Articles | Volume 21, issue 11
https://doi.org/10.5194/acp-21-9089-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-21-9089-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
15 Jun 2021
Research article |
| 15 Jun 2021
| 15 Jun 2021
Urban organic aerosol composition in eastern China differs from north to south: molecular insight from a liquid chromatography–mass spectrometry (Orbitrap) study
State Key Laboratory of Loess and Quaternary Geology (SKLLQG), Center
for Excellence in Quaternary Science and Global Change, and Key Laboratory
of Aerosol Chemistry and Physics, Institute of Earth and Environment,
Chinese Academy of Sciences, Xi'an 710061, China
Institute of Inorganic and Analytical Chemistry, Johannes Gutenberg
University Mainz, Duesbergweg 10–14, Mainz 55128, Germany
Department of Chemistry, Aarhus University, Langelandsgade 140,
8000 Aarhus C, Denmark
Ru-Jin Huang
CORRESPONDING AUTHOR
State Key Laboratory of Loess and Quaternary Geology (SKLLQG), Center
for Excellence in Quaternary Science and Global Change, and Key Laboratory
of Aerosol Chemistry and Physics, Institute of Earth and Environment,
Chinese Academy of Sciences, Xi'an 710061, China
Open Studio for Oceanic-Continental Climate and Environment Changes,
Pilot National Laboratory for Marine Science and Technology (Qingdao),
Qingdao 266061, China
Martin Brüggemann
Atmospheric Chemistry Department (ACD), Leibniz Institute for
Tropospheric Research (TROPOS), Permoserstraße 15, 04318 Leipzig,
Germany
Yun Zhang
Institute of Inorganic and Analytical Chemistry, Johannes Gutenberg
University Mainz, Duesbergweg 10–14, Mainz 55128, Germany
Lu Yang
State Key Laboratory of Loess and Quaternary Geology (SKLLQG), Center
for Excellence in Quaternary Science and Global Change, and Key Laboratory
of Aerosol Chemistry and Physics, Institute of Earth and Environment,
Chinese Academy of Sciences, Xi'an 710061, China
Haiyan Ni
State Key Laboratory of Loess and Quaternary Geology (SKLLQG), Center
for Excellence in Quaternary Science and Global Change, and Key Laboratory
of Aerosol Chemistry and Physics, Institute of Earth and Environment,
Chinese Academy of Sciences, Xi'an 710061, China
Jie Guo
State Key Laboratory of Loess and Quaternary Geology (SKLLQG), Center
for Excellence in Quaternary Science and Global Change, and Key Laboratory
of Aerosol Chemistry and Physics, Institute of Earth and Environment,
Chinese Academy of Sciences, Xi'an 710061, China
Meng Wang
State Key Laboratory of Loess and Quaternary Geology (SKLLQG), Center
for Excellence in Quaternary Science and Global Change, and Key Laboratory
of Aerosol Chemistry and Physics, Institute of Earth and Environment,
Chinese Academy of Sciences, Xi'an 710061, China
Jiajun Han
Department of Chemistry, University of Toronto, 80 St. George Street,
M5S3H6 Toronto, Canada
Merete Bilde
Department of Chemistry, Aarhus University, Langelandsgade 140,
8000 Aarhus C, Denmark
Marianne Glasius
Department of Chemistry, Aarhus University, Langelandsgade 140,
8000 Aarhus C, Denmark
Thorsten Hoffmann
CORRESPONDING AUTHOR
Institute of Inorganic and Analytical Chemistry, Johannes Gutenberg
University Mainz, Duesbergweg 10–14, Mainz 55128, Germany
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- Factors Influencing the Molecular Compositions and Distributions of Atmospheric Nitrogen‐Containing Compounds H. Jiang et al. 10.1029/2021JD036284
