Articles | Volume 22, issue 4
https://doi.org/10.5194/acp-22-2639-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-22-2639-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
25 Feb 2022
Research article |
| 25 Feb 2022
| 25 Feb 2022
The role of organic acids in new particle formation from methanesulfonic acid and methylamine
Rongjie Zhang
Key Laboratory of Industrial Ecology and Environmental Engineering
(Ministry of Education), School of Environmental Science and Technology,
Dalian University of Technology, Dalian 116024, China
Jiewen Shen
Key Laboratory of Industrial Ecology and Environmental Engineering
(Ministry of Education), School of Environmental Science and Technology,
Dalian University of Technology, Dalian 116024, China
Hong-Bin Xie
CORRESPONDING AUTHOR
Key Laboratory of Industrial Ecology and Environmental Engineering
(Ministry of Education), School of Environmental Science and Technology,
Dalian University of Technology, Dalian 116024, China
Jingwen Chen
Key Laboratory of Industrial Ecology and Environmental Engineering
(Ministry of Education), School of Environmental Science and Technology,
Dalian University of Technology, Dalian 116024, China
Jonas Elm
Department of Chemistry and iClimate, Aarhus University,
Langelandsgade 140, 8000 Aarhus C, Denmark
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Cited
25 citations as recorded by crossref.
- Amine-Enhanced Methanesulfonic Acid-Driven Nucleation: Predictive Model and Cluster Formation Mechanism Y. Liu et al. 10.1021/acs.est.2c01639
- Pan-Arctic methanesulfonic acid aerosol: source regions, atmospheric drivers, and future projections J. Pernov et al. 10.1038/s41612-024-00712-3
- The synergistic effect of organic and inorganic sulfonic acids promotes new particle formation Y. Ji et al. 10.1016/j.scitotenv.2023.163611
- HIO3–HIO2-Driven Three-Component Nucleation: Screening Model and Cluster Formation Mechanism R. Zhang et al. 10.1021/acs.est.3c06098
- The role of trifluoroacetic acid in new particle formation from methanesulfonic acid-methylamine Y. Hu et al. 10.1016/j.atmosenv.2023.120001
- Implications for new particle formation in air of the use of monoethanolamine in carbon capture and storage V. Perraud et al. 10.1039/D4CP00316K
- The driving effects of common atmospheric molecules for formation of prenucleation clusters: the case of sulfuric acid, formic acid, nitric acid, ammonia, and dimethyl amine C. Bready et al. 10.1039/D2EA00087C
- Significant contributions of trimethylamine to sulfuric acid nucleation in polluted environments R. Cai et al. 10.1038/s41612-023-00405-3
- Measurement report: Occurrence of aminiums in PM2.5 during winter in China – aminium outbreak during polluted episodes and potential constraints Y. Xu et al. 10.5194/acp-24-10531-2024
- The driving effects of common atmospheric molecules for formation of clusters: the case of sulfuric acid, nitric acid, hydrochloric acid, ammonia, and dimethylamine O. Longsworth et al. 10.1039/D3EA00118K
- Clusteromics III: Acid Synergy in Sulfuric Acid–Methanesulfonic Acid–Base Cluster Formation J. Elm 10.1021/acsomega.2c01396
- Clusteromics V: Organic Enhanced Atmospheric Cluster Formation D. Ayoubi et al. 10.1021/acsomega.3c00251
- Clusteromics IV: The Role of Nitric Acid in Atmospheric Cluster Formation Y. Knattrup & J. Elm 10.1021/acsomega.2c04278
- Characteristics, Origins, and Atmospheric Processes of Amines in Fine Aerosol Particles in Winter in China T. Liu et al. 10.1029/2023JD038974
- Quantum chemical modeling of organic enhanced atmospheric nucleation: A critical review J. Elm et al. 10.1002/wcms.1662
- The role of sulfur cycle in new particle formation: Cycloaddition reaction of SO3 to H2S H. Zhang et al. 10.1016/j.jes.2023.09.010
- Enhancing acid–base–water ternary aerosol nucleation with organic acid: a case of tartaric acid C. Wang et al. 10.1039/D3CP00809F
- Reaction of SO3 with H2SO4 and its implications for aerosol particle formation in the gas phase and at the air–water interface R. Wang et al. 10.5194/acp-24-4029-2024
- Iodine oxoacids enhance nucleation of sulfuric acid particles in the atmosphere X. He et al. 10.1126/science.adh2526
- Vertical profiles of volatile organic compounds and fine particles in atmospheric air by using an aerial drone with miniaturized samplers and portable devices E. Pusfitasari et al. 10.5194/acp-23-5885-2023
- Enhancement of Atmospheric Nucleation Precursors on Iodic Acid-Induced Nucleation: Predictive Model and Mechanism F. Ma et al. 10.1021/acs.est.3c01034
- Organosulfate produced from consumption of SO3 speeds up sulfuric acid–dimethylamine atmospheric nucleation X. Zhang et al. 10.5194/acp-24-3593-2024
- Enhancement of atmospheric nucleation precursors on formic sulfuric anhydride induced nucleation: Theoretical mechanism G. An 10.1016/j.chemosphere.2024.143684
- The driving effects of common atmospheric molecules for formation of clusters: the case of sulfuric acid, formic acid, hydrochloric acid, ammonia, and dimethylamine O. Longsworth et al. 10.1039/D3EA00087G
- Role of substituent on organosulfate/organosulfonate and amide molecules in the initial stage of atmospheric new particle formation S. Ni et al. 10.1016/j.cplett.2024.141691
25 citations as recorded by crossref.
