Articles | Volume 21, issue 21
https://doi.org/10.5194/acp-21-16183-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-21-16183-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
04 Nov 2021
Research article |
| 04 Nov 2021
| 04 Nov 2021
Process-based and observation-constrained SOA simulations in China: the role of semivolatile and intermediate-volatility organic compounds and OH levels
Ruqian Miao
State Key Joint Laboratory of Environmental Simulation and Pollution Control, BIC-ESAT and IJRC, College of Environmental Sciences and Engineering, Peking University, Beijing, 100871, China
State Key Joint Laboratory of Environmental Simulation and Pollution Control, BIC-ESAT and IJRC, College of Environmental Sciences and Engineering, Peking University, Beijing, 100871, China
Manish Shrivastava
Pacific Northwest National Laboratory, Richland, Washington 99352, USA
Youfan Chen
Sichuan Academy of Environmental Policy and Planning, Chengdu, Sichuan, 610041, China
Lin Zhang
Laboratory for Climate and Ocean–Atmosphere Studies, Department of Atmospheric and Oceanic Sciences, School of Physics, Peking University, Beijing, 100871, China
Jianlin Hu
Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control, Jiangsu Engineering Technology Research Center of Environmental Cleaning Materials, Collaborative Innovation Center of Atmospheric Environment and Equipment Technology, School of Environmental Science and Engineering, Nanjing University of Information Science and Technology, Nanjing, Jiangsu, 210044, China
Yan Zheng
State Key Joint Laboratory of Environmental Simulation and Pollution Control, BIC-ESAT and IJRC, College of Environmental Sciences and Engineering, Peking University, Beijing, 100871, China
Keren Liao
State Key Joint Laboratory of Environmental Simulation and Pollution Control, BIC-ESAT and IJRC, College of Environmental Sciences and Engineering, Peking University, Beijing, 100871, China
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Cited
15 citations as recorded by crossref.
- Sources of organic aerosols in eastern China: a modeling study with high-resolution intermediate-volatility and semivolatile organic compound emissions J. An et al. 10.5194/acp-23-323-2023
- Contribution of intermediate-volatility organic compounds from on-road transport to secondary organic aerosol levels in Europe S. Manavi & S. Pandis 10.5194/acp-24-891-2024
- Bias correction of OMI HCHO columns based on FTIR and aircraft measurements and impact on top-down emission estimates J. Müller et al. 10.5194/acp-24-2207-2024
- Characteristics, sources of volatile organic compounds, and their contributions to secondary air pollution during different periods in Beijing, China S. Liang et al. 10.1016/j.scitotenv.2022.159831
- Satellite Evidence for Glyoxal Depletion in Elevated Fire Plumes C. Lerot et al. 10.1029/2022GL102195
- Intermediate-volatility aromatic hydrocarbons from the rubber products industry in China Z. Zhang et al. 10.1016/j.scitotenv.2023.165583
- Spatial variability of air pollutants in a megacity characterized by mobile measurements R. Khuzestani et al. 10.5194/acp-22-7389-2022
- Unveiling the underestimated direct emissions of nitrous acid (HONO) Q. Zhang et al. 10.1073/pnas.2302048120
- Modeling Secondary Organic Aerosols in China: State of the Art and Perspectives J. Li et al. 10.1007/s40726-022-00246-3
- Modeling of secondary organic aerosols (SOA) based on two commonly used air quality models in China: Consistent S/IVOCs contribution but large differences in SOA aging L. Huang et al. 10.1016/j.scitotenv.2023.166162
- Direct radiative forcing of light-absorbing carbonaceous aerosols in China L. Yang et al. 10.1016/j.atmosres.2024.107396
- Secondary organic aerosols from oxidation of 1-methylnaphthalene: Yield, composition, and volatility W. Xiang et al. 10.1016/j.scitotenv.2024.170379
- Simulation of organics in the atmosphere: evaluation of EMACv2.54 with the Mainz Organic Mechanism (MOM) coupled to the ORACLE (v1.0) submodel A. Pozzer et al. 10.5194/gmd-15-2673-2022
- Secondary Formation of Submicron and Supermicron Organic and Inorganic Aerosols in a Highly Polluted Urban Area Y. Zheng et al. 10.1029/2022JD037865
- Comprehensive Assessment for the Impacts of S/IVOC Emissions from Mobile Sources on SOA Formation in China J. Zhao et al. 10.1021/acs.est.2c07265
15 citations as recorded by crossref.
- Sources of organic aerosols in eastern China: a modeling study with high-resolution intermediate-volatility and semivolatile organic compound emissions J. An et al. 10.5194/acp-23-323-2023
- Contribution of intermediate-volatility organic compounds from on-road transport to secondary organic aerosol levels in Europe S. Manavi & S. Pandis 10.5194/acp-24-891-2024
- Bias correction of OMI HCHO columns based on FTIR and aircraft measurements and impact on top-down emission estimates J. Müller et al. 10.5194/acp-24-2207-2024
- Characteristics, sources of volatile organic compounds, and their contributions to secondary air pollution during different periods in Beijing, China S. Liang et al. 10.1016/j.scitotenv.2022.159831
- Satellite Evidence for Glyoxal Depletion in Elevated Fire Plumes C. Lerot et al. 10.1029/2022GL102195
- Intermediate-volatility aromatic hydrocarbons from the rubber products industry in China Z. Zhang et al. 10.1016/j.scitotenv.2023.165583
- Spatial variability of air pollutants in a megacity characterized by mobile measurements R. Khuzestani et al. 10.5194/acp-22-7389-2022
- Unveiling the underestimated direct emissions of nitrous acid (HONO) Q. Zhang et al. 10.1073/pnas.2302048120
- Modeling Secondary Organic Aerosols in China: State of the Art and Perspectives J. Li et al. 10.1007/s40726-022-00246-3
- Modeling of secondary organic aerosols (SOA) based on two commonly used air quality models in China: Consistent S/IVOCs contribution but large differences in SOA aging L. Huang et al. 10.1016/j.scitotenv.2023.166162
- Direct radiative forcing of light-absorbing carbonaceous aerosols in China L. Yang et al. 10.1016/j.atmosres.2024.107396
- Secondary organic aerosols from oxidation of 1-methylnaphthalene: Yield, composition, and volatility W. Xiang et al. 10.1016/j.scitotenv.2024.170379
- Simulation of organics in the atmosphere: evaluation of EMACv2.54 with the Mainz Organic Mechanism (MOM) coupled to the ORACLE (v1.0) submodel A. Pozzer et al. 10.5194/gmd-15-2673-2022
- Secondary Formation of Submicron and Supermicron Organic and Inorganic Aerosols in a Highly Polluted Urban Area Y. Zheng et al. 10.1029/2022JD037865
- Comprehensive Assessment for the Impacts of S/IVOC Emissions from Mobile Sources on SOA Formation in China J. Zhao et al. 10.1021/acs.est.2c07265
Latest update: 25 Apr 2024
Short summary
We apply process-based and observation-constrained schemes to simulate organic aerosol in China and conduct comprehensive model–observation comparisons. The results show that anthropogenic semivolatile and intermediate-volatility organic compounds (SVOCs and IVOCs) are the main sources of secondary organic aerosol (SOA) in polluted regions, for which the residential sector is perhaps the predominant contributor. The hydroxyl radical level is also important for SOA modeling in polluted regions.
We apply process-based and observation-constrained schemes to simulate organic aerosol in China...
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