Articles | Volume 21, issue 13
https://doi.org/10.5194/acp-21-10375-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-21-10375-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
09 Jul 2021
Research article |
| 09 Jul 2021
| 09 Jul 2021
Contrasting effects of secondary organic aerosol formations on organic aerosol hygroscopicity
Institute for Environmental and Climate Research, Jinan University, Guangzhou 511443, China
Guangdong-Hongkong-Macau Joint Laboratory of Collaborative Innovation for Environmental Quality, Guangzhou 511443, China
Institute for Environmental and Climate Research, Jinan University, Guangzhou 511443, China
Guangdong-Hongkong-Macau Joint Laboratory of Collaborative Innovation for Environmental Quality, Guangzhou 511443, China
Biao Xue
Institute for Environmental and Climate Research, Jinan University, Guangzhou 511443, China
Guangdong-Hongkong-Macau Joint Laboratory of Collaborative Innovation for Environmental Quality, Guangzhou 511443, China
Biao Luo
Institute for Environmental and Climate Research, Jinan University, Guangzhou 511443, China
Guangdong-Hongkong-Macau Joint Laboratory of Collaborative Innovation for Environmental Quality, Guangzhou 511443, China
Qicong Song
Institute for Environmental and Climate Research, Jinan University, Guangzhou 511443, China
Guangdong-Hongkong-Macau Joint Laboratory of Collaborative Innovation for Environmental Quality, Guangzhou 511443, China
Wei Chen
State Key Laboratory of Organic Geochemistry and Guangdong Key Laboratory of Environmental Protection and Resources Utilization, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China
Weiwei Hu
State Key Laboratory of Organic Geochemistry and Guangdong Key Laboratory of Environmental Protection and Resources Utilization, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China
Wei Li
Institute for Environmental and Climate Research, Jinan University, Guangzhou 511443, China
Guangdong-Hongkong-Macau Joint Laboratory of Collaborative Innovation for Environmental Quality, Guangzhou 511443, China
Pusheng Zhao
Institute of Urban Meteorology, China Meteorological Administration, Beijing 100089, China
Mingfu Cai
Institute for Environmental and Climate Research, Jinan University, Guangzhou 511443, China
Guangdong-Hongkong-Macau Joint Laboratory of Collaborative Innovation for Environmental Quality, Guangzhou 511443, China
Yuwen Peng
Institute for Environmental and Climate Research, Jinan University, Guangzhou 511443, China
Guangdong-Hongkong-Macau Joint Laboratory of Collaborative Innovation for Environmental Quality, Guangzhou 511443, China
Jipeng Qi
Institute for Environmental and Climate Research, Jinan University, Guangzhou 511443, China
Guangdong-Hongkong-Macau Joint Laboratory of Collaborative Innovation for Environmental Quality, Guangzhou 511443, China
Tiange Li
Institute for Environmental and Climate Research, Jinan University, Guangzhou 511443, China
Guangdong-Hongkong-Macau Joint Laboratory of Collaborative Innovation for Environmental Quality, Guangzhou 511443, China
Sihang Wang
Institute for Environmental and Climate Research, Jinan University, Guangzhou 511443, China
Guangdong-Hongkong-Macau Joint Laboratory of Collaborative Innovation for Environmental Quality, Guangzhou 511443, China
Duohong Chen
Guangdong Ecological and Environmental Monitoring Center, State Environmental Protection Key Laboratory of Regional Air Quality Monitoring, Guangzhou 510308, China
Dingli Yue
Guangdong Ecological and Environmental Monitoring Center, State Environmental Protection Key Laboratory of Regional Air Quality Monitoring, Guangzhou 510308, China
Institute for Environmental and Climate Research, Jinan University, Guangzhou 511443, China
Guangdong-Hongkong-Macau Joint Laboratory of Collaborative Innovation for Environmental Quality, Guangzhou 511443, China
Min Shao
CORRESPONDING AUTHOR
Institute for Environmental and Climate Research, Jinan University, Guangzhou 511443, China
Guangdong-Hongkong-Macau Joint Laboratory of Collaborative Innovation for Environmental Quality, Guangzhou 511443, China
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Cited
19 citations as recorded by crossref.
