Articles | Volume 21, issue 20
https://doi.org/10.5194/acp-21-15901-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-21-15901-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
26 Oct 2021
Research article |
| 26 Oct 2021
| 26 Oct 2021
Exploring the sensitivity of atmospheric nitrate concentrations to nitric acid uptake rate using the Met Office's Unified Model
Anthony C. Jones
CORRESPONDING AUTHOR
Met Office, Fitzroy Road, Exeter, EX1 3PB, UK
Adrian Hill
Met Office, Fitzroy Road, Exeter, EX1 3PB, UK
Samuel Remy
HYGEOS, Lille, France
N. Luke Abraham
National Centre for Atmospheric Science, Leeds, LS2 9PH, UK
Department of Chemistry, University of Cambridge, Lensfield Road,
Cambridge, CB2 1EW, UK
Mohit Dalvi
Met Office, Fitzroy Road, Exeter, EX1 3PB, UK
Catherine Hardacre
Met Office, Fitzroy Road, Exeter, EX1 3PB, UK
Alan J. Hewitt
Met Office, Fitzroy Road, Exeter, EX1 3PB, UK
Ben Johnson
Met Office, Fitzroy Road, Exeter, EX1 3PB, UK
Jane P. Mulcahy
Met Office, Fitzroy Road, Exeter, EX1 3PB, UK
Steven T. Turnock
Met Office, Fitzroy Road, Exeter, EX1 3PB, UK
Met Office Strategic Research Group, School of
Earth and Environment, University of Leeds, Leeds, LS2 9JT, UK
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Cited
10 citations as recorded by crossref.
- Investigating the contribution of grown new particles to cloud condensation nuclei with largely varying preexisting particles – Part 1: Observational data analysis X. Wei et al. 10.5194/acp-23-15325-2023
- The Air Pollution Human Health Burden in Different Future Scenarios That Involve the Mitigation of Near‐Term Climate Forcers, Climate and Land‐Use S. Turnock et al. 10.1029/2023GH000812
- Marine aerosol in Aotearoa New Zealand: implications for air quality, climate change and public health L. Revell et al. 10.1080/03036758.2024.2319753
- Radiative impact of improved global parameterisations of oceanic dry deposition of ozone and lightning-generated NOx A. Luhar et al. 10.5194/acp-22-13013-2022
- Description and evaluation of the tropospheric aerosol scheme in the Integrated Forecasting System (IFS-AER, cycle 47R1) of ECMWF S. Rémy et al. 10.5194/gmd-15-4881-2022
- Large simulated future changes in the nitrate radical under the CMIP6 SSP scenarios: implications for oxidation chemistry S. Archer-Nicholls et al. 10.5194/acp-23-5801-2023
- Below-cloud scavenging of aerosol by rain: a review of numerical modelling approaches and sensitivity simulations with mineral dust in the Met Office's Unified Model A. Jones et al. 10.5194/acp-22-11381-2022
- NUMAC: Description of the Nested Unified Model With Aerosols and Chemistry, and Evaluation With KORUS‐AQ Data H. Gordon et al. 10.1029/2022MS003457
- Impact of East Asian Summer Atmospheric Warming on PM<sub>2.5</sub> Aerosols S. Kim et al. 10.5467/JKESS.2024.45.1.1
- Inequalities in Air Pollution Exposure and Attributable Mortality in a Low Carbon Future C. Reddington et al. 10.1029/2023EF003697
10 citations as recorded by crossref.
- Investigating the contribution of grown new particles to cloud condensation nuclei with largely varying preexisting particles – Part 1: Observational data analysis X. Wei et al. 10.5194/acp-23-15325-2023
- The Air Pollution Human Health Burden in Different Future Scenarios That Involve the Mitigation of Near‐Term Climate Forcers, Climate and Land‐Use S. Turnock et al. 10.1029/2023GH000812
- Marine aerosol in Aotearoa New Zealand: implications for air quality, climate change and public health L. Revell et al. 10.1080/03036758.2024.2319753
- Radiative impact of improved global parameterisations of oceanic dry deposition of ozone and lightning-generated NOx A. Luhar et al. 10.5194/acp-22-13013-2022
- Description and evaluation of the tropospheric aerosol scheme in the Integrated Forecasting System (IFS-AER, cycle 47R1) of ECMWF S. Rémy et al. 10.5194/gmd-15-4881-2022
- Large simulated future changes in the nitrate radical under the CMIP6 SSP scenarios: implications for oxidation chemistry S. Archer-Nicholls et al. 10.5194/acp-23-5801-2023
- Below-cloud scavenging of aerosol by rain: a review of numerical modelling approaches and sensitivity simulations with mineral dust in the Met Office's Unified Model A. Jones et al. 10.5194/acp-22-11381-2022
- NUMAC: Description of the Nested Unified Model With Aerosols and Chemistry, and Evaluation With KORUS‐AQ Data H. Gordon et al. 10.1029/2022MS003457
- Impact of East Asian Summer Atmospheric Warming on PM<sub>2.5</sub> Aerosols S. Kim et al. 10.5467/JKESS.2024.45.1.1
- Inequalities in Air Pollution Exposure and Attributable Mortality in a Low Carbon Future C. Reddington et al. 10.1029/2023EF003697
Latest update: 25 Apr 2024
Short summary
Ammonium nitrate is hard to model because it forms and evaporates rapidly. One approach is to relate its equilibrium concentration to temperature, humidity, and the amount of nitric acid and ammonia gases. Using this approach, we limit the rate at which equilibrium is reached using various condensation rates in a climate model. We show that ammonium nitrate concentrations are highly sensitive to the condensation rate. Our results will help improve the representation of nitrate in climate models.
Ammonium nitrate is hard to model because it forms and evaporates rapidly. One approach is to...
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