Atmospheric Chemistry and Physics
Atmospheric Chemistry and Physics
ACP
Articles | Volume 22, issue 23
Articles | Volume 22, issue 23
https://doi.org/10.5194/acp-22-15449-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-22-15449-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
Articles | Volume 22, issue 23
Research article
 | 
07 Dec 2022
Research article |  | 07 Dec 2022

Observation-based constraints on modeled aerosol surface area: implications for heterogeneous chemistry

Rachel A. Bergin, Monica Harkey, Alicia Hoffman, Richard H. Moore, Bruce Anderson, Andreas Beyersdorf, Luke Ziemba, Lee Thornhill, Edward Winstead, Tracey Holloway, and Timothy H. Bertram

Viewed

Total article views: 2,021 (including HTML, PDF, and XML)
HTML PDF XML Total Supplement BibTeX EndNote
1,477 486 58 2,021 73 64 46
  • HTML: 1,477
  • PDF: 486
  • XML: 58
  • Total: 2,021
  • Supplement: 73
  • BibTeX: 64
  • EndNote: 46
Views and downloads (calculated since 22 Jun 2022)
Cumulative views and downloads (calculated since 22 Jun 2022)

Viewed (geographical distribution)

Total article views: 2,021 (including HTML, PDF, and XML) Thereof 2,021 with geography defined and 0 with unknown origin.
Country # Views %
  • 1
1
 
 
 
 

Cited

Latest update: 04 Feb 2025
Download
Short summary
Correctly predicting aerosol surface area concentrations is important for determining the rate of heterogeneous reactions in chemical transport models. Here, we compare aircraft measurements of aerosol surface area with a regional model. In polluted air masses, we show that the model underpredicts aerosol surface area by a factor of 2. Despite this disagreement, the representation of heterogeneous chemistry still dominates the overall uncertainty in the loss rate of molecules such as N2O5.
Read more
Share
Altmetrics
Final-revised paper
Preprint