Articles | Volume 22, issue 20
https://doi.org/10.5194/acp-22-13495-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-22-13495-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Ozone depletion events in the Arctic spring of 2019: a new modeling approach to bromine emissions
Maximilian Herrmann
Interdisciplinary Center for Scientific Computing, Heidelberg University, Im Neuenheimer Feld 205, 69120 Heidelberg, Germany
Moritz Schöne
Max-Planck Institute for Chemistry, Hahn-Meitner-Weg 1, 55128 Mainz, Germany
Institute of Environmental Physics, Heidelberg University, Im Neuenheimer Feld 229, 69120 Heidelberg, Germany
Christian Borger
Max-Planck Institute for Chemistry, Hahn-Meitner-Weg 1, 55128 Mainz, Germany
Simon Warnach
Max-Planck Institute for Chemistry, Hahn-Meitner-Weg 1, 55128 Mainz, Germany
Institute of Environmental Physics, Heidelberg University, Im Neuenheimer Feld 229, 69120 Heidelberg, Germany
Thomas Wagner
Max-Planck Institute for Chemistry, Hahn-Meitner-Weg 1, 55128 Mainz, Germany
Institute of Environmental Physics, Heidelberg University, Im Neuenheimer Feld 229, 69120 Heidelberg, Germany
Ulrich Platt
Institute of Environmental Physics, Heidelberg University, Im Neuenheimer Feld 229, 69120 Heidelberg, Germany
Heidelberg Center for the Environment, Heidelberg University, Im Neuenheimer Feld 130.1, 69120 Heidelberg, Germany
Eva Gutheil
CORRESPONDING AUTHOR
Interdisciplinary Center for Scientific Computing, Heidelberg University, Im Neuenheimer Feld 205, 69120 Heidelberg, Germany
Heidelberg Center for the Environment, Heidelberg University, Im Neuenheimer Feld 130.1, 69120 Heidelberg, Germany
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Cited
10 citations as recorded by crossref.
- On the dynamics of ozone depletion events at Villum Research Station in the High Arctic J. Pernov et al. 10.5194/acp-24-13603-2024
- Incorporation of multi-phase halogen chemistry into the Community Multiscale Air Quality (CMAQ) model K. Kim et al. 10.5194/acp-25-10293-2025
- Modelling the coupled mercury-halogen-ozone cycle in the central Arctic during spring S. Ahmed et al. 10.1525/elementa.2022.00129
- A new accurate retrieval algorithm of bromine monoxide columns inside minor volcanic plumes from Sentinel-5P TROPOMI observations S. Warnach et al. 10.5194/amt-16-5537-2023
- Global Observations of Tropospheric Bromine Monoxide (BrO) Columns From TROPOMI Y. Chen et al. 10.1029/2023JD039091
- A three-dimensional simulation and process analysis of tropospheric ozone depletion events (ODEs) during the springtime in the Arctic using CMAQ (Community Multiscale Air Quality Modeling System) L. Cao et al. 10.5194/acp-23-3363-2023
- The use of δ 13C in CO to determine removal of CH4 by Cl radicals in the atmosphere * T. Röckmann et al. 10.1088/1748-9326/ad4375
- Source mechanisms and transport patterns of tropospheric bromine monoxide: findings from long-term multi-axis differential optical absorption spectroscopy measurements at two Antarctic stations U. Frieß et al. 10.5194/acp-23-3207-2023
- Global retrieval of stratospheric and tropospheric BrO columns from the Ozone Mapping and Profiler Suite Nadir Mapper (OMPS-NM) on board the Suomi-NPP satellite H. Chong et al. 10.5194/amt-17-2873-2024
- Implications of Snowpack Reactive Bromine Production for Arctic Ice Core Bromine Preservation S. Zhai et al. 10.1029/2023JD039257
10 citations as recorded by crossref.
- On the dynamics of ozone depletion events at Villum Research Station in the High Arctic J. Pernov et al. 10.5194/acp-24-13603-2024
- Incorporation of multi-phase halogen chemistry into the Community Multiscale Air Quality (CMAQ) model K. Kim et al. 10.5194/acp-25-10293-2025
- Modelling the coupled mercury-halogen-ozone cycle in the central Arctic during spring S. Ahmed et al. 10.1525/elementa.2022.00129
- A new accurate retrieval algorithm of bromine monoxide columns inside minor volcanic plumes from Sentinel-5P TROPOMI observations S. Warnach et al. 10.5194/amt-16-5537-2023
- Global Observations of Tropospheric Bromine Monoxide (BrO) Columns From TROPOMI Y. Chen et al. 10.1029/2023JD039091
- A three-dimensional simulation and process analysis of tropospheric ozone depletion events (ODEs) during the springtime in the Arctic using CMAQ (Community Multiscale Air Quality Modeling System) L. Cao et al. 10.5194/acp-23-3363-2023
- The use of δ 13C in CO to determine removal of CH4 by Cl radicals in the atmosphere * T. Röckmann et al. 10.1088/1748-9326/ad4375
- Source mechanisms and transport patterns of tropospheric bromine monoxide: findings from long-term multi-axis differential optical absorption spectroscopy measurements at two Antarctic stations U. Frieß et al. 10.5194/acp-23-3207-2023
- Global retrieval of stratospheric and tropospheric BrO columns from the Ozone Mapping and Profiler Suite Nadir Mapper (OMPS-NM) on board the Suomi-NPP satellite H. Chong et al. 10.5194/amt-17-2873-2024
- Implications of Snowpack Reactive Bromine Production for Arctic Ice Core Bromine Preservation S. Zhai et al. 10.1029/2023JD039257
Latest update: 17 Sep 2025
Short summary
Ozone depletion events (ODEs) are a common occurrence in the boundary layer during Arctic spring. Ozone is depleted by bromine species in an autocatalytic reaction cycle. Previous modeling studies assumed an infinite bromine source at the ground. An alternative emission scheme is presented in which a finite amount of bromide in the snow is tracked over time. The Weather Research and Forecasting model coupled with Chemistry (WRF-Chem) is used to study ODEs in the Arctic from February to May 2019.
Ozone depletion events (ODEs) are a common occurrence in the boundary layer during Arctic...
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