Articles | Volume 21, issue 4
https://doi.org/10.5194/acp-21-2959-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-21-2959-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
26 Feb 2021
Research article |
| 26 Feb 2021
Organosulfates in atmospheric aerosols in Shanghai, China: seasonal and interannual variability, origin, and formation mechanisms
School of Environmental Science and Engineering, Shanghai Jiao Tong
University, Shanghai 200240, China
School of Environmental Science and Engineering, Shanghai Jiao Tong
University, Shanghai 200240, China
Shanghai Institute of Pollution Control and Ecological Security,
Shanghai 200092, China
Yuchen Wang
Division of Environment & Sustainability, Hong Kong University of
Science & Technology, Hong Kong SAR, China
Jian-Zhen Yu
Division of Environment & Sustainability, Hong Kong University of
Science & Technology, Hong Kong SAR, China
Department of Chemistry, Hong Kong University of Science &
Technology, Hong Kong SAR, China
Jingyuan Shao
College of Flight Technology, Civil Aviation University of China,
Tianjin 300300, China
Ping Liu
School of Environmental Science and Engineering, Shanghai Jiao Tong
University, Shanghai 200240, China
Wenfei Zhu
School of Environmental Science and Engineering, Shanghai Jiao Tong
University, Shanghai 200240, China
Zhen Cheng
School of Environmental Science and Engineering, Shanghai Jiao Tong
University, Shanghai 200240, China
School of Environmental Science and Engineering, Shanghai Jiao Tong
University, Shanghai 200240, China
Naiqiang Yan
School of Environmental Science and Engineering, Shanghai Jiao Tong
University, Shanghai 200240, China
Shanghai Institute of Pollution Control and Ecological Security,
Shanghai 200092, China
Huayun Xiao
School of Environmental Science and Engineering, Shanghai Jiao Tong
University, Shanghai 200240, China
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Cited
25 citations as recorded by crossref.
- Molecular Characterization of Organosulfate-Dominated Aerosols over Agricultural Fields from the Southern Great Plains by High-Resolution Mass Spectrometry G. Vandergrift et al. 10.1021/acsearthspacechem.2c00043
- Optical properties and molecular composition of wintertime atmospheric water-soluble organic carbon in different coastal cities of eastern China H. Chen et al. 10.1016/j.scitotenv.2023.164702
- Stability assessment of organic sulfur and organosulfate compounds in filter samples for quantification by Fourier- transform infrared spectroscopy M. Anunciado et al. 10.5194/amt-16-3515-2023
- A review of secondary organic aerosols formation focusing on organosulfates and organic nitrates W. Fan et al. 10.1016/j.jhazmat.2022.128406
- Chemical transformation of <i>α</i>-pinene-derived organosulfate via heterogeneous OH oxidation: implications for sources and environmental fates of atmospheric organosulfates R. Xu et al. 10.5194/acp-22-5685-2022
- Organosulfur compounds in ambient fine particulate matter in an urban region: Findings of a nontargeted approach A. Li et al. 10.1016/j.scitotenv.2023.164114
- Important Roles and Formation of Atmospheric Organosulfates in Marine Organic Aerosols: Influence of Phytoplankton Emissions and Anthropogenic Pollutants Y. Wang et al. 10.1021/acs.est.3c01422
- Daytime SO 2 chemistry on ubiquitous urban surfaces as a source of organic sulfur compounds in ambient air H. Deng et al. 10.1126/sciadv.abq6830
- Online Liquid Chromatography and FT-ICR MS Enable Advanced Separation and Profiling of Organosulfates in Dissolved Organic Matter Y. Qi et al. 10.1021/acsestwater.1c00162
- Identification and semi-quantification of nitrooxy organosulfates in aerosol particles by HPLC-MS/MS W. Li et al. 10.1039/D2AY00460G
