Articles | Volume 21, issue 10
https://doi.org/10.5194/acp-21-8273-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-21-8273-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
28 May 2021
Research article |
| 28 May 2021
| 28 May 2021
Source apportionment of carbonaceous aerosols in Beijing with radiocarbon and organic tracers: insight into the differences between urban and rural sites
Siqi Hou
School of Geography Earth and Environmental Science, University of Birmingham, Birmingham, B15 2TT, UK
Di Liu
School of Geography Earth and Environmental Science, University of Birmingham, Birmingham, B15 2TT, UK
now at: Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing, 100029, China
Jingsha Xu
School of Geography Earth and Environmental Science, University of Birmingham, Birmingham, B15 2TT, UK
Tuan V. Vu
School of Geography Earth and Environmental Science, University of Birmingham, Birmingham, B15 2TT, UK
now at: School of Public Health, Imperial College London, London, UK
Xuefang Wu
School of Earth Sciences and Resources, China University of Geosciences, Xueyuan Road 29, Beijing, 100083, China
Deepchandra Srivastava
School of Geography Earth and Environmental Science, University of Birmingham, Birmingham, B15 2TT, UK
Pingqing Fu
Institute of Surface-Earth System Science, Tianjin University, Tianjin, 300072, China
Linjie Li
State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry Institute of Atmospheric, Physics, Chinese Academy of Sciences, Beijing, 100029, China
now at: Department of Chemistry and Molecular Biology, University of Gothenburg, Gothenburg 41296, Sweden
State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry Institute of Atmospheric, Physics, Chinese Academy of Sciences, Beijing, 100029, China
Athanasia Vlachou
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, Villigen PSI, 5232, Switzerland
Vaios Moschos
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, Villigen PSI, 5232, Switzerland
Gary Salazar
Department of Chemistry and Biochemistry & Oeschger Centre for Climate Change Research, University of Bern, Bern, 3012, Switzerland
Sönke Szidat
Department of Chemistry and Biochemistry & Oeschger Centre for Climate Change Research, University of Bern, Bern, 3012, Switzerland
André S. H. Prévôt
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, Villigen PSI, 5232, Switzerland
School of Geography Earth and Environmental Science, University of Birmingham, Birmingham, B15 2TT, UK
also at: Department of Environmental Sciences/Centre of Excellence in Environmental Studies, King Abdulaziz University, P.O. Box 80203, Jeddah, 21589, Saudi Arabia
School of Geography Earth and Environmental Science, University of Birmingham, Birmingham, B15 2TT, UK
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Cited
19 citations as recorded by crossref.
- Is biomass burning always a dominant contributor of fine aerosols in upper northern Thailand? W. Song et al. 10.1016/j.envint.2022.107466
- On the fossil and non-fossil fuel sources of carbonaceous aerosol with radiocarbon and AMS-PMF methods during winter hazy days in a rural area of North China plain Y. Zhang et al. 10.1016/j.envres.2021.112672
- Molecular composition and the impact of fuel moisture content on fresh primary organic aerosol emissions during laboratory combustion of ponderosa pine needles M. Jaoui et al. 10.1071/EN23013
- The characterization of ambient levoglucosan in Beijing during summertime: Dynamic variation and source contributions under strong cooking influences J. Wang et al. 10.1016/j.jes.2024.08.029
- Fossil and Nonfossil Sources of Winter Organic Aerosols in the Regional Background Atmosphere of China Y. Zhang et al. 10.1021/acs.est.3c08491
- Enhanced PM2.5 episodes in a small residential city of South Korea: Effects of biomass burning and secondary formations S. Choi et al. 10.1016/j.apr.2022.101562
- Quantification of fossil and non-fossil sources to the reduction of carbonaceous aerosols in the Yangtze River Delta, China: Insights from radiocarbon analysis during 2014–2019 M. Yu et al. 10.1016/j.atmosenv.2022.119421
- Characterization of paddy-residue burning derived carbonaceous aerosols using dual carbon isotopes M. Devaprasad et al. 10.1016/j.scitotenv.2022.161044
- Rapid decline in atmospheric organic carbon deposition in rural Beijing, North China between 2016 and 2020 J. Cao et al. 10.1016/j.atmosenv.2022.119030
- Quantitative evaluation for the sources and aging processes of organic aerosols in urban Guangzhou: Insights from a comprehensive method of dual‑carbon isotopes and macro tracers F. Jiang et al. 10.1016/j.scitotenv.2023.164182
- Outdoor charcoal grilling: Particulate and gas-phase emissions, organic speciation and ecotoxicological assessment C. Alves et al. 10.1016/j.atmosenv.2022.119240
- Spatio-temporal distribution of particulate matter and wood-smoke tracers in Temuco, Chile: A city heavily impacted by residential wood-burning M. Quinteros et al. 10.1016/j.atmosenv.2022.119529
- Characterization and sources of carbonaceous aerosol in ambient PM1 in Qingdao, a coastal megacity of northern China from 2017 to 2022 J. Du et al. 10.1016/j.atmosenv.2024.120666
- Geochemical characteristics and socioeconomic associations of carbonaceous aerosols in coal-fueled cities with significant seasonal pollution pattern F. Xie et al. 10.1016/j.envint.2023.108179
- Apportionment of black and brown carbon spectral absorption sources in the urban environment of Athens, Greece, during winter D. Kaskaoutis et al. 10.1016/j.scitotenv.2021.149739
- Biomass Burning Greatly Enhances the Concentration of Fine Carbonaceous Aerosols at an Urban Area in Upper Northern Thailand: Evidence From the Radiocarbon‐Based Source Apportionment on Size‐Resolved Aerosols W. Song et al. 10.1029/2023JD040692
- Contributions of fossil and non-fossil fractions to total carbon in urban aerosols in Bratislava (Slovakia) I. Kontul et al. 10.1016/j.jenvrad.2024.107512
- Space–Time Evaluation of Atmospheric Black Carbon in Chinese Urban Environment: Influence of Land Use and Air Pollution Policies A. Shaheen et al. 10.1007/s41748-024-00380-6
- Impacts of severe residential wood burning on atmospheric processing, water-soluble organic aerosol and light absorption, in an inland city of Southeastern Europe D. Kaskaoutis et al. 10.1016/j.atmosenv.2022.119139
19 citations as recorded by crossref.
