Molecular-scale description of interfacial mass transfer in phase-separated aqueous secondary organic aerosol
Mária Lbadaoui-Darvas,Satoshi Takahama,and Athanasios Nenes
Mária Lbadaoui-Darvas
Laboratory of Atmospheric Processes and their Impacts, School of Architecture, Civil and Environmental Engineering, Swiss Federal Institute of Technology, 1015 Lausanne, Switzerland
Laboratory of Atmospheric Processes and their Impacts, School of Architecture, Civil and Environmental Engineering, Swiss Federal Institute of Technology, 1015 Lausanne, Switzerland
Laboratory of Atmospheric Processes and their Impacts, School of Architecture, Civil and Environmental Engineering, Swiss Federal Institute of Technology, 1015 Lausanne, Switzerland
Center of Studies on Air quality and Climate Change, Institute of Chemical Engineering Sciences, Foundation for Research and Technology Hellas, Patras, 26504, Greece
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Total article views: 2,927 (including HTML, PDF, and XML)
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Aerosol–cloud interactions constitute the most uncertain contribution to climate change. The uptake kinetics of water by aerosol is a central process of cloud droplet formation, yet its molecular-scale mechanism is unknown. We use molecular simulations to study this process for phase-separated organic particles. Our results explain the increased cloud condensation activity of such particles and can be generalized over various compositions, thus possibly serving as a basis for future models.
Aerosol–cloud interactions constitute the most uncertain contribution to climate change. The...
