Articles | Volume 21, issue 20
https://doi.org/10.5194/acp-21-15375-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-21-15375-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Organic and inorganic bromine measurements around the extratropical tropopause and lowermost stratosphere: insights into the transport pathways and total bromine
Meike K. Rotermund
CORRESPONDING AUTHOR
Institute of Environmental Physics, University of Heidelberg, Heidelberg, Germany
Vera Bense
Institute for Atmospheric Physics, Johannes Gutenberg University Mainz, Mainz, Germany
Martyn P. Chipperfield
School of Earth and Environment, University of Leeds, Leeds, UK
National Centre for Earth Observation, University of Leeds, Leeds, UK
Andreas Engel
Institute for Atmospheric and Environmental Science, Goethe University Frankfurt, Frankfurt, Germany
Jens-Uwe Grooß
Institute of Energy and Climate Research – Stratosphere (IEK-7), Forschungszentrum Jülich, Jülich, Germany
Peter Hoor
Institute for Atmospheric Physics, Johannes Gutenberg University Mainz, Mainz, Germany
Tilman Hüneke
Institute of Environmental Physics, University of Heidelberg, Heidelberg, Germany
now at: Encavis AG, Hamburg, Germany
Timo Keber
Institute for Atmospheric and Environmental Science, Goethe University Frankfurt, Frankfurt, Germany
Flora Kluge
Institute of Environmental Physics, University of Heidelberg, Heidelberg, Germany
Benjamin Schreiner
Institute of Environmental Physics, University of Heidelberg, Heidelberg, Germany
Tanja Schuck
Institute for Atmospheric and Environmental Science, Goethe University Frankfurt, Frankfurt, Germany
Bärbel Vogel
Institute of Energy and Climate Research – Stratosphere (IEK-7), Forschungszentrum Jülich, Jülich, Germany
Andreas Zahn
Institute for Meteorology and Climate Research, Karlsruhe Institute of Technology (KIT), Karlsruhe, Germany
Klaus Pfeilsticker
Institute of Environmental Physics, University of Heidelberg, Heidelberg, Germany
Data sets
HALO database; editing status 2020-09-23 re3data.org https://doi.org/10.17616/R39Q0T
Short summary
Airborne total bromine (Brtot) and tracer measurements suggest Brtot-rich air masses persistently protruded into the lower stratosphere (LS), creating a high Brtot region over the North Atlantic in fall 2017. The main source is via isentropic transport by the Asian monsoon and to a lesser extent transport across the extratropical tropopause as quantified by a Lagrange model. The transport of Brtot via Central American hurricanes is also observed. Lastly, the impact of Brtot on LS O3 is assessed.
Airborne total bromine (Brtot) and tracer measurements suggest Brtot-rich air masses...
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