A predictive thermodynamic framework of cloud droplet activation for chemically unresolved aerosol mixtures, including surface tension, non-ideality, and bulk–surface partitioning
Nønne L. Prisle
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Total article views: 2,087 (including HTML, PDF, and XML)
Thereof 2,063 with geography defined
and 24 with unknown origin.
Total article views: 984 (including HTML, PDF, and XML)
Thereof 984 with geography defined
and 0 with unknown origin.
Total article views: 1,103 (including HTML, PDF, and XML)
Thereof 1,079 with geography defined
and 24 with unknown origin.
A mass-based Gibbs adsorption model is presented to enable predictive Köhler calculations of droplet growth and activation with considerations of surface partitioning, surface tension, and non-ideal water activity for chemically complex and unresolved surface active aerosol mixtures, including actual atmospheric samples. The model is used to calculate cloud condensation nuclei (CCN) activity of aerosol particles comprising strongly surface-active model atmospheric humic-like substances (HULIS).
A mass-based Gibbs adsorption model is presented to enable predictive Köhler calculations of...