- Modeling Secondary Organic Aerosols in China: State of the Art and Perspectives J. Li et al. 10.1007/s40726-022-00246-3
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- Measurement report: Characteristics of nitrogen-containing organics in PM2.5 in Ürümqi, northwestern China – differential impacts of combustion of fresh and aged biomass materials Y. Ma et al. 10.5194/acp-24-4331-2024
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- Particulate matter pollution and non-targeted analysis of polar compounds in three regions of Brazil S. Pozza et al. 10.1016/j.chemosphere.2023.139839
- Aqueous secondary organic aerosol formation from the direct photosensitized oxidation of vanillin in the absence and presence of ammonium nitrate B. Mabato et al. 10.5194/acp-22-273-2022
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- More water-soluble brown carbon after the residential “coal-to-gas” conversion measure in urban Beijing W. Yuan et al. 10.1038/s41612-023-00355-w
- Insight into the Role of NH3/NH4+ and NOx/NO3– in the Formation of Nitrogen-Containing Brown Carbon in Chinese Megacities D. Wang et al. 10.1021/acs.est.3c10374
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- Non-targeted analysis (NTA) and suspect screening analysis (SSA): a review of examining the chemical exposome K. Manz et al. 10.1038/s41370-023-00574-6
- Comparison of aqueous secondary organic aerosol (aqSOA) product distributions from guaiacol oxidation by non-phenolic and phenolic methoxybenzaldehydes as photosensitizers in the absence and presence of ammonium nitrate B. Mabato et al. 10.5194/acp-23-2859-2023
- Molecular characteristics of ambient organic aerosols in Shanghai winter before and after the COVID-19 outbreak W. Wen et al. 10.1016/j.scitotenv.2023.161811
- Abundant nitrogenous secondary organic aerosol formation accelerated by cloud processing Z. Liu et al. 10.1016/j.isci.2023.108317
- Particle characterization and quantification of organic and inorganic compounds from Chinese and Iranian aerosol filter samples using scanning laser desorption/ionization mass spectrometry C. Barth et al. 10.1007/s00216-022-04275-1
- Molecular characterization of nitrogen-containing organic compounds in the winter North China Plain J. Mao et al. 10.1016/j.scitotenv.2022.156189
- Molecular characteristics, sources, and formation pathways of organosulfur compounds in ambient aerosol in Guangzhou, South China H. Jiang et al. 10.5194/acp-22-6919-2022
- Interfacial Ozone Oxidation Chemistry at a Riverine Surface Microlayer as a Source of Nitrogen Organic Compounds Y. Wang et al. 10.1021/acs.estlett.2c00130
- Unveiling the Molecular Characteristics, Origins, and Formation Mechanism of Reduced Nitrogen Organic Compounds in the Urban Atmosphere of Shanghai Using a Versatile Aerosol Concentration Enrichment System M. Abudumutailifu et al. 10.1021/acs.est.3c04071
- Discovery of emerging organic pollutants in the atmosphere through an omics approach Z. Cheng et al. 10.1007/s11783-023-1645-9
- Molecular characterization of organic aerosols in Taiyuan, China: Seasonal variation and source identification W. Wang et al. 10.1016/j.scitotenv.2021.149419
- Evolution of organic carbon during COVID-19 lockdown period: Possible contribution of nocturnal chemistry Z. Feng et al. 10.1016/j.scitotenv.2021.152191
27 citations as recorded by crossref.