- Synergistic Effects of SO2 and NH3 Coexistence on SOA Formation from Gasoline Evaporative Emissions T. Chen et al. 10.1021/acs.est.3c01921
- Displacement of Strong Acids or Bases by Weak Acids or Bases in Aerosols: Thermodynamics and Kinetics Z. Chen et al. 10.1021/acs.est.2c03719
- Abundance and Fractional Solubility of Aerosol Iron During Winter at a Coastal City in Northern China: Similarities and Contrasts Between Fine and Coarse Particles H. Zhang et al. 10.1029/2021JD036070
- Aerosol liquid water in PM2.5 and its roles in secondary aerosol formation at a regional site of Yangtze River Delta R. Shi et al. 10.1016/j.jes.2023.04.030
- Interactions of organosulfates with water vapor under sub- and supersaturated conditions C. Peng et al. 10.5194/acp-21-7135-2021
- PM2.5-bound organosulfates in two Eastern Mediterranean cities: The dominance of isoprene organosulfates P. Kanellopoulos et al. 10.1016/j.chemosphere.2022.134103
- Molecular Characteristics of Atmospheric Organosulfates During Summer and Winter Seasons in Two Cities of Southern and Northern China Y. Lin et al. 10.1029/2022JD036672
- SO2 enhances aerosol formation from anthropogenic volatile organic compound ozonolysis by producing sulfur-containing compounds Z. Yang et al. 10.5194/acp-23-417-2023
- Chemical characteristics and sources of organosulfates, organosulfonates, and carboxylic acids in aerosols in urban Xi'an, Northwest China M. Glasius et al. 10.1016/j.scitotenv.2021.151187
- Importance of Oxidants and Temperature in the Formation of Biogenic Organosulfates and Nitrooxy Organosulfates D. Bryant et al. 10.1021/acsearthspacechem.1c00204
- Molecular characterization of organic aerosols in Taiyuan, China: Seasonal variation and source identification W. Wang et al. 10.1016/j.scitotenv.2021.149419
- Biogenic and anthropogenic sources of isoprene and monoterpenes and their secondary organic aerosol in Delhi, India D. Bryant et al. 10.5194/acp-23-61-2023
- Molecular characterization of organic aerosol in winter from Beijing using UHPLC-Orbitrap MS Z. Wang et al. 10.1016/j.scitotenv.2021.151507
- Chemical transformation of a long-chain alkyl organosulfate via heterogeneous OH oxidation: a case study of sodium dodecyl sulfate S. Madeleine Ng et al. 10.1039/D2EA00026A
- A New Structural Classification Scheme for Dissolved Organic Sulfur in Urban Snow from North China S. Su et al. 10.1021/acs.estlett.2c00153
25 citations as recorded by crossref.
- Molecular Characterization of Organosulfate-Dominated Aerosols over Agricultural Fields from the Southern Great Plains by High-Resolution Mass Spectrometry G. Vandergrift et al. 10.1021/acsearthspacechem.2c00043
- Optical properties and molecular composition of wintertime atmospheric water-soluble organic carbon in different coastal cities of eastern China H. Chen et al. 10.1016/j.scitotenv.2023.164702
- Stability assessment of organic sulfur and organosulfate compounds in filter samples for quantification by Fourier- transform infrared spectroscopy M. Anunciado et al. 10.5194/amt-16-3515-2023
- A review of secondary organic aerosols formation focusing on organosulfates and organic nitrates W. Fan et al. 10.1016/j.jhazmat.2022.128406
- Chemical transformation of <i>α</i>-pinene-derived organosulfate via heterogeneous OH oxidation: implications for sources and environmental fates of atmospheric organosulfates R. Xu et al. 10.5194/acp-22-5685-2022
- Organosulfur compounds in ambient fine particulate matter in an urban region: Findings of a nontargeted approach A. Li et al. 10.1016/j.scitotenv.2023.164114
