical review of laboratory studies F. Li et al. 10.1016/j.scitotenv.2022.158895
- Review of the Mechanisms of Liquid-Phase Transformation of Atmospheric Phenolic Compounds: Implications for Air Quality and Environmental Health Y. Yang et al. 10.3390/atmos15091040
- Influence of urban heat islands on seasonal aerosol acidity and aerosol liquid water content in humid subtropical Hong Kong, South China T. Nah & Y. Lam 10.1016/j.atmosenv.2022.119321
- High spatiotemporal resolution ammonia emission inventory from typical industrial and agricultural province of China from 2000 to 2020 C. Zhu et al. 10.1016/j.scitotenv.2024.170732
- Aqueous-Phase Photoreactions of Mixed Aromatic Carbonyl Photosensitizers Yield More Oxygenated, Oxidized, and less Light-Absorbing Secondary Organic Aerosol (SOA) than Single Systems B. Go et al. 10.1021/acs.est.3c10199
- Complexities of Photosensitization in Atmospheric Particles Z. Liang et al. 10.1021/acsestair.4c00112
- Aqueous photochemical aging of water-soluble smoke particles from crop straws burning Z. Ye et al. 10.1016/j.atmosenv.2024.120897
- Single-particle Raman spectroscopy for studying physical and chemical processes of atmospheric particles Z. Liang et al. 10.5194/acp-22-3017-2022
- Comparison of aqueous secondary organic aerosol (aqSOA) product distributions from guaiacol oxidation by non-phenolic and phenolic methoxybenzaldehydes as photosensitizers in the absence and presence of ammonium nitrate B. Go et al. 10.5194/acp-23-2859-2023
- Photoaging of phenolic secondary organic aerosol in the aqueous phase: evolution of chemical and optical properties and effects of oxidants W. Jiang et al. 10.5194/acp-23-7103-2023
- Photochemical Reactions of Glyoxal during Particulate Ammonium Nitrate Photolysis: Brown Carbon Formation, Enhanced Glyoxal Decay, and Organic Phase Formation R. Zhang et al. 10.1021/acs.est.1c07211
- Production of Volatile Organic Compounds by Ozone Oxidation Chemistry at the South China Sea Surface Microlayer Y. Wang et al. 10.1021/acsearthspacechem.3c00102
- The High Pressure Inside Aerosol Particles Enhances Photochemical Reactions of Biomass Burning Compounds C. Dubois et al. 10.1021/acsearthspacechem.4c00011
- Reactivity of aminophenols in forming nitrogen-containing brown carbon from iron-catalyzed reactions H. Al-Abadleh et al. 10.1038/s42004-022-00732-1
- The complexation of atmospheric Brown carbon surrogates on the generation of hydroxyl radical from transition metals in simulated lung fluid Y. Lyu et al. 10.1016/j.envint.2023.108240
- Heterogeneous chemistry of ozone with floor cleaning agent: Implications of secondary VOCs in the indoor environment J. Xu et al. 10.1016/j.scitotenv.2022.160867
- Optical and chemical properties and oxidative potential of aqueous-phase products from OH and <sup>3</sup>C<sup>∗</sup>-initiated photooxidation of eugenol X. Li et al. 10.5194/acp-22-7793-2022
- Enhanced HONO Formation from Aqueous Nitrate Photochemistry in the Presence of Marine Relevant Organics: Impact of Marine-Dissolved Organic Matter (m-DOM) Concentration on HONO Yields and Potential Synergistic Effects of Compounds within m-DOM S. Mora García et al. 10.1021/acsestair.4c00006
- Aqueous Photosensitization of Syringaldehyde: Reactivity, Effects of Environmental Factors, and Formation of Brown Carbon Products F. Li et al. 10.1021/acsearthspacechem.4c00004
- Sulfate Formation in Incense Burning Particles: A Single-Particle Mass Spectrometric Study Z. Liang et al. 10.1021/acs.estlett.2c00492
- Wavelength-resolved quantum yields for vanillin photochemistry: self-reaction and ionic-strength implications for wildfire brown carbon lifetime G. Drozd et al. 10.1039/D4EA00002A
- Chemical evolution of primary and secondary biomass burning aerosols during daytime and nighttime A. Yazdani et al. 10.5194/acp-23-7461-2023
- Photoinduced Reactions of Nitrate in Aqueous Microdroplets by Triplet Energy Transfer P. Kim et al. 10.1021/acs.jpclett.3c02178
- Sulfate formation via aerosol-phase SO2 oxidation by model biomass burning photosensitizers: 3,4-dimethoxybenzaldehyde, vanillin and syringaldehyde using single-particle mixing-state analysis L. Zhou et al. 10.5194/acp-23-5251-2023
- Co-photolysis of mixed chromophores affects atmospheric lifetimes of brown carbon Y. Wang et al. 10.1039/D3EA00073G
