Articles | Volume 21, issue 22
https://doi.org/10.5194/acp-21-16955-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-21-16955-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Cloud-scale modelling of the impact of deep convection on the fate of oceanic bromoform in the troposphere: a case study over the west coast of Borneo
Paul D. Hamer
CORRESPONDING AUTHOR
Norwegian Institute for Air Research (NILU), Kjeller, Norway
Centre National de Recherches Météorologiques, Université
de Toulouse, Météo-France, CNRS, Toulouse, France
Virginie Marécal
Centre National de Recherches Météorologiques, Université
de Toulouse, Météo-France, CNRS, Toulouse, France
Ryan Hossaini
Lancaster Environment Centre, Lancaster University, Lancaster, LA1
4YQ, UK
Michel Pirre
Laboratoire de Physique et Chimie de l'Environnement et de l'Espace,
CNRS and University of Orléans, UMR7328, Orléans, France
retired
Gisèle Krysztofiak
Laboratoire de Physique et Chimie de l'Environnement et de l'Espace,
CNRS and University of Orléans, UMR7328, Orléans, France
Franziska Ziska
GEOMAR Helmholtz Centre for Ocean Research Kiel, Kiel, Germany
Andreas Engel
Institute for Atmospheric and Environmental Sciences, University of
Frankfurt, Altenhöferallee 1, 60438 Frankfurt, Germany
Stephan Sala
Institute for Atmospheric and Environmental Sciences, University of
Frankfurt, Altenhöferallee 1, 60438 Frankfurt, Germany
Timo Keber
Institute for Atmospheric and Environmental Sciences, University of
Frankfurt, Altenhöferallee 1, 60438 Frankfurt, Germany
Harald Bönisch
Institute for Atmospheric and Environmental Sciences, University of
Frankfurt, Altenhöferallee 1, 60438 Frankfurt, Germany
Elliot Atlas
University of Miami, 4600 Rickenbacker Causeway, Miami, FL 33149, USA
Kirstin Krüger
Department of Geosciences, University of Oslo, Postboks 1022,
Blindern, 0315 Oslo, Norway
Martyn Chipperfield
School of Earth
and Environment, University of Leeds, Leeds, UK
Valery Catoire
Laboratoire de Physique et Chimie de l'Environnement et de l'Espace,
CNRS and University of Orléans, UMR7328, Orléans, France
Azizan A. Samah
National Antarctic Research Centre, University of Malaya, Kuala
Lumpur 50603, Malaysia
Institute of Ocean and Earth Sciences, University of Malaya, 50603
Kuala Lumpur, Malaysia
Marcel Dorf
Department of Atmospheric
Chemistry, Max Planck Institute for Chemistry, Mainz, Germany
Phang Siew Moi
Institute of Ocean and Earth Sciences, University of Malaya, 50603
Kuala Lumpur, Malaysia
Hans Schlager
Institut für Physik der Atmosphäre, Deutsches Zentrum für Luft- und Raumfahrt (DLR), Atmosphärische Spurenstoffe, Münchner
Straße 20, 82234 Oberpfaffenhofen-Wessling, Germany
Klaus Pfeilsticker
Institute of Environmental Physics, Ruprecht-Karls-Universität
Heidelberg, Im Neuenheimer Feld 229, 69120 Heidelberg, Germany
Data sets
MTSAT-2 cloud-top height product estimated by geostationary satellite CEReS http://database.rish.kyoto-u.ac.jp/arch/ctop/index_e.html
Short summary
Bromoform is a stratospheric ozone-depleting gas released by seaweed and plankton transported to the stratosphere via convection in the tropics. We study the chemical interactions of bromoform and its derivatives within convective clouds using a cloud-scale model and observations. Our findings are that soluble bromine gases are efficiently washed out and removed within the convective clouds and that most bromine is transported vertically to the upper troposphere in the form of bromoform.
Bromoform is a stratospheric ozone-depleting gas released by seaweed and plankton transported...
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