- Important Roles and Formation of Atmospheric Organosulfates in Marine Organic Aerosols: Influence of Phytoplankton Emissions and Anthropogenic Pollutants Y. Wang et al. 10.1021/acs.est.3c01422
- Daytime SO 2 chemistry on ubiquitous urban surfaces as a source of organic sulfur compounds in ambient air H. Deng et al. 10.1126/sciadv.abq6830
- Online Liquid Chromatography and FT-ICR MS Enable Advanced Separation and Profiling of Organosulfates in Dissolved Organic Matter Y. Qi et al. 10.1021/acsestwater.1c00162
- Identification and semi-quantification of nitrooxy organosulfates in aerosol particles by HPLC-MS/MS W. Li et al. 10.1039/D2AY00460G
- Synergistic Effects of SO2 and NH3 Coexistence on SOA Formation from Gasoline Evaporative Emissions T. Chen et al. 10.1021/acs.est.3c01921
- Displacement of Strong Acids or Bases by Weak Acids or Bases in Aerosols: Thermodynamics and Kinetics Z. Chen et al. 10.1021/acs.est.2c03719
- Abundance and Fractional Solubility of Aerosol Iron During Winter at a Coastal City in Northern China: Similarities and Contrasts Between Fine and Coarse Particles H. Zhang et al. 10.1029/2021JD036070
- Aerosol liquid water in PM2.5 and its roles in secondary aerosol formation at a regional site of Yangtze River Delta R. Shi et al. 10.1016/j.jes.2023.04.030
- Interactions of organosulfates with water vapor under sub- and supersaturated conditions C. Peng et al. 10.5194/acp-21-7135-2021
- PM2.5-bound organosulfates in two Eastern Mediterranean cities: The dominance of isoprene organosulfates P. Kanellopoulos et al. 10.1016/j.chemosphere.2022.134103
- Molecular Characteristics of Atmospheric Organosulfates During Summer and Winter Seasons in Two Cities of Southern and Northern China Y. Lin et al. 10.1029/2022JD036672
- SO2 enhances aerosol formation from anthropogenic volatile organic compound ozonolysis by producing sulfur-containing compounds Z. Yang et al. 10.5194/acp-23-417-2023
- Chemical characteristics and sources of organosulfates, organosulfonates, and carboxylic acids in aerosols in urban Xi'an, Northwest China M. Glasius et al. 10.1016/j.scitotenv.2021.151187
- Importance of Oxidants and Temperature in the Formation of Biogenic Organosulfates and Nitrooxy Organosulfates D. Bryant et al. 10.1021/acsearthspacechem.1c00204
- Molecular characterization of organic aerosols in Taiyuan, China: Seasonal variation and source identification W. Wang et al. 10.1016/j.scitotenv.2021.149419
- Biogenic and anthropogenic sources of isoprene and monoterpenes and their secondary organic aerosol in Delhi, India D. Bryant et al. 10.5194/acp-23-61-2023
- Molecular characterization of organic aerosol in winter from Beijing using UHPLC-Orbitrap MS Z. Wang et al. 10.1016/j.scitotenv.2021.151507
- Chemical transformation of a long-chain alkyl organosulfate via heterogeneous OH oxidation: a case study of sodium dodecyl sulfate S. Madeleine Ng et al. 10.1039/D2EA00026A
- A New Structural Classification Scheme for Dissolved Organic Sulfur in Urban Snow from North China S. Su et al. 10.1021/acs.estlett.2c00153
Latest update: 02 Oct 2023
Short summary
Organosulfates (OSs) are important constituents and tracers of secondary organic aerosols (SOAs) in the atmosphere. Here we characterized the OS species in ambient aerosols in Shanghai, China. We find that the contributions of OSs and SOAs to organic aerosols have increased in recent years and that OS production was largely controlled by the oxidant level (Ox), particularly in summer. We infer that mitigation of Ox pollution can effectively reduce the production of OSs and SOAs in eastern China.
Organosulfates (OSs) are important constituents and tracers of secondary organic aerosols (SOAs)...
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