- The Significant Contribution of Polycyclic Aromatic Nitrogen Heterocycles to Light Absorption in the Winter North China Plain Y. Cheng et al. 10.3390/su15118568
- Chemical Characterization of Rural Organic Aerosol in the North China Plain Using Ultrahigh-Resolution Mass Spectrometry Y. Zhang et al. 10.3390/atmos14111636
- Factors Influencing the Molecular Compositions and Distributions of Atmospheric Nitrogen‐Containing Compounds H. Jiang et al. 10.1029/2021JD036284
- Modeling Secondary Organic Aerosols in China: State of the Art and Perspectives J. Li et al. 10.1007/s40726-022-00246-3
- Chemical composition of secondary organic aerosol particles formed from mixtures of anthropogenic and biogenic precursors Y. Shao et al. 10.5194/acp-22-9799-2022
- Enhanced Production of Organosulfur Species during a Severe Winter Haze Episode in the Guanzhong Basin of Northwest China Y. Han et al. 10.1021/acs.est.3c02914
- Molecular Characteristics of Atmospheric Organosulfates During Summer and Winter Seasons in Two Cities of Southern and Northern China Y. Lin et al. 10.1029/2022JD036672
- Measurement report: Characteristics of nitrogen-containing organics in PM2.5 in Ürümqi, northwestern China – differential impacts of combustion of fresh and aged biomass materials Y. Ma et al. 10.5194/acp-24-4331-2024
- Characteristics of dissolved organic matter (DOM) in Chinese farmland soils under different climate zone types: A molecular perspective B. Han et al. 10.1016/j.jenvman.2023.119695
- Particulate matter pollution and non-targeted analysis of polar compounds in three regions of Brazil S. Pozza et al. 10.1016/j.chemosphere.2023.139839
- Aqueous secondary organic aerosol formation from the direct photosensitized oxidation of vanillin in the absence and presence of ammonium nitrate B. Mabato et al. 10.5194/acp-22-273-2022
- Molecular Signatures and Sources of Fluorescent Components in Atmospheric Organic Matter in South China H. Jiang et al. 10.1021/acs.estlett.2c00629
- More water-soluble brown carbon after the residential “coal-to-gas” conversion measure in urban Beijing W. Yuan et al. 10.1038/s41612-023-00355-w
- Insight into the Role of NH3/NH4+ and NOx/NO3– in the Formation of Nitrogen-Containing Brown Carbon in Chinese Megacities D. Wang et al. 10.1021/acs.est.3c10374
- Nontarget Screening Exhibits a Seasonal Cycle of PM2.5 Organic Aerosol Composition in Beijing J. Ma et al. 10.1021/acs.est.1c06905
- Non-targeted analysis (NTA) and suspect screening analysis (SSA): a review of examining the chemical exposome K. Manz et al. 10.1038/s41370-023-00574-6
- Comparison of aqueous secondary organic aerosol (aqSOA) product distributions from guaiacol oxidation by non-phenolic and phenolic methoxybenzaldehydes as photosensitizers in the absence and presence of ammonium nitrate B. Mabato et al. 10.5194/acp-23-2859-2023
- Molecular characteristics of ambient organic aerosols in Shanghai winter before and after the COVID-19 outbreak W. Wen et al. 10.1016/j.scitotenv.2023.161811
- Abundant nitrogenous secondary organic aerosol formation accelerated by cloud processing Z. Liu et al. 10.1016/j.isci.2023.108317
- Particle characterization and quantification of organic and inorganic compounds from Chinese and Iranian aerosol filter samples using scanning laser desorption/ionization mass spectrometry C. Barth et al. 10.1007/s00216-022-04275-1
- Molecular characterization of nitrogen-containing organic compounds in the winter North China Plain J. Mao et al. 10.1016/j.scitotenv.2022.156189
- Molecular characteristics, sources, and formation pathways of organosulfur compounds in ambient aerosol in Guangzhou, South China H. Jiang et al. 10.5194/acp-22-6919-2022
- Interfacial Ozone Oxidation Chemistry at a Riverine Surface Microlayer as a Source of Nitrogen Organic Compounds Y. Wang et al. 10.1021/acs.estlett.2c00130
- Unveiling the Molecular Characteristics, Origins, and Formation Mechanism of Reduced Nitrogen Organic Compounds in the Urban Atmosphere of Shanghai Using a Versatile Aerosol Concentration Enrichment System M. Abudumutailifu et al. 10.1021/acs.est.3c04071
- Discovery of emerging organic pollutants in the atmosphere through an omics approach Z. Cheng et al. 10.1007/s11783-023-1645-9
- Molecular characterization of organic aerosols in Taiyuan, China: Seasonal variation and source identification W. Wang et al. 10.1016/j.scitotenv.2021.149419
- Evolution of organic carbon during COVID-19 lockdown period: Possible contribution of nocturnal chemistry Z. Feng et al. 10.1016/j.scitotenv.2021.152191
Latest update: 25 Apr 2024
Short summary
Here we present the detailed molecular composition of the organic aerosol collected in three eastern Chinese cities from north to south, Changchun, Shanghai and Guangzhou, by applying LC–Orbitrap analysis. Accordingly, the aromaticity degree of chemical compounds decreases from north to south, while the oxidation degree increases from north to south, which can be explained by the different anthropogenic emissions and photochemical oxidation processes.
Here we present the detailed molecular composition of the organic aerosol collected in three...
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