Articles | Volume 21, issue 9
https://doi.org/10.5194/acp-21-6839-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-21-6839-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
05 May 2021
Research article |
| 05 May 2021
| 05 May 2021
Dilution impacts on smoke aging: evidence in Biomass Burning Observation Project (BBOP) data
Anna L. Hodshire
CORRESPONDING AUTHOR
Department of Atmospheric Science, Colorado State University, Fort
Collins, CO 80523, United States
Emily Ramnarine
Department of Atmospheric Science, Colorado State University, Fort
Collins, CO 80523, United States
Ali Akherati
Department of Mechanical Engineering, Colorado State University, Fort
Collins, CO 80523, United States
Matthew L. Alvarado
Atmospheric and Environmental Research, Inc., Lexington, MA 02421,
United States
Delphine K. Farmer
Department of Chemistry, Colorado State University, Fort Collins, CO
80523, United States
Shantanu H. Jathar
Department of Mechanical Engineering, Colorado State University, Fort
Collins, CO 80523, United States
Sonia M. Kreidenweis
Department of Atmospheric Science, Colorado State University, Fort
Collins, CO 80523, United States
Chantelle R. Lonsdale
Atmospheric and Environmental Research, Inc., Lexington, MA 02421,
United States
Timothy B. Onasch
Aerodyne Research Inc., Billerica, MA 01821, United States
Stephen R. Springston
Environmental and Climate Sciences Department, Brookhaven National
Laboratory, Upton, NY 11973, United States
Jian Wang
Environmental and Climate Sciences Department, Brookhaven National
Laboratory, Upton, NY 11973, United States
now at: Center for Aerosol Science and Engineering, Washington
University, St. Louis, MO 63130, United States
Yang Wang
Center for Aerosol Science and Engineering, Washington University, St.
Louis, MO 63130, United States
now at: Department of Civil, Architectural and Environmental
Engineering, Missouri University of Science and Technology, Rolla, Missouri
65409, United States
Lawrence I. Kleinman
Environmental and Climate Sciences Department, Brookhaven National
Laboratory, Upton, NY 11973, United States
Arthur J. Sedlacek III
Environmental and Climate Sciences Department, Brookhaven National
Laboratory, Upton, NY 11973, United States
Jeffrey R. Pierce
Department of Atmospheric Science, Colorado State University, Fort
Collins, CO 80523, United States
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Cited
26 citations as recorded by crossref.
- Spatially Resolved Photochemistry Impacts Emissions Estimates in Fresh Wildfire Plumes B. Palm et al. 10.1029/2021GL095443
- Hourly biomass burning emissions product from blended geostationary and polar-orbiting satellites for air quality forecasting applications F. Li et al. 10.1016/j.rse.2022.113237
- Using the Black Carbon Particle Mixing State to Characterize the Lifecycle of Biomass Burning Aerosols A. Sedlacek et al. 10.1021/acs.est.2c03851
- Rate of atmospheric brown carbon whitening governed by environmental conditions E. Schnitzler et al. 10.1073/pnas.2205610119
- Optical properties of biomass burning aerosol during the 2021 Oregon fire season: comparison between wild and prescribed fires A. Marsavin et al. 10.1039/D2EA00118G
- Wildfire plume ageing in the Photochemical Large Aerosol Chamber (PHOTO-LAC) H. Czech et al. 10.1039/D3EM00280B
- Understanding the Evolution of Smoke Mass Extinction Efficiency Using Field Campaign Measurements P. Saide et al. 10.1029/2022GL099175