- Is biomass burning always a dominant contributor of fine aerosols in upper northern Thailand? W. Song et al. 10.1016/j.envint.2022.107466
- On the fossil and non-fossil fuel sources of carbonaceous aerosol with radiocarbon and AMS-PMF methods during winter hazy days in a rural area of North China plain Y. Zhang et al. 10.1016/j.envres.2021.112672
- Molecular composition and the impact of fuel moisture content on fresh primary organic aerosol emissions during laboratory combustion of ponderosa pine needles M. Jaoui et al. 10.1071/EN23013
- The characterization of ambient levoglucosan in Beijing during summertime: Dynamic variation and source contributions under strong cooking influences J. Wang et al. 10.1016/j.jes.2024.08.029
- Fossil and Nonfossil Sources of Winter Organic Aerosols in the Regional Background Atmosphere of China Y. Zhang et al. 10.1021/acs.est.3c08491
- Enhanced PM2.5 episodes in a small residential city of South Korea: Effects of biomass burning and secondary formations S. Choi et al. 10.1016/j.apr.2022.101562
- Quantification of fossil and non-fossil sources to the reduction of carbonaceous aerosols in the Yangtze River Delta, China: Insights from radiocarbon analysis during 2014–2019 M. Yu et al. 10.1016/j.atmosenv.2022.119421
- Characterization of paddy-residue burning derived carbonaceous aerosols using dual carbon isotopes M. Devaprasad et al. 10.1016/j.scitotenv.2022.161044
- Rapid decline in atmospheric organic carbon deposition in rural Beijing, North China between 2016 and 2020 J. Cao et al. 10.1016/j.atmosenv.2022.119030
- Quantitative evaluation for the sources and aging processes of organic aerosols in urban Guangzhou: Insights from a comprehensive method of dual‑carbon isotopes and macro tracers F. Jiang et al. 10.1016/j.scitotenv.2023.164182
- Outdoor charcoal grilling: Particulate and gas-phase emissions, organic speciation and ecotoxicological assessment C. Alves et al. 10.1016/j.atmosenv.2022.119240
- Spatio-temporal distribution of particulate matter and wood-smoke tracers in Temuco, Chile: A city heavily impacted by residential wood-burning M. Quinteros et al. 10.1016/j.atmosenv.2022.119529
- Characterization and sources of carbonaceous aerosol in ambient PM1 in Qingdao, a coastal megacity of northern China from 2017 to 2022 J. Du et al. 10.1016/j.atmosenv.2024.120666
- Geochemical characteristics and socioeconomic associations of carbonaceous aerosols in coal-fueled cities with significant seasonal pollution pattern F. Xie et al. 10.1016/j.envint.2023.108179
- Apportionment of black and brown carbon spectral absorption sources in the urban environment of Athens, Greece, during winter D. Kaskaoutis et al. 10.1016/j.scitotenv.2021.149739
- Biomass Burning Greatly Enhances the Concentration of Fine Carbonaceous Aerosols at an Urban Area in Upper Northern Thailand: Evidence From the Radiocarbon‐Based Source Apportionment on Size‐Resolved Aerosols W. Song et al. 10.1029/2023JD040692
- Contributions of fossil and non-fossil fractions to total carbon in urban aerosols in Bratislava (Slovakia) I. Kontul et al. 10.1016/j.jenvrad.2024.107512
- Space–Time Evaluation of Atmospheric Black Carbon in Chinese Urban Environment: Influence of Land Use and Air Pollution Policies A. Shaheen et al. 10.1007/s41748-024-00380-6
- Impacts of severe residential wood burning on atmospheric processing, water-soluble organic aerosol and light absorption, in an inland city of Southeastern Europe D. Kaskaoutis et al. 10.1016/j.atmosenv.2022.119139
Latest update: 13 Dec 2024
Short summary
This study provides a newly developed method which combines radiocarbon (14C) with organic tracers to enable source apportionment of primary and secondary fossil vs. non-fossil sources of carbonaceous aerosols at an urban and a rural site of Beijing. The source apportionment results were compared with those by chemical mass balance and AMS/ACSM-PMF methods. Correlations of WINSOC and WSOC with different sources of OC were also performed to elucidate the formation mechanisms of SOC.
This study provides a newly developed method which combines radiocarbon (14C) with organic...
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