Articles | Volume 21, issue 17
https://doi.org/10.5194/acp-21-13031-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-21-13031-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
A global study of hygroscopicity-driven light-scattering enhancement in the context of other in situ aerosol optical properties
Andalusian Institute for Earth System Research, University of Granada, 18006, Granada, Spain
Department of Applied Physics, University of Granada, 18071, Granada, Spain
María A. Burgos
Department of Environmental Science, Stockholm University, Stockholm, Sweden
Bolin Centre for Climate Research, Stockholm University, Stockholm, Sweden
Paul Zieger
Department of Environmental Science, Stockholm University, Stockholm, Sweden
Bolin Centre for Climate Research, Stockholm University, Stockholm, Sweden
Lucas Alados-Arboledas
Andalusian Institute for Earth System Research, University of Granada, 18006, Granada, Spain
Department of Applied Physics, University of Granada, 18071, Granada, Spain
Urs Baltensperger
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, Villigen, Switzerland
Anne Jefferson
Cooperative Institute for Research in Environmental Studies, University of Colorado, Boulder, CO 80309, USA
James Sherman
Department of Physics and Astronomy, Appalachian State University, Boone, NC, USA
Ernest Weingartner
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, Villigen, Switzerland
now at: Institute for Sensing and Electronics, University of Applied Sciences, Windisch, Switzerland
Bas Henzing
Netherlands Organisation for Applied Scientific Research (TNO), Princetonlaan 6, 3584 Utrecht, the Netherlands
Krista Luoma
Institute for Atmospheric and Earth System Research/Physics, Faculty of Science, University of Helsinki, P.O. Box 68, 00014 Helsinki, Finland
Colin O'Dowd
School of Physics, Ryan Institute's Centre for Climate and Air Pollution Studies, National University of Ireland Galway, University Road, H91 CF50 Galway, Ireland
Alfred Wiedensohler
Department Experimental Aerosol & Cloud Microphysics, Leibniz Institute for Tropospheric Research, 04318 Leipzig, Germany
Elisabeth Andrews
Cooperative Institute for Research in Environmental Studies, University of Colorado, Boulder, CO 80309, USA
Global Monitoring Laboratory, National Oceanic and Atmospheric Administration, Boulder, CO 80305, USA
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Cited
23 citations as recorded by crossref.
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- Optical Properties of Boundary Layer Aerosols From High Spectral Resolution Lidar Measurements in a Polluted Urban Environment (Seoul, Korea) S. Park et al.
- The characterization of particle size evolution of atmospheric aerosol during the hygroscopic growth: A review J. Liu et al.
- Lidar-based investigation of aerosol hygroscopic growth characteristics using fluorescence capacity W. Yufeng et al.
- Hygroscopic enhancement of suburban aerosol light scattering measured using a single-nephelometer system in Central Europe L. Suchánková et al.
- Effects of hygroscopicity on aerosol optical properties and direct radiative forcing in Beijing: Based on two-year observations C. Xia et al.
- Machine learning-based retrieval of aerosol size and hygroscopicity using horizontal scanning LiDAR and PM data J. Shin et al.
- Dynamic decoupling of temperature and humidity effects for enhanced real-time aerosol optical inversion G. Wang et al.
- A machine learning-based model for aerosol scattering hygroscopic growth factor (f(RH)) prediction in Beijing urban area H. Tong et al.
- Joint increase of aerosol scattering efficiency and aerosol hygroscopicity aggravate visibility impairment in the North China Plain B. Xue et al.
- Divergent changes in aerosol optical hygroscopicity and new particle formation during a heatwave of summer 2022 Y. Hao et al.
- Measurement report: Characterization of aerosol hygroscopicity over Southeast Asia during the NASA CAMP2Ex campaign G. Lorenzo et al.
- Tutorial: Electrodynamic balance methods for single particle levitation and the physicochemical analysis of aerosol R. Kaur Kohli et al.
- Aerosol light-scattering enhancement and liquid water content in a tropical coastal atmosphere S. Kompalli & S. Babu
- Revisiting integrating nephelometer measurements W. Malm et al.
- Subsaturated aerosol hygroscopicity over the northwest Atlantic: Impacts of seasonal factors, offshore location, and clouds G. Lorenzo et al.