- Impacts of a Prescribed Fire on Air Quality in Central New Mexico C. Carrico & J. Karacaoglu 10.3390/atmos14020316
- Ultraviolet Irradiation Can Increase the Light Absorption and Viscosity of Primary Brown Carbon from Biomass Burning H. Al-Mashala et al. 10.1021/acsearthspacechem.3c00155
- Intense formation of secondary ultrafine particles from Amazonian vegetation fires and their invigoration of deep clouds and precipitation M. Shrivastava et al. 10.1016/j.oneear.2024.05.015
- Optical Characterization of Fresh and Photochemically Aged Aerosols Emitted from Laboratory Siberian Peat Burning M. Iaukea-Lum et al. 10.3390/atmos13030386
- Dilution and photooxidation driven processes explain the evolution of organic aerosol in wildfire plumes A. Akherati et al. 10.1039/D1EA00082A
- An attribution of the low single-scattering albedo of biomass burning aerosol over the southeastern Atlantic A. Dobracki et al. 10.5194/acp-23-4775-2023
- Mass spectrometric analysis of unprecedented high levels of carbonaceous aerosol particles long-range transported from wildfires in the Siberian Arctic E. Schneider et al. 10.5194/acp-24-553-2024
- New particle formation in the tropical free troposphere during CAMP2Ex: statistics and impact of emission sources, convective activity, and synoptic conditions Q. Xiao et al. 10.5194/acp-23-9853-2023
- Wildfire particulate matter as a source of environmentally persistent free radicals and reactive oxygen species T. Fang et al. 10.1039/D2EA00170E
- Chemical Fingerprinting of Biomass Burning Organic Aerosols from Sugar Cane Combustion: Complementary Findings from Field and Laboratory Studies E. Hartner et al. 10.1021/acsearthspacechem.3c00301
- Aerosol size distribution changes in FIREX-AQ biomass burning plumes: the impact of plume concentration on coagulation and OA condensation/evaporation N. June et al. 10.5194/acp-22-12803-2022
- Air Pollution Interactions with Weather and Climate Extremes: Current Knowledge, Gaps, and Future Directions C. He et al. 10.1007/s40726-024-00296-9
- Emission factors for polycyclic aromatic hydrocarbons from laboratory biomass-burning and their chemical transformations during aging in an oxidation flow reactor D. Sengupta et al. 10.1016/j.scitotenv.2023.161857
- Remote sensing and model analysis of biomass burning smoke transported across the Atlantic during the 2020 Western US wildfire season X. Ceamanos et al. 10.1038/s41598-023-39312-1
- Impact of the Atmospheric Photochemical Evolution of the Organic Component of Biomass Burning Aerosol on Its Radiative Forcing Efficiency: A Box Model Analysis T. Zhuravleva et al. 10.3390/atmos12121555
- The characterization of long-range transported North American biomass burning plumes: what can a multi-wavelength Mie–Raman-polarization-fluorescence lidar provide? Q. Hu et al. 10.5194/acp-22-5399-2022
- Important role of stratospheric injection height for the distribution and radiative forcing of smoke aerosol from the 2019–2020 Australian wildfires B. Heinold et al. 10.5194/acp-22-9969-2022
- Rapid evolution of aerosol particles and their optical properties downwind of wildfires in the western US L. Kleinman et al. 10.5194/acp-20-13319-2020
- Aging of Atmospheric Brown Carbon Aerosol R. Hems et al. 10.1021/acsearthspacechem.0c00346
24 citations as recorded by crossref.
