Articles | Volume 21, issue 24
https://doi.org/10.5194/acp-21-18351-2021
https://doi.org/10.5194/acp-21-18351-2021
Research article
 | 
17 Dec 2021
Research article |  | 17 Dec 2021

Development and evaluation of a new compact mechanism for aromatic oxidation in atmospheric models

Kelvin H. Bates, Daniel J. Jacob, Ke Li, Peter D. Ivatt, Mat J. Evans, Yingying Yan, and Jintai Lin

Data sets

geoschem/geos-chem: GEOS-Chem 12.3.2 (12.3.2) Bob Yantosca https://doi.org/10.5281/zenodo.2658178

Model code and software

Code and files for "Development and evaluation of a new reduced mechanism for aromatic oxidation in atmospheric models" K. H. Bates https://doi.org/10.7910/DVN/0UQYOI

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Short summary
Simple aromatic compounds (benzene, toluene, xylene) have complex gas-phase chemistry that is inconsistently represented in atmospheric models. We compile recent experimental and theoretical insights to develop a new mechanism for gas-phase aromatic oxidation that is sufficiently compact for use in multiscale models. We compare our new mechanism to chamber experiments and other mechanisms, and implement it in a global model to quantify the impacts of aromatic oxidation on tropospheric chemistry.
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