Articles | Volume 21, issue 10
https://doi.org/10.5194/acp-21-8357-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-21-8357-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
01 Jun 2021
Research article |
| 01 Jun 2021
| 01 Jun 2021
Isotopic constraints on atmospheric sulfate formation pathways in the Mt. Everest region, southern Tibetan Plateau
Kun Wang
State Key Laboratory of Cryospheric Science, Northwest Institute of Eco-Environment and Resources, Chinese Academy of Sciences (CAS), Lanzhou 730000, China
Department of Chemical Science and Engineering, School of Materials and Chemical Technology, Tokyo Institute of Technology, 4259 Nagatsuta-cho, Midori-ku, Yokohama, Kanagawa 226-8502, Japan
University of Chinese Academy of Sciences, Beijing 100049, China
Shohei Hattori
CORRESPONDING AUTHOR
Department of Chemical Science and Engineering, School of Materials and Chemical Technology, Tokyo Institute of Technology, 4259 Nagatsuta-cho, Midori-ku, Yokohama, Kanagawa 226-8502, Japan
Department of Chemical Science and Engineering, School of Materials and Chemical Technology, Tokyo Institute of Technology, 4259 Nagatsuta-cho, Midori-ku, Yokohama, Kanagawa 226-8502, Japan
State Key Laboratory of Isotope Geochemistry, Guangzhou Institute of Geochemistry, CAS, Guangzhou 510640, China
CAS Center for Excellence in Deep Earth Science, Guangzhou 510640, China
Sakiko Ishino
Department of Chemical Science and Engineering, School of Materials and Chemical Technology, Tokyo Institute of Technology, 4259 Nagatsuta-cho, Midori-ku, Yokohama, Kanagawa 226-8502, Japan
National Institute of Polar Research, Research Organization of Information and Systems, Tokyo 190-8518, Japan
Becky Alexander
Department of Atmospheric Sciences, University of Washington, Seattle, WA 98195, USA
Kazuki Kamezaki
Department of Chemical Science and Engineering, School of Materials and Chemical Technology, Tokyo Institute of Technology, 4259 Nagatsuta-cho, Midori-ku, Yokohama, Kanagawa 226-8502, Japan
Faculty of Science and Technology, Sophia University, 7-1 Kioi-cho, Chiyoda-ku, Tokyo 102-8554, Japan
Naohiro Yoshida
Department of Chemical Science and Engineering, School of Materials and Chemical Technology, Tokyo Institute of Technology, 4259 Nagatsuta-cho, Midori-ku, Yokohama, Kanagawa 226-8502, Japan
Earth-Life Science Institute, Tokyo Institute of Technology, Meguro-ku, Tokyo 152-8551, Japan
National Institute of Information and Communications Technology, Koganei, Tokyo 184-8795, Japan
Shichang Kang
CORRESPONDING AUTHOR
State Key Laboratory of Cryospheric Science, Northwest Institute of Eco-Environment and Resources, Chinese Academy of Sciences (CAS), Lanzhou 730000, China
CAS Center for Excellence in Tibetan Plateau Earth Sciences, Beijing 100101, China
University of Chinese Academy of Sciences, Beijing 100049, China
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19 citations as recorded by crossref.
- 40 years of theoretical advances in mass-independent oxygen isotope effects and applications in atmospheric chemistry: A critical review and perspectives M. Lin & M. Thiemens 10.1016/j.apgeochem.2023.105860
- Atmospheric sulfur cycle elucidated by isotopologue measurements S. HATTORI et al. 10.3724/j.issn.1007-2802.20240068
- Gypsum formation from calcite in the atmosphere recorded in aerosol particles transported and trapped in Greenland ice core sample is a signature of secular change of SO2 emission in East Asia C. Miyamoto et al. 10.1016/j.atmosenv.2022.119061
- Tracing the origin of elevated springtime atmospheric sulfate on the southern Himalayan-Tibetan plateau S. Dasari et al. 10.1039/D3VA00085K
- Ground-based vertical profile observations of atmospheric composition on the Tibetan Plateau (2017–2019) C. Xing et al. 10.5194/essd-13-4897-2021
- Role of Dust and Iron Solubility in Sulfate Formation during the Long-Range Transport in East Asia Evidenced by 17O-Excess Signatures S. Itahashi et al. 10.1021/acs.est.2c03574
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- Significant formation of sulfate aerosols contributed by the heterogeneous drivers of dust surface T. Wang et al. 10.5194/acp-22-13467-2022
- Sulfate sources, biologic cycling, and mobility in Atacama Desert soils revealed by isotope signatures S. Klipsch et al. 10.1016/j.gloplacha.2023.104290
- Analysis of Atmospheric Radiosulfur at Natural Abundance by a New-Type Liquid Scintillation Counter Equipped with Guard Compensation Technology X. Lin et al. 10.1021/acsearthspacechem.2c00104
- Acidity and the multiphase chemistry of atmospheric aqueous particles and clouds A. Tilgner et al. 10.5194/acp-21-13483-2021
- SE‐Dome II Ice Core Dating With Half‐Year Precision: Increasing Melting Events From 1799 to 2020 in Southeastern Greenland K. Kawakami et al. 10.1029/2023JD038874
- The Earth's atmosphere – A stable isotope perspective and review J. Hoefs & R. Harmon 10.1016/j.apgeochem.2022.105355
- Isotopic Constraints on SO2 Oxidation Rates and Their Potential Relationship with Sulfate Formation Pathways in the Planetary Boundary Layer Z. Niu & M. Lin 10.1021/acsenvironau.4c00070
- Latitudinal difference in sulfate formation from methanesulfonate oxidation in Antarctic snow imprinted on 17O-excess signature S. Hattori et al. 10.1016/j.apgeochem.2024.105901
- Significant overestimation of black carbon concentration caused by high organic carbon in aerosols of the Tibetan Plateau Z. Hu et al. 10.1016/j.atmosenv.2022.119486
- Transported aerosols regulate the pre-monsoon rainfall over north-east India: a WRF-Chem modelling study N. Barman & S. Gokhale 10.5194/acp-23-6197-2023
- Himalayas as a global hot spot of springtime stratospheric intrusions: Insight from isotopic signatures in sulfate aerosols K. Wang et al. 10.1016/j.rcar.2024.03.002
- Record of pre-industrial atmospheric sulfate in continental interiors Y. Peng et al. 10.1038/s41561-023-01211-5
19 citations as recorded by crossref.
