Articles | Volume 21, issue 5
https://doi.org/10.5194/acp-21-3395-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-21-3395-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
05 Mar 2021
Research article |
| 05 Mar 2021
| 05 Mar 2021
Future changes in isoprene-epoxydiol-derived secondary organic aerosol (IEPOX SOA) under the Shared Socioeconomic Pathways: the importance of physicochemical dependency
Cooperative Institute for Research in Environmental Sciences
(CIRES), University of Colorado, Boulder, CO, USA
Department of Chemistry, University of Colorado, Boulder, CO, USA
Atmospheric Chemistry Observations and Modeling Laboratory, National Center for Atmospheric Research, Boulder, CO, USA
Alma Hodzic
Atmospheric Chemistry Observations and Modeling Laboratory, National Center for Atmospheric Research, Boulder, CO, USA
Louisa K. Emmons
Atmospheric Chemistry Observations and Modeling Laboratory, National Center for Atmospheric Research, Boulder, CO, USA
Simone Tilmes
Atmospheric Chemistry Observations and Modeling Laboratory, National Center for Atmospheric Research, Boulder, CO, USA
Rebecca H. Schwantes
Atmospheric Chemistry Observations and Modeling Laboratory, National Center for Atmospheric Research, Boulder, CO, USA
now at: Cooperative Institute for Research in Environmental
Sciences, University of Colorado, Boulder, CO, USA
now at: Chemical Sciences Laboratory, National Oceanic and Atmospheric
Administration, Boulder, CO, USA
Michael J. Mills
Atmospheric Chemistry Observations and Modeling Laboratory, National Center for Atmospheric Research, Boulder, CO, USA
Pedro Campuzano-Jost
Cooperative Institute for Research in Environmental Sciences
(CIRES), University of Colorado, Boulder, CO, USA
Department of Chemistry, University of Colorado, Boulder, CO, USA
Weiwei Hu
Cooperative Institute for Research in Environmental Sciences
(CIRES), University of Colorado, Boulder, CO, USA
Department of Chemistry, University of Colorado, Boulder, CO, USA
now at: State Key Laboratory of Organic Geochemistry, Guangzhou
Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou, China
Rahul A. Zaveri
Atmospheric Sciences and Global Change Division, Pacific Northwest
National Laboratory, Richland, WA, USA
Richard C. Easter
Atmospheric Sciences and Global Change Division, Pacific Northwest
National Laboratory, Richland, WA, USA
Balwinder Singh
Atmospheric Sciences and Global Change Division, Pacific Northwest
National Laboratory, Richland, WA, USA
Zheng Lu
Department of Atmospheric Sciences, Texas A&M University,
College Station, Texas
Christiane Schulz
Particle Chemistry Department, Max Planck Institute for Chemistry,
Mainz, Germany
Leibniz Institute for Tropospheric Research, Leipzig, Germany
Johannes Schneider
Particle Chemistry Department, Max Planck Institute for Chemistry,
Mainz, Germany
John E. Shilling
Atmospheric Sciences and Global Change Division, Pacific Northwest
National Laboratory, Richland, WA, USA
Armin Wisthaler
Department of Chemistry, University of Oslo, Oslo, Norway
Institute for Ion Physics and Applied Physics, University of
Innsbruck, Innsbruck, Austria
Jose L. Jimenez
Cooperative Institute for Research in Environmental Sciences
(CIRES), University of Colorado, Boulder, CO, USA
Department of Chemistry, University of Colorado, Boulder, CO, USA
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Cited
20 citations as recorded by crossref.
- Impacts of changes in climate, land use, and emissions on global ozone air quality by mid-21st century following selected Shared Socioeconomic Pathways H. Bhattarai et al. 10.1016/j.scitotenv.2023.167759
- Improvements to the representation of BVOC chemistry–climate interactions in UKCA (v11.5) with the CRI-Strat 2 mechanism: incorporation and evaluation J. Weber et al. 10.5194/gmd-14-5239-2021
- Molecular dynamics investigation of IEPOX chemical behavior at the interface and in the bulk phase of acidic aerosols X. Liu et al. 10.1016/j.chemosphere.2024.143586
- The C5–Alkene Triol Conundrum: Structural Characterization and Quantitation of Isoprene-Derived C5H10O3 Reactive Uptake Products M. Frauenheim et al. 10.1021/acs.estlett.2c00548
- Nocturnal survival of isoprene linked to formation of upper tropospheric organic aerosol P. Palmer et al. 10.1126/science.abg4506
- Emerging investigator series: surfactants, films, and coatings on atmospheric aerosol particles: a review K. Wokosin et al. 10.1039/D2EA00003B
- Comparison of Urban Air Quality Simulations During the KORUS‐AQ Campaign With Regionally Refined Versus Global Uniform Grids in the Multi‐Scale Infrastructure for Chemistry and Aerosols (MUSICA) Version 0 D. Jo et al. 10.1029/2022MS003458
- Responses of fine particulate matter (PM2.5) air quality to future climate, land use, and emission changes: Insights from modeling across shared socioeconomic pathways H. Bhattarai et al. 10.1016/j.scitotenv.2024.174611
- Analysis of secondary organic aerosol simulation bias in the Community Earth System Model (CESM2.1) Y. Liu et al. 10.5194/acp-21-8003-2021
- Widespread 2013-2020 decreases and reduction challenges of organic aerosol in China Q. Chen et al. 10.1038/s41467-024-48902-0
- Tight Coupling of Surface and In-Plant Biochemistry and Convection Governs Key Fine Particulate Components over the Amazon Rainforest M. Shrivastava et al. 10.1021/acsearthspacechem.1c00356
- Global modeling of aerosol nucleation with a semi-explicit chemical mechanism for highly oxygenated organic molecules (HOMs) X. Shao et al. 10.5194/acp-24-11365-2024
- Kinetics and Products of Heterogeneous Hydroxyl Radical Oxidation of Isoprene Epoxydiol-Derived Secondary Organic Aerosol J. Yan et al. 10.1021/acsearthspacechem.3c00073
- Evaluation of Biogenic Organic Aerosols in the Amazon Rainforest Using WRF‐Chem With MOSAIC J. Mao et al. 10.1029/2021JD034913
- Chemical Composition of Secondary Organic Aerosol Formed from the Oxidation of Semivolatile Isoprene Epoxydiol Isomerization Products M. Frauenheim et al. 10.1021/acs.est.4c06850
- Evaluating the Impact of Chemical Complexity and Horizontal Resolution on Tropospheric Ozone Over the Conterminous US With a Global Variable Resolution Chemistry Model R. Schwantes et al. 10.1029/2021MS002889
- Global Health and Climate Effects of Organic Aerosols from Different Sources D. Jo et al. 10.1021/acs.est.3c02823
- Exploring the Factors Controlling the Long‐Term Trend (1988–2019) of Surface Organic Aerosols in the Continental United States by Simulations Y. Liu et al. 10.1029/2022JD037935
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- Description and performance of a sectional aerosol microphysical model in the Community Earth System Model (CESM2) S. Tilmes et al. 10.5194/gmd-16-6087-2023
20 citations as recorded by crossref.