- Spatially Resolved Photochemistry Impacts Emissions Estimates in Fresh Wildfire Plumes B. Palm et al. 10.1029/2021GL095443
- Hourly biomass burning emissions product from blended geostationary and polar-orbiting satellites for air quality forecasting applications F. Li et al. 10.1016/j.rse.2022.113237
- Using the Black Carbon Particle Mixing State to Characterize the Lifecycle of Biomass Burning Aerosols A. Sedlacek et al. 10.1021/acs.est.2c03851
- Rate of atmospheric brown carbon whitening governed by environmental conditions E. Schnitzler et al. 10.1073/pnas.2205610119
- Optical properties of biomass burning aerosol during the 2021 Oregon fire season: comparison between wild and prescribed fires A. Marsavin et al. 10.1039/D2EA00118G
- Wildfire plume ageing in the Photochemical Large Aerosol Chamber (PHOTO-LAC) H. Czech et al. 10.1039/D3EM00280B
- Understanding the Evolution of Smoke Mass Extinction Efficiency Using Field Campaign Measurements P. Saide et al. 10.1029/2022GL099175
- Impacts of a Prescribed Fire on Air Quality in Central New Mexico C. Carrico & J. Karacaoglu 10.3390/atmos14020316
- Ultraviolet Irradiation Can Increase the Light Absorption and Viscosity of Primary Brown Carbon from Biomass Burning H. Al-Mashala et al. 10.1021/acsearthspacechem.3c00155
- Intense formation of secondary ultrafine particles from Amazonian vegetation fires and their invigoration of deep clouds and precipitation M. Shrivastava et al. 10.1016/j.oneear.2024.05.015
- Optical Characterization of Fresh and Photochemically Aged Aerosols Emitted from Laboratory Siberian Peat Burning M. Iaukea-Lum et al. 10.3390/atmos13030386
- Dilution and photooxidation driven processes explain the evolution of organic aerosol in wildfire plumes A. Akherati et al. 10.1039/D1EA00082A
- An attribution of the low single-scattering albedo of biomass burning aerosol over the southeastern Atlantic A. Dobracki et al. 10.5194/acp-23-4775-2023
- Mass spectrometric analysis of unprecedented high levels of carbonaceous aerosol particles long-range transported from wildfires in the Siberian Arctic E. Schneider et al. 10.5194/acp-24-553-2024
- New particle formation in the tropical free troposphere during CAMP2Ex: statistics and impact of emission sources, convective activity, and synoptic conditions Q. Xiao et al. 10.5194/acp-23-9853-2023
- Wildfire particulate matter as a source of environmentally persistent free radicals and reactive oxygen species T. Fang et al. 10.1039/D2EA00170E
- Chemical Fingerprinting of Biomass Burning Organic Aerosols from Sugar Cane Combustion: Complementary Findings from Field and Laboratory Studies E. Hartner et al. 10.1021/acsearthspacechem.3c00301
- Aerosol size distribution changes in FIREX-AQ biomass burning plumes: the impact of plume concentration on coagulation and OA condensation/evaporation N. June et al. 10.5194/acp-22-12803-2022
- Air Pollution Interactions with Weather and Climate Extremes: Current Knowledge, Gaps, and Future Directions C. He et al. 10.1007/s40726-024-00296-9
- Emission factors for polycyclic aromatic hydrocarbons from laboratory biomass-burning and their chemical transformations during aging in an oxidation flow reactor D. Sengupta et al. 10.1016/j.scitotenv.2023.161857
- Remote sensing and model analysis of biomass burning smoke transported across the Atlantic during the 2020 Western US wildfire season X. Ceamanos et al. 10.1038/s41598-023-39312-1
- Impact of the Atmospheric Photochemical Evolution of the Organic Component of Biomass Burning Aerosol on Its Radiative Forcing Efficiency: A Box Model Analysis T. Zhuravleva et al. 10.3390/atmos12121555
- The characterization of long-range transported North American biomass burning plumes: what can a multi-wavelength Mie–Raman-polarization-fluorescence lidar provide? Q. Hu et al. 10.5194/acp-22-5399-2022
- Important role of stratospheric injection height for the distribution and radiative forcing of smoke aerosol from the 2019–2020 Australian wildfires B. Heinold et al. 10.5194/acp-22-9969-2022
Latest update: 20 Nov 2024
Short summary
Biomass burning emits particles and vapors that can impact both health and climate. Here, we investigate the role of dilution in the evolution of aerosol size and composition in observed US wildfire smoke plumes. Centers of plumes dilute more slowly than edges. We see differences in concentrations and composition between the centers and edges both in the first measurement and in subsequent measurements. Our findings support the hypothesis that plume dilution influences smoke aging.
Biomass burning emits particles and vapors that can impact both health and climate. Here, we...
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