Cloud-scale modelling of the impact of deep convection on the fate of oceanic bromoform in the troposphere: a case study over the west coast of Borneo

Hamer, Paul D.; Marécal, Virginie; Hossaini, Ryan; Pirre, Michel; Krysztofiak, Gisèle; Ziska, Franziska; Engel, Andreas; Sala, Stephan; Keber, Timo; Bönisch, Harald; Atlas, Elliot; Krüger, Kirstin; Chipperfield, Martyn; Catoire, Valery; Samah, Azizan A.; Dorf, Marcel; Siew Moi, Phang; Schlager, Hans; Pfeilsticker, Klaus

doi:https://doi.org/10.5194/acp-21-16955-2021

Articles | Volume 21, issue 22

https://doi.org/10.5194/acp-21-16955-2021

© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.

https://doi.org/10.5194/acp-21-16955-2021

© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.

Articles | Volume 21, issue 22

Research article

|

23 Nov 2021

Research article |

| 23 Nov 2021

Cloud-scale modelling of the impact of deep convection on the fate of oceanic bromoform in the troposphere: a case study over the west coast of Borneo

Paul D. Hamer, Virginie Marécal, Ryan Hossaini, Michel Pirre, Gisèle Krysztofiak, Franziska Ziska, Andreas Engel, Stephan Sala, Timo Keber, Harald Bönisch, Elliot Atlas, Kirstin Krüger, Martyn Chipperfield, Valery Catoire, Azizan A. Samah, Marcel Dorf, Phang Siew Moi, Hans Schlager, and Klaus Pfeilsticker

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Final revised paper (published on 23 Nov 2021)
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Preprint (discussion started on 01 Sep 2020)
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Interactive discussion

Status: closed

AC: Author comment | RC: Referee comment | SC: Short comment | EC: Editor comment

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RC1: 'Review', Anonymous Referee #1, 16 Sep 2020
- RC3: 'missing points in previous review', Anonymous Referee #1, 27 Oct 2020
- AC1: 'Reply to RC1 and RC3 combined', Paul Hamer, 07 Sep 2021
RC2: 'review', Anonymous Referee #2, 29 Sep 2020
- AC2: 'Reply to RC2', Paul Hamer, 07 Sep 2021

Peer-review completion

AR: Author's response | RR: Referee report | ED: Editor decision

AR by Paul Hamer on behalf of the Authors (08 Sep 2021) Author's response Author's tracked changes Manuscript

ED: Referee Nomination & Report Request started (14 Sep 2021) by Rolf Müller

RR by Anonymous Referee #2 (04 Oct 2021)

ED: Publish subject to technical corrections (09 Oct 2021) by Rolf Müller

AR by Paul Hamer on behalf of the Authors (21 Oct 2021) Manuscript

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Short summary

Bromoform is a stratospheric ozone-depleting gas released by seaweed and plankton transported to the stratosphere via convection in the tropics. We study the chemical interactions of bromoform and its derivatives within convective clouds using a cloud-scale model and observations. Our findings are that soluble bromine gases are efficiently washed out and removed within the convective clouds and that most bromine is transported vertically to the upper troposphere in the form of bromoform.