Articles | Volume 22, issue 15
https://doi.org/10.5194/acp-22-10023-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Special issue:
https://doi.org/10.5194/acp-22-10023-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
04 Aug 2022
Research article |
| 04 Aug 2022
| 04 Aug 2022
Secondary aerosol formation in marine Arctic environments: a model measurement comparison at Ny-Ålesund
Carlton Xavier
CORRESPONDING AUTHOR
Institute for Atmospheric and Earth Systems Research, University of
Helsinki, P.O. Box 64, 00014 Helsinki, Finland
Metin Baykara
Institute for Atmospheric and Earth Systems Research, University of
Helsinki, P.O. Box 64, 00014 Helsinki, Finland
Climate and Marine Sciences Department, Eurasia Institute of Earth
Sciences, Istanbul Technical University, Maslak 34469, Istanbul, Turkey
Robin Wollesen de Jonge
Division of Nuclear Physics, Department of Physics, Lund University,
P.O. Box 118, 221 00 Lund, Sweden
Barbara Altstädter
Institute of Flight Guidance, Technische Universität Braunschweig,
38108 Braunschweig, Germany
Petri Clusius
Institute for Atmospheric and Earth Systems Research, University of
Helsinki, P.O. Box 64, 00014 Helsinki, Finland
Ville Vakkari
Atmospheric Chemistry Research Group, Chemical Resource Beneficiation,
North-West University, Potchefstroom, South Africa
Finnish Meteorological Institute, P.O. Box 503, 00101 Helsinki,
Finland
Roseline Thakur
Institute for Atmospheric and Earth Systems Research, University of
Helsinki, P.O. Box 64, 00014 Helsinki, Finland
Lisa Beck
Institute for Atmospheric and Earth Systems Research, University of
Helsinki, P.O. Box 64, 00014 Helsinki, Finland
Silvia Becagli
Department of Chemistry, University of Florence, Sesto Fiorentino,
50019 Florence, Italy
Mirko Severi
Department of Chemistry, University of Florence, Sesto Fiorentino,
50019 Florence, Italy
Rita Traversi
Department of Chemistry, University of Florence, Sesto Fiorentino,
50019 Florence, Italy
Radovan Krejci
Department of Environmental Science, Stockholm University, Stockholm,
Sweden
Bolin Centre for Climate Research, Stockholm University, Stockholm,
Sweden
Peter Tunved
Department of Environmental Science, Stockholm University, Stockholm,
Sweden
Bolin Centre for Climate Research, Stockholm University, Stockholm,
Sweden
Mauro Mazzola
National Research Council of Italy, Institute of Polar Sciences
(CNR-ISP), Bologna, Italy
Birgit Wehner
Institute of Tropospheric Research, 04318 Leipzig, Germany
Mikko Sipilä
Institute for Atmospheric and Earth Systems Research, University of
Helsinki, P.O. Box 64, 00014 Helsinki, Finland
Markku Kulmala
Institute for Atmospheric and Earth Systems Research, University of
Helsinki, P.O. Box 64, 00014 Helsinki, Finland
Michael Boy
Institute for Atmospheric and Earth Systems Research, University of
Helsinki, P.O. Box 64, 00014 Helsinki, Finland
LUT School of Engineering Science, Lappeenranta-Lahti University of
Technology, P.O. Box 20, 53851 Lappeenranta, Finland
Pontus Roldin
CORRESPONDING AUTHOR
Division of Nuclear Physics, Department of Physics, Lund University,
P.O. Box 118, 221 00 Lund, Sweden
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Cited
6 citations as recorded by crossref.
- Revealing the chemical characteristics of Arctic low-level cloud residuals – in situ observations from a mountain site Y. Gramlich et al. 10.5194/acp-23-6813-2023
- Arctic observations of hydroperoxymethyl thioformate (HPMTF) – seasonal behavior and relationship to other oxidation products of dimethyl sulfide at the Zeppelin Observatory, Svalbard K. Siegel et al. 10.5194/acp-23-7569-2023
- Spatial distribution and variability of boundary layer aerosol particles observed in Ny-Ålesund during late spring in 2018 B. Harm-Altstädter et al. 10.5194/ar-1-39-2023
- Role of Iodine-Assisted Aerosol Particle Formation in Antarctica C. Xavier et al. 10.1021/acs.est.3c09103
- A new implementation of FLEXPART with Enviro-HIRLAM meteorological input, and a case study during a heavy air pollution event B. Foreback et al. 10.1080/20964471.2024.2316320
- Atmospherically Relevant Chemistry and Aerosol box model – ARCA box (version 1.2) P. Clusius et al. 10.5194/gmd-15-7257-2022
6 citations as recorded by crossref.
- Revealing the chemical characteristics of Arctic low-level cloud residuals – in situ observations from a mountain site Y. Gramlich et al. 10.5194/acp-23-6813-2023
- Arctic observations of hydroperoxymethyl thioformate (HPMTF) – seasonal behavior and relationship to other oxidation products of dimethyl sulfide at the Zeppelin Observatory, Svalbard K. Siegel et al. 10.5194/acp-23-7569-2023
- Spatial distribution and variability of boundary layer aerosol particles observed in Ny-Ålesund during late spring in 2018 B. Harm-Altstädter et al. 10.5194/ar-1-39-2023
- Role of Iodine-Assisted Aerosol Particle Formation in Antarctica C. Xavier et al. 10.1021/acs.est.3c09103
- A new implementation of FLEXPART with Enviro-HIRLAM meteorological input, and a case study during a heavy air pollution event B. Foreback et al. 10.1080/20964471.2024.2316320
- Atmospherically Relevant Chemistry and Aerosol box model – ARCA box (version 1.2) P. Clusius et al. 10.5194/gmd-15-7257-2022
Latest update: 25 Apr 2024
Short summary
The focus of this work is to study and improve our understanding of processes involved in the formation and growth of new particles in a remote Arctic marine environment. We run the 1D model ADCHEM along air mass trajectories arriving at Ny-Ålesund in May 2018. The model finds that ion-mediated H2SO4–NH3 nucleation can explain the observed new particle formation at Ny-Ålesund. The growth of particles is driven via H2SO4 condensation and formation of methane sulfonic acid in the aqueous phase.
The focus of this work is to study and improve our understanding of processes involved in the...
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