Articles | Volume 20, issue 13
Atmos. Chem. Phys., 20, 8201–8225, 2020
https://doi.org/10.5194/acp-20-8201-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Atmos. Chem. Phys., 20, 8201–8225, 2020
https://doi.org/10.5194/acp-20-8201-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
16 Jul 2020
Research article
| 16 Jul 2020
Predicting secondary organic aerosol phase state and viscosity and its effect on multiphase chemistry in a regional-scale air quality model
Ryan Schmedding et al.
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Cited
18 citations as recorded by crossref.
- A computationally efficient model to represent the chemistry, thermodynamics, and microphysics of secondary organic aerosols (simpleSOM): model development and application to α-pinene SOA S. Jathar et al. 10.1039/D1EA00014D
- Fluorescence Aerosol Flow Tube Spectroscopy to Detect Liquid–Liquid Phase Separation P. Ohno et al. 10.1021/acsearthspacechem.1c00061
- Direct observation and assessment of phase states of ambient and lab-generated sub-micron particles upon humidification Z. Cheng et al. 10.1039/D1RA02530A
- Measurements of the partitioning of nitric acid and sulfuric acid in aqueous/organic phase-separated systems B. Deming & P. Ziemann 10.1039/D0EA00003E
- Diurnal and Seasonal Variations in the Phase State of Secondary Organic Aerosol Material over the Contiguous US Simulated in CMAQ Y. Li et al. 10.1021/acsearthspacechem.1c00094
- Humidity-Dependent Viscosity of Secondary Organic Aerosol from Ozonolysis of β-Caryophyllene: Measurements, Predictions, and Implications A. Maclean et al. 10.1021/acsearthspacechem.0c00296
- Global Distribution of the Phase State and Mixing Times within Secondary Organic Aerosol Particles in the Troposphere Based on Room-Temperature Viscosity Measurements A. Maclean et al. 10.1021/acsearthspacechem.1c00296
- Viscosity and phase state of aerosol particles consisting of sucrose mixed with inorganic salts Y. Song et al. 10.5194/acp-21-10215-2021
- Representation of Multiphase OH Oxidation of Amorphous Organic Aerosol for Tropospheric Conditions J. Li & D. Knopf 10.1021/acs.est.0c07668
- Dynamics of Liquid–Liquid Phase Separation in Submicrometer Aerosol T. Kucinski et al. 10.1021/acs.jpca.1c01985
- Modeling Volatility-Based Aerosol Phase State Predictions in the Amazon Rainforest Q. Rasool et al. 10.1021/acsearthspacechem.1c00255
- Modeling the Size Distribution and Chemical Composition of Secondary Organic Aerosols during the Reactive Uptake of Isoprene-Derived Epoxydiols under Low-Humidity Condition M. Octaviani et al. 10.1021/acsearthspacechem.1c00303
- Evaluation of Biogenic Organic Aerosols in the Amazon Rainforest Using WRF‐Chem With MOSAIC J. Mao et al. 10.1029/2021JD034913
- Viscosity and liquid–liquid phase separation in healthy and stressed plant SOA N. Smith et al. 10.1039/D0EA00020E
- Determining the Role of Acidity, Fate and Formation of IEPOX-Derived SOA in CMAQ P. Vasilakos et al. 10.3390/atmos12060707
- Molecular-scale description of interfacial mass transfer in phase-separated aqueous secondary organic aerosol M. Lbadaoui-Darvas et al. 10.5194/acp-21-17687-2021
- Prediction of Phase State of Secondary Organic Aerosol Internally Mixed with Aqueous Inorganic Salts Z. Yu et al. 10.1021/acs.jpca.1c06773
- Predictions of the glass transition temperature and viscosity of organic aerosols from volatility distributions Y. Li et al. 10.5194/acp-20-8103-2020
17 citations as recorded by crossref.
- A computationally efficient model to represent the chemistry, thermodynamics, and microphysics of secondary organic aerosols (simpleSOM): model development and application to α-pinene SOA S. Jathar et al. 10.1039/D1EA00014D
- Fluorescence Aerosol Flow Tube Spectroscopy to Detect Liquid–Liquid Phase Separation P. Ohno et al. 10.1021/acsearthspacechem.1c00061
- Direct observation and assessment of phase states of ambient and lab-generated sub-micron particles upon humidification Z. Cheng et al. 10.1039/D1RA02530A
- Measurements of the partitioning of nitric acid and sulfuric acid in aqueous/organic phase-separated systems B. Deming & P. Ziemann 10.1039/D0EA00003E
- Diurnal and Seasonal Variations in the Phase State of Secondary Organic Aerosol Material over the Contiguous US Simulated in CMAQ Y. Li et al. 10.1021/acsearthspacechem.1c00094
- Humidity-Dependent Viscosity of Secondary Organic Aerosol from Ozonolysis of β-Caryophyllene: Measurements, Predictions, and Implications A. Maclean et al. 10.1021/acsearthspacechem.0c00296
- Global Distribution of the Phase State and Mixing Times within Secondary Organic Aerosol Particles in the Troposphere Based on Room-Temperature Viscosity Measurements A. Maclean et al. 10.1021/acsearthspacechem.1c00296
- Viscosity and phase state of aerosol particles consisting of sucrose mixed with inorganic salts Y. Song et al. 10.5194/acp-21-10215-2021
- Representation of Multiphase OH Oxidation of Amorphous Organic Aerosol for Tropospheric Conditions J. Li & D. Knopf 10.1021/acs.est.0c07668
- Dynamics of Liquid–Liquid Phase Separation in Submicrometer Aerosol T. Kucinski et al. 10.1021/acs.jpca.1c01985
- Modeling Volatility-Based Aerosol Phase State Predictions in the Amazon Rainforest Q. Rasool et al. 10.1021/acsearthspacechem.1c00255
- Modeling the Size Distribution and Chemical Composition of Secondary Organic Aerosols during the Reactive Uptake of Isoprene-Derived Epoxydiols under Low-Humidity Condition M. Octaviani et al. 10.1021/acsearthspacechem.1c00303
- Evaluation of Biogenic Organic Aerosols in the Amazon Rainforest Using WRF‐Chem With MOSAIC J. Mao et al. 10.1029/2021JD034913
- Viscosity and liquid–liquid phase separation in healthy and stressed plant SOA N. Smith et al. 10.1039/D0EA00020E
- Determining the Role of Acidity, Fate and Formation of IEPOX-Derived SOA in CMAQ P. Vasilakos et al. 10.3390/atmos12060707
- Molecular-scale description of interfacial mass transfer in phase-separated aqueous secondary organic aerosol M. Lbadaoui-Darvas et al. 10.5194/acp-21-17687-2021
- Prediction of Phase State of Secondary Organic Aerosol Internally Mixed with Aqueous Inorganic Salts Z. Yu et al. 10.1021/acs.jpca.1c06773
Discussed (final revised paper)
Latest update: 07 Aug 2022
Short summary
Accurate model prediction of aerosol concentrations is a known challenge. It is assumed in many modeling systems that aerosols are in a homogeneously mixed phase state. It has been observed that aerosols do phase separate and can form a highly viscous organic shell with an aqueous core impacting the formation processes of aerosols. This work is a model implementation to determine an aerosol's phase state using glass transition temperature and aerosol composition.
Accurate model prediction of aerosol concentrations is a known challenge. It is assumed in many...
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