Articles | Volume 21, issue 4
https://doi.org/10.5194/acp-21-2329-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-21-2329-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Brown carbon's emission factors and optical characteristics in household biomass burning: developing a novel algorithm for estimating the contribution of brown carbon
Jianzhong Sun
State Key Laboratory of Environmental Criteria and Risk Assessment,
Chinese Research Academy of Environmental Sciences, Beijing 100012, China
School of Physical Education, Shangrao Normal University, Shangrao
334001, China
Yuzhe Zhang
State Key Laboratory of Environmental Criteria and Risk Assessment,
Chinese Research Academy of Environmental Sciences, Beijing 100012, China
Guorui Zhi
CORRESPONDING AUTHOR
State Key Laboratory of Environmental Criteria and Risk Assessment,
Chinese Research Academy of Environmental Sciences, Beijing 100012, China
Regina Hitzenberger
University of Vienna, Faculty of Physics, Boltzmanngasse 5, 1090
Vienna, Austria
Wenjing Jin
State Key Laboratory of Environmental Criteria and Risk Assessment,
Chinese Research Academy of Environmental Sciences, Beijing 100012, China
Shanghai Key Laboratory of Atmospheric Particle Pollution and
Prevention (LAP3), Department of Environmental Science and Engineering,
Fudan University, Shanghai 200438, China
Lei Wang
State Key Laboratory of Environmental Criteria and Risk Assessment,
Chinese Research Academy of Environmental Sciences, Beijing 100012, China
Chongguo Tian
Key Laboratory of Coastal Environmental Processes and Ecological
Remediation, Yantai Institute of Coastal Zone Research, Chinese Academy of
Sciences, Yantai 264003, China
Zhengying Li
State Key Laboratory of Environmental Criteria and Risk Assessment,
Chinese Research Academy of Environmental Sciences, Beijing 100012, China
Rong Chen
College of Physical and Health Education, East China Jiaotong
University, Nanchang 330006, China
Wen Xiao
School of Physical Education, Jiangxi Science & Technology Normal University, Nanchang 330006, China
Yuan Cheng
State Key Laboratory of Urban Water Resource and Environment, School of Environment, Harbin Institute of Technology, Harbin 150001, China
Wei Yang
School of Physical Education, Shangrao Normal University, Shangrao
334001, China
Liying Yao
School of Physical Education, Shangrao Normal University, Shangrao
334001, China
Yang Cao
School of Physical Education, Shangrao Normal University, Shangrao
334001, China
Duo Huang
School of Physical Education, Shangrao Normal University, Shangrao
334001, China
Yueyuan Qiu
School of Physical Education, Shangrao Normal University, Shangrao
334001, China
Jiali Xu
School of Physical Education, Shangrao Normal University, Shangrao
334001, China
Xiaofei Xia
School of Physical Education, Shangrao Normal University, Shangrao
334001, China
Xin Yang
School of Physical Education, Shangrao Normal University, Shangrao
334001, China
Xi Zhang
School of Physical Education, Shangrao Normal University, Shangrao
334001, China
Zheng Zong
Key Laboratory of Coastal Environmental Processes and Ecological
Remediation, Yantai Institute of Coastal Zone Research, Chinese Academy of
Sciences, Yantai 264003, China
Yuchun Song
Jiangxi Sports Hospital, Nanchang 330006, China
Changdong Wu
Jiangxi Sports Hospital, Nanchang 330006, China
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20 citations as recorded by crossref.
- Optical properties, chemical functional group, and oxidative activity of different polarity levels of water-soluble organic matter in PM2.5 from biomass and coal combustion in rural areas in Northwest China S. Huang et al. 10.1016/j.atmosenv.2022.119179
- Light absorption and source apportionment of water soluble humic-like substances (HULIS) in PM2.5 at Nanjing, China M. Bao et al. 10.1016/j.envres.2021.112554
- Global brown carbon emissions from combustion sources R. Xiong et al. 10.1016/j.ese.2022.100201
- Effects of Bio-Coal Briquette for Residential Combustion on Brown Carbon Emission Reduction J. Qi & J. Wu 10.3390/pr11061834
- Modeling Investigation of Brown Carbon Aerosol and Its Light Absorption in China Y. Zhu et al. 10.3390/atmos12070892
- Direct radiative forcing of light-absorbing carbonaceous aerosols in China L. Yang et al. 10.1016/j.atmosres.2024.107396
- Seasonal features of brown carbon in northern China: Implications for BrC emission control L. Wang et al. 10.1016/j.atmosres.2021.105610
- Review of Brown Carbon Aerosols in China: Pollution Level, Optical Properties, and Emissions Q. Wang et al. 10.1029/2021JD035473
- Aromatic Nitration Enhances Absorption of Biomass Burning Brown Carbon in an Oxidizing Urban Environment J. Duan et al. 10.1021/acs.est.4c05558
- Emissions of Carbonaceous Particulate Matter and Ultrafine Particles from Vehicles—A Scientific Review in a Cross-Cutting Context of Air Pollution and Climate Change B. Bessagnet et al. 10.3390/app12073623
- Light absorption characteristics of primary brown carbon during a complete residential biomass combustion process and their links with aerosol composition P. Chen et al. 10.1016/j.fuel.2023.130695
- Contribution of brown carbon to light absorption in emissions of European residential biomass combustion appliances S. Basnet et al. 10.5194/acp-24-3197-2024
- Emission of water soluble brown carbon from different combustion sources: optical properties and functional group characterisation M. Hossen et al. 10.1088/2515-7620/acea1d
- A review of quantification methods for light absorption enhancement of black carbon aerosol Y. Kong et al. 10.1016/j.scitotenv.2024.171539
- Quantifying the Light-Absorption Properties and Molecular Composition of Brown Carbon Aerosol from Sub-Saharan African Biomass Combustion V. Moschos et al. 10.1021/acs.est.3c09378
- The integrating sphere system plus in-situ absorption monitoring: A new scheme to study absorption enhancement of black carbon in ambient aerosols Z. Li et al. 10.1016/j.scitotenv.2023.164355
- Investigation of structural changes of atmospheric aerosol samples during two thermal–optical measurement procedures (EUSAAR2, NIOSH870) T. Haller et al. 10.5194/amt-14-3721-2021
- Light absorption properties of black carbon and brown carbon emitted from biomass combustion at the typical rural cooking stoves in Bangladesh M. Pavel et al. 10.1007/s11869-023-01302-7
- Emission and optical characteristics of brown carbon in size-segregated particles from three types of Chinese ships F. Yang et al. 10.1016/j.jes.2023.05.045
- Concentration, optical characteristics, and emission factors of brown carbon emitted by on-road vehicles R. Huang et al. 10.1016/j.scitotenv.2021.151307
20 citations as recorded by crossref.