- The Effect of Human Occupancy on Indoor Air Quality through Real-Time Measurements of Key Pollutants H. Deng et al. 10.1021/acs.est.2c04609
- Surface Oxidation of Phenolic Aldehydes: Fragmentation, Functionalization, and Coupling Reactions M. Rana & M. Guzman 10.1021/acs.jpca.2c04963
- Role of Direct and Sensitized Photolysis in the Photomineralization of Dissolved Organic Matter and Model Chromophores to Carbon Dioxide S. Buckley et al. 10.1021/acs.est.4c01530
- Photoinduced production of substances with humic-like fluorescence, upon irradiation of water samples from alpine lakes L. Carena et al. 10.1016/j.chemosphere.2023.137972
- Simultaneous Measurement of Gaseous HONO and NO2− in Solutions from Aqueous Nitrate Photolysis Mediated by Organics Y. Zhao et al. 10.3390/atmos15111279
- Role of WSOCs and pH on Ammonium Nitrate Aerosol Efflorescence: Insights into Secondary Aerosol Formation J. Sun et al. 10.1021/acs.est.3c07603
- Contribution of Carbonyl Chromophores in Secondary Brown Carbon from Nighttime Oxidation of Unsaturated Heterocyclic Volatile Organic Compounds K. Chen et al. 10.1021/acs.est.3c08872
- Aqueous-Phase Photooxidation of Vanillin in the Presence of Nitrite: Characteristics, Products, and Mechanism M. Cai et al. 10.1021/acsestair.4c00013
- Daytime SO 2 chemistry on ubiquitous urban surfaces as a source of organic sulfur compounds in ambient air H. Deng et al. 10.1126/sciadv.abq6830
- Metal–organic framework-reduced graphene oxide (Zn-BDC@rGO) composite for selective discrimination among ammonia, carbon monoxide, and sulfur dioxide M. More et al. 10.1007/s00339-023-07103-0
- Enhanced Sulfate Formation through Synergistic Effects of Chlorine Chemistry and Photosensitization in Atmospheric Particles R. Zhang & C. Chan 10.1021/acsestair.3c00030
- Evaluating the potential secondary contribution of photosensitized chemistry to OH production in aqueous aerosols E. Petersen-Sonn et al. 10.1039/D4EA00103F
- pH affects the aqueous-phase nitrate-mediated photooxidation of phenolic compounds: implications for brown carbon formation and evolution J. Yang et al. 10.1039/D2EM00004K
- The interplay of Brown carbon (BrC) surrogates and copper: Implications for the oxidative potential of ambient particles D. Wu et al. 10.1016/j.jhazmat.2024.136276
- Phototransformation of Vanillin in Artificial Snow by Direct Photolysis and Mediated by Nitrite L. Carena et al. 10.1021/acs.est.3c01931
- Effects of copper on chemical kinetics and brown carbon formation in the aqueous ˙OH oxidation of phenolic compounds J. Yang et al. 10.1039/D4EM00191E
- Rapid aqueous-phase dark reaction of phenols with nitrosonium ions: Novel mechanism for atmospheric nitrosation and nitration at low pH B. Cai et al. 10.1093/pnasnexus/pgae385
- Deciphering the key drivers of oxidative potential during ammonium nitrate-mediated aqueous-phase photoreaction of methoxyphenols R. Lai et al. 10.1016/j.atmosenv.2024.120895
- Unsaturated Fatty Acids Enhance Aqueous Atmospheric Oxidation Ability by Producing Oxygen‐Containing Radicals in Fog Droplets N. Yang et al. 10.1029/2022JD038069
- Seasonal variations in the production of singlet oxygen and organic triplet excited states in aqueous PM2.5 in Hong Kong SAR, South China Y. Lyu et al. 10.5194/acp-23-9245-2023
- Significantly alleviated PM2.5 pollution in cold seasons in the Beijing-Tianjin-Hebei and surrounding area: Insights from regional observation Y. Chu et al. 10.1016/j.atmosres.2023.107136
- Decay Kinetics and Absorption Changes of Methoxyphenols and Nitrophenols during Nitrate-Mediated Aqueous Photochemical Oxidation at 254 and 313 nm Y. Wang et al. 10.1021/acsearthspacechem.2c00021
Latest update: 13 Dec 2024
Short summary
Biomass burning (BB) is a global phenomenon that releases large quantities of pollutants such as phenols and aromatic carbonyls into the atmosphere. These compounds can form secondary organic aerosols (SOAs) which play an important role in the Earth’s energy budget. In this work, we demonstrated that the direct irradiation of vanillin (VL) could generate aqueous SOA (aqSOA) such as oligomers. In the presence of nitrate, VL photo-oxidation can also form nitrated compounds.
Biomass burning (BB) is a global phenomenon that releases large quantities of pollutants such as...
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