- Impacts of changes in climate, land use, and emissions on global ozone air quality by mid-21st century following selected Shared Socioeconomic Pathways H. Bhattarai et al. 10.1016/j.scitotenv.2023.167759
- Improvements to the representation of BVOC chemistry–climate interactions in UKCA (v11.5) with the CRI-Strat 2 mechanism: incorporation and evaluation J. Weber et al. 10.5194/gmd-14-5239-2021
- Molecular dynamics investigation of IEPOX chemical behavior at the interface and in the bulk phase of acidic aerosols X. Liu et al. 10.1016/j.chemosphere.2024.143586
- The C5–Alkene Triol Conundrum: Structural Characterization and Quantitation of Isoprene-Derived C5H10O3 Reactive Uptake Products M. Frauenheim et al. 10.1021/acs.estlett.2c00548
- Nocturnal survival of isoprene linked to formation of upper tropospheric organic aerosol P. Palmer et al. 10.1126/science.abg4506
- Emerging investigator series: surfactants, films, and coatings on atmospheric aerosol particles: a review K. Wokosin et al. 10.1039/D2EA00003B
- Comparison of Urban Air Quality Simulations During the KORUS‐AQ Campaign With Regionally Refined Versus Global Uniform Grids in the Multi‐Scale Infrastructure for Chemistry and Aerosols (MUSICA) Version 0 D. Jo et al. 10.1029/2022MS003458
- Responses of fine particulate matter (PM2.5) air quality to future climate, land use, and emission changes: Insights from modeling across shared socioeconomic pathways H. Bhattarai et al. 10.1016/j.scitotenv.2024.174611
- Analysis of secondary organic aerosol simulation bias in the Community Earth System Model (CESM2.1) Y. Liu et al. 10.5194/acp-21-8003-2021
- Widespread 2013-2020 decreases and reduction challenges of organic aerosol in China Q. Chen et al. 10.1038/s41467-024-48902-0
- Tight Coupling of Surface and In-Plant Biochemistry and Convection Governs Key Fine Particulate Components over the Amazon Rainforest M. Shrivastava et al. 10.1021/acsearthspacechem.1c00356
- Global modeling of aerosol nucleation with a semi-explicit chemical mechanism for highly oxygenated organic molecules (HOMs) X. Shao et al. 10.5194/acp-24-11365-2024
- Kinetics and Products of Heterogeneous Hydroxyl Radical Oxidation of Isoprene Epoxydiol-Derived Secondary Organic Aerosol J. Yan et al. 10.1021/acsearthspacechem.3c00073
- Evaluation of Biogenic Organic Aerosols in the Amazon Rainforest Using WRF‐Chem With MOSAIC J. Mao et al. 10.1029/2021JD034913
- Chemical Composition of Secondary Organic Aerosol Formed from the Oxidation of Semivolatile Isoprene Epoxydiol Isomerization Products M. Frauenheim et al. 10.1021/acs.est.4c06850
- Evaluating the Impact of Chemical Complexity and Horizontal Resolution on Tropospheric Ozone Over the Conterminous US With a Global Variable Resolution Chemistry Model R. Schwantes et al. 10.1029/2021MS002889
- Global Health and Climate Effects of Organic Aerosols from Different Sources D. Jo et al. 10.1021/acs.est.3c02823
- Exploring the Factors Controlling the Long‐Term Trend (1988–2019) of Surface Organic Aerosols in the Continental United States by Simulations Y. Liu et al. 10.1029/2022JD037935
- A new simplified parameterization of secondary organic aerosol in the Community Earth System Model Version 2 (CESM2; CAM6.3) D. Jo et al. 10.5194/gmd-16-3893-2023
- Description and performance of a sectional aerosol microphysical model in the Community Earth System Model (CESM2) S. Tilmes et al. 10.5194/gmd-16-6087-2023
Latest update: 30 Dec 2024
Short summary
Secondary organic aerosol (SOA) is a major component of submicron particulate matter, but there are a lot of uncertainties in the future prediction of SOA. We used CESM 2.1 to investigate future IEPOX SOA concentration changes. The explicit chemistry predicted substantial changes in IEPOX SOA depending on the future scenario, but the parameterization predicted weak changes due to simplified chemistry, which shows the importance of correct physicochemical dependencies in future SOA prediction.
Secondary organic aerosol (SOA) is a major component of submicron particulate matter, but there...
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