- Aerosols over East and South Asia: Type Identification, Optical Properties, and Implications for Radiative Forcing Y. Liu & B. Yi
- Aerosol hygroscopicity over the southeast Atlantic Ocean during the biomass burning season – Part 1: From the perspective of scattering enhancement L. Zhang et al.
- Measurement report: Optical properties of supermicron aerosol particles in a boreal environment S. Banerji et al.
- Hygroscopic Growth of Glyoxal Aqueous Aerosol Revealed by Infrared Extinction Spectra K. Liu & L. Chu
- Optical and radiative properties of coated black carbon during hygroscopic growth and retrieval errors of mixing state using single-particle soot photometer J. Liu et al.
- Aerosol microphysical and optical closure study in the Baltic Sea coastal zone K. Markowicz et al.
- Discussion of the spectral slope of the lidar ratio between 355 and 1064 nm from multiwavelength Raman lidar observations M. Haarig et al.
23 citations as recorded by crossref.
- Measurement report: Rapid decline of aerosol absorption coefficient and aerosol optical property effects on radiative forcing in an urban area of Beijing from 2018 to 2021 X. Hu et al.
- Optical Properties of Boundary Layer Aerosols From High Spectral Resolution Lidar Measurements in a Polluted Urban Environment (Seoul, Korea) S. Park et al.
- The characterization of particle size evolution of atmospheric aerosol during the hygroscopic growth: A review J. Liu et al.
- Lidar-based investigation of aerosol hygroscopic growth characteristics using fluorescence capacity W. Yufeng et al.
- Hygroscopic enhancement of suburban aerosol light scattering measured using a single-nephelometer system in Central Europe L. Suchánková et al.
- Effects of hygroscopicity on aerosol optical properties and direct radiative forcing in Beijing: Based on two-year observations C. Xia et al.
- Machine learning-based retrieval of aerosol size and hygroscopicity using horizontal scanning LiDAR and PM data J. Shin et al.
- Dynamic decoupling of temperature and humidity effects for enhanced real-time aerosol optical inversion G. Wang et al.
- A machine learning-based model for aerosol scattering hygroscopic growth factor (f(RH)) prediction in Beijing urban area H. Tong et al.
- Joint increase of aerosol scattering efficiency and aerosol hygroscopicity aggravate visibility impairment in the North China Plain B. Xue et al.
- Divergent changes in aerosol optical hygroscopicity and new particle formation during a heatwave of summer 2022 Y. Hao et al.
- Measurement report: Characterization of aerosol hygroscopicity over Southeast Asia during the NASA CAMP2Ex campaign G. Lorenzo et al.
- Tutorial: Electrodynamic balance methods for single particle levitation and the physicochemical analysis of aerosol R. Kaur Kohli et al.
- Aerosol light-scattering enhancement and liquid water content in a tropical coastal atmosphere S. Kompalli & S. Babu
- Revisiting integrating nephelometer measurements W. Malm et al.
- Subsaturated aerosol hygroscopicity over the northwest Atlantic: Impacts of seasonal factors, offshore location, and clouds G. Lorenzo et al.
- Aerosols over East and South Asia: Type Identification, Optical Properties, and Implications for Radiative Forcing Y. Liu & B. Yi
- Aerosol hygroscopicity over the southeast Atlantic Ocean during the biomass burning season – Part 1: From the perspective of scattering enhancement L. Zhang et al.
- Measurement report: Optical properties of supermicron aerosol particles in a boreal environment S. Banerji et al.
- Hygroscopic Growth of Glyoxal Aqueous Aerosol Revealed by Infrared Extinction Spectra K. Liu & L. Chu
- Optical and radiative properties of coated black carbon during hygroscopic growth and retrieval errors of mixing state using single-particle soot photometer J. Liu et al.
- Aerosol microphysical and optical closure study in the Baltic Sea coastal zone K. Markowicz et al.
- Discussion of the spectral slope of the lidar ratio between 355 and 1064 nm from multiwavelength Raman lidar observations M. Haarig et al.
Saved (final revised paper)
Latest update: 28 Apr 2026
Short summary
This paper investigates the impact of water uptake on aerosol optical properties, in particular the aerosol light-scattering coefficient. Although in situ measurements are performed at low relative humidity (typically at
RH < 40 %), to address the climatic impact of aerosol particles it is necessary to take into account the effect that water uptake may have on the aerosol optical properties.
This paper investigates the impact of water uptake on aerosol optical properties, in particular...
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