- Technical note: Quantified organic aerosol subsaturated hygroscopicity by a simple optical scatter monitor system through field measurements J. Zhang et al. 10.5194/acp-24-13445-2024
- Markedly different impacts of primary emissions and secondary aerosol formation on aerosol mixing states revealed by simultaneous measurements of CCNC, H(/V)TDMA, and SP2 J. Tao et al. 10.5194/acp-24-9131-2024
- Significant impact of water-soluble organic matter on hygroscopicity of fine particles under low relative humidity condition J. Tao et al. 10.1016/j.scitotenv.2023.167980
- Joint increase of aerosol scattering efficiency and aerosol hygroscopicity aggravate visibility impairment in the North China Plain B. Xue et al. 10.1016/j.scitotenv.2022.156279
- Theoretical framework for measuring cloud effective supersaturation fluctuations with an advanced optical system Y. Kuang et al. 10.5194/acp-25-1163-2025
- Strong light scattering of highly oxygenated organic aerosols impacts significantly on visibility degradation L. Liu et al. 10.5194/acp-22-7713-2022
- Impacts of Aerosol Chemical Composition on Cloud Condensation Nuclei (CCN) Activity during Wintertime in Beijing, China Q. Liu et al. 10.3390/rs15174119
- Enhanced daytime secondary aerosol formation driven by gas–particle partitioning in downwind urban plumes M. Cai et al. 10.5194/acp-24-13065-2024
- Aerosol hygroscopicity over the southeast Atlantic Ocean during the biomass burning season – Part 1: From the perspective of scattering enhancement L. Zhang et al. 10.5194/acp-24-13849-2024
- Formation of highly absorptive secondary brown carbon through nighttime multiphase chemistry of biomass burning emissions Y. Kuang et al. 10.5194/acp-25-3737-2025
- Photolysis frequency of nitrophenols derived from ambient measurements Y. Peng et al. 10.1016/j.scitotenv.2023.161810
- Measurement report: Size-resolved particle effective density measured by an AAC-SMPS and implications for chemical composition Y. Song et al. 10.5194/acp-25-4755-2025
- Measurement report: Distinct size dependence and diurnal variation in organic aerosol hygroscopicity, volatility, and cloud condensation nuclei activity at a rural site in the Pearl River Delta (PRD) region, China M. Cai et al. 10.5194/acp-22-8117-2022
- Residential Wood Burning and Vehicle Emissions as Major Sources of Environmentally Persistent Free Radicals in Fairbanks, Alaska K. Edwards et al. 10.1021/acs.est.4c01206
- Hygroscopic behavior and aerosol chemistry of atmospheric particles containing organic acids and inorganic salts F. Tan et al. 10.1038/s41612-024-00752-9
- Measurement report: The variation properties of aerosol hygroscopic growth related to chemical composition during new particle formation days in a coastal city of Southeast China L. Li et al. 10.5194/acp-25-3669-2025
- Parameterizations of size distribution and refractive index of biomass burning organic aerosol with black carbon content B. Luo et al. 10.5194/acp-22-12401-2022
- PM2.5 Source Apportionment and Implications for Particle Hygroscopicity at an Urban Background Site in Athens, Greece E. Diapouli et al. 10.3390/atmos13101685
- Relationships of the Hygroscopicity of HULIS With Their Degrees of Oxygenation and Sources in the Urban Atmosphere R. Zhou et al. 10.1029/2022JD037163
19 citations as recorded by crossref.
- Technical note: Quantified organic aerosol subsaturated hygroscopicity by a simple optical scatter monitor system through field measurements J. Zhang et al. 10.5194/acp-24-13445-2024
- Markedly different impacts of primary emissions and secondary aerosol formation on aerosol mixing states revealed by simultaneous measurements of CCNC, H(/V)TDMA, and SP2 J. Tao et al. 10.5194/acp-24-9131-2024
- Significant impact of water-soluble organic matter on hygroscopicity of fine particles under low relative humidity condition J. Tao et al. 10.1016/j.scitotenv.2023.167980
- Joint increase of aerosol scattering efficiency and aerosol hygroscopicity aggravate visibility impairment in the North China Plain B. Xue et al. 10.1016/j.scitotenv.2022.156279
- Theoretical framework for measuring cloud effective supersaturation fluctuations with an advanced optical system Y. Kuang et al. 10.5194/acp-25-1163-2025
- Strong light scattering of highly oxygenated organic aerosols impacts significantly on visibility degradation L. Liu et al. 10.5194/acp-22-7713-2022
- Impacts of Aerosol Chemical Composition on Cloud Condensation Nuclei (CCN) Activity during Wintertime in Beijing, China Q. Liu et al. 10.3390/rs15174119
- Enhanced daytime secondary aerosol formation driven by gas–particle partitioning in downwind urban plumes M. Cai et al. 10.5194/acp-24-13065-2024
- Aerosol hygroscopicity over the southeast Atlantic Ocean during the biomass burning season – Part 1: From the perspective of scattering enhancement L. Zhang et al. 10.5194/acp-24-13849-2024
- Formation of highly absorptive secondary brown carbon through nighttime multiphase chemistry of biomass burning emissions Y. Kuang et al. 10.5194/acp-25-3737-2025
- Photolysis frequency of nitrophenols derived from ambient measurements Y. Peng et al. 10.1016/j.scitotenv.2023.161810
- Measurement report: Size-resolved particle effective density measured by an AAC-SMPS and implications for chemical composition Y. Song et al. 10.5194/acp-25-4755-2025
- Measurement report: Distinct size dependence and diurnal variation in organic aerosol hygroscopicity, volatility, and cloud condensation nuclei activity at a rural site in the Pearl River Delta (PRD) region, China M. Cai et al. 10.5194/acp-22-8117-2022
- Residential Wood Burning and Vehicle Emissions as Major Sources of Environmentally Persistent Free Radicals in Fairbanks, Alaska K. Edwards et al. 10.1021/acs.est.4c01206
- Hygroscopic behavior and aerosol chemistry of atmospheric particles containing organic acids and inorganic salts F. Tan et al. 10.1038/s41612-024-00752-9
- Measurement report: The variation properties of aerosol hygroscopic growth related to chemical composition during new particle formation days in a coastal city of Southeast China L. Li et al. 10.5194/acp-25-3669-2025
- Parameterizations of size distribution and refractive index of biomass burning organic aerosol with black carbon content B. Luo et al. 10.5194/acp-22-12401-2022
- PM2.5 Source Apportionment and Implications for Particle Hygroscopicity at an Urban Background Site in Athens, Greece E. Diapouli et al. 10.3390/atmos13101685
- Relationships of the Hygroscopicity of HULIS With Their Degrees of Oxygenation and Sources in the Urban Atmosphere R. Zhou et al. 10.1029/2022JD037163
Latest update: 30 May 2025
Short summary
We found that organic aerosol factors with identified sources perform much better than oxidation level parameters in characterizing variations in organic aerosol hygroscopicity, and secondary aerosol formations associated with different sources have distinct effects on organic aerosol hygroscopicity. It reveals that source-oriented organic aerosol hygroscopicity investigations might result in more appropriate parameterization approaches in chemical and climate models.
We found that organic aerosol factors with identified sources perform much better than oxidation...
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