Articles | Volume 22, issue 22
https://doi.org/10.5194/acp-22-14467-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-22-14467-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
15 Nov 2022
Research article |
| 15 Nov 2022
| 15 Nov 2022
Comparison of model and ground observations finds snowpack and blowing snow aerosols both contribute to Arctic tropospheric reactive bromine
Department of Chemistry and Biochemistry and Geophysical Institute,
University of Alaska Fairbanks, Fairbanks, Alaska, USA
Chris D. Holmes
Department of Earth, Ocean and Atmospheric Science, Florida State
University, Tallahassee, Florida, USA
William R. Simpson
Department of Chemistry and Biochemistry and Geophysical Institute,
University of Alaska Fairbanks, Fairbanks, Alaska, USA
Kaitlyn Confer
Department of Atmospheric Sciences, University of Washington, Seattle,
Washington, USA
Louis Marelle
Institut des Géosciences de l'Environnement (IGE), Institut
Polytechnique de Grenoble, Grenoble, France
Laboratoire Atmosphères Observations Spatiales (LATMOS), Sorbonne
Université, Paris, France
Jennie L. Thomas
Institut des Géosciences de l'Environnement (IGE), Institut
Polytechnique de Grenoble, Grenoble, France
Lyatt Jaeglé
Department of Atmospheric Sciences, University of Washington, Seattle,
Washington, USA
Becky Alexander
Department of Atmospheric Sciences, University of Washington, Seattle,
Washington, USA
Shuting Zhai
Department of Atmospheric Sciences, University of Washington, Seattle,
Washington, USA
Qianjie Chen
Department of Civil and Environmental Engineering, Hong Kong
Polytechnic University, Hong Kong, China
Xuan Wang
School of Energy and the Environment, City University of Hong Kong,
Hong Kong, China
Tomás Sherwen
National Centre for Atmospheric Science, University of York, York, UK
Department of Chemistry, University of York, York, UK
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Cited
11 citations as recorded by crossref.
- Global Observations of Tropospheric Bromine Monoxide (BrO) Columns From TROPOMI Y. Chen et al. 10.1029/2023JD039091
- Modelling the coupled mercury-halogen-ozone cycle in the central Arctic during spring S. Ahmed et al. 10.1525/elementa.2022.00129
- Implications of Snowpack Reactive Bromine Production for Arctic Ice Core Bromine Preservation S. Zhai et al. 10.1029/2023JD039257
- Low ozone dry deposition rates to sea ice during the MOSAiC field campaign: Implications for the Arctic boundary layer ozone budget J. Barten et al. 10.1525/elementa.2022.00086
- Arctic halogens reduce ozone in the northern mid-latitudes R. Fernandez et al. 10.1073/pnas.2401975121
- Impact of Changing Arctic Sea Ice Extent, Sea Ice Age, and Snow Depth on Sea Salt Aerosol From Blowing Snow and the Open Ocean for 1980–2017 K. Confer et al. 10.1029/2022JD037667
- Tropospheric bromine monoxide vertical profiles retrieved across the Alaskan Arctic in springtime N. Brockway et al. 10.5194/acp-24-23-2024
- Technical note: Sublimation of frozen CsCl solutions in an environmental scanning electron microscope (ESEM) – determining the number and size of salt particles relevant to sea salt aerosols L. Vetráková et al. 10.5194/acp-23-4463-2023
- Surface snow bromide and nitrate at Eureka, Canada, in early spring and implications for polar boundary layer chemistry X. Yang et al. 10.5194/acp-24-5863-2024
- Arctic tropospheric ozone: assessment of current knowledge and model performance C. Whaley et al. 10.5194/acp-23-637-2023
- Application of Satellite‐Based Detections of Arctic Bromine Explosion Events Within GEOS‐Chem P. Wales et al. 10.1029/2022MS003465
11 citations as recorded by crossref.
- Global Observations of Tropospheric Bromine Monoxide (BrO) Columns From TROPOMI Y. Chen et al. 10.1029/2023JD039091
- Modelling the coupled mercury-halogen-ozone cycle in the central Arctic during spring S. Ahmed et al. 10.1525/elementa.2022.00129
- Implications of Snowpack Reactive Bromine Production for Arctic Ice Core Bromine Preservation S. Zhai et al. 10.1029/2023JD039257
- Low ozone dry deposition rates to sea ice during the MOSAiC field campaign: Implications for the Arctic boundary layer ozone budget J. Barten et al. 10.1525/elementa.2022.00086
- Arctic halogens reduce ozone in the northern mid-latitudes R. Fernandez et al. 10.1073/pnas.2401975121
- Impact of Changing Arctic Sea Ice Extent, Sea Ice Age, and Snow Depth on Sea Salt Aerosol From Blowing Snow and the Open Ocean for 1980–2017 K. Confer et al. 10.1029/2022JD037667
- Tropospheric bromine monoxide vertical profiles retrieved across the Alaskan Arctic in springtime N. Brockway et al. 10.5194/acp-24-23-2024
- Technical note: Sublimation of frozen CsCl solutions in an environmental scanning electron microscope (ESEM) – determining the number and size of salt particles relevant to sea salt aerosols L. Vetráková et al. 10.5194/acp-23-4463-2023
- Surface snow bromide and nitrate at Eureka, Canada, in early spring and implications for polar boundary layer chemistry X. Yang et al. 10.5194/acp-24-5863-2024
- Arctic tropospheric ozone: assessment of current knowledge and model performance C. Whaley et al. 10.5194/acp-23-637-2023
- Application of Satellite‐Based Detections of Arctic Bromine Explosion Events Within GEOS‐Chem P. Wales et al. 10.1029/2022MS003465
Latest update: 20 Nov 2024
Short summary
Radical bromine molecules are seen at higher concentrations during the Arctic spring. We use the global model GEOS-Chem to test whether snowpack and wind-blown snow sources can explain high bromine concentrations. We run this model for the entire year of 2015 and compare results to observations of bromine from floating platforms on the Arctic Ocean and at Utqiaġvik. We find that the model performs best when both sources are enabled but may overestimate bromine production in summer and fall.
Radical bromine molecules are seen at higher concentrations during the Arctic spring. We use the...
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