- 40 years of theoretical advances in mass-independent oxygen isotope effects and applications in atmospheric chemistry: A critical review and perspectives M. Lin & M. Thiemens 10.1016/j.apgeochem.2023.105860
- Atmospheric sulfur cycle elucidated by isotopologue measurements S. HATTORI et al. 10.3724/j.issn.1007-2802.20240068
- Gypsum formation from calcite in the atmosphere recorded in aerosol particles transported and trapped in Greenland ice core sample is a signature of secular change of SO2 emission in East Asia C. Miyamoto et al. 10.1016/j.atmosenv.2022.119061
- Tracing the origin of elevated springtime atmospheric sulfate on the southern Himalayan-Tibetan plateau S. Dasari et al. 10.1039/D3VA00085K
- Ground-based vertical profile observations of atmospheric composition on the Tibetan Plateau (2017–2019) C. Xing et al. 10.5194/essd-13-4897-2021
- Role of Dust and Iron Solubility in Sulfate Formation during the Long-Range Transport in East Asia Evidenced by 17O-Excess Signatures S. Itahashi et al. 10.1021/acs.est.2c03574
- Observations of the vertical distributions of summertime atmospheric pollutants in Nam Co: OH production and source analysis C. Xing et al. 10.5194/acp-24-10093-2024
- Significant formation of sulfate aerosols contributed by the heterogeneous drivers of dust surface T. Wang et al. 10.5194/acp-22-13467-2022
- Sulfate sources, biologic cycling, and mobility in Atacama Desert soils revealed by isotope signatures S. Klipsch et al. 10.1016/j.gloplacha.2023.104290
- Analysis of Atmospheric Radiosulfur at Natural Abundance by a New-Type Liquid Scintillation Counter Equipped with Guard Compensation Technology X. Lin et al. 10.1021/acsearthspacechem.2c00104
- Acidity and the multiphase chemistry of atmospheric aqueous particles and clouds A. Tilgner et al. 10.5194/acp-21-13483-2021
- SE‐Dome II Ice Core Dating With Half‐Year Precision: Increasing Melting Events From 1799 to 2020 in Southeastern Greenland K. Kawakami et al. 10.1029/2023JD038874
- The Earth's atmosphere – A stable isotope perspective and review J. Hoefs & R. Harmon 10.1016/j.apgeochem.2022.105355
- Isotopic Constraints on SO2 Oxidation Rates and Their Potential Relationship with Sulfate Formation Pathways in the Planetary Boundary Layer Z. Niu & M. Lin 10.1021/acsenvironau.4c00070
- Latitudinal difference in sulfate formation from methanesulfonate oxidation in Antarctic snow imprinted on 17O-excess signature S. Hattori et al. 10.1016/j.apgeochem.2024.105901
- Significant overestimation of black carbon concentration caused by high organic carbon in aerosols of the Tibetan Plateau Z. Hu et al. 10.1016/j.atmosenv.2022.119486
- Transported aerosols regulate the pre-monsoon rainfall over north-east India: a WRF-Chem modelling study N. Barman & S. Gokhale 10.5194/acp-23-6197-2023
- Himalayas as a global hot spot of springtime stratospheric intrusions: Insight from isotopic signatures in sulfate aerosols K. Wang et al. 10.1016/j.rcar.2024.03.002
- Record of pre-industrial atmospheric sulfate in continental interiors Y. Peng et al. 10.1038/s41561-023-01211-5
Latest update: 17 Apr 2025
Short summary
Sulfate aerosols play an important climatic role and exert adverse effects on the ecological environment and human health. In this study, we present the triple oxygen isotopic composition of sulfate from the Mt. Everest region, southern Tibetan Plateau, and decipher the formation mechanisms of atmospheric sulfate in this pristine environment. The results indicate the important role of the S(IV) + O3 pathway in atmospheric sulfate formation promoted by conditions of high cloud water pH.
Sulfate aerosols play an important climatic role and exert adverse effects on the ecological...
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