- Optical properties, chemical functional group, and oxidative activity of different polarity levels of water-soluble organic matter in PM2.5 from biomass and coal combustion in rural areas in Northwest China S. Huang et al. 10.1016/j.atmosenv.2022.119179
- Light absorption and source apportionment of water soluble humic-like substances (HULIS) in PM2.5 at Nanjing, China M. Bao et al. 10.1016/j.envres.2021.112554
- Global brown carbon emissions from combustion sources R. Xiong et al. 10.1016/j.ese.2022.100201
- Effects of Bio-Coal Briquette for Residential Combustion on Brown Carbon Emission Reduction J. Qi & J. Wu 10.3390/pr11061834
- Modeling Investigation of Brown Carbon Aerosol and Its Light Absorption in China Y. Zhu et al. 10.3390/atmos12070892
- Direct radiative forcing of light-absorbing carbonaceous aerosols in China L. Yang et al. 10.1016/j.atmosres.2024.107396
- Seasonal features of brown carbon in northern China: Implications for BrC emission control L. Wang et al. 10.1016/j.atmosres.2021.105610
- Review of Brown Carbon Aerosols in China: Pollution Level, Optical Properties, and Emissions Q. Wang et al. 10.1029/2021JD035473
- Aromatic Nitration Enhances Absorption of Biomass Burning Brown Carbon in an Oxidizing Urban Environment J. Duan et al. 10.1021/acs.est.4c05558
- Emissions of Carbonaceous Particulate Matter and Ultrafine Particles from Vehicles—A Scientific Review in a Cross-Cutting Context of Air Pollution and Climate Change B. Bessagnet et al. 10.3390/app12073623
- Light absorption characteristics of primary brown carbon during a complete residential biomass combustion process and their links with aerosol composition P. Chen et al. 10.1016/j.fuel.2023.130695
- Contribution of brown carbon to light absorption in emissions of European residential biomass combustion appliances S. Basnet et al. 10.5194/acp-24-3197-2024
- Emission of water soluble brown carbon from different combustion sources: optical properties and functional group characterisation M. Hossen et al. 10.1088/2515-7620/acea1d
- A review of quantification methods for light absorption enhancement of black carbon aerosol Y. Kong et al. 10.1016/j.scitotenv.2024.171539
- Quantifying the Light-Absorption Properties and Molecular Composition of Brown Carbon Aerosol from Sub-Saharan African Biomass Combustion V. Moschos et al. 10.1021/acs.est.3c09378
- The integrating sphere system plus in-situ absorption monitoring: A new scheme to study absorption enhancement of black carbon in ambient aerosols Z. Li et al. 10.1016/j.scitotenv.2023.164355
- Investigation of structural changes of atmospheric aerosol samples during two thermal–optical measurement procedures (EUSAAR2, NIOSH870) T. Haller et al. 10.5194/amt-14-3721-2021
- Light absorption properties of black carbon and brown carbon emitted from biomass combustion at the typical rural cooking stoves in Bangladesh M. Pavel et al. 10.1007/s11869-023-01302-7
- Emission and optical characteristics of brown carbon in size-segregated particles from three types of Chinese ships F. Yang et al. 10.1016/j.jes.2023.05.045
- Concentration, optical characteristics, and emission factors of brown carbon emitted by on-road vehicles R. Huang et al. 10.1016/j.scitotenv.2021.151307
Latest update: 22 Nov 2024
Short summary
Brown carbon (BrC) emission factors from household biomass fuels were measured with an integrating sphere optics approach supported by iterative calculations. A novel algorithm to directly estimate the absorption contribution of BrC relative to that of BrC + black carbon (FBrC) was proposed based purely on the absorption exponent (AAE)
(FBrC = 0.5519 lnAAE + 0.0067). The FBrC for household biomass fuels was as high as 50.8 % across the strongest solar spectral range of 350−850 nm.
Brown carbon (BrC) emission factors from household biomass fuels were measured with an...
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