Articles | Volume 21, issue 5
https://doi.org/10.5194/acp-21-3395-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-21-3395-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
05 Mar 2021
Research article |
| 05 Mar 2021
| 05 Mar 2021
Future changes in isoprene-epoxydiol-derived secondary organic aerosol (IEPOX SOA) under the Shared Socioeconomic Pathways: the importance of physicochemical dependency
Cooperative Institute for Research in Environmental Sciences
(CIRES), University of Colorado, Boulder, CO, USA
Department of Chemistry, University of Colorado, Boulder, CO, USA
Atmospheric Chemistry Observations and Modeling Laboratory, National Center for Atmospheric Research, Boulder, CO, USA
Alma Hodzic
Atmospheric Chemistry Observations and Modeling Laboratory, National Center for Atmospheric Research, Boulder, CO, USA
Louisa K. Emmons
Atmospheric Chemistry Observations and Modeling Laboratory, National Center for Atmospheric Research, Boulder, CO, USA
Simone Tilmes
Atmospheric Chemistry Observations and Modeling Laboratory, National Center for Atmospheric Research, Boulder, CO, USA
Rebecca H. Schwantes
Atmospheric Chemistry Observations and Modeling Laboratory, National Center for Atmospheric Research, Boulder, CO, USA
now at: Cooperative Institute for Research in Environmental
Sciences, University of Colorado, Boulder, CO, USA
now at: Chemical Sciences Laboratory, National Oceanic and Atmospheric
Administration, Boulder, CO, USA
Michael J. Mills
Atmospheric Chemistry Observations and Modeling Laboratory, National Center for Atmospheric Research, Boulder, CO, USA
Pedro Campuzano-Jost
Cooperative Institute for Research in Environmental Sciences
(CIRES), University of Colorado, Boulder, CO, USA
Department of Chemistry, University of Colorado, Boulder, CO, USA
Weiwei Hu
Cooperative Institute for Research in Environmental Sciences
(CIRES), University of Colorado, Boulder, CO, USA
Department of Chemistry, University of Colorado, Boulder, CO, USA
now at: State Key Laboratory of Organic Geochemistry, Guangzhou
Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou, China
Rahul A. Zaveri
Atmospheric Sciences and Global Change Division, Pacific Northwest
National Laboratory, Richland, WA, USA
Richard C. Easter
Atmospheric Sciences and Global Change Division, Pacific Northwest
National Laboratory, Richland, WA, USA
Balwinder Singh
Atmospheric Sciences and Global Change Division, Pacific Northwest
National Laboratory, Richland, WA, USA
Zheng Lu
Department of Atmospheric Sciences, Texas A&M University,
College Station, Texas
Christiane Schulz
Particle Chemistry Department, Max Planck Institute for Chemistry,
Mainz, Germany
Leibniz Institute for Tropospheric Research, Leipzig, Germany
Johannes Schneider
Particle Chemistry Department, Max Planck Institute for Chemistry,
Mainz, Germany
John E. Shilling
Atmospheric Sciences and Global Change Division, Pacific Northwest
National Laboratory, Richland, WA, USA
Armin Wisthaler
Department of Chemistry, University of Oslo, Oslo, Norway
Institute for Ion Physics and Applied Physics, University of
Innsbruck, Innsbruck, Austria
Jose L. Jimenez
Cooperative Institute for Research in Environmental Sciences
(CIRES), University of Colorado, Boulder, CO, USA
Department of Chemistry, University of Colorado, Boulder, CO, USA
Data sets
IEPOX-SOA and related chemical/meteorological fields simulated by CESM2/CAM-chem under present and future conditions Duseong Jo, Alma Hodzic, Louisa Emmons, Simone Tilmes, Rebecca Schwantes, Michael J. Mills, Pedro Campuzano-Jost, Weiwei Hu, Rahul A. Zaveri, Richard C. Easter, Balwinder Singh, Zheng Lu, Christiane Schulz, Johannes Schneider, John E. Shilling, Armin Wisthaler, and Jose Jimenez https://doi.org/10.5065/7873-2z88
CESM2.1.0 CESM https://github.com/ESCOMP/CESM
Short summary
Secondary organic aerosol (SOA) is a major component of submicron particulate matter, but there are a lot of uncertainties in the future prediction of SOA. We used CESM 2.1 to investigate future IEPOX SOA concentration changes. The explicit chemistry predicted substantial changes in IEPOX SOA depending on the future scenario, but the parameterization predicted weak changes due to simplified chemistry, which shows the importance of correct physicochemical dependencies in future SOA prediction.
Secondary organic aerosol (SOA) is a major component of submicron particulate matter, but there...
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