- Amine-Enhanced Methanesulfonic Acid-Driven Nucleation: Predictive Model and Cluster Formation Mechanism Y. Liu et al. 10.1021/acs.est.2c01639
- Pan-Arctic methanesulfonic acid aerosol: source regions, atmospheric drivers, and future projections J. Pernov et al. 10.1038/s41612-024-00712-3
- The synergistic effect of organic and inorganic sulfonic acids promotes new particle formation Y. Ji et al. 10.1016/j.scitotenv.2023.163611
- HIO3–HIO2-Driven Three-Component Nucleation: Screening Model and Cluster Formation Mechanism R. Zhang et al. 10.1021/acs.est.3c06098
- The role of trifluoroacetic acid in new particle formation from methanesulfonic acid-methylamine Y. Hu et al. 10.1016/j.atmosenv.2023.120001
- Implications for new particle formation in air of the use of monoethanolamine in carbon capture and storage V. Perraud et al. 10.1039/D4CP00316K
- The driving effects of common atmospheric molecules for formation of prenucleation clusters: the case of sulfuric acid, formic acid, nitric acid, ammonia, and dimethyl amine C. Bready et al. 10.1039/D2EA00087C
- Significant contributions of trimethylamine to sulfuric acid nucleation in polluted environments R. Cai et al. 10.1038/s41612-023-00405-3
- Measurement report: Occurrence of aminiums in PM2.5 during winter in China – aminium outbreak during polluted episodes and potential constraints Y. Xu et al. 10.5194/acp-24-10531-2024
- The driving effects of common atmospheric molecules for formation of clusters: the case of sulfuric acid, nitric acid, hydrochloric acid, ammonia, and dimethylamine O. Longsworth et al. 10.1039/D3EA00118K
- Clusteromics III: Acid Synergy in Sulfuric Acid–Methanesulfonic Acid–Base Cluster Formation J. Elm 10.1021/acsomega.2c01396
- Clusteromics V: Organic Enhanced Atmospheric Cluster Formation D. Ayoubi et al. 10.1021/acsomega.3c00251
- Clusteromics IV: The Role of Nitric Acid in Atmospheric Cluster Formation Y. Knattrup & J. Elm 10.1021/acsomega.2c04278
- Characteristics, Origins, and Atmospheric Processes of Amines in Fine Aerosol Particles in Winter in China T. Liu et al. 10.1029/2023JD038974
- Quantum chemical modeling of organic enhanced atmospheric nucleation: A critical review J. Elm et al. 10.1002/wcms.1662
- The role of sulfur cycle in new particle formation: Cycloaddition reaction of SO3 to H2S H. Zhang et al. 10.1016/j.jes.2023.09.010
- Enhancing acid–base–water ternary aerosol nucleation with organic acid: a case of tartaric acid C. Wang et al. 10.1039/D3CP00809F
- Reaction of SO3 with H2SO4 and its implications for aerosol particle formation in the gas phase and at the air–water interface R. Wang et al. 10.5194/acp-24-4029-2024
- Iodine oxoacids enhance nucleation of sulfuric acid particles in the atmosphere X. He et al. 10.1126/science.adh2526
- Vertical profiles of volatile organic compounds and fine particles in atmospheric air by using an aerial drone with miniaturized samplers and portable devices E. Pusfitasari et al. 10.5194/acp-23-5885-2023
- Enhancement of Atmospheric Nucleation Precursors on Iodic Acid-Induced Nucleation: Predictive Model and Mechanism F. Ma et al. 10.1021/acs.est.3c01034
- Organosulfate produced from consumption of SO3 speeds up sulfuric acid–dimethylamine atmospheric nucleation X. Zhang et al. 10.5194/acp-24-3593-2024
- Enhancement of atmospheric nucleation precursors on formic sulfuric anhydride induced nucleation: Theoretical mechanism G. An 10.1016/j.chemosphere.2024.143684
- The driving effects of common atmospheric molecules for formation of clusters: the case of sulfuric acid, formic acid, hydrochloric acid, ammonia, and dimethylamine O. Longsworth et al. 10.1039/D3EA00087G
- Role of substituent on organosulfate/organosulfonate and amide molecules in the initial stage of atmospheric new particle formation S. Ni et al. 10.1016/j.cplett.2024.141691
Latest update: 20 Nov 2024
Short summary
Formic acid is screened out as the species that can effectively catalyze the new particle formation (NPF) of the methanesulfonic acid (MSA)–methylamine system, indicating organic acids might be required to facilitate MSA-driven NPF in the atmosphere. The results are significant to comprehensively understand the MSA-driven NPF and expand current knowledge of the contribution of OAs to NPF.
Formic acid is screened out as the species that can effectively catalyze the new particle...
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